Optical diagnostics in fluid mechanics Metrology of particles

63
Optical diagnostics in fluid mechanics Metrology of particles Part 2: Theories Kuan Fang REN Email: [email protected] tel: 02 32 95 37 43 UMR 6614/ CORIA CNRS - INSA & University of Rouen

Transcript of Optical diagnostics in fluid mechanics Metrology of particles

Page 1: Optical diagnostics in fluid mechanics Metrology of particles

Optical diagnostics in fluid mechanics

Metrology of particles

Part 2: Theories

Kuan Fang RENEmail: [email protected]

tel: 02 32 95 37 43

UMR 6614/ CORIA

CNRS - INSA & University of Rouen

Page 2: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Theories of light scattering

II-2

❑ Rigorous theories• Lorenz-Mie theory

• Generalized Lorenz-Mie theory

❑ Approximate models and theories

• Geometric optics → VCRM

•Diffraction

• Ray theory of waves

• Rayleigh theory

•. . . . . .

❑ Numerical methods• T-matrix, DDA

• MoM, FTDT, FEM, …

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➢ Imaging in daily life:

▪ Image by reflection: mirror in car, water surface, summer route …

▪ Image by refraction: fish, stick in water, mirage in the nature …

➢ Optical instruments:

▪ Camera, telescope, microscope, ..

▪ Industrial measurement systems,

▪ Optical fiber for telecommunication

➢ Scientific research:

▪ Fluid mechanics: PIV, holography, LDV, PDA,

▪ Measurement of temperature, size distribution, …

▪ Biological imaging, …

I-3

What is it used for ?

Geometric optics

Advantages:• Simple

• Object of arbitrary

shape

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Geometric optics

II-4

Conditions :

l ≪ lThe wave length l is much longer than the dimension of the object l.

1. Straight propagation

in a homogeneous medium

Imaging

f’

Photography

d’d

Condition and simple applications

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Geometric optics – reflection and refraction

II-5

Reflection and refraction on a surface between two media

Law of Snell-Descartes

'i i=

The velocity of light v depends

on the refractive index n of the

medium:

cn

v=

Reflection:

sin 'sinn i n r=Refraction:

I

i

r

n

n’>n

R’

R

i’

More refractive

medium

Diopter or

refraction surface

Reflection and refraction laws

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Geometric optics – reflection and refraction

II-6

Critical angle

Forbidden zonen’>n

n

2 1

2 1

:

/ 1/1.333 48.6

/ 1/1.500 41.8

l

l

Examples

n n i

n n i

= =

= =

Total reflection

Critical angle:

Total reflection :

n

n’<n

Critical angle

Total reflection

'arcsin

l

n

ni

=

li i

Applications

▪ Optical fiber• Telecommunication

• Transport de laser beam

▪ Critical angle for

measuring bubbles

▪ Optical gauge

▪ Natural mirage

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Geometric optics – reflection and refraction

II-7

Propagation of a light beam

in a parallel stratified

environment:

ni until ij=90°,

i.e. total reflection.

n1

n2

n3

n4

...

npn1>n2 >n3 >… >np

ij

sinj j

n i C=

Total reflection - applications

Application 1:Optical fiber

Application 2:Effect of mirage

grad T grad n

A

A’

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Geometric optics – reflection and refraction

II-8

( )

( )//

tancos cos

cos cos tan

i tt i i t

i t t i i t

n nr

n n

−− =

+ +

( ) ( )/ /

2 cos 2sin cos

cos cos sin cos

i i t i

i t t i i t i t

nt

n n

=

+ + −

( )( )ti

ti

ttii

ttii

nn

nnr

+

−−=

+

−⊥

sin

sin

coscos

coscos

( )

2 cos 2sin cos

cos cos sin

i i t i

i i t t i t

nt

n n

⊥ =

+ +

Fresnel formulas – relation between the amplitudes of the reflected/refracted and incident waves

iE rE iE⊥

rE⊥

, r t

X XX Xi i

X X

E Er t

E E= =

Relation of amplitudes and intensities

ou polarisation state

: amplitude of incidente wave

, amplitudes of reflected/refracted waves

iX

r rX X

X

E

E E

=⊥

tE

tE⊥

iE rEiE⊥

rE⊥

Page 9: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – reflection and refraction

II-9

Forbidden zonen’>n

n

n

n’<n

Inte

nsi

ty r

atio

of

refl

ecti

on

r2

Incident angle

┴║

Total reflection

Critical angle

┴║

Relation of amplitudes and intensities

Brewster angle: i+r=p/2

Page 10: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – propagation of light in a medium

II-10

ds

A

B

Optical path:

dt=m ds

• Phase difference : SrkmrkAB == t )(

• Absorption: ( ) ( )exp( 2 ) ( )exp( 2 )I B I A k I A km Si i

t= − = −

• If m is constant: r

km S =

0exp( 2 )

iI I km S= −

Propagation of light in a medium:

optical path, phase and intensity

Complex refractive index:

r im m im= −

( ) ( )B

AAB m s dst =

Page 11: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

I-11

Can GO be applied to light scattering ?

YES to the simple particles:

▪ Homogeneous sphere,

▪ Homogeneous circular cylinder

Possible for objects of complex shape:

▪ Pure ray model, precision is very limited

▪ Ray model + electromagnetic integration, much better

▪ Ray model + wave properties ➔ Vectorial Complex Ray Model

→ New concept, very precise and easy to use.

Page 12: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

II-12

OA

B

• Intensity :

where p is the scattering order,

X represents the polarization sate

(⊥ or || ), rX Fresnel coefficients.

• Length of the path in the particle:

• Deviation angle de :

Light scattering by a sphere:

Reflection and refraction in a particle

F

E

D

C

0

1

2 sin 'p pa t =

2 2 'p p t t= −

imp

ort

an

t

Page 13: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

II-13

➢Phases:

• Phase difference due to the difference of the optical paths :

• Jump of phase due to reflection on the surface and the focal lines.

1) Reflection: phase of the complex number: rX,

2) Focal lines: phase jump p/2 at each focal line.

cos sin

sin

ip

p

p

Dd

d

t

t

=➢ Divergence factor :

2 2

0 0, 02 2

cos sin

sin

X i Xs p X p

s p p

I dS I a d d aI I D

dS r d d r

t t t

= = =

Reflection and refraction in a particle

SummaryThese equations are enough to calculate the intensity of each order and the total field.

, ,

0

P

Ni

s t s p

p

A I e −

=

=

imp

ort

an

t

Page 14: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

II-14

• Sphere of water

• Polarization ⊥

• Intensity →

at rainbow angle

Without

interference

between

different

modes

Scattering diagram according to geometrical optics

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Geometric optics – application to light scattering

I-15

Scattering diagram of a water droplet: a=50µm, l=0.6328, m=1.333

Page 16: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

II-16

Scattering diagram of a water droplet: a=200µm, l=0.6328, m=1.333

Forward direction First rainbow

LMT - Rigorous theory

GO – approximate method

Page 17: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

II-17

Total intensity with

interference:

A sphere of water or a air bubble in the water illuminated by a plane wave of wavelength of 0.6328 μm.

Comparison with rigorous theory

A homogeneous

sphere

Page 18: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics – application to light scattering

II-18

Total intensity with interferenceA circular cylinder of water with a radius of 5 μm (left) or 10 μm (right) illuminated by a plane

wave with a wavelength of 0.6328 μm.

Geometric optics still work very well for a ~ 10l.

GOGO

A homogeneous infinite cylinder

Comparison with rigorous theory

Page 19: Optical diagnostics in fluid mechanics Metrology of particles

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Preliminary conclusions

➢ By taking into account correctly the interferences, the Ray

model can predict the scattering diagram in ALL directions.

➢ It can be applied to the scattering of any shaped beam.

➢ It works also for a circular infinite cylinder.

Limitations

NOT appropriate for a spheroid or an ellipsoid particle, as well

NO for any irregular shaped particles.

The key problem is the divergence factor.

Geometric optics – application to light scattering

II-19

How to improve the model ?

Page 20: Optical diagnostics in fluid mechanics Metrology of particles

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Geometric optics VCRM

II-20

Possible candidate?

Rigorous theories: the particle shape must correspond to a coordinates

system

Numerical methods: size limited, very time communing

✓ Ray models: precision to be improved

Key problem: lack of wave properties

Our strategy: Extension of ray model- Inclusion of wave front curvature

- Interference between all the rays.

- Diffraction.

Divergence/

Convergence

Phase in

focal linesVectorial Complex Ray Model

Page 21: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

I-21

• Vectorial Complex Ray Model – new

✓ 5 properties of a ray:

1. direction,

2. amplitude,

3. phase,

4. polarizationCla

ssic

al o

pti

csGeometrical optics + wave form

For details:

- Ren et al, Opt. Lett. 36(3), 2011

- http://www.amocops.eu

5. Wave front curvature New

✓ Advantages:• Objects of any shape with smooth surface,• Incident wave of any form,• Sufficiently precise – scattering in all directions,• All scattering properties of the objet.

imp

ort

an

t

Page 22: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

➢ Vectorial complex Ray :

➢ Wave front – curvature matrix:

➢ Surface of dioptry:

➢ Projection matrix:

( )0

ˆ ˆ ˆ( ) p p

Ni i

s p p

p

S A e A e⊥− − ⊥

=

= +k e e

11 12

21 22

q qQ

q q

=

11 12

21 22

c cC

c c

=

1 1 1 2

2 1 2 2

ˆ ˆˆ ˆ

ˆ ˆˆ ˆ

t s t s

t s t s

=

II-22

10

Sphere :1

0

10

Cylinder :

0 0

:

r

Examples

C

r

C r

=

=

Essential of VCRM

Page 23: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

I-23

The rays remain in the same plane – a main direction of the wave front

and the particle surface:

– Spherical particle

– Infinite cylinder at normal incidence

– Ellipsoidal particle in the symmetric plane.

➢ Curvature matrix:

➢ Wave front equation:

R1

t1

t2 s2

s1

1

Special case of the wave front equation

Page 24: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

▪ Sphere

– Reflection:

– Refraction p =1:

After 1st refraction:

After 2nd refraction:

Divergence factor:

▪ Cylinder: R2=∞

▪ Reflection :

▪ Refraction p=1:

1 2

cos 2 1

2 cos 4

aR R D

a

= − = − → =

2

11 12

cos' '

cos cos cos cos

am amR R

m m

= − = −

− −

21 22

cos 2cos 2 cos ( cos cos )' cos '

2( cos cos ) 2( cos cos )(sin sin sin sin )

m a m mR R

m m

− − −= =

− − −

sin(2 )cos

4sin[2( )](cos cos )

mD

m

=

− −

cos

2

aD

=

cos cos

2(cos cos )

mD

m

=

II-24

Theoretical Validation – divergence factor

Identical to the

classical formula

(page II-13).

Page 25: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

II-25

1. Snell-Descartes law:

'=i iReflection:

sin 'sinn i n r=Refraction:

Reflection surface

I

i

r

n

n’>n

R’

R

i

Basic laws of geometrical optics

( )

( )//

tancos cos

cos cos tan

i tt i i t

i t t i i t

n nr

n n

−− =

+ +

( ) ( )titi

ti

itti

ii

nn

nt

−+=

+

cossin

cossin2

coscos

cos2//

( )( )ti

ti

ttii

ttii

nn

nnr

+

−−=

+

−⊥

sin

sin

coscos

coscos

( )ti

ti

ttii

ii

nn

nt

+=

+⊥

sin

cossin2

coscos

cos2

2. Fresnel’s Equations :

The tangent component of

wave vector is continuous

'k kt t

=

VCRM

Page 26: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

II-26

Summary of VCRM

• Fundamental laws

1. Wave front equation:

2. Law of Snell-Descartes in vectors:

• Amplitude:

• Phase:

• Total field:

1

N

diff i

i

E S S=

= +

A D=

inc fl path = + + +

( ) ' ' ' 'i t T T

n nk k C k Q k Q− = −

t t=i tk k

CQQ’

Divergence factor:

Fresnel coefficients: ε

All expressed in wave vector components.

' '' '1 2' ' 12 22

11 21

12 22 1 2

q q

q q

R RR RD R R

R R R R=

'

'

n n

n n

k kr

k k⊥

−=

+

2 '

2 '

n n

n n

m k kr

m k k

−=

+

Page 27: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

II-27

VCRMEll2D : Vectorial Complex Ray Model (VCRM) for Scattering of

plane wave by an Elliptical particle in the 2D plane

1. Module for ray tracing

Available at www.amocops.eu

Page 28: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

II-28

Without reflectionWith reflection

VCRMEll2D : Vectorial Complex Ray Model (VCRM) for Scattering of

plane wave by an Elliptical particle in the 2D plane

2. Module for scattering diagrams

Raw data in VCRMEll2D_raw.datInput parameters:a= 50.0000, b= 60.0000, c= 100.0000, theta0[deg]= 30.0000

m= 1.3330 + 0.0000i, wl= 0.63280, ki= 9.9292, kr= 13.2356

Ray n°: 0 Incident (x,z): -32.7327 75.5929, eki0: 0.5000 0.8660

Order p : 0

Ce: -1.158E-002 -1.837E-002, Ci: 1.000E-014 1.000E-014

Cl: -1.873E+005 -4.541E-009, Cr: 1.751E-002 1.215E-002

ekl: 0.50000 0.86603, ekr: 0.94773 0.31907

kint: 0.00000 9.92918, krnt: 8.75171 9.92918, rfr: -1.00000 0.0

Amplitude: 3.404E+002 Phase: 9.782E+002

Order p : 1

(x,z): 18.5546 92.8596, ekl: -0.10234 -0.99475

ekr: 0.99588 0.09070, phase:-228.7430

Ce: 2.381E-002 2.337E-002, Ci: -3.324E-001 -3.547E-002

Cl: 3.890E-001 7.477E-002, Cr: -6.744E-001 -5.729E-002

kint: 6.87711 -7.16198, krnt: 11.13046 -7.16198, rfr: 0.23620 0.0

Amplitude: 2.737E-001 Phase: 4.150E+001

Order p : 2

(x,z): -1.2843 -99.9670, ekl: 0.00016 1.00000

… …

Page 29: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

II-29

Toward the Ray theory of wave

p=3, a=100 µm

Fig. 3 Comparison of Airy structure calculated

with the three methods.

VCRM can predict much better Airy structure than the Airy theory and can be

applied directly to non-spherical particle.

p=3, a=50 µm

Caustics of GO to be corrected !

Page 30: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Oblate:

a = c = 139.17 µm

b = 133.86 μm,

a/b = 0.8938, 0.9608, 0.9816 (eq. Vol)

m = 1.4465

λ = 0.6328 µm

Vectorial Complex Ray Model

Experimental set-up results

II-30

Page 31: Optical diagnostics in fluid mechanics Metrology of particles

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Comparison of VCRM and experimental normalized equatorial scattering diagrams for the droplets

of 3 different aspect ratios. From (a) to (c), the droplet's aspect ratio b/a increases and refractive

index decreases when the amplitude of the acoustic field is reduced.

Fig. 3 in Opt. Exp. 2015

Onofri, Ren et al

DEHS: Di-Ethyl-Hexyl-

Sebacat

HUDC: Hyperbolic

Umbilic

Diffraction

Catastrophe

Comparison with VCRM

Vectorial Complex Ray Model

II-31

Caustics of GO to be corrected !

Page 32: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

Scattering of a pendent droplet

Scattering patterns

around rainbow

angles

Experiment

Simulation

with VCRM

Page 33: Optical diagnostics in fluid mechanics Metrology of particles

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Vectorial Complex Ray Model

Scattering patterns in

forward direction

Simulation

with VCRM

Experiment

Page 34: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

− Morphology

(a, b)

− Refractive index

m

− Time evolution

a(t), b(t), m(t)

(a) Principal radii measured with the rainbow refractometer and imaging system

and (b) corresponding evolution of the droplet refractive index during the course

of the experiment.

Application to Characterization of non-spherical droplets

Vectorial Complex Ray Model

II-34

Page 35: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Diffraction

II-35

The diffraction is the behavior of waves when they encounter an obstacle.

The phenomenon of diffraction is manifested when• the dimension of the object is of the order of the wavelength,• there is a brutal variation of the density / amplitude of the wave.

A wave diffracts around an obstacle Diffraction effect in a rainbow.Diffraction by a double slit.

Phenomena of diffraction

Page 36: Optical diagnostics in fluid mechanics Metrology of particles

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Diffraction

II-36

Principle of Huygens–Fresnel(1) The contribution of Huygens (1678)

The wave of light propagates step. Each surface

element reached by it behaves as a secondary source that

emits spherical wavelets. The new wavefront is the envelop

of the wavelets and the amplitude of each wavelet is

proportional to the size of the element.

t+t

(2) The contribution of Fresnel (1818)

The complex amplitude of the wave at one point is

the sum of the complex amplitudes of all the secondary

sources at that point. All these waves interfere to form the

wave at the considered point.

t

Theory of diffraction

Page 37: Optical diagnostics in fluid mechanics Metrology of particles

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Diffraction

II-37

Fresnel diffraction (R is small):

Fraunhofer diffraction (R → infinity):

Theory of diffraction

Page 38: Optical diagnostics in fluid mechanics Metrology of particles

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Diffraction

II-38

Diffraction by circular disk (sphere):

A circular hole of radius r :

Be cause of the revolution symmetry,

we can place in the plane of the disk

with the origin at the center:

( )2

1

0

sin

sin

JI I

=

=2pr/l

Applications

cos , sin ,x y dS dxdy d d = = = =

𝑎 = sin , β = 0

Page 39: Optical diagnostics in fluid mechanics Metrology of particles

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Diffraction

II-39

Rayleigh criterion:

The first minimum of J1(x) is located at x=3.832, i.e.:

1.22

D

l =

D

écran

A1

A2

So it is interesting to have an large opening

for a better resolution (telescope, camera, ...)

Applications

Page 40: Optical diagnostics in fluid mechanics Metrology of particles

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Diffraction and Interference

II-40

Diffraction by a single slit: 2

0 2

sin uI I

u=

Width of the central spot: 0

2DL

a

l=

Yong’s slits: N=2

fringe :D

ib

l=

22

0 2

sincos

u bI I u

au

=

Applications

2 2

0 2 2

sin sin

sin

u NvI I

u v=

sin sin,

a bu v

p p

l l= =

N slits:

Page 41: Optical diagnostics in fluid mechanics Metrology of particles

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VCRM + Phys. Opt. ➔ Reay theory of waves

I-41

Page 42: Optical diagnostics in fluid mechanics Metrology of particles

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VCRM + Phys. Opt. ➔ Reay theory of waves

➢ Physical optics

▪ Recall of Airy theory (1838)

» with approximation the vicinity of 𝜽𝑹 the

phase is a cubic function:

𝑢 =ℎ𝑣3

3𝑎2with ℎ =

𝑝2−1 2

𝑝2𝑝2−𝑚2 1/2

𝑚2−1 3/2

» And assuming a constant amplitude for all

emergent rays, the amplitude of the scattered

wave is give by (extending v to infinity):

• The version of van de Hulst (1957) permits to predict the profile,

• But the absolute or relative intensity?

I

O ( )go m

G.O.

Airy theory

v

u

Page 43: Optical diagnostics in fluid mechanics Metrology of particles

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Ray theory of waves

➢ Physical optics

▪ Reexamination of Airy theory

» Some typical results in the literature:

» Tricker: in the book “Introduction to

meteorological optics” 1970

𝐴~ 𝑎/λ

» Nussenzveig: JOSA 1979 :

𝐴~(𝑎/λ)7/6

» Hovenac & Lock: JOSA A 1992

» R. Lee: Appl. Opt. 1998

Airy & Mie

Perpendicular polarizationHovenac & Lock 1992

Airy differs from Debye and difference increases with p

=1000 → a=160 λ=1000 → a=160 λ

Perpendicular polarizationNussenzveig PRL (1974), JOSA A (1979)

Airy fails for pparallel polarization!!

=1500 → a=240 λ

Page 44: Optical diagnostics in fluid mechanics Metrology of particles

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Ray theory of waves

➢ Physical optics

▪ Airy theory in RTW to remove the two approximations

» Phase: = 𝑄 − 𝐶 − 𝑘𝑃𝑅with

» Amplitude: 𝑨𝑷= 𝑨𝑄𝑮𝑸′

𝑮𝑷

𝑮𝑿 and 𝑮𝑋′ are the Gaussian curvatures at point X before/after interaction.

IV-44

Conclusions:▪ Both phase and amplitude are calculated numerically, so rigorously, ▪ No any hypothesis,▪ Same method for non-spherical particle.

Page 45: Optical diagnostics in fluid mechanics Metrology of particles

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Ray theory of waves

➢ Physical optics

▪ Airy theory in RTW – Validation of the results:

Comparison of the total intensities calculated by four methods

IV-45

perpendicular polarization parallel polarization

The results of Ray Theory of Waves (green curves) are in very good agreement with Debye (black curves).

Page 46: Optical diagnostics in fluid mechanics Metrology of particles

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Application of RTW

➢ Generalized rainbow patterns

IV-46

Duan et al OL 2021

Quantitative comparison of VCRM with experiment.

Excellent agreement in all range.

Zhang, Rozé & Ren, ELS 2021

Page 47: Optical diagnostics in fluid mechanics Metrology of particles

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Rayleigh theory

II-47

1 1 11 cos

2cos

2

d

dr r rr

Electric fields• Two charges +q et – q

• Distance b/t them: d

• Dipole moment : p=qd

2

1 1

4

cos4

dipôle

ext

ext

q

r r

p

r

p

p

+ −

= −

Static field of a dipole

Page 48: Optical diagnostics in fluid mechanics Metrology of particles

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Rayleigh theory

II-48

Electrostatic approximation

Conditions:1. Electric field

• static

• uniform

2. Size of the particle: l<<l

Potential of the induced field:

“Scattered” field:2

3.02

4sin

2

i ext

i ext

E a E er

p

l

−=

+

3

.02

cos2

i extext

i ext

aE

r

−=

+

4 2

2

,

8 1 = Re

3 2ext

d

d mQ

m

l

p

l

+

Field scattered by an induced dipole

Page 49: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Rayleigh theory

II-49

Scattering diagram

Elements of scattering matrix:3

14

ikS

p= −

3

2 cos4

ikS

p= −

Perpendicular polarization Parallel polarization

Field scattered by an induced dipole

Page 50: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Lorenz-Mie Theory - LMT

II-50

Conditions:

1. Incident plane wave

2. Particle :

• Spherical

• Homogeneous or central

stratified

• Isotropic

Electromagnetic field:En = An Rn(r) () ()

Hn = Bn Rn(r) () ()

Boundary conditions :

, , ,

, , ,

i s e

i s e

E E E

H H H

+ =

+ =

Conditions and principle

Page 51: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Lorenz-Mie Theory - LMT

II-51

Incident wave:

( )( )

( ) ( ) ( )

( )( )

( ) ( ) ( )

tp

pt

EE

HH

EE

HH

Sikrkr

Eiba

nn

nikr

kr

EE

Sikrkr

iEiba

nn

nikr

kr

iEE

HE

n

nnnn

n

nnnn

rr

0

0

0

0

1

1

00

2

1

00

sinexpcoscos1

12sinexp

cosexpcoscos1

12cosexp

0

−=

=

−−

=++

+−

−=

−=++

+−=

==

=

=

( )( ) ( )

=+

+

+=

1

1

12 sin

coscos

1

1211

n

nnni

TE

i

TM Pkrnn

n

ikU

U

Scattered field (far region):

an, bn scattering Mie

coefficients dépending on the

proprieties of the particle

tn, pn angular functions

of Legendre

S1, S2 elements of the

scattering matrix

Conditions and principle

Page 52: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Lorenz-Mie Theory - LMT

II-52

Scattered intensities:

I⊥()=|S1|2

I||()=|S2|2

Efficiency sections :

Cext=Csca+Cabs

Radiation pressure :

Cx=Cy=0

Physical quantities

Page 53: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Generalized Lorenz-Mie Theory - GLMT

II-53

Conditions:1. Incident wave: any shape

2. Particle :

• Spherical

• Homogeneous or centrally stratified

• Isotropic

Particularities:1. When the object is big, the illumination

is not uniform,

2. The incident wave is described by two

series of coefficients :

Conditions and principle

Page 54: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Generalized Lorenz-Mie Theory - GLMT

II-54

Scattered field

Elements of scattering matrix:

Expressions of scattered fields

Page 55: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Generalized Lorenz-Mie Theory - GLMT

II-55

Scattering diagram

Scatterin angle [°]

340320300280260240220200180160140120100806040200

log(

I)

7

6

5

4

3

2

1

0

Scattering diagram

Scatterin angle [°]

350300250200150100500

log(

I)

6

5

4

3

2

1

0

-1

-2

-3

Scattering diagram

Scatterin angle [°]

340320300280260240220200180160140120100806040200

log(

I)

6

5

4

3

2

1

0

-1

Particle :

a = 5 µm

m = 1.33

Gaussian beam:

l = 0.6328 µm

w0 = 5 µm

Plane wave

on-axis Gaussian beam

on-axis Gaussian beam: d=w0

Scattering diagram:

On axis - symmetric

Off axis - non-symmetric

Scattered field – plane wave/Gaussian beam

Page 56: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

TLM and TLMG for a sphere

II-56

iE

iH

n,TMgm

n,TEgm

na

nb s

Es

H

I

P

Structure of TLMG

Case of a sphere

Page 57: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

GLMT for a cylinder

II-57

Introduction of the method plane wave expansion

iE

iHn,TM

I (g )

n,TEI (g )

sE

sH IanI, anII

bnI, bnII

Structure of TLMG

Case of an infinite cylinder

Page 58: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Debye theory

II-58

Structure of Debye theory

( )22 22

1 12 2112 21 11

111

1 11 1

2 2 1

p

n n nn n n n n

pn n

a T TR T T R R

b R

=

= − − = − −

' '11

' '

( ) ( ) ( ) ( )

( ) ( ) ( ) ( )

n n n nn

n n n n

x y x yR

x y x y

−= −

' '22

' '

( ) ( ) ( ) ( )

( ) ( ) ( ) ( )

n n n nn

n n n n

x y x yR

x y x y

−= −

12

' '

2

( ) ( ) ( ) ( )n

n n n n

iT

x y x y =

21 1

' '

2

2

( ) ( ) ( ) ( )n

n n n n

n iT

n x y x y =

21 12 1

2' '

2

4

( ) ( ) ( ) ( )n n

n n n n

nT T

n x y x y

−=

1 2/ pour

1 pour

n

n

n n a

b

=

1 2

1 pour

/ pour

n

n

a

n n b

=

The Mie coefficients are developed in series, so it is

a) rigorous,

b) applied to any wave.

An rigorous theory interprets the

scattering in the language of GO.

Page 59: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

ABSphere – software for all physical quantities

II-59

ABSphere

• Plane wave• Gaussian beam• Bessel beam• Dognut beam

✓ Scattering diagrams

✓ Radiation pressure

✓ Efficiency factors

▪ Internal field

▪ External field

▪ Far field

o Total field

o Field of each mode

o Effect of shaped beam

➢ Fluid mechanics

➢ Combustions

➢ Environment science

➢ Life science

➢ … …

- Rainbow refractometry

- Extinction spectroscopy

- Holography

- PDA, PIV,

To be download from:

www.amocops.eu

Page 60: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Scattering of a pulse by a sphere

II-60

t = 3400

t = − 120 t = 20

Internal fieldsHomogeneous sphere

d=40 µm, t=50 fs

Gaussian beam

t = 120 t = 1080

Scattering of a Gaussian beam by a sphere

Page 61: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Scattering of a pulse by a sphere

II-61

t = 3400

t = − 120 t = 20

Internal fieldscoated sphere

de=40 µm, di=20 µm

t=50 fs

Plane wave

t = 120 t = 1060

Scattering of a plane wave by a coated sphere

Page 62: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Scattering of a pulse by a sphere

II-62

Scattering of a Gaussian pulse by a sphere

Page 63: Optical diagnostics in fluid mechanics Metrology of particles

Course M2 EFE – Rouen University

Exercise on geometrical optics

I-63

1. Under what condition can the geometrical optics be used?

2. A light ray arrives on a surface separating two media of different refractive indices. The two figures

below represent the reflection coefficients as a function of the incident angle i in the two cases: from a

more refractive medium to a less refractive and from a less refractive medium to a more refractive.

- To which case does each of these two figures correspond?

- What does each of the two curves represent in the figures?

- Why is there a plateau in the right figure from 41.8°? Deduce the ratio of the refractive indices of the

two media.

- What is the angle of 56.3° in the left figure and 33.7° in the right figure? Explain this phenomenon.

3. A light ray of wavelength l= 0.488 µm penetrates into a medium of index m = 1.35−0.001i. What is the

speed of light in this medium? What is the characteristic depth of penetration defined by I() = I(0)/e2.