On the intercontinental transport of Pollutants; Modeling Studies

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Environmental Modeling Center ______________________________________________ Climate Change and Air Quality Workshop MCNC On the intercontinental transport of Pollutants; Modeling Studies Adel Hanna, Rohit Mathur, Aijun Xiu, Kiran Alapaty, Uma Shankar, and Zac Adelman MCNC-Environmental Modeling Center P.O. Box 12889 Research Triangle Park, NC 27709-2889 USA

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On the intercontinental transport of Pollutants; Modeling Studies. Adel Hanna, Rohit Mathur, Aijun Xiu, Kiran Alapaty, Uma Shankar, and Zac Adelman MCNC-Environmental Modeling Center P.O. Box 12889 Research Triangle Park, NC 27709-2889 USA. Outline. Flux of Pollutants - PowerPoint PPT Presentation

Transcript of On the intercontinental transport of Pollutants; Modeling Studies

Environmental Modeling Center

______________________________________________ Climate Change and Air Quality Workshop

MCNC

On the intercontinental transport of Pollutants; Modeling Studies

Adel Hanna, Rohit Mathur, Aijun Xiu, Kiran Alapaty,

Uma Shankar, and Zac Adelman

 

MCNC-Environmental Modeling Center

P.O. Box 12889

Research Triangle Park, NC 27709-2889

USA 

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Environmental Modeling Center

______________________________________________ Climate Change and Air Quality Workshop

MCNC

Outline

Flux of Pollutants Integrated Modeling Approach Intercontinental Transport Model Evaluation and Remote Sensing Data

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1- Flux of Pollutants Characterization of Synoptic Patterns

Southwest flow at the surface ahead of a cold front approaching the Northeastern US. (e.g., June 7-8 and 10-11, 1995)

A surface high pressure extending over the middle Atlantic and Northeastern US. An OMEGA pattern at 500 mb. Re-circulation over the Southeastern US (e.g. June 16-17-18, 1995)

A surface low pressure over central US June and OMEGA pattern at 500 mb (e.g. June 26 – 27, 1995)

Large-scale circulation with surface high pressure and 500 mb high pressure (e.g., July 14 and 15, 1995)

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Surface and 500 mb MeteorologyJune 7, 1995 June 8, 1995

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O3 Daily Average Flux (June 7 & 8)

July 7, 1995

July 8, 1995

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Vertical Cross-Section of Zonal Flux- O3 (June 7 &8)

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Vertical Distribution of Daily Average Eastward O3 Flux for June-July, 1995

0 500 1000 15000.01

0.1

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10Percentiles of Distribution

5th50th95thMax

Eastward O3 Flux (g m-2 s-1)

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Export of O3 Pollution from Eastern United States

Other Studies– 1.1 Gmol/day [Parrish et al., 1993] ;

measurements– 1.6 Gmol/day [Jacob et al., 1993];

global model– 3.2 Gmol/day [Banic et al., 1996];

measurements

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5 15 25 35 45 55

EastwardNorthward

Days (June/July 1995)

Mean = 2.25 Gmoles/day

June 1 July 31

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2- Online Integrated Meteorology Atmospheric Chemistry Calculations Atmospheric Aerosol Loading: Radiative Effects

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0 5 10 15Concentration (g/m3)

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0.05 0.1 0.15 0.2 0.25 0.3Diameter (m)

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150 200 250 300 350 400 450 500Number Density (Number/cm3)

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3- Intercontinental TransportMAQSIP Pacific Simulations: April 15-30, 1998

Period characterized by two intense dust storms on April 15th and 19th

NASA TOMS Aerosol Index shows large-scale signatures of dust coverage over the Pacific on April 21, 1998

Time period provides an opportunity to examine and study– Transport characteristics of outflow– Effects of superposition of emissions from different regions on pollutant

distribution– Long range transport impacts on chemical composition over the Pacific

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Transport and Chemical Evolution of Sulfate at 850 mb

April 20, 1998

April 21, 1998

April 22, 1998

Daily Average

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Transport and Chemical Evolution of Ozone at 850 mb

April 21, 1998

April 22, 1998

April 23, 1998

Daily Average

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Six Day Back Trajectories

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4- Model Evaluation and Remote Sensing DataObserved and Simulated CO

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Charge Questions

How to obtain reliable emissions which are missing from major urban areas in many countries out side North America and Europe?

How to reconcile the differences between global, regional, and field measurements estimates of pollution export ?

The indirect effects of aerosols and the microphysics of clouds are crudely parameterized in regional air quality models