EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei...

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EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80

Transcript of EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei...

Page 1: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Collaboration NIPNE Bucharest -- LSF LN Legnaro

Studies of N≈Z nuclei above mass 80

Page 2: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

M.Axiotis1, D.Bazzacco2, D.Bucurescu3, G. de Angelis4, E.Farnea2, A.Gadea4, M.Ionescu-Bujor3, A.Iordǎchescu3, W.Krolas5, Th.Kröll6, S.Lenzi2, S.Lunardi2, N.Mǎrginean3,4, T. Martinez4, R.Menegazzo2, D.R.Napoli4, P.Pavan2, B.Quintana7, C.Rossi Alvarez2, C.Rusu3,4, P.Spolaore4, C.A.Ur2,3,

J. Wrzesinski5

recent youngs: C. Mihai3, G. Suliman3

[1] - N.R.C. Demokritos Athens[2] - Università Padova[3] - H.H.-NIPNE Bucharest[4] - INFN, L.N. Legnaro[5] - H.N. – INP Krakow[6] - T.U. München[7] - Universidad Salamanca

The collaboration

Page 3: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Short history of collaboration: Since 1990, γ-ray spectroscopy with fusion-evaporation reactions, first with GAMIPE, then with

GASP. (NIPNE-INFN collab. agreement; since 2000: LSF-TRM)

• High-spin states in different nuclei• Highly-deformed & SD structures (decay out, lifetimes, A≈130)• Spectroscopic studies of nuclei in the exotic region N≈Z, A=80-90• Static moments of isomeric states in exotic nuclei• Spectroscopy of n-rich nuclei with CLARA- PRISMA

Page 4: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Topics(prompt γ-ray spectroscopy of N≈Z nuclei above mass

80)

• T=0 np pairing• Spin-gap isomers• Shell model description• Evolution of collectivity

Page 5: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Experimental Studies of “heavy” N≈Z Nuclei

Production• Fusion-evaporation• Fragmentation

Identification Coincidence with evaporated

particles Direct A and Z measurement

Low cross sections(with stable beams)

High ‘background’

10-5 10-4 10-3 10-2 10-1 100

88Ru 2n

88Tc pn87Tc p2n

88Mo 2p87Mo 2pn

86Mo 85Mo n

87Nb 3p85Nb p

84Nb pn

84Zr 2p82Zr

Relative Yield

Ancillary detectors

γ-ray SpectroscopyGe arraysBeta-decay studies

32S+58Ni, 105 MeV

Charged particle ballsNeutron arraysMass spectrometers

Page 6: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Experimental Facilities

GASP

GASP (config. 1)abs (40 HPGe) 3%

Peak/Total 60%

abs (80 BGO) 76%

ISIS (40 ΔE-E Silicon

telescopes)

p 56-60%

35-38%

N-Ringn 2-5%

Beam

Page 7: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007 p-drip line: G.A.Lalazissis et al, Nucl. Phys. A719,209c(2003): Relativistic HB calc.

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EWON – Prague May 10, 2007

N. Mărginean et al. Phys. Rev. C 63 (2001) 032303(R)

N. Mărginean et al. Phys. Rev. C 65 (2002) 051303(R)

Page 9: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

New data:

72Kr : C.Andreoiu et al., Phys. Rev. C75(2007)041301(R)

76Sr : P.J.Davies et al., Phys. Rev. C75(2007)011302(R)

No evidence for isoscalar (T=0) np pair field

isovector mean-field theory OK (isovector np pairing + isospin symmetry conservation) [ Afanasjev & Frauendorf, PRC71(2005)064318 ] (CRHB calculations)

Signature of T=0 np pairing ?Delayed Alignment in N=Z Nuclei:

J=0 T=1

J=1…2j T=0

Page 10: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Projected Shell Model Calculations

N. Mărginean et al. Phys. Rev. C 65 (2002) 051303(R)

Page 11: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

N=Z+1

81Zr

Experiment: 28Si(90 MeV) + 58NiTarget: 2 x 0.5 mg/cm2 58Ni 81Zr - αn channel, intensity 2·10-4

N. Mărginean et al. Phys. Rev. C 69 (2004) 054301

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EWON – Prague May 10, 2007

N=40[422]5/2

[301]3/2[431]1/2

1 neutron hole + 82Zr

N=40[422]5/2

[301]3/2[431]1/2

1 neutron particle + 80Zr

Fermi

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EWON – Prague May 10, 2007

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Projected Shell Model Calculations

(empty symbols)

N. Mărginean et al. Phys. Rev. C 69 (2004) 054301

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EWON – Prague May 10, 2007

E3 isomeric

decay

95Ag

τisomer > ≈ 1 μs

[predicted by Ogawa, Phys.Rev. C28,958(1983)]

Page 16: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Shell Model Effective Interactions

SLGT0 - Serduke, Lawson, Gloeckner, NPA256(1976)45;

Herndl, Brown, NPA605(1996)195 A>86, N,Z=[38-50] π,υ(2p1/2,1g9/2)

Gross-Frenkel - Gross, Frenkel, NPA267(1976)85

F-FIT, … - Johnstone, Skouras, EPJA11(2001)125 (fit to increased number of exc. energies in mass 86-100 nuclei)

Other SM calculations: Hasegawa et al., P+QQ Hamilt., (2p1/2,1g9/2,1f5/2,2p3/2 ) (88,89,90Ru)

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ν,π(p1/2,g9/2)SLGT0 resid. inter.

C. Rusu et al , Phys. Rev. C 69 (2004) 024307

N.Mǎrginean et al, Phys. Rev. C67(2003)061301(R)

Page 18: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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2.86

2.0 2.25

2.75

2.5

2.0

2.25

1.75

1.5

2.30

2.52

2.84

2.5

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EWON – Prague May 10, 2007

(F. Iachello

Phys. Rev. Letters 85 (2000) 3580)

134Ba

(F. Iachello

Phys. Rev. Letters 87 (2001) 052502)

152Sm

Unharmonic vibrator

Stable quadrupole deformation

-soft

rotor

Axially symmetric

rotor

Shape phases, phase transitions and critical points

Critical points: parameter-free analytical approximations

Page 20: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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Prediction of X(5) nuclei

4.5 < NpNn/(Np+Nn) < 5.5

N=Z = 38,40

(N.V. Zamfir, private comm.)

Page 21: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

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Quasi- bands identified or extended in

78Sr, 80Sr, 82Zr, 84Zr, 86Zr, 86Mo, 88Mo

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Phase Transition in IBA Triangle

2]

~[~~

41

ddsddsQ

LLQQN

naH dIBA

0+

2+

4+ 2+

3+

4+

Fine grid on parameter space

2 merit function including both energy and branching ratios

New parameters:2/7

2/71

1

yx

*

*

82Zr80Sr

78Sr

Page 24: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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Conclusions• N≈Z nuclei, mass 80 - 100: theatre of many interesting nuclear structure phenomena

• First spectroscopic measurements of the heaviest known N=Z (88Ru) and N=Z+1 (81Zr, 85Mo, 89Ru, 91Rh, 93Pd,95Ag) nuclei.

• ”Systematic delay” in alignment frequency in N=Z even-even nuclei. Is it “abnormal”? (T=0 neutron-proton pairing?) need for: - measurements at higher spins; - direct determinations of: s.p. energies, deformations.

• Deformed Odd-A (N=Z+1) nuclei: rich information (more bands) - possible delayed alignment observed. Implications for the N=Z core? (polarization of the mean-field; the T=1 pair field induced by additional neutron in 81Zr).

Page 25: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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• Evolution of the Collectivity: maximum of collectivity (deformation) around N,Z=38,40 but still far from ideal rotor; X(5) “island”? (new “indicators” needed for 76,78Sr, 80Zr, (78Zr) )

• Extensions of these data are necessary (in spin: e.g.,88Ru to higher states; in mass: 92Pd; N=Z+1 nuclei).

• Shell model (Z≥44; N≥45): old residual interactions (SLGT0, GF, JS) in (p1/2,g9/2) space perform reasonably well. Isomers explained. But: yrast π = + (g9/2) states are not so sensitive – not critical tests!

• Exceptional support within LSF LN-Legnaro; full use of the capabilities of GASP and its ancillaries: ISIS and N-wall.

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END

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EWON – Prague May 10, 2007

Page 28: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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Reaction Target Beam intens.

(8+), [pnA]

Trigger

condition

28Si (90 MeV) +

58Ni

2 x 0.5 mg/cm2

142Ge,2BGO

32S (105 MeV) +58Ni

1.1 mg/cm2

62Ge,3BGO

40Ca(130MeV)+ 54Fe

6.5 mg/cm2

4 - 62Ge,1BGO

40Ca(135MeV)+ 58Ni

6.0 mg/cm2

82Ge,1BGO

GASP experiments

Page 29: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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Reaction Channel Studied

Nucleus σ σ (% σF) Status

28Si+58Ni90 MeV

2n 84Mo ~ 7 μb ~ 4 10-5 1 γ known

before

αn 81Zr ~ 0.3 mb ~ 2 10-4 unknown

32S+58Ni105 MeV

2n 88Ru 5-10 μb ~ 4 10-5 unknown

αn 85Mo 0.13 mb 7 10-4 unknown

40Ca+54Fe130 MeV

αn 89Ru ~ 40 μb ~ 1-2 10-4 unknown

p2n 91Rh ~ 65 μb ~ 2-3 10-4 unknown

40Ca+58Ni135 MeV

αn 93Pd unknown

p2n 95Ag unknown

PR C56,2497(1997)PR C65,051303R(2002)

PR C61,024310(2000)PR C69,054301(2004)

PR C63,031303(2001)

PR C65,0334315(2002)

PR C70,044302(2004)

PR C72,014302(2005)

PR C69,024307(2004)

PR C67,061301R(2003)

Simultaneous publications: 93Pd: D.Sohler et al., EPJ A19,169(2004) 95Ag: J.Döring et al., PR C68,034306(2003)

Page 30: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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~ Grodzins estimate β2 ~ A-7/6E(2+)-1/2

Page 31: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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M.Hasegawa et al., Phys. Rev. C69,034324(2004)

Shell model, P+QQ Hamiltonian, (1g9/2,2p1/2,1f5/2,2p3/2)-N

max. dimens. for 88Ru (N=12): 165 x 106

Strengthened isoscalar QQpn interaction

Page 32: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Identification of

N=Z: 88Ru

Experiment: 32S(105 MeV) + 58Ni– Target: 1.1 mg/cm2 58Ni on 10 mg/cm2 Au– 88Ru populated as 2n channel, intensity 4·10-5

– Four gamma-ray cascade identified by coincidence with neutrons and anticoincidence with charged particles

Sum of gates 616 + 800 +964 keV:

GASP + ISIS + 6 n-detectors

N. Mărginean et al. Phys. Rev. C 63 (2001) 031303(R)

Matrix projection

Page 33: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

τisomer > ≈ 1 μs

N=Z+1, 9547Ag48 approaching N,Z=50 : spin gap isomer

N. Mărginean et al. Phys. Rev. C 67 (2003) 061301(R)

1p2n channel predicted Ogawa PR C28,958(1983)

Page 34: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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Page 35: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

Estimate for the alignment frequency of 80Zr

Missing alignment

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EWON – Prague May 10, 2007

Page 37: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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JΠ Ex (keV) SLGT0 GF F-FIT

(9/2+) 0 0 0 0

(13/2+) 840 112 22 56

(17/2+) 1787 48 -116 -42

(21/2+) 2655 -81 -308 -226

(25/2+) 3103 -75 -316 -241

(29/2+) 4136 -1 -365 -245

(1/2-) 173 112 186

(5/2-) 792 195 330 187

(9/2-) 1292 258 368 208

(13/2-) 1905 82 168 2

(17/2-) 2278 97 190 46

EXP. Ecalc. - Eexp. (keV)

91Rh – comparison with 3 Shell Model calculations

Page 38: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

91Rh

Johnstone-Skouras (2001) – F-FIT eff. inter.

πυ(2p1/21g9/2)

N. Mărginean et al. Phys. Rev. C 72 (2005) 014302

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(preliminary)

Page 40: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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General structure of a collective nucleus:Basic information on:

g.s.b. 02

+ - band (quasi-beta band)

2γ+ - band (quasi-gamma band)

Energy ratios: E(41+)/ E(21

+); E(02+)/E(21

+); E(2γ+)/E(21

+); etc.

Elmag. trans. Probab.: B(E2; 2γ --> 01)/ B(E2; 21 --> 01);

B(E2; 2γ --> 01)/ B(E2; 21 --> 21); etc.

Ex.: U(5) R(4/2) = 2.0 R(02+/21

+) = a (~2) R(22+/21

+) = a (~2)

O(6) 2.5 a (>~2.0) a (>~2.0)

SU(3) 3.33 a (>~12) a (>~12)

X(5) 2.91 5.67 4.23

E(5) 2.19 3.03 2.20

a = depends on additional Hamiltonian parameters

Page 41: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

56Ni + 40Ca ---> 88Ru + 2α

88Ru cross-sections : with 56Ni beam : ~ 30 mb with 32S beam: 5-10 μb --------------------------------------- R ~ 3 x 103 (56Ni/32S)

Beam 56Ni : [~ 3 x 107 ions/sec (2003, ANL)] ------→ ~ 1011 (FAIR)

Beam 32S (GASP): ~ 6 pnA ≈ 4 x 1010 ions/sec ----------------------------------------

R ~ 1 (56Ni/32S)

Overall gain with 56Ni : ~3000 (assuming GASP (3%) γ-efficiency and same target !) with Ge-array of increased efficiency :

gain >> ~ 3000 !

N=Z 88Ru with RIB:

Page 42: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

S.Takami et al., Phys. Lett. B431,242(1998)M.Yamagami et al., Nucl Phys. A693,579(2001)J.Dudek et al., Phys. Rev. Lett. 88,252502(2002)

Exotic deformation: ~ 80Zr : tetrahedral deformation (spin-gap isomers?)

Page 43: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

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23/2+

N=Z+1; odd-Z

Page 44: EWON – Prague May 10, 2007 Collaboration NIPNE Bucharest -- LSF LN Legnaro Studies of N≈Z nuclei above mass 80.

EWON – Prague May 10, 2007

N=Z+1; even-Z