PHYSICAL REVIEW ACCELERATORS AND BEAMS 23, 093402 (2020)

9
Semiempirical zero-dimensional approach for the estimation of beam features from plasma parameters in proton sources G. Castro INFN Laboratori Nazionali del Sud, via S. Sofia 62, 95123 Catania, Italy (Received 3 June 2020; accepted 9 September 2020; published 28 September 2020) Beam intensity, proton fraction, and beam emittance represent the most important characteristics of a beam extracted by a proton source. Beam parameters are strongly related to the parameters of the plasma from which the beam is extracted. The recent improvement of plasma diagnostics devoted to compact ion sources, and, in particular, the development of optical emission spectroscopy, allows an ever more reliable measurement of plasma parameters, also during source operations. In this paper, a zero-dimensional approach able to estimate the beam intensity and the ion fraction from plasma parameters in a proton source is introduced. The model is based on a simplified solution of the balance equation system in a hydrogen plasma achieved by including the electron density, the electron temperature, and the relative neutral abundance ratio H=H 2 within the equations. This approach permits one to reduce the balance equation system to four equations in four unknowns, namely, the H þ ,H þ 2 , and H þ 3 density and the confinement time. The balance equation system is solved by means of a homemade numerical code. The model has been applied to the beam generated by the Proton Source for the European Spallation Source (PS-ESS), during its commissioning at Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali del Sud in Catania. The extracted current and ion fraction estimated by this approach have been compared with the experimental results obtained by the PS-ESS beam diagnostics. The proton confinement time estimated by this approach has been compared with the results of a theoretical model based on a diffusion model. The comparison demonstrates that the model has achieved a surprising capability of estimation. The paper discusses the main characteristics of the zero-dimensional approach together with its main advantages and limits. The perspectives for further improvement of the model are also discussed. DOI: 10.1103/PhysRevAccelBeams.23.093402 I. INTRODUCTION Microwave discharge ion sources (MDIS) and electron cyclotron resonance ion sources (ECRIS) are currently the most used devices to feed particle accelerators because of their compactness and reliability [1]. MDIS are usually used for the generation of protons, H þ 2 , and light ion beams characterized by low emittance, high stability, and beam intensity up to 100 mA [26]. To be able to improve the ion source performances, it is of great value to have an in-depth understanding of the mechanism occurring in the plasma. This can be achieved by the implementation of diagnostic techniques, such as Langmuir probe diagnostics, x-ray diagnostics, interfero- polarimetry, and optical emission spectroscopy (OES) [7]. Among them, OES is probably the most remarkable for application in working ECRIS and MDIS: It requires very little room for operation (just a quartz window to access the plasma light), it does not directly affect nor is affected by plasma (although indirect effects due to the optical windows can arise), and it operates also in high-voltage conditions, i.e., the usual working conditions in ECRIS and MDIS. According to the sensitivity of the instrumentation, OES allows one to evaluate the plasma emission lines that, analyzed with a proper collisional radiative model, enable achieving the electron density n e , the electron temperature T e of the cold electron population (0100 eV) [8,9], the ion temperature T i [10], the neutral relative abundances, the rotovibrational molecular spectrum [11], and the concen- tration of highly charged ions in plasmas by acquiring the electromagnetic spectrum emitted by the plasma in the optical domain. Figure 1 shows a typical spectrum acquired in a MDIS ion source: Balmer lines and a Fulcher band are evidenced. More information on the OES technique and its appli- cations can be found in Refs. [12,13]. The goal of this paper is to introduce a zero-dimensional semiempirical approach able to relate univocally the beam parameters to the plasma parameters in proton sources and, Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published articles title, journal citation, and DOI. PHYSICAL REVIEW ACCELERATORS AND BEAMS 23, 093402 (2020) 2469-9888=20=23(9)=093402(9) 093402-1 Published by the American Physical Society

Transcript of PHYSICAL REVIEW ACCELERATORS AND BEAMS 23, 093402 (2020)

Semiempirical zero-dimensional approach for the estimation of beamfeatures from plasma parameters in proton sources

G. CastroINFN Laboratori Nazionali del Sud, via S. Sofia 62, 95123 Catania, Italy

(Received 3 June 2020; accepted 9 September 2020; published 28 September 2020)

Beam intensity, proton fraction, and beam emittance represent the most important characteristics of abeam extracted by a proton source. Beam parameters are strongly related to the parameters of the plasmafrom which the beam is extracted. The recent improvement of plasma diagnostics devoted to compact ionsources, and, in particular, the development of optical emission spectroscopy, allows an ever more reliablemeasurement of plasma parameters, also during source operations. In this paper, a zero-dimensionalapproach able to estimate the beam intensity and the ion fraction from plasma parameters in a proton sourceis introduced. The model is based on a simplified solution of the balance equation system in a hydrogenplasma achieved by including the electron density, the electron temperature, and the relative neutralabundance ratio H=H2 within the equations. This approach permits one to reduce the balance equationsystem to four equations in four unknowns, namely, the Hþ, Hþ

2 , and Hþ3 density and the confinement time.

The balance equation system is solved by means of a homemade numerical code. The model has beenapplied to the beam generated by the Proton Source for the European Spallation Source (PS-ESS), duringits commissioning at Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali del Sud in Catania. Theextracted current and ion fraction estimated by this approach have been compared with the experimentalresults obtained by the PS-ESS beam diagnostics. The proton confinement time estimated by this approachhas been compared with the results of a theoretical model based on a diffusion model. The comparisondemonstrates that the model has achieved a surprising capability of estimation. The paper discusses themain characteristics of the zero-dimensional approach together with its main advantages and limits. Theperspectives for further improvement of the model are also discussed.

DOI: 10.1103/PhysRevAccelBeams.23.093402

I. INTRODUCTION

Microwave discharge ion sources (MDIS) and electroncyclotron resonance ion sources (ECRIS) are currently themost used devices to feed particle accelerators because oftheir compactness and reliability [1]. MDIS are usuallyused for the generation of protons, Hþ

2 , and light ion beamscharacterized by low emittance, high stability, and beamintensity up to 100 mA [2–6].To be able to improve the ion source performances, it is

of great value to have an in-depth understanding of themechanism occurring in the plasma. This can be achievedby the implementation of diagnostic techniques, such asLangmuir probe diagnostics, x-ray diagnostics, interfero-polarimetry, and optical emission spectroscopy (OES) [7].Among them, OES is probably the most remarkable forapplication in working ECRIS and MDIS: It requires very

little room for operation (just a quartz window to access theplasma light), it does not directly affect nor is affectedby plasma (although indirect effects due to the opticalwindows can arise), and it operates also in high-voltageconditions, i.e., the usual working conditions in ECRIS andMDIS.According to the sensitivity of the instrumentation, OES

allows one to evaluate the plasma emission lines that,analyzed with a proper collisional radiative model, enableachieving the electron density ne, the electron temperatureTe of the cold electron population (0–100 eV) [8,9], the iontemperature Ti [10], the neutral relative abundances, therotovibrational molecular spectrum [11], and the concen-tration of highly charged ions in plasmas by acquiring theelectromagnetic spectrum emitted by the plasma in theoptical domain. Figure 1 shows a typical spectrum acquiredin a MDIS ion source: Balmer lines and a Fulcher band areevidenced.More information on the OES technique and its appli-

cations can be found in Refs. [12,13].The goal of this paper is to introduce a zero-dimensional

semiempirical approach able to relate univocally the beamparameters to the plasma parameters in proton sources and,

Published by the American Physical Society under the terms ofthe Creative Commons Attribution 4.0 International license.Further distribution of this work must maintain attribution tothe author(s) and the published article’s title, journal citation,and DOI.

PHYSICAL REVIEW ACCELERATORS AND BEAMS 23, 093402 (2020)

2469-9888=20=23(9)=093402(9) 093402-1 Published by the American Physical Society

therefore, to permit the real-time estimation of the beamparameters from plasma parameters. In past decades,numerical simulations have already become a valuabletool for improving the understanding of discharge physicsand can provide theoretical predictions, especially in caseswhere diagnostic devices are expensive or difficult toinclude in an experimental setup. Zero-dimensional modelsapplied to hydrogen discharges have been already reported[14–20]. Four fundamental conservation laws are usuallyused in the formulation of a zero-dimensional mode:(i) mass conservation, described via a particle balancefor each species except for the H2 molecules; (ii) chargeconservation, reduced to the quasineutrality condition;(iii) neutral density conservation, determined by the equa-tion of state for the total particle number density; and(iv) the energy conservation law, expressed through powerbalance. The resulting balance conditions consist of asystem of 24 coupled nonlinear ordinary differentialequations which can be numerically solved to obtainrelevant plasma parameters [14].This paper simplifies the aforementioned balance equa-

tion system by including the plasma parameters evaluatedby OES diagnostics and the neutral pressure as inputparameters. This approach has allowed estimation of thein-plasma density of Hþ, Hþ

2 , and Hþ3 ions. The classical

Child-Langmuir law conditions allow one to estimate theconcentration of Hþ, Hþ

2 , and Hþ3 ions in the beam

extracted from and the total current [21].To validate this semiempirical approach, the MDIS

proton source for the European Spallation Source (PS-ESS) has been used as a test bench [22]. PS-ESS wasdesigned, built, and commissioned in the framework of theESS project at the Istituto Nazionale di Fisica Nucleare,Laboratori Nazionali del Sud (INFN-LNS) to become theinjector of the ESS linac. PS-ESS works in pulsed waves(6 ms pulse length, 14 Hz repetition rate) and produces

more than 100 mA of proton current with an emittancelower than 0.2 π · mm · mrad, according to the ESS projectrequirements. More information about PS-ESS and itscharacteristics can be found in Refs. [23,24].During the commissioning phase, four diagnostics have

been used to characterize the beam extracted by PS-ESS.In particular, we measured (i) the total current from a high-voltage power supply by a wide-bandwidth ac currenttransformer (ACCT); (ii) the species fraction in the low-energy beam transport (LEBT) by a Doppler-shift meas-urement unit; (iii) the beam intensity at the end of the LEBTby a Faraday cup; and (iv) the beam emittance by anemittance measurement unit.Measurements of PS-ESS plasma parameters by OES

have been also performed. The electron density ne, theelectron temperature Te, and the neutral relative abundan-ces NH=NH2

(NH and NH2being the density of atomic

hydrogen H and molecular hydrogen H2, respectively) havebeen estimated by comparing the differences betweenexperimental and theoretical line ratios (Yacora package[25]) of Balmer lines and the Fulcher band for anyoperative configuration. The statistical error in the mini-mization procedure allows one to evaluate the plasmaparameter error (see Ref. [26] for further information).A comparison between beam parameters estimated by

the semiempirical approach and experimental data acquiredin the same experimental conditions has been used tovalidate the approach. Either the extracted current or the ionfractions are predicted with accuracy. Moreover, the con-finement time estimated by the semiempirical approach hasbeen compared with a theoretical diffusion model in MDIS.Plasma parameters used as input parameters in this workare available in Ref. [26].

II. HYPOTHESIS AND ASSUMPTIONS

The semiempirical approach presented in this workconnects the plasma parameters (ne, Te, and NH=NH2

) tothe beam parameters under a number of hypotheses,approximations, and assumptions regarding the beamgeneration from plasma and the characteristics of theplasma parameters evaluated by OES that will be discussedin this section.

A. Assumptions concerning the beam generationfrom plasma

Generation and extraction of an ion beam from ECRISplasma is a topic discussed for several decades. In thiswork, a series of reasonable approximations have beenintroduced to simplify the physical problem: (1) Ionsmove along a flux tube parallel to the magnetic field witha radius equal to the extraction hole r (see Fig. 2). Thishypothesis is based on the consideration that, in MDIS,the parallel diffusion coefficient Dk is much larger than theradial diffusion coefficient D⊥. Therefore, plasma can be

FIG. 1. Example of hydrogen spectrum used for achieving thePS-ESS plasma parameters.

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considered frozen to the magnetic field lines [27–29].(2) Ion motion is isotropic along the axial direction. Ionshave equal probability to move toward the extraction holeor toward the opposite direction. Therefore, just one-half ofthe ions in the magnetic flux tube move toward extraction.(3) All ions in the flux tube approaching the plasmameniscus are extracted. (4) Ions enter the extraction regionwith Bohm velocity vBohm [28]. This is the velocity withwhich ions enter the plasma sheath. viBohm depends on theelectron temperature Te and ion temperature Ti (measuredin eV) and on ion mass Mi as follows:

viBohm ¼ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffieðTi þ TeÞ

Mi

s: ð1Þ

(5) The Child-Langmuir hypothesis is assumed: Duringextraction, the beam current density JiðzÞ (where thesubscript i represents each one of the three species thatconstitute the extracted beam, i.e., Hþ, Hþ

2 , and Hþ3 , and z is

the distance from the extraction sheath) does not depend onthe position z in the gap [21]. Current density conservationimplies that JiðzÞ can be evaluated in any point of the gapand, in particular, at the position z ¼ 0. It follows that

JiðzÞ ¼ Jiðz ¼ 0Þ ¼ qniviBohm: ð2Þ

This strategy allows one to avoid any consideration aboutthe influence of the geometry of the extraction system. Inparticular, one can assume the current value supplied by theACCT as the total extracted beam current. It is well knownthat the ACCT current is due to two contributions, thepositive ion current exiting the ion source and the electroncurrent (generated by residual gas ionization in the LEBT)entering the source. However, the second contribution isgenerally much smaller than the first one, and, for the scopeof this work, it can be neglected.

B. Assumptions concerning plasma parameters

The mode operation of PS-ESS and the experimentalapproach used to measure the plasma parameters imply theuse of further approximations and hypothesis concerningplasma characteristics: (1) Plasma parameters are assumedto not change considerably with the chamber radius.

Indeed, the first hypothesis concerning the beam generationrequires plasma parameters to be ideally evaluated alongthe magnetic flux tube from which ions are extracted. Inreal experiments, this measurement cannot be performedbecause of mechanical constraints. In the case of thePS-ESS test bench [26], OES plasma parameters havebeen evaluated by means of an opportune optical fiberconnection to the gas input. This has implied a determi-nation of plasma parameters from an oblique cone of viewintercepting the extraction hole, as shown in Fig. 3. Thehypothesis of small dependence of plasma parameters fromthe radius allows considering OES measurements asrepresentative of a measurement performed along themagnetic flux tube. (2) Although PS-ESS is operated ina 6 ms pulsed wave, we suppose that the variation of plasmaparameters during plasma turn on and off phases isnegligible. Figure 4 shows the 6 ms beam pulse measuredby the ACCT for values of microwave power increasingfrom 100 to 1200 W through 10 W steps. Extracted currentis almost constant in the temporal interval 0.4–6 ms for

FIG. 2. Schematic view of a magnetic flux tube in a protonsource. Because of the negligible radial diffusion, ions movealong a magnetic tube flux tube toward the extraction hole [27].

FIG. 3. Sketch of the OES experimental setup including thearrangement of the diagnostics.

FIG. 4. PS-ESS beam pulse measured by the ACCT for valuesof microwave power increasing from 100 to 1200 W through10 W steps. ACCT current is almost constant from 0.4 to 6 ms formicrowave power larger than 150 W.

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microwave power larger than 150 W. Moreover, rise andfall times are of the order of few hundreds of microseconds,much smaller than the pulse length. Several works showthat plasma parameters reach steady state conditions in∼0.6 ms after plasma switch on [30,31]. Therefore, forthe purposes of this work, PS-ESS plasma can be assumedin steady state conditions during OES measurements.(3) During the OES experimental campaign on thePS-ESS proton source, it was not possible to measurethe neutral and ion temperature. Yonesu et al. [32]performed measurements of neutral and ion temperaturein experimental conditions very close to PS-ESS. Theyfound a neutral temperature Tn ∼ 0.05 eV and ion temper-ature Ti ∼ 0.4 eV at 1 × 10−3 mbar operative pressure and2.5 kWmicrowave power. The value of neutral temperaturehas been confirmed also by measurements reported inRef. [11]. In this work, we hypothesize that Tn and Tiassume similar values as given by the previous references.(4) Ion lifetime τ is assumed to be proportional to thesquare root of the ion mass. Indeed, τ is inversely propor-tional to the ambipolar diffusion coefficient, which, in turn,is inversely proportional to the square root of the ion mass(more information in Refs. [27,28,33]). Therefore, thefollowing relation holds:

τHþ∶τHþ2∶τHþ

3¼ 1∶

ffiffiffi2

p∶

ffiffiffi3

p: ð3Þ

III. MODEL DESCRIPTION

The estimation of the beam parameters from plasmaparameters has been performed through a three-stageprocedure.

A. Stage 1

Neutral pressure is measured in the low-energybeam transport. However, if the hydrogen flow rate inthe plasma chamber and the geometry of the proton sourceare known, it is possible to evaluate an average value of theneutral pressure inside the plasma chamber. Neutral pres-sure P depends on the neutral density and temperature asfollows:

P ¼ NHTn þ NH2Tn: ð4Þ

According to hypothesis (iii) of Sec. II B, we assume aconstant neutral temperature, while the ratio NH=NH2

isknown from the OES measurements. This allows one toevaluate the absolute value of NH and NH2

for anyexperimental value of NH=NH2

.

B. Stage 2

In this stage, the following nonlinear balance equa-tion system in the unknowns nHþ , nHþ

2, nHþ

3, and τHþ is

solved:

ne ¼ nHþ þ nHþ2þ nHþ

3;

Xi

RiHþ −

nHþ

τHþ¼ 0;

Xi

RiHþ

2

−nHþ

2

τHþ2

¼Xi

RiHþ

2

−nHþ

2ffiffiffi2

pτHþ

¼ 0;

Xi

RiHþ

3

−nHþ

3

τHþ3

¼Xi

RiHþ

3

−nHþ

3ffiffiffi3

pτHþ

¼ 0; ð5Þ

nHþ , nHþ2, and nHþ

3being the density of Hþ, Hþ

2 , and Hþ3 ,

respectively, in plasma, and τHþ , τHþ2, and τHþ

3are the

confinement times for the three species. τHþ2and τHþ

3have

been replaced, respectively, withffiffiffi2

pτHþ and

ffiffiffi3

pτHþ

according to hypothesis (iv) of Sec. II B.Ri represents the volume creation or loss rate of the

generic reactions i for each ion species. In particular, Ri isdefined as

Ri ¼ nAnBQi; ð6Þ

where nA and nB are the densities of the interacting speciesand Qi is known as the reaction rate coefficient. For aMaxwellian distribution, Qi is only a function of Te [33]:

QiðTeÞ ¼Z

0

σifðvÞvdv ¼ 6.7 × 107

× T−3=2e

Z∞

0

Eσie−E=TedE: ð7Þ

In this work, we have considered 13 reactions having across section larger than 10−18 cm2 in the energy domain0–100 eV [34]. A list of the reactions is presented inTable I. Figure 5 shows the cross sections as a function ofthe electron temperature. In this picture, σ10 is a constant,because it does not depend on the electron temperature buton the ion temperature, assumed to be a constant. σ10 has

TABLE I. List of the cross sections taken into account forproton fraction estimation [34].

Reaction Process

σ1 H2 þ e− → Hþ Hþ e− Dissociative excitationσ2 H2 þ e− → Hþ

2 þ 2e− Ionizationσ3 H2 þ e− → Hþ þ Hþ 2e− Dissociative ionizationσ4 Hþ

2 þ e− → Hþ þ Hþ e− Dissociative excitationσ5 Hþ

2 þ e− → 2Hþ þ 2e− Dissociative ionizationσ6 Hþ e− → Hþ þ 2e− Ionizationσ7 Hþ e− → H2s þ e− Excitation to H2s stateσ8 H2s þ e− → Hþ þ 2e− Ionization from H2s stateσ9 Hþ

2 þ e− → 2H Dissociative recombinationσ10 Hþ

2 þ H → Hþ3 þ H Ion generation

σ11 Hþ3 þ e− → Hþ þ 2Hþ e− Dissociative excitation

σ12 Hþ3 þ e− → 3H Dissociative recombination

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been evaluated by replacing the electron temperature withthe ion temperature in Eq. (7). Consequently, the solutionof the nonlinear balance equation system (nHþ , nHþ

2, nHþ

3,

and τHþ) is a function of the input experimental para-meters ne, Te, NH, and NH2

. Since the input parametersare affected by experimental errors, Eq. (5) has beensolved within the whole interval [ne � Δne, Te � ΔTe,NH=NH2

� ΔðNH=NH2Þ]. This approach has allowed us to

evaluate the error bars of the solution of Eq. (5) and,therefore, the error of the estimated beam parameters.

C. Stage 3

The evaluation of the ion density in the previous stageenables us to evaluate the overall beam intensity and the ionspecies fractions.According to Eqs. (1) and (2), it is possible to estimate

the extracted current for any ion species as

IiðzÞ ¼ Iiðz ¼ 0Þ ¼ 1

2qπr2niviBohm: ð8Þ

The total extracted current Iextr is the sum of the partialcurrents:

Iextr ¼Xi

Ii: ð9Þ

Finally, the ion species fractions are estimated as

Hþð%Þ ¼ IHþ

Iextr;

Hþ2 ð%Þ ¼ IHþ

2

Iextr;

Hþ3 ð%Þ ¼

IHþ3

Iextr: ð10Þ

IV. COMPARISON BETWEEN EXPERIMENTALRESULTS AND CODE ESTIMATION

In this section, the extracted current and species fractionsestimated by the semiempirical approach are comparedwith the experimental results obtained on the PS-ESSproton source. Extracted beam characterization and OESmeasurements have been performed in the same workingconditions for a microwave power increasing from 150to 1200 W and a neutral pressure P ¼ 1 × 10−3 mbar.Unfortunately, for microwave power higher than 800 W,OES did not allow us to evaluate the NH=NH2

, due to a toosmall signal to noise ratio. For this reason, a complete set ofOES plasma parameters to be used as input in Eq. (5) wasavailable only in the range 150–800 W.The measured extracted current has been evaluated from

data in Fig. 4. Pulse stability ΔIpextr=Iextr during the 6 msinterval is always in the range 1%–4% for any value ofmicrowave power, while pulse to pulse stability ΔIp2pextr =Iextrdoes not overcome 2%. Therefore, the error on Iextr has

been evaluated asffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiðΔIpextr=IextrÞ2 þ ðΔIp2pextr =IextrÞ2

q.

The Doppler-shift unit gives a measurement of thespecies fraction averaged in 4 s, a time much higher thanthe duration of a single pulse. The comparison betweendifferent measurements, performed at constant microwavepower, shows a very high parameter stability and repeat-ability (<1%). Therefore, the error on the measurementof species fraction is negligible for the scope of thepresent paper.Figure 6 shows the comparison between the total

extracted current measured by ACCT and the value oftotal current estimated from the semiempirical approach.The value of extracted current is predicted with goodaccuracy in most of the experimental conditions. Figure 7shows the comparison between the species fraction

FIG. 5. Cross section of the 13 main reactions in a hydrogenplasma in the energy domain typical of MDIS [34].

FIG. 6. Comparison between the experimental value of ex-tracted current measured by ACCT and total current predicted bymeans of Eqs. (8) and (9).

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measured by the Doppler-shift measurement unitand the species fraction estimated by the semiempiricalapproach. Also in this case, a good prediction capabilityis found for a large part of the experimental values. Theresults are less accurate at higher power. A possible reasonis the decrease of the plasma electron temperature athigh power. This causes the Hþ

2 and Hþ3 generation and

destruction reactions (related to cross sections σ4, σ9, andσ12) to become more and more relevant with respect to theother reactions. Hþ

2 and Hþ3 generation and destruction

reactions depend on Tn and Ti, here assumed to beconstants. Consequently, any systematic error concerningthe value of Tn and Ti may play a role and negativelyaffect the results.The solution of the semiempirical balance equation

system gives, together with the beam species currents, alsoan estimation of the proton lifetime τHþ . To support thisresult, we made a theoretical estimation of the confinementtime expected in the PS-ESS proton source.In MDIS, the magnetic field of proton sources is almost

flat and does not confine particles. So, the confinement timeis mainly determined by the peculiar diffusion mechanismsof magnetized plasmas [1].In the presence of a magnetic field, particle diffusion

takes place via interaction with a self-generated electricfield, which modifies opportunely electron and ion lossfluxes to maintain the plasma quasineutrality [28].Two different diffusion mechanisms can arise: (i) Simon

diffusion.—A surplus of positive loss fluxes across themagnetic field is matched by a surplus of negative lossfluxes along the magnetic field. Surface currents, called theSimon currents, guarantee overall charge neutralization [35].

(ii) Ambipolar diffusion.—If Simon currents cannotflow due to insulated walls, positive and negative lossfluxes have to match along any diffusion direction, i.e.,either along and across the magnetic field [28,36]. Ithas been experimentally proven that ambipolar diffusionoptimizes MDIS performances [27].More informationabout plasma diffusion in ion sources can be found inRefs. [28,36].In PS-ESS, the injection and extraction sides of the

plasma chamber are constituted by two boron nitride disks,avoiding Simon currents to flow. Therefore, the ambipolardiffusion can be considered as the preferential diffusionmechanism [27]. Furthermore, according to Refs. [27,28],ambipolar diffusion across the magnetic field is negligiblewith respect to ambipolar diffusion along the magneticfield. Consequently, the proton confinement time inPS-ESS can be evaluated as the average time for protonsto diffuse from the position where they are generated to theextraction electrode along a flux tube of length L and radiusr under ambipolar diffusion conditions.In particular, for an ion generated at a distance x from

extraction, confinement time τðxÞ is [28]

τðxÞ ¼ x2

2Dambk

; ð11Þ

whereDambk is the ambipolar diffusion coefficient along the

magnetic field [28]. The evaluation of the mean confine-ment time requires one to average over all the possiblepositions where ions are generated. This treatment isbeyond the scope of the present paper. However, the twoextreme cases are considered. In the first case, we hypoth-esize that ions are generated homogeneously within thetube flux. In such a case, the average theoretical confine-ment time τtheor1Hþ is

τtheor1Hþ ¼Z

L

0

x2niπr2dx2Damb

1

niπr2L¼ L2

6Dambk

; ð12Þ

where niπr2dx is the number of ions in a circular slab ofwidth dx and radius r placed at distance x from the wallsand niπr2L is the total number of particles in the tube flux.In the second case, we hypothesize that ions are

generated mainly at the microwave injection, where theelectric field is larger and an ECR layer is placed [37]. Insuch a case, the confinement time is

τtheor2Hþ ¼ L2

2Dambk

: ð13Þ

It is reasonable that the real confinement τ time is includedin the range τtheor1Hþ < τ < τtheor2Hþ .Damb

k can be expressed as a function of the ion andelectron mobility coefficients μi and μe, respectively, and of

FIG. 7. Comparison between experimental values of the speciesfraction measured by Doppler-shift measurement unit and thevalues predicted by code.

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the electron and ion diffusion coefficients along magneticfield Dki and Dke:

Dambk ¼ μiDke þ μeDki

μi þ μe: ð14Þ

In proton sources, the largest part of the collisions inplasmas are long-range Coulomb scatters and ion-neutralcollisions (the latter include elastic and charge exchangecollisions) [1]. Consequently, μi, μe, Dke, and Dki can bewritten as [1]

μe ¼1

MeðνSpitzee þ νSpitzei Þ ;

μi ¼1

MiðνSpitzii þ νSpitzei þ νinÞ;

Dke ¼Te

MeðνSpitzee þ νSpitzei Þ ;

Dki ¼Ti

MiðνSpitzii þ νSpitzei þ νinÞ; ð15Þ

where νSpitzee , νSpitzii , and νSpitzei are the Spitzer collisionfrequencies for electron-electron, ion-ion, and electron-ion collisions, respectively; νin is the ion-neutral collisionfrequency. νSpitzee , νSpitzii , and νSpitzei are functions of ne, Te,and Ti and can be easily evaluated from the literature[1,28]. Figure 8 compares the code estimation τHþ obtainedas a solution of the balance equation system with τtheor1Hþ andτtheor2Hþ obtained by Eqs. (12) and (13).τHþ is between τtheor1Hþ and τtheor2Hþ for the largest part of the

values.

The good agreement between the results obtained bythe two different approaches supports the value of confine-ment time estimated by the semiempirical approach. τHþ

increases slightly from ∼10 μs at 180 W to ∼30þ35−15 μs at

800W. The percentage error increases also with microwavepower, and it is of the order of 100% at 600 and 800 W. Asin the case of the extracted current, the error is caused bythe error in the evaluation of the electron temperature byOES [26].

V. CONCLUSIONS AND PERSPECTIVES

This work introduces a semiempirical strategy aimed atthe estimation of the beam features from plasma param-eters. The balance equation system in a proton source hasbeen reduced and simplified by introducing experimentalplasma parameters as input parameters. In this work,plasma parameters have been measured by OES, whichallows an accurate and noninvasive measurement of ne, Te,and nH=nH2

. In particular, the solution of the balanceequation system has allowed estimating the total extractedcurrent, the species fractions, and the confinement timeunder a series of assumptions and hypothesis discussed inSecs. II A and II B. The comparison between the valuespredicted by the semiempirical approach and the exper-imental values measured on the PS-ESS source has shown asurprising agreement, although PS-ESS works in pulsedwaves. This result can be considered as a validation of thestrategy that underlies the semiempirical approach.A value of the proton confinement time, slightly increas-

ing from ∼10 to ∼30 μs with microwave power, is alsofound as a solution of the balance equation system. It hasbeen compared with two theoretical values of confinementtime in ambipolar diffusion conditions. Also in this case,the theoretical approach confirms the results of the semi-empirical approach.Therefore, we can state that the semiempirical approach

allows one to estimate with good accuracy the features ofthe beam generated by a MDIS proton source. Furtherimprovements can be obtained by including experimentalneutral and ion temperature within the input parameter set.Measurements of Tn and Ti can be performed by OES byusing a spectrometer with a FWHM of the order of 10 pm[11] (PS-ESS measurements were carried out with a 1 nmFWHM spectrometer [26]).The semiempirical approach requires also to be accu-

rately tested in continuous wave MDIS proton sources.Indeed, steady state working conditions allow one to reducethe number of approximations in Secs. II A and II B.In perspective, the semiempirical approach, applied in

synergy with OES diagnostics, could boost the R&D in thefield of MDIS proton sources. It could allow a real-time,cost-effective, and small footprint diagnostics of the beamproperties, also in the absence of an extraction system, andlead to an overall decrease of the beam commissioning timein proton accelerators.

FIG. 8. Proton confinement time τHþ estimated by the semi-empirical approach is supported by the comparison with the twoborderline values of theoretical confinement time. τtheor1Hþ < τHþ <τtheor2Hþ in the largest part of cases.

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ACKNOWLEDGMENTS

The support of the Ministero dell’Istruzione,dell’Universita e della Ricerca through the ESS-Miurexperiment is gratefully acknowledged. The contributionand suggestions of L. Neri, L. Celona, G. D’Agostino, andM. Mazzaglia have been essential for the preparation of thepresent work.

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