Assessment of Contribution to PM10 Concentrations from ...€¦ · •Mohan, M. and S. Bhati...
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Table 1: Directional profile of PM10 for summer 2008-2010
Figure 2: Simulation Domains classified as (A) NorthIndia, (B) India, (C) Asia and (D) Large domain (Asia,Africa and Australia).
Table 2: Maximum level of PM10 obtained and percentage contribution of geographical region (max. observed PM10 value is 1134.5 µg m-3)
Figure 1: Simulated Wind and Pollution Roses for (A) 2-3 May, (B) 4-6 May and (C) 1-4 June 2008-2010 at Delhi
Wind
Direction
PM10 Concentration (the no. shows the
max. avg. value achieved ) (µg m-3)Regions located in the specified
direction2008 2009 2010
E ≤ 25 ≤ 25 ≤ 25 Nepal, China
ESE ≤ 25 ≤ 25 ≤ 25 Bangladesh, Burma, Thailand
ENE ≤ 25 ≤ 25 ≤ 25 China
NW ≤ 75 ≤ 25 ≤ 75 Pakistan, Afghanistan, Russia
W ≤ 300 ≤ 300 ≤ 400 Pakistan, Iran, Saudi Arabia
WNW ≤ 400 ≤ 300 ≤ 300 Pakistan, Afghanistan, Iran
WSW 25-200 ≤ 25 ≤ 50 Pakistan, Saudi Arabia
4. Conclusions
•Based on the simulations for different synoptic conditions during selected summer periods in May-June, 2008-
10, it was observed that high concentrations of PM10 were found to be associated with winds coming from
WNW and West directions. The hourly averaged values of PM10 ranges approximately from 25-400 µg m-3.
PM10 concentrations are lower in cases of winds coming from East direction as compared to winds from West
direction.
• The influence of geographical domain on PM10 based on model simulations revealed that the contributions
due to long range transport outside Indian domain can be as high as 40%. It can be inferred that the high levels
of PM10 concentration is not only due to local pollution but is also highly influenced by remote sources. This
however, shows the contribution to PM10 concentrations from Multiscale Transport.
• It is suggested to perform such simulation studies for other seasons as well as other synoptic conditions, so
that factors that influence PM10 concentrations can be understood.
• In megacity Delhi, particulate matter levels remain persistently high. The regulatory measures should
therefore give due importance to regional and long range transport in policy interventions.
Assessment of Contribution to PM10 Concentrations from Multiscale Transport of Pollutants Using WRF/Chem for A Tropical Urban Airshed
Manju Mohan and Medhavi GuptaCentre for Atmospheric Sciences, Indian Institute of Technology Delhi, India
email: [email protected]
(ii) Influence of different geographical domains on PM10 concentrations
• Table 2 shows the percentage contribution to maximum PM10 concentration simulated due to varying
geographical domain for 3rd June 2010, when highest PM10 value was observed i.e. 1134.5 µg m-3. The
geographical domains are shown in Figure 2.
• Figure 3 represents annually averaged global emission for PM10 for the year 2008.
• In Table 2, the maximum PM10 values achieved for varying domains i.e. Large domain (which includes Asia,
Africa and Australia), Asia, India and North India are shown. Since there is not much difference in the
maximum values of Large and Asia domain it can be said that there is not much influence due to Africa,
Australia and surrounding regions PM10.
• It can be inferred that the high levels of PM10 concentration is not only due to local pollution but is also
highly influenced by remote sources. This however, shows the contribution to PM10 concentrations from
Multiscale Transport. About 60% concentration is due to Indian domain.
• Table 3 gives the statistical analysis of PM10 representing the influence of varying geographical domain for
the simulation leading to maximum concentration in 2010 and shows a reasonable model performance.
3. Results and Discussion
(i) Influence of Synoptic conditions on PM10 concentrations for year 2008-2010
summer season
• 3 periods during summer of 3 years (2008-10) are selected which broadly covered 7
prominent wind directions. Table 1 shows the regions associated to these directions while
Figure 1 depicts wind rose and corresponding pollution rose for these 9 cases. The emissions
are maintained at 2008 level in all cases to extract the impact of only the met. It is inferred
that high concentrations of PM10 are associated with winds coming from WNW and West
direction. PM10 concentrations are lower in cases of winds coming from East direction as
compared to winds from West direction.
1. Introduction and Objective
• The analysis of PM10 with respect to National Air Quality Standards (NAAQS) in India during 2009 revealed that
24-hourly average concentrations exceed standard (100 μg m-3) at 85% of the stations under consideration.
• It is expected that variation of PM10 is not only controlled by the emission rate in PM10 sources at local level alone,
but also by the long range transport as also the met. conditions, dust storms etc. that prevails over Delhi.
• Suitable regulatory mechanisms should include the contributions of various sources and their emissions impacting
the receptors in a given region of interest.
• The main objective of this study is to understand the impact of different geographical domains on PM10
concentration and thereby assess contributions due to multiscale transport over a highly polluted tropical urban
airshed viz; megacity Delhi with due consideration to influences of varying synoptic conditions in the region.
2. Modelling Tools and Simulation Details
• Model: WRF/Chem Version 3.2
• Domains: Three domains of resolution (90km, 30km, 10km)
• Physics option: Lin et al (1983) microphysics, Kain Fritsch
cumulus parameterization, Dudhia shortwave radiation scheme,
RRTM longwave radiation scheme and MM5 Similarity surface
layer- Noah LSM chosen based on sensitivity studies performed
over Delhi (Mohan and Bhati, 2011)
• Chemistry option: RACM gas phase mechanism and
MADE/SORGAM aerosol module
Figure 3: PM10 emissions for 2008 (tons/year). Source: EDGAR
Statistical Parameter
Large Asia IndiaNorth India
Reported values from other studies(Reference)
MNGE (%) 53 50 60 67 <=56 (Zhang et al., 2006)FB (%) -72 -59 -83 -95 ±60 (Spak and Holloway, 2009)
R 0.8 0.77 0.76 0.75 0.57 to 0.92 (Spak and Holloway, 2009)MNB (%) -38 -29 -42 -45 -38 to 35(Zhang et al., 2006)
Table 3: Statistical Parameters evaluation for PM10
References• Mohan, M. and S. Bhati (2011), Analysis of WRF Model Performance over
Subtropical Region of Delhi, India, Advances in Meteorology 2011, 13
• Spak, S. N. and T. Holloway (2009), Seasonality of speciated aerosol transport
over the Great Lakes region, Journal of Geophysical Research 114
• Zhang, Y., P. Liu, A. Queen, C. Misenis, B. Pun, C. Seigneur and S. Wu
(2006), A comprehensive performance evaluation of MM5-CMAQ for the
Summer 1999 Southern Oxidants Study episode—Part II: Gas and aerosol
predictions, Atmospheric Environment 40, 4839–4855
Parent Domain
Maximum
Simulated PM10
(µg m-3)
Percentage
Contribution
(%)
Large (Asia, Africa and Australia) 1041.6 100
Asia 1011 97
India 653.4 62.7
North India 472.3 45.3
Global Atmospheric Watch (GAW) 2013 Symposium and Task Force on
Hemispheric Transport of Air Pollution March 18-22, 2013; WMO, Geneva