SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author:...
Transcript of SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author:...
![Page 1: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/1.jpg)
Quantum Dots
vertical dot
metal grain
metallic SET
nanotube
self assembled
MBE grown
lateral
![Page 2: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/2.jpg)
an electrical engineerspoint of view
lateral vs. vertical
![Page 3: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/3.jpg)
Lateral Dots: Formed in GaAs/AlGaAs 2DEG
CONTACT
Electrons travel in sub-surface layer:
CONTACTGATE
Only lowestsub-band occupiedat low T
++++++++ + + +
Surface
doping layer
Al0.3Ga0.7As GaAs
Fermienergy
Negative voltage on gates depletes underlying electrons & defines dot cavity
GaAs
I (pA)
![Page 4: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/4.jpg)
point contacts
A
B
C 1
2
3
A,B,C : control quantum point contactstransmission to reservoirs
1,2,3: control confinement potential / energy levels only
A
B
C 1 2X
X control dot-internal tunneling rate
gate defined dots
![Page 5: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/5.jpg)
-0.7
-0.6
-0.5
-0.4
-0.3
-0.2
-0.1
VN
OS
E (
V)
-0.6 -0.4 -0.2 0.0VQPC1 (V)
0
2
4 6 8
86420 g (e2/h)
Quantum Point Contact Leads
-300
-200
-100
0
100
200
300
Nos
e (m
V)
-200 0 200QPC2 (mV)
Not all QPCs are beautiful:
6
4
2
0
g (e
2 /h)
150100500VG (mV)
VNOSE
VQPC1
T
1 µmI
slide from A. Huibers, Thesis (1999)
![Page 6: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/6.jpg)
Open vs. Closed
Open Dot Closed Dot
•Vgate set to allow ≥ 2e2/h conductance through each point contact
•Dot is well-connected to reservoirs
•Transport measurements exhibit CF and Weak Localization
•Vgate set to require tunnelling across point contacts
•Dot is isolated from reservoirs, contains discrete energy levels
•Transport measurements exhibit Coulomb Blockade
point contacts
![Page 7: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/7.jpg)
Coulomb Blockade in Closed Dots
Finite energy Ec=e2/Cdot is needed to add an additional electron to the dot. When kT<<Ec charging blocks conduction in valleys.
0.15
0.10
0.05
0.00-200 -198 -196 -194
V (mV)
g (e
2 /h)
N N+1 N+2 . . .
V
1 µm2
Coulomb blockade peaks:resonant transport through dot levels
![Page 8: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/8.jpg)
Electrostatic Energy
apply voltages
what is potential on dot?
voltage divider...
can use Vg to shift dot energy!!
![Page 9: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/9.jpg)
Charging Energy
capacitance of dot to world = C
energy stored in capacitor
charging energy can range from~0 to many meV
Classical Effect, NOT quantum
![Page 10: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/10.jpg)
Constant Interaction Model
: interaction of electron k with rest
constant inteaction: model φk with CΣ
![Page 11: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/11.jpg)
Confinement Energy
harmonic potential
µeV to meV
complicated potential
average level spacing
x
E
quantum mechanical effect!!
![Page 12: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/12.jpg)
Constant Interaction Model
el.chemical potentialµ=0: change Ncurrent flows
total dot energy
addition energy
![Page 13: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/13.jpg)
0.20
0.15
0.10
0.05
0.00-250 -200 -150 -100 -50 0
Quantum Coulomb Blockade
For kT < ∆, each peak describes tunnelling into a single eigenstate. Wavefunction amplitude fluctuations lead to peak height fluctuations.
V (mV)
g (e
2 /h)
V
B=0 mTB=20 mT
kT ~ 3µeV∆ ~ 10µeVEc ~ 200µeV
slide from J. Folk (2002)
![Page 14: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/14.jpg)
Coulomb Diamonds
200nm
VSD
I
kT ~ 1.5µeV∆ ~ 1000µeVEc ~ 2000µeV
differential conductance: peaks when current through dot is changing
![Page 15: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/15.jpg)
Coulomb Diamonds
-eVSD
200nm
VSD
I
peaks in g appearwhen dot levelaligned with eithersource or drainchemical potential
![Page 16: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/16.jpg)
Coulomb Diamonds, Sequential Tunneling Transport
electrons tunnel on / off dotone by one(charging energy)
electrons do not changeenergy when tunneling
dot energy unchanged
![Page 17: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/17.jpg)
Coulomb Diamonds
two slopes, each associated with its respective dot-lead capacitance
Eadd
![Page 18: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/18.jpg)
Excited State Spectroscopy
GS1ES2ES
-eVSDGS1ES2ES
-eVSDGS1ES2ES
-eVSD
only one electron excess electron can be on dot (charging energy)
lab to investigatequantum levelsin device!!
A B C
A B C
quantum confinement energies
internal excitations (spin)
![Page 19: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/19.jpg)
Cotunneling Transport
-eVSD
∆
-eVSD
∆
VSD>∆
white lines: inelastic cotunnelingdot energy changesonly possible for VSD>∆
higher order process: two electrons tunnel and change energy
elastic cotunneling (blue circle)
before tunneling after
dot energy unchanged
dot nowin excitedstate
before tunneling
after
![Page 20: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/20.jpg)
Temperature Regimes
no charging effects, no Coulomb blockade
classical Coulomb blockade (metallic CB)temperature broadenedtransport through several quantum dot energy levels
peak conductance idependent of TFWHM ~ 4.35kT
Γ = ΓL + ΓR escape broadening (tunneling rates)
![Page 21: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/21.jpg)
quantum Coulomb blockadetemperature broadended regimeresonant tunnelingtransport through only one dot level
Temperature Regimes
peak conductance 1/TFWHM ~ 3.5kT
quantum Coulomb blockadelifetime broadended regimetransport through only one dot level
peak conductance e2/h indep. of TFWHM ~ Γ
![Page 22: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/22.jpg)
Temperature Dependence: Theory
∆= 0.01 e2/CkT / e2Ca 0.075b 0.15c 0.3d 0.4e 1f 2
van Houten, Beenakker & Staring, NATO ASI Series
![Page 23: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/23.jpg)
Temperature Dependence: Experiment
Foxman et al., PRB50, 14193 (1994)
crossover 3.5 to 4.3kT peak widthpeak g 1/T dependence: quantum regime T independent: cassical regime
3.5 kT
4.4 kT
inve
rse
peak
hei
ght
peak
wid
th
![Page 24: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/24.jpg)
Line Shapes: Experiments
Foxman et al., PRB47, 10020 (1993)
T-broadened lifetimebroadened
![Page 25: SS06 MesoDots lecture5 - unibas.ch · Microsoft PowerPoint - SS06_MesoDots_lecture5.ppt Author: Dominik Zumbuhl Created Date: 4/20/2006 7:13:21 PM ...](https://reader030.fdocuments.in/reader030/viewer/2022041017/5ecaac4ee047113c4d484f71/html5/thumbnails/25.jpg)
Charge Switching / Telegraph Noise
Elzermann, 2003