Theory of STM on Unconventional Superconductorskreisel/Kreisel_STM_SC_kit.pdf · Theory of STM on...
Transcript of Theory of STM on Unconventional Superconductorskreisel/Kreisel_STM_SC_kit.pdf · Theory of STM on...
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Theory of STM on Unconventional Superconductors
Andreas KreiselInstitut für Theoretische Physik, Universität Leipzig, Germany
T. BerlijnCNMS, Oak Ridge Nat. Lab., USA
W. KuDept. of Phys. and Astr.,
Shanghai Jiao Tong U., China
P.J. HirschfeldDept. of Physics, U. Florida, USA
B.M. AndersenNiels Bohr Institute, U. Copenhagen, Denmark
P. Choubey, et al., Phys. Rev. B 90, 134520 (2014)A. Kreisel, et al., Phys. Rev. Lett. 114, 217002 (2015)A. Kreisel, et al., Phys. Rev. B 94, 224518 (2016)P. Choubey, et al.. Phys. Rev. B 96, 174523 (2017)
P. ChoubeyIndian Institute of Science, Bengaluru 560012, India
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Outline
● Motivation– STM: impurities as probe for electronic
structure, order parameter and more
– layered superconductors, complications
● Theoretical methods to investigate impurity physics in superconductors– using wavefunction information in layered
superconductors: Wannier method
– Applications● LiFeAs (multiband, s-wave)● Cuprates: Bi2Sr2CaCu2O8 , Ca2CuO2Cl2
● Inelastic tunneling
s± s++
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Scanning tunneling microscopy
J. Tersoff and D. R. Hamann, PRB 31, 805 (1985)
J. Hoffman Rep. Prog. Phys. 74 124513 (2011)
I(V; x; y; z) = ¡4¼e~½t(0)jM j2
Z eV
0
½(x; y; z; ²)d²
Tunneling current:
Local Density Of States (LDOS)of sample at given energy at the tip position
STMtip
samplee.g.SC
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STM: examples
● Cuprates: Zn impurity in BSCCO
● Fe-SCFeSe: topograph of Fe centered impurity
Song et al., Science 332, 1410 (2011)
Can-Li Song, et al. PRL 109, 137004 (2012)
spectra and conductance map
Pan et al., Nature 403, 746 (2000)
LiFeAs: Fe centered impurity
S. Grothe, et al., PRB 86, 174503 (2012)
-200 -100 0 100 2000.0
0.5
1.0
1.5
2.0
2.5
Diff
ere
ntia
l Con
duct
anc
e (
nS)
Sample Bias (mV)
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Layered superconductors
● 2 examples: surface atoms ≠ superconducting layer
Cuprates Iron based superconductors
Bi-2212
LiFeAs
“111”
Fe
As
Li
surface: Li, As?
surface: BiO
states at theFermi levelCu-planeFe-plane
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Theoretical approaches: Cuprates
● LDOS: impurity in d-wave superconductor– local LDOS: 4 fold pattern
– low energy bound state
● Comparison to experiment
A. V. Balatsky, M. I. Salkola, and A. Rosengren Phys. Rev. B 51, 15547 (1995)
J. M. Byers, M. E. Flatté, and D. J. Scalapino Phys. Rev. Lett. 71, 3363 (1993)
Stamp, Journal of Magnetism and Magnetic Materials, 63, 429 - 431 (1987) (p-wave)
-200 -100 0 100 2000.0
0.5
1.0
1.5
2.0
2.5
Diff
eren
tial C
ondu
ctan
ce (
nS)
Sample Bias (mV)Pan et al., Nature 403, 746 (2000)
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Theoretical approaches: Cuprates
● LDOS: impurity in d-wave superconductor– local LDOS: 4 fold pattern
– low energy bound state
● Comparison to experiment
A. V. Balatsky, M. I. Salkola, and A. Rosengren Phys. Rev. B 51, 15547 (1995)
J. M. Byers, M. E. Flatté, and D. J. Scalapino Phys. Rev. Lett. 71, 3363 (1993)
Stamp, Journal of Magnetism and Magnetic Materials, 63, 429 - 431 (1987) (p-wave)
Cu-Cu
Cu-Cu-200 -100 0 100 2000.0
0.5
1.0
1.5
2.0
2.5
Diff
eren
tial C
ondu
ctan
ce (
nS)
Sample Bias (mV)Pan et al., Nature 403, 746 (2000)
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Theoretical approaches: Cuprates
● extended impurity potentials(magnetic Ni impurity)
● Correlations: “Kondo screening” (magnetic impurity)
● “Filter function”: STM tip probes states in the superconducting layer by tunneling matrix elements
● Large tight binding basis set of orbitals + Greens function method to calculate tunneling matrix elements
J. Nieminen, et al., PRB 80, 134509 (2009)
Martin et al., PRL 88, 097003 (2002)
Jian-Ming Tang and Michael E. Flatté PRB 66, 060504(R) (2002)
Anatoli Polkovnikov PRB 65, 064503 (2002)
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Theoretical approaches: Fe-SC
● Identification of nature of impurities in FeSe monolayer (non-SC) by ab-initio calculations
● Inelastic tunneling– coupling to bosonic mode
– signatures of spin fluctuations (real space)
● Wannier method (this talk)
normal state
superconductingstate
Dennis Huang et al., Nano Lett., 16 (7), 4224 (2016)
See also: “holographic maps”Dalla Torre, He, DemlerNat. Phys., 12, 1052 (2016) unravel intra-unitcell
information
S. Chi, et al., Nat. Commun. 8, 15996 (2017)
J. R. Kirtley and D. J. Scalapino, PRL 65, 798 (1990); J. R. Kirtley, PRB 47, 11379 (1993)P. Hlobil, et al., Phys. Rev. Lett. 118, 167001 (2017)
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Wannier method: example LiFeAs
● Ab-initio calculation– band structure
5 band model
– Wannier functions(including glideplane symmetry)
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Superconductivity
● superconducting order parameter from spin- fluctuation theory
● calculate Green's function in superconducting state
Real space Greens function by Fourier transform
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Impurity → engineered
● ab-initio calculation of impurity potential for Co, Ni, Mn in LiFeAs (engineered impurity)
● T-matrix approach to obtain Green's function other methods also possible– BdG
– Gutzwiller mean field
lattice Green function (state of the art)
Kreisel et al., Phys. Rev. Lett. 114, 217002 (2015)Choubey et al., New J. Phys. 19, 013028 (2017)
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cLDOS
● Basis transformation
lattice Green functioncontinuum position
nonlocal contributions
surface Wannier function with phases
continuum Local Density Of States (cLDOS)of sample at given energy at the tip position
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LiFeAs: Questions
● Properties of the orderparameter (sign-change)
antiphase s±Z. P. Yin, K. Haule, G. KotliarNature Physics 10, 845 (2014)
conventional s± Y. Wang, A. Kreisel, et al.,Phys. Rev. B 88, 174516 (2013)A. Kreisel, et al., Phys. Rev. B 95, 174504 (2017)
novel s± F. Ahn, et al., Phys. Rev. B 89, 144513 (2014)
conventional s++T. Saito, et al. Phys. Rev. B 90, 035104 (2014)
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LiFeAs: Questions
● Interpretation of– impurity shapes
– registered “surface lattice” in STM
“Dot” “Trench” “Dumbbell”
Hanaguri, unpublished (KITP 2011)R. Schlegel, et al., Phys. Status Solidi B, 254: 1600159 (2017)
Shun Chi, et al., PRL 109, 087002 (2012)T. Hanaguri, et al. PRB 85, 214505 (2012)S. Grothe, et al., PRB 86, 174503 (2012)J. -X. Yin, et al., arXiv, 1602.04949 (2016)
LiFeAs: Li or As lattice?
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LiFeAs: spectra
● evidence for sign-changing order parameter by in-gap state with engineered impurity
conventional calculation:lattice LDOS: strongresponse at negative bias
S. Chi, (...) , A. Kreisel, et al. Phys. Rev. B 94, 134515 (2016)
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LiFeAs: spectra
● sequence of impurity potentials from ab-initio calculation correct, but overall renormalization downwards required[correlation effects]
relative spectraNi impurity
P. O. Sprau, …, A. Kreisel, et al., Science, 357, 75 (2017)A. Kreisel, et al., Phys. Rev. B 95, 174504 (2017)A. Kostin, et al., arXiv:1802.02266 S. Chi, (...) , A. Kreisel, et al.
Phys. Rev. B 94, 134515 (2016)
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Height and current dependence of topographs
● experiment: Li or As lattice?
Shun Chi, et al., PRL 109, 087002 (2012)T. Hanaguri, et al. PRB 85, 214505 (2012)S. Grothe, et al., PRB 86, 174503 (2012)J. -X. Yin, et al., arXiv, 1602.04949 (2016)
height maxima at Li positions!?counter-intuitive from chemistry point of view
R. Schlegel, et al., Phys. Status Solidi B, 254: 1600159 (2017)
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Further experimental evidences?
Ronny Schlegel, Dissertation, TU Dresden(thanks to C. Hess)
expe
rimen
t (cu
rren
t m
aps)
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Further experimental evidences?
Ronny Schlegel, Dissertation, TU Dresden(thanks to C. Hess)
expe
rimen
t (cu
rren
t m
aps)
theo
ry
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Simulation of topographs
● solve for
● switching of height maxima as a function of bias voltage
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Resultsregistered surface lattice in STM
● tunneling into states describedby Wannier functions
● registered lattice switchesas function of bias and current
measured topographies
simulated topographies
“Li lattice” “As lattice”
measured topographyclose to Ni
simulated topography close to strong imp.
bias
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Inelastic tunneling
● well known propertyincreasing conductance at large bias
● deduction of collective modes?
J. R. Kirtley and D. J. Scalapino, PRL 65, 798 (1990); J. R. Kirtley, PRB 47, 11379 (1993)P. Hlobil, et al., Phys. Rev. Lett. 118, 167001 (2017)
Nag et al, Scientific Reports 6, 27926 (2016)
spectraDensity of states
Chi et al, Nat. Commun. 8, 15996 (2017)
normal state
superconductingstate
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Inelastic tunneling in FeSC:coupling to spin fluctuations
● Inelastic contribution
● Dip-hump feature
Spin fluctuations: two gap superconductor (LiFeAs), double resonance
J. R. Kirtley and D. J. Scalapino, PRL 65, 798 (1990); J. R. Kirtley, PRB 47, 11379 (1993)P. Hlobil, et al., Phys. Rev. Lett. 118, 167001 (2017)
M. M. Korshunov, et al., Phys. Rev. B 94, 094517 (2016)
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Imaging spin fluctuations in real space
● real space structure
● in presence of impurity
Fast spatial decay of impurity resonance, slow decay of dip-hump → spin fluctuations (real space)
S. Chi, (…) AK, et al., Nat. Commun. 8, 15996 (2017)
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Cuprates: Questions
● signatures of strong impurity in d-wave SC
● universalities across materials
Cu-Cu
Cu-Cu
Kohsaka et al. Nature, 454, 1072 (2008)
Crossover between U-shaped andV-shaped spectra
same properties for tunneling!
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Wannier method: CupratesSurfaceBiO vs. CaCland tunneling path very different
Ab initio calculation:1 band model+Wanner function
similar properties dictated by crystal symmetry
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Superconductivity
● superconducting order parameter(d-wave) (phenomenology orcalculation fx. mean-field)
● continuum Green function
lattice Green functioncontinuum position
nonlocal contributions
surface Wannier function with phases
½(r; !) ´ ¡ 1¼ImG(r;r;!)
local density of states (LDOS)
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BSCCO: ResultsSTM maps and spectra
● d-wave order parameter● Zn impurity:
Vimp=-5 eVresonance: -3.6 meV
resonance at NN
resonance at impurity
Zhu et al., PRB 67, 094508 (2003)
-200 -100 0 100 2000.0
0.5
1.0
1.5
2.0
2.5
Diff
eren
tial C
ondu
ctanc
e (n
S)
Sample Bias (mV)
Pan et al., Nature 403, 746 (2000)
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STM Spectra: homogeneous SC
● overdoped: U-shape, lower doping: V-shape
● Analytical result– Spectral function
– Wannier transformation
– dx²-y² Wannier function
– only cubic contribution
Kohsaka et al.Nature, 454, 1072 (2008)
Alldredge et al.Nature Physics, 4, 319 (2008) BdG+W:
U-shape enters naturally within Wannier transformation
A. Kreisel, et al., Phys. Rev. Lett. 114, 217002 (2015)
P. Choubey, et al.. Phys. Rev. B 96, 174523 (2017)
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Bi2Sr
2CaCu
2O
8 ↔ Ca
2CuO
2Cl
2
● superconductivity:d-wave order parameter
● T-matrix calculation+ Wannier method
● strong impurityspectra + conductance map
Kreisel et al., Phys. Rev. Lett. 114, 217002 (2015)Choubey et al., New J. Phys. 19, 013028 (2017)P. Choubey, et al.. Phys. Rev. B 96, 174523 (2017)
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Summary
Acknowledgments
● Wannier method: basis transformation of the lattice Green function
● Qualitative correct (symmetry) and quantitative predictive results
● Impurities and homogeneous lattice in LiFeAs
● inelastic tunneling● Universality in cuprates● method to detect sign change of
order parameter in STM
● Nematicity in Fe-based SC
S. Chi, (...) , A. Kreisel, et al. Phys. Rev. B 94, 134515 (2016)A. Kreisel, et al. Phys. Rev. B 94, 224518 (2016)
Kreisel et al., Phys. Rev. Lett. 114, 217002 (2015)Choubey et al., New J. Phys. 19, 013028 (2017)Choubey, et al.. Phys. Rev. B 96, 174523 (2017)
S. Chi, (…) AK, et al., Nat. Commun. 8, 15996 (2017)
Martiny, Kreisel, Hirschfeld, Andersen Phys. Rev. B 95, 184507 (2017)Sprau, et al. Science, 357, 75 (2017)
A. Kostin,et al., arXiv:1802.02266