Civil Aviation Alternate Fuels Contrails and Emissions ...

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Aerospace Civil Aviation Alternate Fuels Contrails and Emissions Research – Operations and Contrail Observations LR-FRL-2018-0013 A P Brown, M Bastian, F Femia, M Salib, F Ghatala, J Olfert, R Beunis, M Valk and N Gaudet Flight Research Laboratory

Transcript of Civil Aviation Alternate Fuels Contrails and Emissions ...

Aerospace

Civil Aviation Alternate Fuels

Contrails and Emissions Research –

Operations and Contrail

Observations

LR-FRL-2018-0013

A P Brown, M Bastian, F Femia, M Salib, F Ghatala, J Olfert,

R Beunis, M Valk and N Gaudet

Flight Research Laboratory

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Table of Contents

Table of Figures .............................................................................................................................. 4

Abbreviations .................................................................................................................................. 8

Abstract ......................................................................................................................................... 11

1.0 Introduction ............................................................................................................................. 12

2.0 CAAFCER consortium operational responsibilities ............................................................... 12

3.0 SkyNRG HEFA biofuel acquisition and blending .................................................................. 13

4.0 Air Canada CAAFCER flight operations ............................................................................... 13

4.1 Flight operational period ..................................................................................................... 13

4.2 Air Canada flight procedures .............................................................................................. 13

4.3 Air Canada flight listing ...................................................................................................... 14

4.4 Wing-tank fuel samples....................................................................................................... 15

4.5 Flight profile & data ............................................................................................................ 15

4.6 Supplemental flight details .................................................................................................. 15

5.0 University of Alberta calibration operations........................................................................... 16

5.1 Particle Loss estimations ..................................................................................................... 16

6.0 NRC CT-133 flight operations................................................................................................ 17

6.1 NRC CT-133 Research Aircraft and Instrumentation......................................................... 17

6.2 CAAFCER NRC CT-133 flights......................................................................................... 19

7.0 A data overview and examples of CAAFCER contrail flight data ......................................... 21

7.1 General ................................................................................................................................ 21

7.2 Atmospheric influence ........................................................................................................ 21

7.3 Data analysis ....................................................................................................................... 21

7.3.1 General.......................................................................................................................... 21

7.3.2 Spatial re-construction .................................................................................................. 21

7.3.3 Time-trace analysis ....................................................................................................... 22

7.4 25th April flight .................................................................................................................... 23

7.4.1 Biofuel contrail ............................................................................................................. 23

8.0 Contrail Video Imagery .......................................................................................................... 24

8.1 Biofuel contrail, 3rd May flight ........................................................................................... 24

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8.2 Jet A1 contrail, B763, 3rd May ............................................................................................ 26

8.3 Biofuel contrail, A320, 4th May, afternoon flight ................................................................ 27

8.4 Jet A1 contrail, A320, 11th May .......................................................................................... 31

9.0 Data review and analysis......................................................................................................... 34

9.1 Data example, biofuel contrail, 25th April 2017.................................................................. 34

9.1.1 Inertial and Air data ...................................................................................................... 34

9.1.2 Wake vortex data .......................................................................................................... 34

9.1.3 Dynamic phase, contrail length 10-17 km .................................................................... 37

9.1.4 Biofuel contrail, 25th April 2017, 18-26 km length ...................................................... 44

9.1.5 Biofuel contrail, 25th APRIL 2017, 27-37 km length ................................................... 49

9.1.6 Biofuel contrail, 25th APRIL 2017, 37-50 km .............................................................. 53

9.1.7 Biofuel contrail, 25th APRIL 2017, 50-55 km length ................................................... 57

9.2 Overview, assembly & comparison, CN data ..................................................................... 61

9.2.1 Biofuel contrail, 25th April, to 55 km length ................................................................ 61

9.2.2 Contrail FSSP data assemblage .................................................................................... 62

10.0 Conclusions ........................................................................................................................... 64

11.0 Acknowledgements ............................................................................................................... 65

12.0 References ............................................................................................................................. 65

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Table of Figures Figure 1. NRC CT-133 research jet, equipped with contrail and emissions measurement sensors; strike -through text depicts the configuration changes of successive sensor developmental cycles – text in red (2016ff) depicts CAAFCER configuration. Figure 2 – CAAFCER inflight pictures of contrail states, left, slanted-veil state, and right, laterally-spreading crown of cirrocumulus character. Figure 3 – top, left to right, typical contrail cross-section, and vertical distribution of ice particles; mid, left to right, ice particle size spectra, bottom, left to right, MED contrail cross-section, behaviour of MED with contrail length. Figure 4 – plot of CAAFCER contrail AEIn7 values, for the FSSP-100 against CN, CPC & CPCnv values. Figure 5 – plot of all contrail AEIn values, derived from contrail cross-sections, measured by the NRC CT-133, and compared to CN EIn. Figure 6 – plot of nvPM EIm against total hydrogen content (normalised by 15.3%) for five jet fuels tested in the altitude chamber of the Gas Turbine Lab of the NRC1; curve-fit is the variation nvPM EIm ~ (total hydrogen)-27.9. Figure 7 – plot of contrail FSSP-100 AEIn against total hydrogen content; ordinate direction spread includes the effect of variations in atmospheric conditions, such as RH iice, individual aircraft, engines, power settings+3%; the log-log linearization shown is for CAAFCER JetA1 and ACCESS II Jet A and HEFA-blend., resulting in a power index of -36. Figure 8 – plot of normalised emitted PM EIn against sulphur content, estimated from Aerodyne/NASA data2. Figure 9(a) –trailing vortex pair core passages at 11 km wake length, plotted against crossplane

projection of the CT-133 flight-path (this data was used for the open path integral of Figure 8)..

Figure 9(b) – re-constructed cross-plane view of trailing vortex pair (of Figure 9(a)), observed in the signature of induced vertical wind: showing the relatively large-scale of the vortices and relatively short distance between vortex cores, approximately 10 metres.

Figure 10 – plot of CAAFCER & ACCESS II NRC data of FSSP-100 AEIn against atmospheric temperature. Figure 11 – plot of CAAFCER & ACCESS II NRC data of FSSP-100 AEIn against atmospheric RHICE Figure 12 – plot of CAAFCER & ACCESS II NRC data of FSSP-100 AEIn against atmospheric RH lapse rate,

RH/z.

Figure 13 – plots of ARH/zaTSbRHice

c = log10[FSSP EIn], identifications for each of the two separate fuel type CAAFCER contrail data-sets (ACCESS data is not included in the statistical identification, merely presented for comparison).

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Figure 14 – plot of ARH/zaTSbRHice

c identified separately for each of the two fuel types, against contrail cross-section data-point age Figure 15 – plots of CAAFCER & ACCESS II NRC data of FSSP-100 AEIm against atmospheric temperature

TS, RH lapse rate RH/z and relative humidity over ice RHICE.

Figure 16 – plots of log-normal (by 108 µg/kg) ARH/zaTSbRHice

c = log10[FSSP AEIm], identifications of contrail spherically-assumed ice-mass, for each of the two separate fuel type contrails Figure 17 – plot of ARH/zaTS

bRHicec identified separately for each of the two fuel types, against contrail

cross-section data-point age. Figure 18 – contrail ice particle spectra, FSSP-100, in homogenous sections of the contrail, at various contrail lengths:- top, left to right, 15 nm, 18 nm, 22 nm; bottom, left to right, 35 nm, 45 nm Figure 19(a) – contour crossplane plots of contrail FSSP-100 ice particle spectral MED (43%HEFA contrail, 3rd May 2017), showing size growth in the UJW and sublimation in the TWV regions over increasing contrail length:- top, left to right, 8 nm, 12 nm; bottom, left to right, 15 nm, 18 nm. Figure 19(b) – contour crossplane plots of contrail FSSP-100 ice particle spectral MED (Jet A1 contrail, 3rd May 2017), showing size growth in the UJW and sublimation in the TWV regions over increasing contrail length:- top, left to right, 123nm, 16 nm; bottom, left to right, 19 nm, 22 nm. Figure 20 – plots of median MED for each contrail cross-sections, plotted against top left, contrail age (and along-track spatial changes) and atmospheric parameters, top right, TS, bottom left, RHice, bottom

right, RH/z. Figure 21 – plots of identified power-law parametric variations of contrail cross-section median MED with atmospheric properties, for the two fuel types used on CAAFCER, Figure 22 – CAAFCER #1, 18-27 km contrail cross-sections, biofuel nvPM CPC3776 >2.5 nano-m (left) and CN 7610 >10 nano-m CN (right) concentration. Figure 23 – CAAFCER #1, 18-27 km contrail cross-section lateral integrations, biofuel nvPM CPC3776 >2.5 nano-m (left) and CN 7610 >10 nano-m CN concentration (right). Figure 24 – CAAFCER #1, 18-27 km contrail, biofuel, ratio of FSSP ice particle count density to nvPM particle count, with contrail length (left) and a contrail cross-sectional contour plot (right). Figure 25 – CAAFCER #1, 18-27 km contrail cross-section and lateral integration, CO2 plume. Figure 26 – CAAFCER #1, 18-27 km contrail cross-section and lateral integration, BC plume. Figure 27 – CAAFCER #1, 18-27 km contrail cross-section and lateral integration, ice-mass, assuming sphericity. Figure 28 – CAAFCER #1, 18-27 km contrail cross-sectional MED distribution (left) and behaviour of MED with contrail length (right).

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Figure 29 – CAAFCER #1, 18-27 km contrail cross-sections of RH (left) and RHi (right). Figure 30 – CAAFCER #1, 27-37 km contrail cross-section of CN and lateral integrand distribution Figure 31(a) – CAAFCER #1, 27-37 km contrail cross-section of CPC3776 PM and lateral integrand distribution. Figure 31(b) – CAAFCER #1, 27-37 km contrail cross-section of CO2 and lateral integrand distribution. Figure 32 – CAAFCER #1, 27-37 km contrail cross-section of FSSP-100 ice particles and lateral integrand vertical distribution thereof. Figure 33 – CAAFCER #1, 27-37 km contrail cross-sectional distribution of ice particle MED. Figure 34 – CAAFCER #1, 27-37 km contrail cross-sections of RH (left) and RHi (right). Figure 35 – CAAFCER #1, 37-50 km contrail cross-section of CN and lateral integrand, vertical distribution. Figure 36 – CAAFCER #1, 37-50 km contrail cross-section of CPC3776 nvPM and lateral integrand, vertical distribution Figure 37 – CAAFCER #1, 37-50 km contrail cross-section of CO2 and lateral integrand, vertical distribution Figure 38 – CAAFCER #1, 37-50 km contrail cross-section of BC and lateral integrand, vertical distribution. Figure 39 – CAAFCER #1, 37-50 km contrail cross-section of ice particles and # lateral integrand, vertical distribution Figure 40 – CAAFCER #1, 37-50 km contrail cross-section of MED. Figure 41 – CAAFCER #1, 37-50 km contrail nvPM/FSSP activation (left) and re-constructed cross-section of the activation (right). Figure 42 – CAAFCER #1, 37-50 km contrail cross-sections of RH (left) and RHi(right). Figure 43 – CAAFCER #1, 50-55 km contrail cross-section of CN aerosol # (left) lateral integrand, vertical distribution (right). Figure 44 – CAAFCER #1, 50-55 km contrail cross-section of CPC total ultrafine aerosol # ( left) lateral integrand, vertical distribution (right). Figure 45 – CAAFCER #1, 50-55 km contrail cross-section of CO2 (left) lateral integrand, vertical distribution (right).

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Figure 46 – CAAFCER #1, 50-55 km contrail cross-section of BC (left) lateral integrand, vertical distribution (right). Figure 47 – CAAFCER #1, 50-55 km contrail cross-section of ice particle count (top left) lateral integrand, vertical distribution (top right), and MED cross-section (bottom left). Figure 48 – CAAFCER #1, 50-55 km contrail cross-sections of RH (left) and RHi (right). Figure 49 – CAAFCER #1, biofuel contrail assembly and comparison of CN EIn data, plotted against cruise altitude, with that of other flight campaigns. Figure 50 – CAAFCER #1, biofuel contrail assembly and comparison of CN EIn data, plotted against engine EGT/TS, a measure of engine thrust level. Figure 51 – CAAFCER #1, biofuel contrail FSSP-100 AEIn, (top) and spherical-AEIm (bottom), cross-plotted against cruise altitude, and compared with AEIn of other contrails measured by the NRC CT-133 upon earlier flight campaigns. Figure 52 – CAAFCER #1, biofuel contrail FSSP-100 AEIn, cross-plotted against CN aerosol EIn and compared with AEIn ~ CN EIn of other contrails measured by the NRC CT-133 upon earlier flight campaigns.

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Abbreviations

ACA Air Canada flight ACCESS II NASA project Alternativee Fuel Effects on Contrails &

Cruise Emissions, Phase II

ADS Air data system AEIn Apparent Emissions Index of contrail ice particle number

per kg of fuel burned, for ice particles >0.5µm in size as measured by the NRC CT-133 FSSP-100 probe

ASTM D7566 Standard Specification for Aviation Turbine Fuel of the

American Society for Testing & Materials ATC Air traffic control

bv Lateral separation of the trailing vortex pair BC Black carbon particles (soot) BL-NCE Business Led Network of Centres of Excellence

CAAFCER Civil Aviation Alternate Fuel Contrails and Emissions Research

CN 7610 Condensation nuclei counter, model 7610, counting aerosol particles of greater than 10 nano-metres, in size

CPC 3776 Condensation particle counter, model 3776 operated on a

sheath airflow principle, to count ultrafine particles of greater than 2.5 nano-metres, in size

CT-133 NRC research jet aeroplane DAS Data acquisition system DND Department of National Defence of Canada

ECCC Environment and Climate Change Canada EI or EIm Emission Index by mass per kg fuel burned

EIn Number Emission index by number per kg of fuel burned FIRNS FRL inertial reference and navigations system (integrated

HG1700 IMU, Novatel GPS and DRP system)

FL Flight level, aircraft altitude in 100 feet units above sea level, e.g., F300=30,000 feet altitude

FMS Flight management system FSSP-100 Forward scattering spectrometric probe -100 part number

sizing 0.5-47 µm

GARDN Green Aviation Research & Development Network, a non-profit organization funded by the Business-Led Network of

Centres of Excellence (BL-NCE) of the Government of Canada and the Canadian aerospace industry

HAARC NRC High altitude atmospheric research capability

HEFA Hydro-processed Esters and Fatty Acids LOF Line of flight

LVW Lower viscous wake (wake regime below the TWV) M Mach Number MED Median effective diameter – the spherical ice particle

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diameter equating to the 50th percentile of the FSSP-100 cumulative volumetric distribution of the particle size

spectrum MFC Mass-flow controller

MLE Maximum likelihood estimator NOx Total NO, NO2, and HONO compounds, measured by full

conversion to NO2 by the Thermo 42I analyser one sample

per twenty seconds in this mode, which is not used on the CAAFCER project

NOy Nitric oxides measured by the Thermo 42I analyser, operating in 1 Hz streaming mode (i.e. incomplete conversion), ref. para 5.1.5

NRC National Research Council of Canada N1 Engine gas generator rotational speed (%)

nm Nano-metres Nm Nautical miles NMR Nuclear magnetic resonance measurement of total

hydrogen content nvPM Non-volatile particulate matter (such as black carbon)

PDP NRC particle detection probe PIREP Pilot report of inflight conditions of icing, turbulence, air

temperature

PM Particulate matter emissions PS Atmospheric static air pressure

PT Atmospheric total air temperature QAR Quick access recorder, part of the aircraft flight data

recorder

QETE Quality Engineering Test Establishment of the Department of National Defence

RH Relative humidity RHice RH over ice TAT Total air temperature

TGT Engine turbine gas temperature THC Total hydrogen content

TOPC Top of climb TOPD Top of descent TS Static air temperature

TWV Trailing wake vortex crossplane flow region UofA The University of Alberta

UJW Upper jet wake; generally the UJW in cross-sectional shape is a ‘T’, the lateral being the UJW crown, the vertical being the UJW stem, and the foot being the TWV region.

UTLS Upper troposphere lower stratosphere V True airspeed

vPM Volatile particulate matter WV Trailing pair of wake vortices

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wa Vortex-induced velocity component in the contrail axial direction, [x]

wC Vortex-induced velocity component in the contrail crossplane, or lateral, direction [y]

wZ Vortex-induced velocity component in the contrail normal direction [z]

YOW Ottawa Airport

YUL Montreal Pierre Elliott Trudeau Airport YVO Val d’Or Airport, Quebec

YYZ Toronto Pearson Airport Contrail axis system:

[x] Projection of the CT-133 mean LOF axis direction onto the horizontal plane (upstream is positive); mean LOF is

aligned with the contrail mean axial direction projection onto the horizontal plane (in cruising flight at constant Flight Level, the difference in elevation is negligible)

[y] Lateral direction (to the right is positive, looking upstream), orthogonal to [x]

[z] Normal direction (upwards is positive)

Free airflow incidence angle (angle-of-attack) to the NRC

CT-133

Free airflow sideslip angle to the NRC CT-133

Vortex circulation

Free airflow density

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Abstract

In 2017, the NRC undertook GARDN project CAAFCER, Civil Aviation Alternate Fuels Contrails and Emissions Research, in conjunction with Air Canada, The Waterfall Group, The

University of Alberta, SkyNRG, and The Boeing Company, with the scientific objective of comparing the characteristics of persistent contrails formed from petroleum jet fuel and biofuel.

The NRC CT-133 research jet undertook flight measurements of contrail ice particle size and number, particulate and gaseous emissions from Air Canada A320 series jets in cruise, flying

respectively on bulk JetA1 and pre-blended 43% HEFA-biofuel-JetA1 blend. The HEFA was supplied by AltAir, Air Canada conducted the blend in Montreal. Intertek conducted full ASTM

analyses of the fuel blend. Aircraft departed Montreal Airport for Toronto. The NRC CT-133 flew from Ottawa Airport, intercepting the Air Canada jets at top-of-climb.

Fuel from the wing-tanks of each project Air Canada flight were sampled and analysed by QETE

DND, for hydrogen content, aromatics, sulphur, naphthalene and heat of combustion – biofuel blend flights were fuel-sampled following refuelling and prior to despatch, JetA1 inbound flights were fuel-sampled following shutdown at the arrival gates in Montreal Airport.

Biofuel contrails were successfully obtained and measured to 90 kilometres in length; JetA1

contrails to 55 kilometres in length.

The ground and flight operations are summarized. Included are examples of measured emission data and a range of particulate emissions and contrail characteristics flight data.

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1.0 Introduction

The Civil Aviation Alternate Fuels Contrail and Emissions Research project (CAAFCER),

addressed the flight research of high altitude contrails formed by jet transport aeroplanes, and, in

particular, the comparison between contrails formed by petroleum jet fuel and biofuel. The

CAAFCER project was a 2016 award from The Green Aviation Research and Development

Network (GARDN), a non-profit organization funded by the Business-Led Network of Centres

of Excellence (BL-NCE) of the Government of Canada and the Canadian aerospace industry.

The research was conducted by a consortium, led by The Waterfall Group. Additional

consortium members were the National Research Council Canada (NRC), Air Canada, SkyNRG,

the University of Alberta and Boeing. Flight research consisted of the flight measurement of

contrails and emissions produced by Jet A1 and by a biofuel blend, consisting of 43% hydro-

processed ester fatty acid (HEFA) biofuel and 57% Jet A1.

The data acquisition Operations Phase of GARDN CAAFCER extended from the 20 th April to

the 4th May, for the last biofuel flight, and a subsequent Jet A1 flight on 11th May 2017. The

overall operational phase covered fuel acquisition, delivery, blending and usage operations.

These operations are briefly described herein.

Fuel usage and consumption consisted of line flight operations of Air Canada A320 series

aircraft, operating Montreal Airport (YUL) to Toronto Airport (YYZ) on 43% HEFA / Jet A1

blend and Toronto to Montreal on Jet A1, refueled in Toronto. The NRC CT-133 research jet

aeroplane measured contrail and emissions characteristics.

The principal goal of this project was to measure and compare contrail characteristics from

different jet transport fuels, namely petroleum and biofuel blend. For such a comparison, the

determinant parameters are the types of jet fuel, individual engine, aircraft and atmospheric

conditions. The comparative analysis considers the parametric variants of fuel properties (for the

JetA1 and 43%HEFA blend used on the experiment) and atmospheric conditions.

2.0 CAAFCER consortium operational responsibilities In the CAAFCER consortium, the following entities undertook operations or operations support:

(1) The Waterfall Group – project management, liaison and coordination

(2) SkyNRG – management of fuel acquisition and blending with Air Canada

(3) Air Canada – conduct of biofuel blending with SkyNRG and conducting line flight

operations, integration of the biofuel flights

(4) NRC – flight measurement and analysis of contrails and emissions from the Air

Canada flights

(5) University of Alberta – management and analysis of the CPC 3776 aerosol counter

and denuder operations,

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(6) Boeing – providing technical input in the planning and execution of the CAAFCER

flights, notably fuel property and flight process optimization and quality assurance.

(7) QETE of DND – undertaking analysis of fuel samples, for the measurement of fuel

properties.

3.0 SkyNRG HEFA biofuel acquisition and blending The HEFA biofuel acquired for CAAFCER was produced by Alt-Air bio-refinery in Los

Angeles Airport, using a feedstock of used cooking oil. The HEFA was shipped per ISO

container via rail, to Montreal railyards, where it was blended with Jet A1, produced by the

Valero jet-fuel refinery, in early April 2017.

The 43%HEFA- Jet Al blend was required, by ASTM D7566 standards, to comply with all Jet

A1 specifications. Marginal fuel specification compliance characteristics centred upon aromatics

content and fuel freezing point; the latter dictated the final blend of 43% HEFA.

The analysis of the 43% HEFA / 57% Jet A1 blend is included as Appendix A.

4.0 Air Canada CAAFCER flight operations

4.1 Flight operational period

The planned CAAFCER flight operations period covered the 20th April to the 5th May, inclusive.

Five biofuel flights were conducted over this period. As explained below, the operational period

was extended to the 11th of May, in an attempt to utilize the residual HEFA blend, after the five

flights.

The residual biofuel quantity was 3,000 kg in the biofuel bowser, operated by the Air Canada

contractor at YUL, Swissport. In an effort to utilise the residual quantity (in a wing-tank mix

that would be approximately 35% HEFA / Jet A1 blend), the operational period was extended to

11th May. However, the residual biofuel was not able to be uploaded, due to insufficient pump-

priming head (fuel depth) for a flight on that data. The NRC CT-133 nevertheless flew on that

date, surveying an ACA A320 contrail generated on Jet A1.This was the sixth and final

CAAFCER flight.

4.2 Air Canada flight procedures When contrail conditions were forecast to occur, a CAAFCER biofuel flight was scheduled, by

the afternoon of the day before the flight. Generally, this was the early flight from YUL, which

had been gated overnight at one of three suitable Gates (for the size of the biofuel bowser) at the

Air Canada terminal at YUL.

In early morning on the flight day, Air Canada defueled the designated aircraft (to an undrainable

fuel level of approximately 200 litres Jet A1), then refueled with biofuel-blend for flight

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operations dispatch of the aircraft. The wing fuel was sampled for analysis by DND QETE, for

(i) calorific value, (ii) total hydrogen, (iii) aromatics, (iv) naphthalene and (v) sulphur content.

The biofuel aircraft QAR was fitted with a flash-card for recording flight parameters – engine,

inertial and air data. The flash-card was removed and archived, upon arrival of the aircraft, at the

terminal gate in YYZ.

In the second week of CAAFCER flight operations, two middle-of-the-day flights were prepared

and despatched from YUL, in order to achieve all CAAFCER flights (due to limitations on

suitable atmospheric conditions). The middle-of-the-day flight operations were considerably

more demanding upon flight- line resources, due to the time limitations on aircraft-turnarounds.

Greater human resources were applied, in order to achieve these flights. The Jet A1 YYZ-YUL

flights, following arrival at the designated gate in YUL, had wing-tank fuel sampled for DND

QETE analysis. The QAR flight data flash-card, with recorded engine, inertial and air data, was

removed and archived, following arrival of the aircraft at the terminal gate at YYZ.

4.3 Air Canada flight listing Table 1 lists the Air Canada flights, biofuel from YUL and Jet A1 from YYZ. In addition to the

list, a project flight functional check was conducted on the 20th April, with an A320 (flight

ACA411) JetA1 contrail being measured, but wing-tank fuel not being sampled for fuel

properties testing.

Table 1 – Air Canada CAAFCER flight details.

Date, 2017 Flight, YUL-YYZ (43% HEFA/JetA1) Flight, YYZ-YUL (Jet A1)

Flt No. Aircraft Engines, Type Flt No. Aircraft Engines, Type

25th April ACA401 C-GPWG A320-211

ACA402 C-GITY A321-211

28th April ACA401 C-FGKN

A321-211

CFM56-5B3-P ACA402 C-GJWD

A321-211

FIN457

CFM56-5B3-P

3rd May ACA411 C-FNVU

A320-211

CFM56-5A1

ACA412

C-FPCA

B767-375 FIN637

CF6-80C2 B1F/B6F

4th May ACA401 C-FDRH

A320-211

CFM56-5A1 ACA402 C-FXCD

A320-214 FIN239

CFM56-5B4/P

4th May ACA413

A320-211

CFM56-5A1 ACA414

A320-211

11th May nil nil Nil nil ACA402 A320 - -

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4.4 Wing-tank fuel samples The wing-tank fuel samples, that were taken by flight- line personnel from each of the biofuel

flights despatched from YUL, and for each of the arrival Jet A1 flights from YYZ (with the

exception of flight ACA402 on the 11th May 2017), were packaged and transported to DND

QETE, for analysis.

4.5 Flight profile & data

All Air Canada (AC) flights followed the same profile, routing (as shown in Figure 1) and

itemized below, between a number of sequential flight route waypoints and arrival procedure

into YYZ:

a. YUL-YYZ: via TORNI-RAGID3ARR, and

b. YYZ-YUL: via DEDKI-SANIN-MIGLO, onwards to YUL (not sampled by the NRC

CT-133).

ACA flights were flown to the same cost index programmed into the FMS, and thus followed

similar thrust schedules. In particular, this dictated normal cruise Mach Numbers, c.0.76.

However, variations in profile (generally, lower cruising altitude) occurred in response to

atmospheric turbulence forecasts and PIREPs. This impeded measurements on the 4th May

biofuel flight (morning flight), whereupon the cruising altitude was initially below contrail-

generating altitude.

The biofuel and Jet A1 QAR flashcard data recorded on the CAAFCER flights was downloaded

and delivered to the NRC on 8th of May 2017.

Generally, YUL-YYZ flights flew higher, in higher RH conditions (more conducive to

thickened, persistent contrail formation), with greater time in-cruise, because of headwinds.

However, YYZ-YUL flights had less time in cruise and flew at lower altitudes, somewhat less

conducive to thick contrail formation. In addition, aerodrome works at YYZ caused greater

delays, so that YYZ-YUL flights tended to have greater time imperative. Overall, time-extent of

Jet A1 contrail data was approximately half that of 43% HEFA/Jet A1 contrail data.

4.6 Supplemental flight details The first NRC CT-133 flight was conducted, on 20th April, as a post-maintenance and sensor

flight functional check. For this, the aircraft was flown on the CAAFCER flight profile (of

Figure 1), including the sampling of the contrail from a YUL-YYZ flight on Jet A1. Analysis of

this data, as far as possible (given the wing-tank fuel was not sampled nor analysed for this

particular flight – nor, also for the Jet A1 contrail of the 11th May) was included in the

CAAFCER contrail and emissions flight data assemblage.

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Figure 1 – Air Canada & NRC flight tracks for CAAFCER flights, indicating the ACA routes and CT-133

contrail measurement segments of cruising flight.

5.0 University of Alberta calibration operations

5.1 Particle Loss estimations

Through the course of 2016, the University of Alberta (UAlberta) conducted detailed estimations

of particle losses for the CPC 3776 and denuder installations in the starboard pod of the CT-133.

The method of inflight operation involved using a pair of pinch (low particle loss) valves, for

bypass or in-line operation of the denuder (which was kept at operating temperature >300C

throughout), to obtain total ultrafine aerosol counts and non-volatile particle counts, respectively.

At the NRC Flight Research Laboratory, UAlberta conducted inter-comparative calibrations for

particle sizes >10 nm, between the CN 7610 and CPC 3776 counters. A fully flight-

representative calibration was not possible, because of the difficulty of static representation of

flight (wherefore, isokinetic probe operation is driven by airspeed, i.e. a positive pressure at the

inlet). However, the inter-comparisons did indicate similarity of measurements between the

counters – a similar result to previous inter-comparisons between the CN7610 and an ECCC

CPC.

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The CPC 3776 and denuder performed very well inflight, following initial performance flight

testing on the 20th April flight. Initially the dissipative heat exchanger of the Peltier cooler did

not receive sufficient cooling – a mini cooling fan assembly (consisting of two mini-axial- flow

fans) was designed, installed, and successfully provided sufficient forced convection to rectify

the condition. Furthermore, to maintain the denuder temperature above 300C, the denuder

heater temperature was set higher, from 350C to 430 C

6.0 NRC CT-133 flight operations

6.1 NRC CT-133 Research Aircraft and Instrumentation

The NRC CT-133 research aeroplane contrail and emissions equipage, together with the sensor

data acquisition rates, are shown in the photograph of Figure 2, which captions the

instrumentation configuration for the measurement of emissions and contrail ice particles, as

used upon the GARDN CAAFCER biofuel contrails project.

Most of the contrail and emissions sensors were contained in the port and starboard underwing

pods. The exceptions were the CO2 and water vapour sensor (a Licor 840A, located in the

aircraft nose), the wing glove on the port wing, for dynamic loads measurements, and the LOF

video camera.

The aircraft inertial, airdata and data acquisition systems were contained in the aircraft nose and

cockpit. The sensors are described below (note that the locations are significant, given that the

principal methodology of NRC contrail and emissions data analysis involves contrail/plume

cross-sectional, spatiotemporal reconstruction):-

a. PORT wing:-

(1) Wing glove with pressure sensors for measuring wake vortex loads;

b. PORT HAARC pod:-

(1) Isokinetic sampling system (consisting of isokinetic probe, manifold, bypass,

and MFC); and (2) LII300 black carbon sensor (operated in High Sensitivity mode);

c. STARBOARD HAARC pod:-

(1) isokinetic sampling system (as above); (2) CN 7610 counter;

(3) Thermo 42 I NOx analyser;; (4) FSSP-100 particle probe; (5) CPC 3776 ultrafine particle counter, detecting particles of size >2.5 nm; and

(6) Denuder, for vaporising volatile particles, thereby allowing the CPC 3776 to count the non-volatile particle sub-set of overall ultrafine particle count.

18

d. AIRCRAFT NOSE:-

(1) airdata boom, sensors TAT, PS, PT ,

(2) inertial system; (3) back-up DAS;

(4) LICOR 840A, measuring CO2 and water vapour; (5) NRC ice Particle Detector Probe (PDP); (6) GPS antenna and receiver.

e. AIRCRAFT COCKPIT:-

(1) DAS; and

(2) Line-of-flight video camera.

Figure 2 – NRC CT-133 contrail and emissions measurement instrumentation, configuration of the GARDN

CAAFCER project.

Pre-operational period, the FSSP-100 contrail ice particle counting and sizing probe was

calibrated for spherical water particles – particular attention was paid to the optical set-up and

instrument calibration (to spherical water particles), such that confidence was placed in the

smallest bin sizing of 0.5μm. A density correction, water to ice, was applied to the calibration, in

19

order to correctly size the measured ice particles of the contrails. FSSP-100 data was gathered at

10 Hz.

The 42I NOx analyser measures the luminescence of the reaction between NO and ozone (the

luminescence level is proportional to concentration), the complete NOx determination firstly

requires the catalytic conversion of any NO2 to NO, a relatively long process (one reading

available each 20 seconds).

In relation to operation of the 42I: without conversion, an NOx reading would be available each

second in streaming mode – the reading would be sensitive to NO and some other nitric

compounds such as HONO, but would not be sensitive to NO2; on the other hand, in fresh

aircraft emission plumes, the majority of nitric oxide compounds is generally present as NO and

oxidises slowly, negligibly over an elapsed contrail survey time of several minutes.

On the NRC CT-133, the NOx analyser was always operated in 1 Hz streaming mode on

CAAFCER flights. To reflect data acquisition in the streaming mode, without sensitivity to the

presence of any NO2, the measured parameter is identified as NOy (rather than NOx).

6.2 CAAFCER NRC CT-133 flights The operational status of the CT-133 and sensors upon all CAAFCER flights, together with

atmospheric conditions, is presented in Table 2.

Note that although the first flight was a post-maintenance and flight functional check of systems

and sensors, it has been designated as Flight Number CAAFCER #0, insofar as it followed the

CAAFCER flight profile and surveyed a Jet A1 contrail from an ACA A320 westward-bound to

YYZ. The wing-tank fuel was not sampled. Thus, in analyzing the contrail data against fuel

properties, the average of Jet A1 fuel analyses has been used. This analysis has been conducted

elsewhere, other than this report. It compared favourably with the other CAAFCER Jet A1

contrails.

20

Table 2 – NRC CT-133 flight details summary (light blue coloured flight details denote post-maintenance and

functional flight test of the CT-133, with a Jet A1 A320 contrail surveyed).

# Date

(2017) Flight

duration

(hrs)

AC flights (from Table 1) Notes:- instrumentation & atmospheric YUL-YYZ

type

altitude

contrail length

YYZ-YUL

type

altitude

contrail length

Pre-CAAFCER flight

0 20th

April

1.5

ACA411 A320 –

YUL JetA1

FL260

6-17 Nm

Nil Used for CPC & denuder flight development, generally

satisfactory, denuder required a higher temp setting for SAE

compliance at high altitude; full FSSP data throughout this &

all flights; no LOF video taken. On ground test on 21st

April

2017, it was apparent that the CPC condenser temperature was

too warm, so that two mini-fans were installed (24th

April 2017)

to successfully provide additional cooling.

Contrail at 8 km height surveyed 10-30 km in length. FSSP

recorded 1 Hz, contrail, AEIn1013

.

CAAFCER flights

1 25th

April

2.5

ACA401

A320-211 -

biofuel

FL340

6-apprr.40 Nm

Nil (late

dispatch from

YYZ due to

ground works

program)

NOy unreliable due to limited settling time after ground power

interruptions; CN 7610, CPC 3776+denuder functional CN,

PM, nvPM; no LOF video taken..

Contrail persistent, optically thinner in the visual range,

dynamic character, AEIn1015

-1013

in jet-stream dynamics

2 28th

April

2.3

ACA401

A321 - biofuel

FL340

Sublimated by c.

4 nm

ACA402

A321 - JetA1

FL330

Contrail

remnants at 8

nm

Starboard pod pumps failed, reset (some loss of CN; loss of

NOy due to off-condition time duration).

CPC data with denuder in-bypass; LOF video;

JetA1 visible contrail limited to trailing vortices only at 15 km

length; 43%HEFA contrail visibly sublimated by 7 km;

however, non-visible ice particles were numerous, resulting in

AEIn values of the order of 108 #/kg. These non-persistent,

non-visible contrails were very useful in data analysis,

conducted elsewhere.

3 3rd

May

2.0

ACA411

A320 - biofuel

FL300

6-c.20 nm

(descent)

ACA412

B763 – JetA1

FL290

8-c.20 nm

(descent)

On climb – starboard pod pump OFF difficulties, resolved

promptly; full comparative sets of CN, NOy, CPC + denuder,

BC, CO2, water vapour data; LOF video.

4 4th

May

2.2

ACA401

A320 – biofuel

FL240 – FL280

No intercept

ACA402

A320 – JetA1

FL310

6-c.12 nm

ACA401 flight planned low altitude due to atmospheric

turbulence, eventually climbed FL280, however not in a

position to obtain contrail data; LOF video.

Full data-set for YYZ JetA1.

5 4th

May

1.8

ACA413

A320 – biofuel

FL320

6-36 nm

ACA414

A320 – JetA1

FL330

c.20-30 nm

Comparative (between Jet A1 and 43%HEFA contrails) sets of

CN, NOy, CPC + denuder, BC, CO2, H2O data; LOF video.

Contrails formed at the top of the troposphere in light

background cirrus.

6 11th

May

2.3

Nil

Background

cirrus (high

aerosol)

ACA402

A320 – JetA1

FL330-350

c.10-24 nm

YYZ Jet A1 sets of CN, NOy, CPC + denuder, BC, CO2, water

vapour data; LOF video.

Contrail formed at the top of the troposphere in background

cirrus with high aerosol content

21

7.0 A data overview and examples of CAAFCER contrail flight data

7.1 General

NRC CT-133 contrail and emissions data has been analysed in detail by the NRC and the

University of Alberta. Examples of data obtained and video images is presented here, in order to

present the atmospheric conditions encountered and the characteristics of the contrails generated

by the ACA flights.

7.2 Atmospheric influence The YYZ-YOW-YUL-YVO area of the St Lawrence Seaway valley is typically influenced by

the North American Jetstream. The NRC has conducted high altitude atmospheric research

flights in this area for wake turbulence research since 2004 (requiring contrail conditions to

delineate wake vortex position), for emissions since 2011, and for contrails, since 2014.

Furthermore, the NRC has conducted mid-altitude atmospheric research in the region for

approximately five decades, with a resultant, substantive local atmospheric knowledge. In

particular, inflight and ground observations of UTLS cloud and contrail characteristics have

enabled the NRC FRL to characterize the UTLS atmospheric nature and dynamics of the St

Lawrence Seaway. The jet-stream influence typically leads to dynamic effects involving water

phase changes, such as high ice particle growth rates during rapid deposition events, ice particle

gravity fall-out and sublimation, convective uplift and cirrocumulus development, and humidity

pooling. Along track, these effects can vary over relatively-small spatial scales of approximately

20-80 km.

High contrail ice particle growth rates have previously been measured (2014/2015) by the NRC

CT-133 in flights to the north of Ottawa[1,2]. As an example of ice particle growth rates,

compared with CT-133 measurements in NASA ACCESS II, DC-8 vortex-dominated

condensate spectra had median effective diameter (MED) values of 1-2 µm as measured by the

FSSP-100, whereas B773 spectra north of YOW had MED of 7 µm. As mentioned below,

CAAFCER flight A320, A321 and B763 contrail ice particle spectra likewise had comparatively

high MED, 5-10 µm.

7.3 Data analysis

7.3.1 General

Two methods of data anlaysis have been applied to CAAFCER contrail and emissions data:

a. Spatial re-construction, and

b. Time-trace analysis.

7.3.2 Spatial re-construction

Contrail and emissions cruise flight data for biofuel and petroleum jet fuel, has been analysed in

the spatiotemporal domain, for which the dominant spatial variable of dynamic change is in the

lateral and vertical directions, orthogonal to the contrail axis. In particular, contrail and emissions

22

plume cross-sections were re-constructed from concatenated sub-sets of nine passes across the

contrail, each occupying a duration of 2-5 seconds (overall, an elapsed time of, typically, two

minutes, at a contrail lengthening rate of 3.5 km per minute, over an air distance of 10 km per

minute). This experimental technique has been matured over four years of flight technique and

data-analysis development [1,2].

FSSP-100 data is recorded at 10 Hz, which is equivalent to a crossplane displacement increment

of 1-2.5 metres per data point. Some of the passes, in the cross-plane, overlapped. Contour plots

have been derived by Matlab delauney triangulation of data points. Therefore, spatial re-

construction is an averaging process. As such, this reduces the inaccuracy effects of

uncertainties such as contrail lateral meandering) and vertical reference (whether geo-centric or

wake vortex referenced [1,2]). Nevertheless, these uncertainties determine the process to be

stochastic. For example, there are differences in the contour plot integrations and hence the

derived contrail AEIn values whether the contrail was assessed in a geo-centric reference (when

the dynamic effects of entrainment were subsiding and detrainment onset occurring) or in a wake

vortex height frame of reference. Assessments [1,2] indicate that the error involved could be

within the range of +10% over this intermediate contrail state of subsiding entrainment-

increasing detrainment.

By this methodology, spatiotemporal re-constructions of GARDN CAAFCER contrail cross-

sections have been conducted for four biofuel (43% HEFA / JetA1 blend) contrails and six

baseline JetA1 flight data, using a total of 10 different aircraft, of three types (A320, A321 and a

B763). Analysis therefore can be based under the premise of considering contrail characteristics

variations and potential parameterisations with fuel properties and atmospheric properties, across

the range of individual engines, engine types and aircraft types.

7.3.3 Time-trace analysis

Included in the CAAFCER flightpath segment train was occasional dwell-time (occupying 15-40

seconds) in a relatively constant position in the contrail, typically near the stem-crown juncture

of the UJW, wherein it was found the ice particle count was reasonably homogenous (e.g., in the

time-slice 1360-1390 seconds of Figure 3). For contrails and emissions flight data analysis,

homogeneity is a desirable pre-requisite for time domain analysis, as it reduces variations (and

hence the standard deviation of an averaging process) over a sampling period, using sensors

operating at different bandwidths and acquisition rates. These segments thus would be amenable

to time-domain analysis of the FSSP-100, CN or CPC data, using the co-located NOy signal

(with an internal, pneumatic lag of 8 seconds) as the intermediary species for the determination

of EIn or, for contrail ice particle number, AEIn in the time domain.

23

7.4 25th April flight

7.4.1 Biofuel contrail

The contrail intercept by the CT-133 occurred from above (by the ACA flight climbing through

the CT-133 flight level, 5 Nm ahead). A time-slice example of contrail ice particle and

particulate matter data is presented in Figure 3.

Concerning CT-133 height, it is seen that the survey height, as time progressed, is biased towards

the UJW domain – this is symptomatic of tracking the presence of ice particles, and in particular

the occurrence of ice particle sublimation in the TWV region, as the vortices descend into, on

this occasion, air of lower RH and higher pressure as the vortex circulation decays.

For every persistent contrail and emissions plume measured by the NRC CT-133, the top of the

contrail and UJW have remained at the emitter aircraft altitude. The vertical traverse at time

c.1500 sec of Figure 3 illustrates this point: it is seen that the FSSP-100 activity count (roughly

proportional to the number of ice particles validly observed by the FSSP-100) diminished with

height downwards, whilst the CN and ultrafine aerosol each maintained two concentrations – one

in the UJW crown and one in the TWV remnant region, with a diminution of concentrations in

the UJW stem.

Concerning contrail ice particle density, in data snapshot terms, the metric ‘FSSP activity count’

is related proportionately, ‘Max’ relating to local thickness, ‘Mean’ and ‘Median’ (all shown in

Figure 3) relating statistically to the overall contrail, including the time spent outside the contrail,

in order to delineate the contrail dimensions and to measure local background atmospheric

parameters. It is seen in Figure 3 that the Max value is 47, occurring in the TWV region of the

fresh contrail. Maximum values in the UJW crown of the persistent contrail were in the range of

30-33.

24

Figure 3 – CAAFCER #1 data time-slice (as recorded inflight, i.e. non-time correlated for differing internal pneumatic lags between sensors):- top downwards, CT-133 height, CN 7610 >10 nano-m data, FSSP-100

activity count, CPC 3776 ultrafine aerosol data.

8.0 Contrail Video Imagery Examples of contrail imagery, viewed in the LOF direction, are presented in this section, to

illustrate examples of contrail ice particle perspectives and state-transformations encountered on

the CAAFCER flights.

8.1 Biofuel contrail, 3rd May flight The intercept was conducted with the NCR CT-133 above the ACA flight, following which the

ACA flight climbed through the CT-133 flight level, when 9 km ahead of the CT-133 (Figure 4).

25

Figure 4(a) – 3rd

May 2017 CAFACER flight, at intercept of the ACA flight, from above (ACA flight is 9 km

ahead).

Figure 4(b) – LOF contrail appearance, from below, at approximately 19 km contrail length.

26

Figure 4(c) – contrail at approximately 30 km length: diminution of trailing vortex condensate, and

development of crown condensate in UJW (note the slanted-downwards to the left inclination of the contrail,

due to background crosswind and shear).

Figure 4(d) – contrail limited to UJW crown region, with optically thinning due to sublimating ice particles.

8.2 Jet A1 contrail, B763, 3rd May The LOF appearance of the contrail is shown in Figure 5, for a contrail length of approximately

28 km. The NRC CT-133 is below the UJW, flying in the trailing vortex region (with little

condensate in this region) at the moment of the image. The UJW appearance to the contrail

27

indicates non-homogeneity, ‘lumpiness’ of ice particle appearance, which might be

representative of a cumuliform, or convective, character.

Figure 5 – 3rd

May 2017, B763 JetA1 contrail UJW crown region, viewed from below, at a contrail length of

approximately 28 km.

8.3 Biofuel contrail, A320, 4th May, afternoon flight The progression of states of this contrail is depicted in the sequence of images presented in

Figure 6. Generally the contrail state is a stem or veil of ice particles from the UJW crown to the

lower TWV region. Progressively, the stem sublimates. The UJW crown is then seen (Figure

6(e)) to develop in lateral spreading, with optical appearances characteristic of cirro-cumuliform

ice cloud patches (i.e., a convective development process).

28

Figure 6(a) – 4th

May 2017 afternoon flight, A320 HEFA-blend biofuel contrail, viewed from below, at a

contrail length of approximately 10 km.

Figure 6(b) – contrail viewed during a vertical traverse, near the top of the contrail, of a veil or UJW-stem

type of structure shape at this stage, approximately 15 km length.

29

Figure 6(c) – contrail viewed from below, the transformation of the contrail, from a veil shape to a laterally-

developing UJW crown is seen, approximately 30 km length.

Figure 6(d) – contrail viewed from amidst the UJW crown of the contrail, approximately 35 km length.

30

Figure 6(e) –with the contrail age approximately 3 minutes and length 42 km, the contrail has transformed to

a UJW lateral crown of contrail cirrocumulus (distinct small-spatial scale ‘puffy’ shapes).

Figure 6(f) – amidst the UJW laterally-spreading crown (below), it can be seen that the lateral spread is

slanted, indicative of interaction with background atmospheric crossflow-vertical shear, length

approximately 50 km.

31

Figure 6(g) – NRC CT-133 landing back at Ottawa, Runway 25, in a light southerly crosswind:-

8.4 Jet A1 contrail, A320, 11th May Contrail images are shown in Figure 7 for a Jet A1-fueled A320 ACA flight, measured by the

NRC CT-133 on a flight on the 11th May 2017. It is a good example of the varying states of

contrail characteristics, and the influence of varying background air-mass conditions, typical of

the St Lawrence Seaway jet-stream-dominated atmospheric conditions.

Figure 7(a) – seen from below, whilst holding near Toronto, for the ACA402 Jet A1 flight, contrail from an

overflying regional jet, 2,000 feet above the NRC CT-133 (shown on the port wing, in orange, is the wing

glove, fitted with pressure transducers to measure the unsteady wake vortex loads on the wing):-

32

Figure 7(b) – ACA402 JetA1 contrail, viewed from below, at interception (at a contrail length of

approximately 18 km); non-uniform nature of the contrail veil is evident, because of the entrainment

dynamics effect of the trailing vortices in long-wave, linking instability, typically excited by background

atmospheric turbulence (of a ‘light to moderate ‘chop’ nature).

Figure 7(c) – ACA402 JetA1 contrail, viewed from below, at a length of approximately 25 km, picture taken

with the CT-133 in the lower part of the contrail, vicinity of trailing vortices, which have induced a roll ont eh

Ct-133..

33

Figure 7(d) – ACA402 JetA1 contrail at viewed from below, at a length of approximately 35 km; contrail

abruptly spatially-transformed into an homogenous slanted veil shape.

Figure 7(e) – ACA402 JetA1 contrail, seven minutes after sampling is evident above the NRC CT-133 port

wing tip fuel tank, at the edge of the background cirrus mass, which abruptly dissipated eastwards, into a dry

air, with some level of observed turbulent mixing.

34

9.0 Data review and analysis

9.1 Data example, biofuel contrail, 25th April 2017

CT-133 acquired data analysis is reviewed, to illustrate the development and quantify the

measured characteristics of CAFACER contrails and emissions. For this, the data has been

analysed in the format of NRC ACCESS II contrail and emissions data [1,2].

Data quantified and presented herein is representative of the nature of spatially reconstructed

CAAFCER contrail and emissions plume data, presented for the illustrative purposes of the

present report.

9.1.1 Inertial and Air data

Inertial data was reliably acquired at 600 samples per second (i.e., 600 Hz) throughout all flights.

Likewise, air data was reliably recorded, with the exception of probable ice contamination or

blocking, which occurred on the final flight, 11th May, and which was evidenced in the

derivation of α and β. Nevertheless, re-construction of air data for this condition was

successfully conducted using inertial acceleration and velocity data.

9.1.2 Wake vortex data

At 600 Hz, the measured inertial and derived air data vectors have been differenced, then

spatially-correlated (using inertial position information, transformed to the wake vortex axis

system, concurrent with mean direction-of-flight), to provide trailing vortex data for port and

starboard vortices, from which wake vortex characteristics have been usefully derived.

Trailing vortex cores were relatively large in diameter (1 to 4 metres diameter, which varied in

vortex vented, funnel-shaped short-wave instability modes3). Lateral separation between

vortices was relatively small, typically 20 m, centre-to-centre. The separation varied with long-

wave instability excitation, as typical of wake vortex states. At 56% of wingspan, this vortex

separation was significantly less than that for an elliptically-loaded wing (/4, or 79% of

wingspan).

Lateral proximity of the vortices to each other would tend to suggest that geometric wingspan

would not be a scaling parameter for vortex size nor diameter. It would also be expected to

result in greater short and long wave instability modes, and result in greater generated vortex

circulation. Generated circulation, =W/(Vbv), was typically (for ACA A320 flights on

CAAFCER) 250 m2/s (which agreed with the circulation derived from the open path integral of

the approach segment of the CT-133 flight-path [4], Figure 8 refers).

35

Figure 8 – open path line integral, deriving vortex circulation, for a typical CAAFCER contrail survey flight-

path.

Figure 9(a) shows 3-velocity components to the vortices. Most unusual is the dominance of axial

velocity peaks (in green, peak magnitudes 9-17 m/s; tangential velocity component, 5-7 m/s).

Possibly this could be attributable to the relative proximity of vortices to each other, in driving

helical vorticity associated with elliptical modes. Figure 9(b) presents the vertical wind

component, highlighting the relatively large-scale of the vortices cross-section, and relatively

small distance between them (approximately 10 metres in this re-construction). The relatively

small ratio of separation to core radius could be the mechanism providing stimulation of

particular mutual instability modes which might drive the axial velocity observations.

The circumferentially non-uniform distribution of velocity peaks is considered to be associated

with such elliptical modes of instability. Characteristics of axial variation of vortex core state

include venting, funneling contractions of vortex cores, and circumferential discretization of

vorticity into ‘strings of pearl’ vortices [3].

100 200 300 400 500 600 700 800 900

-600

-400

-200

0

200

400

t (sec)

(

m2s

-1)

Crossplane open path integral, wCZ

sds, A320

36

Figure 9(a) –trailing vortex pair core passages at 11 km wake length, plotted against crossplane projection of

the CT-133 flight-path (this data was used for the open path integral of Figure 8)..

Figure 9(b) – re-constructed cross-plane of vortex-induced velocity magnitude (m/s), delineating a view of

trailing vortex pair (of Figure 9(a)), observed in the signature of induced vertical wind: showing the

relatively large-scale of the vortices and relatively short distance between vortex cores, approximately 10-15

metres.

345 350 355 360 365 370 375

-10

-5

0

5

10

15

dsa-sum, crossplane arc distance

wc

w

a

w

Z

wc

wa

wZ

37

9.1.3 Dynamic phase, contrail length 10-17 km

9.1.3.1 CN 7610 aerosol counter data

The time-trace of CN7610 aerosol data is presented in Figure 10. It is seen that there was

gradual , non-monotonic diminishment of values with time (i.e. with the contrail length

increasing at a rate of 3.5 km/minute). The progression was non-monotonic, because vortex

entrainment resulted in large spatial variations of concentration – maxima values occurring in the

trailing vortex core edges. This is highlighted in the following spatial re-construction.

The first nine passes through the contrail have been used to re-construct the CN concentration

cross-sectional shape, shown in Figure 11. Peak gross concentrations of 14,000 per cc were

measured in the TWV – at the vortex core edges (averaged by the contour plot algorithm to peak

values of 11,000 per cc).

In Figure 12, is the lateral integral of the plume. Vertical integration of this shape then is used,

via TAS and ACA401 fuel-flow, to derive the EIn for CN, namely 1.4622e+16 per kg fuel.

Figure 10 – time-trace of CAAFCER #1 biofuel CN 7610 >10 nano-m aerosol concentration (# per m3).

38

Figure 11 – CAAFCER #1 biofuel CN 7610 concentration per cc, cross-plane emission plume re-construction.

Figure 12 – CAAFCER #1 biofuel CN 7610 lateral integrals – giving vertical distribution to the CN plume.

9.1.3.2 CPC 3776, denuder by-passed

The University of Alberta CPC3776 was operated in denuder-bypassed operation for this

segment of the contrail (10-17 km length), thereby registering all ultra-fine aerosols, volatile and

non-volatile, > 2.5 nm in size. The data is plotted bin re-constructed cross-plane form, in Figure

y (m)

z,

geo-h

eig

ht

(m)

A320 CN concentrations, no./cm3, wake length 6-9 nm nm)

-50 0 50

-50

0

50

100

150

1000

2000

3000

4000

5000

6000

7000

8000

9000

10000

11000

-0.5 0 0.5 1 1.5 2 2.5 3 3.5 4

x 1011

-300

-200

-100

0

100

200

300

net CN, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zFA

20 (

m)

39

13. The vertical profile of the lateral integrand shows greater entrainment within the trailing

wake vortex region (presumably a reflection of the smaller aerosol size).

Figure 13 – CAAFCER #1 biofuel CPC3776 total ultrafine aerosol data, left, re-constructed plume cross-

section of data, right, lateral integrals – giving vertical distribution to the CPC3776 denuder-bypassed plume.

The EIn derived from integration of the concatenated plume cross-section (as with other species)

was 4.2647e+16 per kg fuel, which is approximately four times the CN (>10 nm) EIn, implying

the aerosol count between 2.5-10 nm in size is thrice that >10 nm in size. Likewise, at 70,000

per cc, peak number concentrations of ultra-fines were 4x those >10 nano-metres.

9.1.3.3 CO2 data

The CO2 plume re-constructed cross-section is shown in Figure 14. Peak concentrations were in

the trailing vortices, with only an apparently relatively small amount in the UJW. The cross-

section laterally- integrates to that vertical distribution shown in Figure 14 also. It integrated to

an EI of 3.2621 kg/kg fuel – although this is an interactive loop processing, to account for plume

wavering under atmospheric forcing, necessary for CO2 because of the low signal-to-noise (S/N)

ratio of the C02 measurement (and hence lower experimental accuracy).

y (m)

z,

geo-h

eig

ht

(m)

A320 CPC concentrations, no./cm3, wake length 6-9 nm)

-60 -40 -20 0 20 40

-60

-40

-20

0

20

40

60

80

100

120

140

0

1

2

3

4

5

6

7x 10

4

-1 0 1 2 3 4 5 6 7 8

x 1011

-100

-50

0

50

100

150

200

net CPC, no./m3, 6-9 nmheig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

40

Figure 14 – CAAFCER #1 biofuel CO2 cross-sectional plume (left), cross-sectional plume lateral integrand,

showing vertical profile (right).

9.1.3.4 Black carbon (BC) data

The BC plume re-constructed cross-sectional profile is shown in Figure 15, for 10-17 km contrail

length contrail. Compared to the CN and CPC plumes, the re-constructed BC profile lacks some

correlation, likely related to low-concentration levels of BC, and including optical turbulence

effects in the sensor optical cell. Integration of the profile yielded an EI of 212+50 mg/kg, with

an uncertainty that relates to the minimum concentration sensitivity of the sensor.

y (m)

z (

m)

A320 CO2 concentrations, ppb, wake length 6-9 nm

-60 -40 -20 0 20 40

-60

-40

-20

0

20

40

60

80

100

120

140

366

368

370

372

374

376

378

-2 0 2 4 6 8 10 12 14 16 18

x 10-5

-300

-200

-100

0

100

200

300

CO2, m3

heig

ht

above/b

elo

w A

320 p

lane,

zFA

20 (

m)

CO2 ppm Grand total minus CO

2,ppb Background

y (m)

z,

geo-h

eig

ht

(m)

A320 BC concentration, mg/m3, wake length 6-9 nm)

-80 -60 -40 -20 0 20 40 60

-50

0

50

100

150

0.5

1

1.5

2

2.5

x 10-3

0 0.005 0.01 0.015 0.02 0.025 0.03 0.035 0.04-100

-50

0

50

100

150

200

BC, mg/m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

41

Figure 15 – CAAFCER #1 biofuel BC: Left: BC cross-sectional plume (left), cross-sectional plume lateral

integrand, showing vertical profile (right); Right (blue relates to data for the complete contrail survey; red

relates to the data sub-set which is only used for the 10-17 km contrail length): lateral distribution of BC

readings (left), vertical distribution (right).

9.1.3.5 Contrail ice particle data, 6-9 nm

The FSSP-100 contrail ice particle (>0.5µm size) number (#) density is shown in Figure 16, and

the lateral integrand in Figure 16 likewise, which integrated to an AEIn of 1.3244e+14 #/kg fuel

from ACA401, at this location & length of contrail. Ice aprticle number densities were of the

order of 200 #/cc. The contrail ice distribution was predominantly vertically-oriented. The

shape could be described as an amorphous, ‘lumpy’ veil, with no lateral crown developed at this

stage, a one minute old contrail.

However the TWV region had smaller ice particles than the UJW (and eventually, the TWV ice

particles ceased growing and sublimated). Typical spectra are shown in Figure 17.

The spectra can be integrated to derive the median effective diameter of the ice particles (MED),

the distribution of which is shown in Figure 18 – it is seen that the smaller particles occurred in

the TWV region (and were sized 1-2 µm MED), larger occurred in the UJW, with a progressive

vertical distribution in MED. With increasing contrail length – there is a general growth in

average MED (Figure 18) and in the difference between MAX and MIN MED values, over the

cross-section of the contrail.

42

Figure 16 – CAAFCER #1 biofuel contrail cross-sectional shape (left) and lateral integrand (right), showing

vertical distribution.

Figure 17 – CAAFCER #1 biofuel contrail ice particle spectra, left, TWV, right, UJW stem.

y (m)

z (

m)

A320 FSSP concentrations, no./cm3, wake length 6-9 nm)

-30 -20 -10 0 10 20 30

-50

0

50

100

150

0

20

40

60

80

100

120

140

160

0 2 4 6 8 10 12 14 16 18

x 108

-100

-50

0

50

100

150

200

FSSP, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

0 1 2 3 4 5 6 7 8 90

5

10

15

20

25

30

35

size (m)

#/c

c

0 1 2 3 4 5 6 7 8 90

5

10

15

20

25

size (m)

#/c

c

43

Figure 18 – CAAFCER #1 biofuel contrail ice particle MED left, spatial distribution, right, as a function of

contrail length.

The ice particle spectra can be integrated into an ice mass concentration, the cross-sectional

distribution of which is shown in Figure 19. With the larger particle size in the UJW, the ice

mass fraction of the whole, contained in the UJW, is greater. At this length, 10-17 km, the

contrail had an ice-mass (for =1,000 kg/m3, likely an over-estimate due to air bubble

entrapment in the ice nucleation process) AEIm of 9.1494e+08 µg/kg fuel.

Figure 19 – CAAFCER #1 biofuel contrail ice mass left, spatial distribution, right vertical profile.

y (m)

z (

m)

A320 FSSP Median Vol. Diameter, wake length 6-9 nm)

-80 -60 -40 -20 0 20 40 60

-50

0

50

100

150

1

1.5

2

2.5

3

3.5

4

4.5

5x 10

-6

5 10 15 20 25 30 350

1

2

3

4

5

6

7

8x 10

-6

length of wake (m)

ME

D (

m)

y (m)

z (

m)

A320 FSSP ICE MASS, g/m3, wake length 6-9 nm)

-60 -40 -20 0 20 40

-50

0

50

100

150

0

100

200

300

400

500

600

700

800

900

0 0.5 1 1.5 2 2.5 3

x 104

-300

-200

-100

0

100

200

300

ICE, cumulative g/m2

heig

ht

above/b

elo

w A

320 p

lane,

zFA

20 (

m)

44

9.1.3.6 Water vapour, Licor 840A

The water vapour RH and RH over ice, RHi, data obtained from the Licor 840A in the CT-133, is

presented in Figure 20, in re-constructed cross-sectional distribution. At the TWV region (z=0),

the RH is irregular, with depletion-region shape definition that appears to be that of the trailing

vortex pair. In the UJW, super-saturation to 120% is evident, and is laterally-spread, a precursor

to the eventual lateral spread of the contrail UJW crown.

Figure 20 – CAAFCER #1 biofuel contrail measured cross -section of RH and RHICE.

9.1.4 Biofuel contrail, 25th April 2017, 18-26 km length

9.1.4.1 CN 7610 aerosol data

For the same contrail, but at a longer length (older age and different relative-atmospheric

location, approximately 35 km air-track distance further to the west), the CN7610 data re-

constructed plume and contrail cross-section are presented in Figure 21. Compared to the same

contrail at 10-17 km length, perhaps there is slightly greater lateral extent of the particle plume, a

lessening effect of the TWV and a growing detrainment effect (greatest lateral integration was no

longer in the TWV, but occurred at mid-height of the plume).

y (m)

z (

m)

A320 RHw

, wake length 6-9 nm)

-80 -60 -40 -20 0 20 40 60

-50

0

50

100

150

30

35

40

45

50

55

60

65

70

75

y (m)

z (

m)

A320 RHi, wake length 6-9 nm)

-80 -60 -40 -20 0 20 40 60

-50

0

50

100

150

50

60

70

80

90

100

110

120

45

Figure 21 – CAAFCER #1 biofuel contrail measured cross -section of aerosol, CN.

9.1.4.2 CN 7610 & denuded CPC3776 data

Presented in Figure 22 are the contrail cross-section reconstructions for CN (>10 nm) and non-

volatile ultrafine particles, nvPM, (>2.5 nm), The vertical distribution of accumulations is

shown in Figure 23. nvPM particles could be expected to have been principally soot, BC.

Figure 22 – CAAFCER #1, 18-27 km contrail cross-sections of PM concentrations (#/cc), biofuel nvPM CPC3776 >2.5 nm (left) and CN 7610 >10 nm CN (right).

It is seen that nvPM concentrations were approximately 15% of CN concentrations. As

described earlier, CPC3776 counts, with denuder bypassed, were 4x CN counts, if similarity is

y (m)

z,

geo-h

eig

ht

(m)

A320 CN concentrations, no./cm3, wake length 10-14 nm)

-80 -60 -40 -20 0 20 40 60 80-100

-50

0

50

100

150

1000

2000

3000

4000

5000

6000

7000

8000

-2 0 2 4 6 8 10 12 14 16 18

x 1010

-100

-50

0

50

100

150

200

net CN, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

46

assumed over the contrail distance increase, these figures imply that nvPM were approximately

4+2% (accounting for the CPC3776 measurement error of +40%) of overall ultrafine aerosols.

Figure 23 – CAAFCER #1, 18-27 km contrail cross-section lateral integrations, biofuel nvPM CPC3776 >2.5 nano-m (left) and CN 7610 >10 nano-m CN concentration (right).

Figure 24 presents the re-constructed cross-sectional contrail of FSSP 3 per cc, and the ratio of

FSSP ice particle number density to nvPM number density. It can be expected that the nvPM

principally consisted of soot particles. Therefore the ratio would represent the activation count

of soot particles for ice nucleation. The mean activation is seen to have increased with contrail

length, and varied with location in the plume cross-section. Recognising that the FSSP-100 only

registered ice particles >0.5 µm, these two observations are likely to reflect, at least in part, the

progressive growth in ice particle, from below to beyond 0.5 µm in size.

Figure 24 – CAAFCER #1, 18-27 km contrail, biofuel, ratio of FSSP ice particle count density to nvPM particle count, with contrail length (left) and a contrail cross-sectional contour plot (right).

0 2 4 6 8 10 12 14 16 18

x 109

-100

-50

0

50

100

150

200

net CPCnv, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

-2 0 2 4 6 8 10 12 14 16 18

x 1010

-100

-50

0

50

100

150

200

net CN, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

9 10 11 12 13 14 15 160

0.05

0.1

0.15

0.2

0.25

0.3

0.35

0.4

0.45

ratio

contrail length

Activation representation, ratio of FSSP/CPCnv

47

9.1.4.3 CO2, cross-section

The CO2 plume is shown in Figure 25, for this segment of the contrail length. The bulk of the

CO2 is observed to reside in the lower half of the cross-section.

Figure 25 – CAAFCER #1, 18-27 km contrail cross-section and lateral integration, CO2 plume.

9.1.4.4 BC, cross-section

The BC re-constructed plume cross-section for this contrail segment is presented in Figure 26.

Figure 26 – CAAFCER #1, 18-27 km contrail cross-section and lateral integration, BC plume.

y (m)

z (

m)

A320 CO2 concentrations, ppb, wake length 10-14 nm

-60 -40 -20 0 20 40 60

-50

0

50

100

150

363

364

365

366

367

368

369

370

371

372

373

374

-4 -2 0 2 4 6 8

x 10-5

-100

-50

0

50

100

150

200

CO2, m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

CO2 ppm Grand total minus CO

2,ppb Background

0 0.002 0.004 0.006 0.008 0.01 0.012 0.014 0.016 0.018 0.02-100

-50

0

50

100

150

200

BC, mg/m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

48

9.1.4.5 FSSP-100 ice-mass

Integration of the ice particle count (Figure 24) of the contrail cross-section, assuming sphericity,

resulted in a value AEIn = 1.0914e+14, which is about 25% less than 10-17 km length. The

cross-sectional distribution is shown in Figure 27. The cross-sectional distribution of MED and

the behaviour with contrail length are shown in Figure 28. MED was more homogenous over the

cross-section, with smaller values in the TWV (likely sublimation) and at the UJW crown lateral

limits (likely growth).

Figure 27 – CAAFCER #1, 18-27 km contrail cross-section and lateral integration, ice-mass, assuming

sphericity.

Figure 28 – CAAFCER #1, 18-27 km contrail cross-sectional MED distribution (left) and behaviour of MED

with contrail length (right).

0 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8 2

x 109

-100

-50

0

50

100

150

200

FSSP, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

5 10 15 20 25 30 350

1

2

3

4

5

6

7

8x 10

-6

length of wake (m)

ME

D (

m)

49

9.1.4.6 Licor 840A Water vapour

Water vapour RH and RHi are shown in Figure 29, for 18-27 km contrail length. The

distribution of RH and RHi is seen to have changed, compared to the shorter length contrail

(Figure 20), denoting not only the production of ice particles, and interaction with background

humidity, but also the change in background humidity and humidity lapse rate, with geographic

location in the jet-stream.

Figure 29 – CAAFCER #1, 18-27 km contrail cross-sections of RH (left) and RHi (right).

9.1.5 Biofuel contrail, 25th APRIL 2017, 27-37 km length

9.1.5.1 CN data

In cross-sectional shape, the CN emissions plume (Figure 30) had somewhat transformed to a

squat-shape (principally, a lateral spread, vertical extent was 240 metres, similar to the shorter

wake). Peak concentrations were 8,000 #/cc.

Figure 30 – CAAFCER #1, 27-37 km contrail cross-section of CN and lateral integrand distribution.

-5 0 5 10 15 20

x 1010

-100

-50

0

50

100

150

200

250

net CN, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

50

9.1.5.2 CPC3776 PM data, i.e. denuder bypassed

The cross-sectional profile, Figure 31, of ultrafine aerosol PM (i.e., total, volatile and non-

volatile) was similar to that of CN, and peak concentrations were ~30,000 #/cc, once again

roughly 4 x that of CN, implying ~3 x CN were particles between 2.5 and 10 nano-m in size.

Figure 31(a) – CAAFCER #1, 27-37 km contrail cross-section of CPC3776 PM and lateral integrand

distribution.

9.1.5.3 CO2 data

CO2 dilution was evidenced at the greater contrail length. Elevated CO2 concentrations (to peak

values of 374 ppb, against the background of 364 ppb) were more prevalent in the lower-half of

the wake (refer to Figure 31(b)), compared to CN and ultrafine PM. Licor 840A repeatability

was specified at +2% - the elevated concentrations were therefore at the limit of the sensor

accuracy.

-1 0 1 2 3 4 5

x 1011

-100

-50

0

50

100

150

200

250

net CPC, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

51

Figure 31(b) – CAAFCER #1, 27-37 km contrail cross-section of CO2 and lateral integrand distribution.

9.1.5.4 FSSP-100 ice particle data

Compared to 18-27 km contrail length, an FSSP AEIn = 1.2574e+15 indicated the re-

establishment of ice particle growth, perhaps from <FSSP-sensing size (0.5 µm), a further

example of the interaction of emitted water vapour and background atmospheric RH.

Figure 32 – CAAFCER #1, 27-37 km contrail cross-section of FSSP-100 ice particles and lateral integrand

vertical distribution thereof.

The contour plot of MED (Figure 33) indicated different characteristics, compared to the shorter

contrail. Vertically, the MED distribution was reasonably homogenous, but significantly lower

y (m)

z (

m)

A320 CO2 concentrations, ppb, wake length 14-19 nm

-100 -50 0 50 100-100

-50

0

50

100

150

200

364

365

366

367

368

369

370

371

372

373

374

-4 -2 0 2 4 6 8 10

x 10-5

-100

-50

0

50

100

150

200

250

CO2, m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

CO2 ppm Grand total minus CO

2,ppb Background

0 2 4 6 8 10 12 14 16 18

x 109

-100

-50

0

50

100

150

200

250

FSSP, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

52

MED values were prevalent at the sides of the contrail, likely to have been indicative of fresh ice

particle growth occurring laterally (i.e., a lateral spread of the contrail).

Figure 33 – CAAFCER #1, 27-37 km contrail cross-sectional distribution of ice particle MED.

9.1.5.6 Licor 840A Water vapour

High RH values remained prevalent (Figure 34) across the UJW crown of the contrail, which

would be expected to support continued lateral growth of the crown.

Figure 34 – CAAFCER #1, 27-37 km contrail cross-sections of RH (left) and RHi (right).

53

9.1.6 Biofuel contrail, 25th APRIL 2017, 37-50 km

9.1.6.1 CN data

The CN cross-section was integrated to an EIn of 1.4522e+16. However, the plume (Figure 35)

showed that the integration may have been truncated in the 4-5 o’clock position, in which case

the cross-section integration could be expected to be an under-estimate.

Figure 35 – CAAFCER #1, 37-50 km contrail cross-section of CN and lateral integrand, vertical distribution.

9.1.6.2 CPC data, non-volatile (i.e. denuder in-line)

On the other hand, the CPC3776 nvPM plume (Figure 36) would appear to have been fully

captured. Of further note for the vector of nine traverses used in the cross-sectional re-

construction was the observation that background CN data points differed from background non-

volatile data points (indicative of some difference in background aerosol constituents, and the

presence of volatile particles in particular). EIn for CPCnv was 1.2978e+15 /kg.

Figure 36 – CAAFCER #1, 37-50 km contrail cross-section of CPC3776 nvPM and lateral integrand, vertical

distribution

-0.5 0 0.5 1 1.5 2 2.5

x 1011

-100

-50

0

50

100

150

200

250

300

net CN, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

0 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8 2

x 1010

-100

-50

0

50

100

150

200

250

300

net CPCnv, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

54

9.1.6.3 CO2 data, 19-26 nm

For CO2, as seen below, the re-construction suffered from delauney triangulation streaking in the

contour-interpolation process, which was evidence of non-optimum flight-path traversing, for

CO2. Therefore the integration can be expected to be unrealistically high, which it was, at 5.0

kg/kg, an error of approximately 60%.

Figure 37 – CAAFCER #1, 37-50 km contrail cross-section of CO2 and lateral integrand, vertical distribution

9.1.6.4 BC data

The BC re-constructed cross-section (Figure 38) was integrated to give an EI of 346 mg/kg.

Figure 38 – CAAFCER #1, 37-50 km contrail cross-section of BC and lateral integrand, vertical distribution.

9.1.6.5 FSSP ice particle data

The FSSP-100 ice particle re-constructed cross-section would appear (Figure 39) to have

captured the contrail cross-section fully, and integrated to AEIn = 1.2062e+14 #/kg. Assuming

y (m)

z (

m)

A320 CO2 concentrations, ppb, wake length 19-26 nm

-100 -50 0 50

50

100

150

200

250

365

366

367

368

369

370

371

372

373

-6 -4 -2 0 2 4 6 8 10 12 14

x 10-5

-100

-50

0

50

100

150

200

250

300

CO2, m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

CO2 ppm Grand total minus CO

2,ppb Background

0 0.005 0.01 0.015 0.02 0.025 0.03 0.035 0.04 0.045-100

-50

0

50

100

150

200

250

300

BC, mg/m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

55

sphericity (likely to be significantly in error for this contrail length), ice mass integrated to AEIm

= 1.5291e+09 µg/kg. With a hydrogen content of 14.6% for the 43%HEFA-blend (c.f. 13.8% for

Jet A1), a water vapour emission index of approximately 1.3 kg/kg could be expected. An

exceedance of this implies background atmospheric water vapour deposition. However, the

AEIm integration of 1.53 kg/kg could also have reflected an experimental error due to

asphericity.

Figure 39 – CAAFCER #1, 37-50 km contrail cross-section of ice particles and # lateral integrand, vertical

distribution

MED was mostly of the order 2.5-4 µm. The MED distribution (Figure 40) delineated growth in

the lateral spread of the UJW crown, to +100 metres in extent.

Figure 40 – CAAFCER #1, 37-50 km contrail cross-section of MED.

0 0.5 1 1.5 2 2.5

x 109

-100

-50

0

50

100

150

200

250

300

FSSP, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

56

The ratio of FSSP ice particle number density to that of nvPM (i.e., CPC with denuder in-line, as

stated above) is shown in Figure 41. Peak ratios are seen to be lower than 19-27 km contrail

length, 0.2 (c.f. 0.3), implying some sublimation. Examination of the contour plot of the ratio

(Figure 41), in comparison to Figure 24 (shorter contrail) indicates that the sublimation occurred

in the TWV region. On the other hand, ratios at lateral extremities of the contrail had risen from

values of 0.05 (Figure 24) to 0.1, representing for FSSP sensed ice particle sizes, greater

activation associated with the lateral spread of the contrail.

Figure 41 – CAAFCER #1, 37-50 km contrail nvPM/FSSP activation (left) and re-constructed cross-section of

the activation (right).

9.1.6.6 Licor 840A water vapour

The RH cross-section (Figure 42) shows strong water vapour depletion in the areas of the

contrail. The RHi distribution (Figure 42) shows the surrounding environment to have no super-

saturation. Sublimation can be expected to be in-process.

57

Figure 42 – CAAFCER #1, 37-50 km contrail cross-sections of RH (left) and RHi(right).

9.1.7 Biofuel contrail, 25th APRIL 2017, 50-55 km length

7.1.7.1 CN data

The CN re-constructed plume cross-section for 50-55 km length is shown in Figure 43.

Although there was a five-fold increase in contrail length from the initial traverses, peak CN

concentrations had reduced (by dilution) only 40%, from 11,000 (Figure 11) to 7,000 /cc. This

indicated that the concentrating effect of vorticity remains significant at the 50-55 lm length of

contrail. EIn was derived by area integration, as 9.3385e+15 #/kg.

Figure 43 – CAAFCER #1, 50-55 km contrail cross-section of CN aerosol # (left) lateral integrand, vertical

distribution (right).

-1 0 1 2 3 4 5 6 7 8

x 1010

-200

-150

-100

-50

0

50

100

150

200

250

300

net CN, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

58

9.1.7.2 CPC PM data, denuder bypassed

For ultrafine aerosols (both volatile plus non-volatile), the re-constructed plume cross-section is

shown in Figure 44, and integrates to EIn = 1.8588e+16, or approximately twice the CN EIn.

Figure 44 – CAAFCER #1, 50-55 km contrail cross-section of CPC total ultrafine aerosol # (left) lateral

integrand, vertical distribution (right).

9.1.7.3 CO2 data

The cross-section of Figure 45 integrated to an EIm of 3.3467 kg/kg, when iterated against

refinements to the background concentration curve-fitting. Background CO2 had increased in

this location to a mean 370 ppb, with a negative lapse rate, from 372 ppb, 200 m below vortex

reference height, to 368 ppb, 200 m above vortex reference height. Elevations in CO2

concentration above this (to peak values of 373 ppb) were within the resolution of the Licor

840A. Thus, the re-constructed plume was non-deterministic.

Figure 45 – CAAFCER #1, 50-55 km contrail cross-section of CO2 (left) lateral integrand, vertical

distribution (right).

0 2 4 6 8 10 12 14 16

x 1010

-200

-150

-100

-50

0

50

100

150

200

250

300

net CPC, no./m3heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

y (m)

z (

m)

A320 CO2 concentrations, ppb, wake length 26-28 nm

-30 -20 -10 0 10 20 30 40 50

-150

-100

-50

0

50

100

150

200

250

366

367

368

369

370

371

372

373

-2 -1 0 1 2 3 4 5 6 7

x 10-5

-200

-150

-100

-50

0

50

100

150

200

250

300

CO2, m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

CO2 ppm Grand total minus CO

2,ppb Background

59

9.1.7.4 BC data

For the BC plume cross-section (Figure 46), EIm was integrated to a BC EIm value of 303

mg/kg.

9.1.7.5 FSSP-100 data

The contrail cross-section, Figure 47, was also bifurcated vertically (like that observed for CN

and CPC data), into lower and upper lobes, joined on the port side, and slanted to the starboard

side. Integration gave AEIn = 5.5113e+13 /kg. By mass, assuming sphericity, AEIm =

7.1758e+08 µg/kg. The MVD distribution (below) showed size homogeneity through the height

of the contrail, 3.5-4 µm.

Figure 46 – CAAFCER #1, 50-55 km contrail cross-section of BC (left) lateral integrand distribution (right).

Figure continued over-page, with caption.

0 0.002 0.004 0.006 0.008 0.01 0.012 0.014 0.016 0.018-200

-150

-100

-50

0

50

100

150

200

250

300

BC, mg/m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

0 1 2 3 4 5 6 7

x 108

-200

-150

-100

-50

0

50

100

150

200

250

300

FSSP, no./m3

heig

ht

above/b

elo

w A

320 p

lane,

zA

320 (

m)

60

Figure 47 – CAAFCER #1, 50-55 km contrail cross-section of ice particle count (top left) lateral integrand,

vertical distribution (top right), and MED cross-section (bottom left).

9.1.7.6 Licor 840A Water Vapour

Relative humidity and RHi distributions are shown in Figure 48. Water vapour depletion is

observed within the midst of the contrail. The surrounding air adjacent to the UJW crown is

super-saturated and, therefore, could be expected to support further contrail crown growth.

Figure 48 – CAAFCER #1, 50-55 km contrail cross-sections of RH (left) and RHi (right).

61

9.2 Overview, assembly & comparison, CN data

9.2.1 Biofuel contrail, 25th April, to 55 km length

An overview is herein provided of CN 7610 aerosol data, which has been assembled for the 25th

April biofuel contrail and plotted with data from other flight campaigns.

As illustrated in Figure 49, CN EIn cross-plotted against cruise altitude. It is seen that there is a

wide range if EIn values, more than two orders of magnitude spread. This covers a variety of jet

fuel compositions (varying Sulphur, for example) and a wide range of various engine and

airframe types. It also includes data from individual engines (on the same airframe), namely the

singular NRC Falcon 20 (two GE CF700 engines) and the NASA DC-8 (four CFM56 engines)

on NASA ACCESS II. The ACCESS II measurements were made from very low Sulphur

content fuels (both 50%HEFA-blend and Jet A), whereas CAAFCER fuels were significant

Sulphur (order of 0.05% Sulphur content). As mentioned, a wide range of engine technology is

also employed in the measurements of Figure 49, covering four decades of development.

The CN EIn data, for a range of contrails, is plotted against engine thrust in Figure 50. Together

with the ACCESS II NRC data points, these were higher thrust levels, representative of typical

jet air transport high altitude cruise (wherefore, optimum cruise Mach Number is in the range of

0.71-0.84, depending upon the type of jet aircraft). On the other hand, the a priori Falcon NRC

data was at lower thrust levels (and Mach Numbers, in the range 0.5-0.6).

Figure 49 – CAAFCER #1, biofuel contrail assembly and comparison of CN EIn data, plotted against cruise

altitude, with that of other flight campaigns.

62

Figure 50 – CAAFCER #1, biofuel contrail assembly and comparison of CN EIn data, plotted against engine

EGT/TS, a measure of engine thrust level.

9.2.2 Contrail FSSP data assemblage

For illustration, the FSSP-100 ice particle count and spherical-mass data of the present biofuel

contrail example has been assembled with other contrail data, and plotted against cruise altitude,

in Figure 51. The data represent the largest ice particle count AEIn and AEIm measured in any

contrail by the NRC CT-133.

3.1 3.2 3.3 3.4 3.5 3.6 3.7 3.8 3.9 4 4.1

1014

1015

1016

ratio of engine exhaust gas temperature / air temperature (K/K)

CN

EIn

#/k

g

Falcon,JetA1,flight #8

" ",JetA1,flight #8

" ",50/50,flight #8

" ",JetA1,flight #6

" ",60/40,flight #6

" ",JetA1,ARA flt

" ",ReadiJet

DC8,JetA,ACCESS

DC8,HEFA,ACCESS

CAAFCER,25thApril

63

Figure 51 – CAAFCER #1, biofuel contrail FSSP-100 AEIn, (top) and spherical-AEIm (bottom), cross-plotted

against cruise altitude, and compared with AEIn of other contrails measured by the NRC CT-133 upon

earlier flight campaigns.

64

FSSP-100 AEIn for the 25th April biofuel contrail is plotted against CN EIn in Figure 52,

illustrating the simultaneously high values of CN aerosol EIn, measured in conjunction with the

contrail ice particle count (AEIn).

Figure 52 – CAAFCER #1, biofuel contrail FSSP-100 AEIn, cross-plotted against CN aerosol EIn and

compared with AEIn ~ CN EIn of other contrails measured by the NRC CT-133 upon earlier flight

campaigns.

10.0 Conclusions The Operations Phase of GARDN project CAAFECR involved biofuel fuel acceptance,

blending, storage, wing-sampling, usage in Air Canada A320/321?B763 aircraft and

measurement of contrails and emissions by the NRC CT-133 flight data, including ultrafine

volatile and non-volatile particulate matter by the University of Alberta CPC3776 counter and

denuder.

These experimental processes, as well as data analysis processes have been described. An

example of contrail analysis, in particular cross-sectional spatial re-construction has been

presented in detail. The methodology has been followed for all biofuel and Jet A1 CAAFCER

contrails and reported upon, separately.

The CAAFCER example contrail had the highest ice particle number (AEIn) and spherical

integration volume (AEIm) of all contrails measured by the NRC CT-133 aircraft, measured a

priori.

1014

1015

1016

1010

1012

1014

CNEIn (#/kg)

FS

SP

-100 E

In n

o./

kg

FSSP-100 EIn ~ CNEIn

FA20,JetA1,7/4/14

JetA,B773,11/4/14

JetA,ACCESS

HEFA,ACCESS

JetA,B763,25/6/14

JetA,A343,27/10/14

JetA,A388,4/12/14

JetA,DC8,I/B

HEFA,DC8,I/B

CAAFCER,25thApril

65

11.0 Acknowledgements CAAFCER project funding has been provided by the Green Aviation Research and Development

Network (GARDN), a non-profit organization funded by the Business-Led Network of Centres

of Excellence (BL-NCE) of the Government of Canada and the Canadian aerospace industry

Technical assistance provided by Steve Baughcum of Boeing has been very influential on the

success of the CAAFCER project. Successful conduct of CAAFCER flight operations (and

quantity of data gathered) involved a huge undertaking and commitment by Air Canada.

12.0 References

1. A P Brown, Matthew Bastian, Mike Pryor, Per Talgoy, “NRC CT-133 ACCESS II

DATA ANALYSIS:- GASEOUS, AEROSOL AND CONTRAIL

CHARACTERISTICS,” Flight Research Laboratory, NRC IFAR NASA ACCESS II Data Workshop, Kissimmee, FL, 9th January 2015

2. A. P. Brown, M. Bastian, S. Alavi, M Wasey, “FLIGHT RESEARCH REPORT:-

PROJECTS AEAFFR, CAAFER AND NASA ACCESS II JET TRANSPORT EMISSIONS MEASUREMENTS,’ NRC LTR-FRL-2015-0054, March 2015.

3. Brown, A.P., “Flight data of axial flows in wake vortex instability,” AIAA AVIATION Forum, 13-17 June 2016, Washington D.C., 8th AIAA Atmospheric and Space Environments Conference, 10.2514/6.2016-3435.

4. Brown, A.P. and Bastian, M., “Derivation of Wake Vortex Circulation from Flight Data using Path Integrals,” AIAA 2007-286, 45th AIAA Aerospace Sciences Meeting

and Exhibit, 8 - 11 January 2007, Reno, Nevada.