Soft X-ray Lensless Imaging and Resonant Imaging Endstation · study of phase transitions –...
Transcript of Soft X-ray Lensless Imaging and Resonant Imaging Endstation · study of phase transitions –...
3/2/2009 2LCLS/SSRL Users' Meeting 2008
Outline
study of phase transitions – single shot experimentsstudy of ultrafast electronic and spin dynamics –pump-probe experiments
soft x-ray resonant imaging endstation (low fluence)plans for high fluence or single shot experiments
3/2/2009 3LCLS/SSRL Users' Meeting 2008
Solid state and its excitations
E. Beaurepaire, et al.,PRL
76, p4250 (1996)
•Electron-Lattice Dynamics•Magnetization Dynamics
3/2/2009 5LCLS/SSRL Users' Meeting 2008
Soft X-ray Fourier Transform Holography
S. Eisebitt, J. Lüning, W. F. Schlotter, M. Lörgen, O. Hellwig, W. Eberhardt, J. Stöhr, Nature 432, 885 (2004)
3/2/2009 7LCLS/SSRL Users' Meeting 2008
Phase Hologram
absorption
phase
absorption reducedby order of magnitudefor comparable image
quality
3/2/2009 8LCLS/SSRL Users' Meeting 2008
Optical Constants
A. Scherz, et al., submitted.
Co L3
n = 1 ¡ ± + i¯Refractive Index
E (eV)776.5 779.5
Re( T )
Im( T )t = 1 ¡ ¹ + iÁweak contrast
3/2/2009 9LCLS/SSRL Users' Meeting 2008
frompump – probe where
time resolution is essentialto
imaging of critical fluctuations wherenumber of photons is essential
3/2/2009 10LCLS/SSRL Users' Meeting 20082D Ising model
T=TC
M=M
0
 = 1kT
Pr ±¾r ±¾0
FMFM PMPM
TC =RT
Cu/Co/Cu(1 1 17)
single shotsingle shotat instant of timeat instant of time
5 μm 2.5 ML Co
FM - PM phase transition
3/2/2009 12LCLS/SSRL Users' Meeting 2008
Dynamics of Critical Fluctuations
¿(Tc )¿o
=³
»(Tc )»o
´ z= 2
»(Tc) » 0.1 ¹ m
¿(Tc) » 80 ¹ s
(T ¡ Tc)=Tc ¼ 10¡ 3
2D Ising Model real spacereciprocal space
3/2/2009 13LCLS/SSRL Users' Meeting 2008
Requirements / Limits for imaging fluctuations
imaging magnetic fluctuations – need the full pulse intensityno “movie” possible, since the pulse drives the system out of equilibriumXPCS may then be possible using (cw) source with average high brightness
3/2/2009 15LCLS/SSRL Users' Meeting 2008
NEW PHASE DIAGRAM
OLD PHASE DIAGRAM
S. Kivelson,Nature materials (News and Views) 5,343 (2006)
Electronic liquid crystal:S.A.Kivelson et al, Nature 393, 550 (1998)
High-Tc superconductor
3/2/2009 16LCLS/SSRL Users' Meeting 2008
BL13-3 Coherent X-ray Scattering
a. Cryostat and sample holderb. in-vacuum CCD on linear stagec. Guard Apertures and magnetd. Coherence apertures / filters
Sample Environment
Soft X-ray coherent Scatteringresonant, polarization dependentX-ray Holography, MAD ImagingX-ray Photon Correlation Spectroscopy
Specs:Energy range 200-1200 eVCCD N.A. = 0.031 - 0.545max. q at 800eV: 2.3 nm-1
30nm resolution demonstrated at cryogenic temperatures
Covers important K and L edges forPolymers, Magnetic Nanostructures, Correlated Materials, Nanocrystals, Biominerals
Experiments
superparamagnetic array of 18nm Fe/FeO nanocubes
T= 15K
resolution ~30nm
SEM
1um
FTH
3/2/2009 18LCLS/SSRL Users' Meeting 2008
CCD Detector
Commercial CCD13.5um pixel size2048x2048 pixels2MHz pixel readout
for 850eV (1.46nm)1.7nm image pixel size @ 30mm18.5nm image pixel size @ 350mm
extras1um Al cover (optical filter)movable beamstop
PI-MTE
3/2/2009 19LCLS/SSRL Users' Meeting 2008
Radiation Damage
unfocused KB system<10uJ/cm2
focused KB system>10uJ/cm2
reflecting beamstop
3/2/2009 20LCLS/SSRL Users' Meeting 2008
Timeline
system using unfocused LCLS beam ready in July ‘09testing at BL 13, SSRL before summer shutdown