How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0...

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How much dust? And which dust? From grain-size data (and bulk density) to aeolian mass fractions Michael Dietze 1 1 - GFZ German Research Centre for Geosciences, Section 5.1 Geomorphology

Transcript of How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0...

Page 1: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

How much dust? And which dust?

From grain-size data (and bulk density)to aeolian mass fractions

Michael Dietze1

1 - GFZ German Research Centre for Geosciences, Section 5.1 Geomorphology

Page 2: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A (more or less) typical loess section

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 3: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A (more or less) typical loess sectionA (more or less) typical loess section

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 4: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A (more or less) typical loess sectionA (more or less) typical loess section

0.001 1 100

0.00.5

1.01.5

2.02.5

3.0

size(µm)

Vol.-

%

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 5: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A (more or less) typical loess sectionA (more or less) typical loess section

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 6: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A more conceptual formulation of the problem

dust(s)

other

proxi-mal

distalre-

mote

1. How much solid is there?

2. How much of it is "dust"?

3. Which types/sources are there?

4. What are its average densities?

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 7: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A conceptual estimate of potential consequences

0.001 1 100

0.00.5

1.01.5

2.02.5

3.0

size(µm)

Vol.-

%

"dust fraction" Cutting off at fixed boundaries may lead to:

- underestimation of the target fraction's total vol.-%

- contamination of the target fraction, by - tail(s) of coarser fractions - contribution of smaller fractions

- bias in the resulting time series of dust

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 8: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

5e−02 5e−01 5e+00 5e+01 5e+02

01

23

45

Grain size (µm)

Vol.−

%

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020

4060

8010

0

Time/sample IDR

elat

ive c

once

ntra

tion

A simple test of the contamination hypothesis – Setup A

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 9: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A simple test of the contamination hypothesis – Setup B

5e−02 5e−01 5e+00 5e+01 5e+02

01

23

45

Grain size (µm)

Vol.−

%

0 20 40 60 80 100

020

4060

8010

0

Time/sample IDR

elat

ive c

once

ntra

tion

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 10: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A simple test of the contamination hypothesis – Resulting mixed data sets

5e−02 5e−01 5e+00 5e+01 5e+02

01

23

45

Grain−size

Vol.−

%

5e−02 5e−01 5e+00 5e+01 5e+02

01

23

4

Grain−sizeVo

l.−%

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 11: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

A simple test of the contamination hypothesis – Resulting "dust" fractions (< 4 µm)

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0

Time/sample ID

Rel

ative

con

cent

ratio

n

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elat

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tion

true fraction

apparent fraction

true fraction

apparent fraction

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 12: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

One approach to tackling the problem – parametric curve fitting

5e−02 5e−01 5e+00 5e+01 5e+02

01

23

4

Grain−size

Vol.−

%

µ1, σ1, c1µ2, σ2, c2µ3, σ3, c3

Fitting n parametric distributions (log-normal, Weibull, Gamma, ...)

Attractive, because we get unmixed time se- ries and parametric end-member definition

But, for each sample we can get different µ, σ. So which one is the right one?

What if a sample has more than n compo- nents, or less?

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 13: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Another approach to tackling the problem – eigen space based decomposition (EMMA)

Considers an entire data set as input and describes it as linear combination of eigen vectors (V) and their scores (M) plus an error matrix (E).

Based on eigen space decomposition (PCA), extended to optimisation and reduction (FA), framed by scaling to real units (EMMA).

Attractive, because we get unmixed time series and unconstrained end-member definition

MX

V

X = M V + E• T

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 14: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Another approach to tackling the problem – eigen space based decomposition (EMMA)

Lumi-nescence

RLumModel

BayLum

ADmin

sandbox EMMAgeo PUMAgeo

RLumShiny

rbacon

Basic and advanced data analysis

Luminescence model implementation

Bayesian age calculations

Bayesian age depth models

Advanced age data visualisation

Age error type separation

Virtual sediment section modelling

Compositional data analysis

Age-depth to proxy uncertainty propagation

Bchron

clam

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 15: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Another approach to tackling the problem – eigen space based decomposition (EMMA)

FAPCA

EMMA

Online course: micha-dietze.de/pages/r_courses.html

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 16: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Another approach to tackling the problem – eigen space based decomposition (EMMA)

0 5 10 15

0.0

0.4

0.8

Class−wise explained variance (mean = 89 %)

Class

R2

0 20 40 60 80 100

0.85

0.95

Sample−wise explained variance (mean = 97 %)

Samples

R2

0 5 10 15

01

23

45

67

End−member loadings

Class

Rel

ative

am

ount

s

5 15 25 35 45 55 65 75 85 95

End−member scores

Samples

Rel

ative

am

ount

s

0.0

0.2

0.4

0.6

0.8

1.0

End−member ID (mode position | explained variance)EM1 (6.1 | 23 %) EM2 (4.7 | 19 %) EM3 (1.6 | 30 %) EM4 (1 | 28 %)

0 5 10 15

0.0

0.4

0.8

Class−wise explained variance (mean = 89 %)

Class

R2

0 20 40 60 80 100

0.70

0.85

1.00

Sample−wise explained variance (mean = 93 %)

Samples

R2

0 5 10 15

01

23

45

67

Robust end−member loadings

Class

Rel

ative

am

ount

s

Robust end−member scores

Samples

Rel

ative

am

ount

s pe

r end

−mem

ber

0 20 40 60 80 100

00

00

End−member ID (mode position | explained variance)EM1 (64 | 14 %) EM2 (74 | 27 %) EM3 (98 | 26 %) EM4 (100 | 33 %)

Deterministic mode ("I know the number of components") Robust mode ("I fully allow for parameter uncertainty")

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 17: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 18: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 19: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 20: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 21: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 22: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 23: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 24: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

Let's apply the technique – Welcome to a special kind of dusty deposit

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 25: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

So?... Some recapitulation ... And a look ahead

Aeolian deposits usually comprise a mixture of components from different sources, transport pathways and transport processes, and have undergone syn- and postdepositional alteration.

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 26: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

So?... Some recapitulation ... And a look ahead

Aeolian deposits usually comprise a mixture of components from different sources, transport pathways and transport processes, and have undergone syn- and postdepositional alteration.

Simple, subjectively defined size boundaries inevitably introduce bias, which is why we need robust approaches to unmixing data into inhertent components.

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 27: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

So?... Some recapitulation ... And a look ahead

Aeolian deposits usually comprise a mixture of components from different sources, transport pathways and transport processes, and have undergone syn- and postdepositional alteration.

Simple, subjectively defined size boundaries inevitably introduce bias, which is why we need robust approaches to unmixing data into inhertent components.

After a decision which components represent the "dust fraction(s)" of interest, it is crucial to investigate the spatial heterogeneity (or spatial autocorrelation function of the data).

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 28: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

So?... Some recapitulation ... And a look ahead

Aeolian deposits usually comprise a mixture of components from different sources, transport pathways and transport processes, and have undergone syn- and postdepositional alteration.

Simple, subjectively defined size boundaries inevitably introduce bias, which is why we need robust approaches to unmixing data into inhertent components.

After a decision which components represent the "dust fraction(s)" of interest, it is crucial to investigate the spatial heterogeneity (or spatial autocorrelation function of the data).

With spatially "scaled" volume percentages of distinct dust fractions, one can engage with i) removing the non-solid volume fractions (water, air), ii) propagating solid volumes to age-depth-space, and iii) robustly estimating size- and component-specific material density, to produce mass deposition rates.

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 29: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

So?... Some recapitulation ... And a look ahead

Aeolian deposits usually comprise a mixture of components from different sources, transport pathways and transport processes, and have undergone syn- and postdepositional alteration.

Simple, subjectively defined size boundaries inevitably introduce bias, which is why we need robust approaches to unmixing data into inhertent components.

After a decision which components represent the "dust fraction(s)" of interest, it is crucial to investigate the spatial heterogeneity (or spatial autocorrelation function of the data).

With spatially "scaled" volume percentages of distinct dust fractions, one can engage with i) removing the non-solid volume fractions (water, air), ii) propagating solid volumes to age-depth-space, and iii) robustly estimating size- and component-specific material density, to produce mass deposition rates. Thanks

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 30: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries

DARTDust Accumulation Rate Tackling

Thanks

THE PROBLEM | ONE SOLUTION | ANOTHER SOLUTION | APPLICATION | SYNTHESIS

Michael Dietze @ GFZ Potsdam > Geomorphology Section > Sediment unmixing > Workshop on dust mass accumulation rates

Page 31: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries
Page 32: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries
Page 33: How much dust? And which dust? · A conceptual estimate of potential consequences 0.001 1 100 0.0 0.5 1.0 1.5 2.0 2.5 3.0 size(µm) Vol.-% "dust fraction" Cutting off at fixed boundaries