Electromagnetic scattering laws in Weyl...
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Electromagnetic scattering laws in Weyl systemsMing Zhou1, Lei Ying1, Ling Lu2, Lei Shi3, Jian Zi3 & Zongfu Yu1
Wavelength determines the length scale of the cross section when electromagnetic waves
are scattered by an electrically small object. The cross section diverges for resonant scat-
tering, and diminishes for non-resonant scattering, when wavelength approaches infinity. This
scattering law explains the colour of the sky as well as the strength of a mobile phone signal.
We show that such wavelength scaling comes from the conical dispersion of free space at
zero frequency. Emerging Weyl systems, offering similar dispersion at non-zero frequencies,
lead to new laws of electromagnetic scattering that allow cross sections to be decoupled from
the wavelength limit. Diverging and diminishing cross sections can be realized at any target
wavelength in a Weyl system, providing the ability to tailor the strength of waveโmatter
interactions for radiofrequency and optical applications.
DOI: 10.1038/s41467-017-01533-0 OPEN
1 Department of Electrical and Computer Engineering, University of Wisconsin, Madison, Madison, 53705, USA. 2 Institute of Physics, Chinese Academy ofSciences and Beijing National Laboratory for Condensed Matter Physics, Beijing, 100190, China. 3 Department of Physics, Fudan University, Shanghai,200433, China. Correspondence and requests for materials should be addressed to Z.Y. (email: [email protected])
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E lectromagnetic scattering is a fundamental process thatoccurs when waves in a continuum interact with an elec-trically small scatterer. Scattering is weak under non-
resonant conditions; an example is Rayleigh scattering, which isresponsible for the colours of the sky. Conversely, scatteringbecomes much stronger with resonant scatterers, which have aninternal structure supporting localized standing waves, such asantennas, optical nanoresonators, and quantum dots. Resonantscatterers have wide application because the resonance allowsphysically small scatterers to capture wave energy from a largearea. As such, large electromagnetic cross sections, ฯ, are alwaysdesirable: a larger ฯ value means, for example, stronger mobilephone signals1 and higher absorption rates for solar cells2.
The maximum cross section of resonant scattering is boundedby the fundamental limit of electrodynamics. One might be
tempted to enlarge the scatterer to increase the cross section, butthis strategy only works for non-resonant scattering, or elec-trically large scatterers. In resonant scattering, physical size onlyaffects spectral bandwidth, while the limit of cross section isdetermined by the resonant wavelength ฮป as3:
ฯmax ยผDฯฮป2 รฐ1ร
The directivity D describes the anisotropy of the scattering; D = 1for isotropic scatterers. Equation 1 shows that an atom4 can havea ฯmax similar to that of an optical antenna5, despite the sub-nanometre size of the atom. This also means that optical scat-terers cannot attain resonant cross sections as large as those ofradiofrequency (RF) antennas, due to the smaller wavelengthsinvolved.
k k
Weyl point
Atom
RF antenna
1 1
!2 โ!2โ!
Weyl pointDC
a b
c
!
! !
!=ck
" "
!
Fig. 1 The length scale of cross section and its relation to dispersion. a In free space, the resonant cross section scales according to ฯ $ ฮป2 or $ 1=ฯ2. Largecross sections always favour low frequencies. For example, the cross section of an optical transition in an atom is small (~10%12 m2) because of theassociated short wavelength (~ฮผm). The cross section of an RF antenna is much larger (~10%4 m2) due to a much longer wavelength (~cm). Diverging crosssections are obtained around the DC point, which happens to be the apex of a conical dispersion. The double lines indicate double degeneracy due topolarization. b By embedding the resonant scatterer in a medium where the dispersion of the continuum exhibits conical dispersions located away from theDC point, diverging cross sections can be realized at high frequencies. The cross section scales according to $ 1=ฮฯ2, where ฮฯ is the relative detuningbetween the resonant frequency of the scatterer and the Weyl point. In both a and b, regions with stronger colour indicate larger resonant scattering crosssection. c Schematic of extraordinarily large cross section created by an electrically small resonant scatterer (red dot) placed inside Weyl photonic crystal
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Overcoming the limit just described has far-reaching implica-tions for RF and optoelectronic applications. Many efforts havebeen devoted to realizing this goal, including the use of enhanceddirectivity D6โ10, degenerate resonances11, decreased dielectricconstants12 ฯต and materials with negative refractive index13.While these approaches exploit certain trade-offs to slightlyincrease the pre-factor in Eq. (1), the fundamental limit of ฮป2
remains, which can be proven directly from Maxwellโs equationswithout requiring specific scatterer details5. Until now, extremelylarge cross sections have only been obtained at long wavelengthsnear the DC frequency.
Here we show that the scattering laws in Weyl systems14 allowsthe cross section to be decoupled from the wavelength limit. Thisopens a new path to realizing strong waveโmatter interaction,providing potential benefits to RF and optoelectronic devices thatrely on resonant scattering. Moreover, the scattering effect dis-covered here is equally applicable to acoustic or electronicwaves15โ17.
ResultsLength scale of the cross section. In free space, the dispersiondirectly leads to the wavelength limit of the cross section, which isshown by Eq. (1). Specifically, the DC point, which is located atthe apex of the conical dispersion relation as shown in Fig. 1a,gives rise to the diverging cross sections at low frequencies. The
apex of the conic dispersion can be also realized at other spectralregimes, such as that shown in Fig. 1b. All the special scatteringproperties associated with the DC point can be reproduced,resulting in diverging cross sections and exceptionally stronglightโmatter interactions at high frequencies. Weyl points14, 18โ28,the three-dimensional (3D) analogy of Dirac points, have recentlybeen shown to exhibit such conical dispersion relations. Thescattering laws in Weyl systems allows the cross section to bedecoupled from the wavelength limit. Extraordinarily large crosssection can be realized even for very small scatterers inside a Weylphotonic crystal, which is schematically illustrated in Fig. 1c.Unlike the lensing effect that can concentrate incident waves to afixed focus, the scatterer concentrates incident waves to itself nomatter where it is placed inside the Weyl photonic crystal.
Conservation law of resonant scattering. To illustrate theunderlying physics of the relation between the dispersion andcross section, we will first show a conservation law of resonantscattering. We start by considering the resonant cross section of adipole antenna (Fig. 2a). Without losing generality, we only dis-cuss the scattering cross section, assuming zero absorption.Similar conclusions can be drawn for the absorptive case, with themaximum absorption cross section 1
4 that of the scattering crosssection29.
The dipole antenna is anisotropic due to its elongated shape, sothe cross section ฯรฐฮธ;ฯร depends on the incident direction of thewave. At a normal direction, when ฮธ ยผ ฯ=2, it reaches itsmaximum value5 of ฯmax ยผ 3ฮป2=2ฯ. Along the axial direction,when ฮธ ยผ 0, the cross section vanishes. While it is straightfor-ward to calculate the cross section of a dipole antenna, it is notimmediately apparent why the cross section follows the ฮป2 ruleand diverges around the DC frequency.
Figure 2b shows the real-space representation of ฯรฐฮธ;ฯร at theresonant frequency ฯ0. We can also represent ฯรฐฮธ;ฯร inmomentum space as ฯรฐkร, with k located on the isosurfacedefined by ฯ ยผ ฯ0. As shown in Fig. 2c, the isosurface is a spherewith jkj ยผ ฯ0=c. To visualize the momentum-space representa-tion, ฯรฐkร is indicated by the colour intensity on the isosurface inFig. 2d. As we show in Supplementary Note 1, the resonant crosssection satisfies the following conservation law:
โฌs:ฯ kรฐ รยผฯ0
ฯ kรฐ รds ยผ 16ฯ2 รฐ2ร
The integration is performed on the isosurface ฯ kรฐ ร ยผ ฯ0. Ourproof is based on quantum electrodynamics30, so it applies toclassical scatterers such as antennas, as well as to quantumscatterers such as electronic transitions that absorb and emit light.More importantly, the continuum, in which the scatterer isembedded, does not need to be free space; it can be anisotropicmaterials, or even photonic crystals31, as long as a well-defineddispersion relation ฯ ยผ ฯรฐkร exists.
Equation 2 dictates the scaling of ฯ with respect to the resonantfrequency ฯ0 of the scatterer. As ฯ0 decreases, the area of theisosurface shrinks. To conserve the value of the integration over asmaller isosurface, the cross section ฯ kรฐ ร must increase accord-ingly. For example, Fig. 2e and f show the isosurfaces of dipoleantennas with resonant frequencies at ฯ0=2 and ฯ0=3, respec-tively. The cross sections, indicated by colour intensity, mustincrease proportionally to maintain a constant integration overthese smaller isosurfaces. This can also be seen by the averagecross section in the momentum space:
ฯ &โฌ ฯ kรฐ รdsโฌ ds
ยผ 16ฯ2
Sรฐ3ร
Real spacea b
c d
e f
z
yx
kz
ky
kx
#
Incident
"(k)ds
Momentum space
Isosurface
Dipoleantenna
k
$
"($, #)
"(k)/"d
"(k)
!0
!0/3!0/2
1.0
0.8
0.6
0.4
0.2
Fig. 2 Scaling law of resonant cross sections in momentum space. aSchematic of a dipole antenna in free space. b Real-space representation ofscattering cross section ฯ ฮธ;ฯรฐ ร. c In the momentum space, the crosssection is represented by ฯรฐkร, with k located on the isosurface defined bythe resonant frequency. d The cross section ฯรฐkร of the dipole antenna isrepresented by the colour intensity on the isosurface. e The cross section ofa dipole antenna operating at a lower resonant frequency of ฯ0=2. Theisosurface shrinks by half compared to d. The cross section increases asindicated by stronger colours. f Same as e but with an even smallerresonant frequency of ฯ0=3. d, e and f all use the same colour map so thatthe cross section can be directly compared. The cross section is normalizedby ฯd ยผ 27ฮป20=2ฯ
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Here, S & โฌ ds is the area of the isosurface. When approachingthe apex of the conical dispersion relation, the isosurfacediminishes, i.e., S ! 0. As a result, the cross section divergesaround the DC point (Fig. 1a).
Resonant scattering in Weyl photonic crystal. Recent demon-strations of Weyl points in photonic crystals18 show that thedispersion of a 3D continuum can exhibit conical dispersion atany designed frequency (Fig. 1b). The Hamiltonian for the con-tinuum around the Weyl point is given byH qรฐ ร ยผ vxqxฯx รพ vyqyฯy รพ vzqzฯz , where ฯx;y;z are Pauli matrices.The momentum q qx; qy; qz
! "ยผ k % kWeyl defines the distance to
the Weyl point in the momentum space, and q= 0 at the Weylpoint. The linear dispersion described by this Hamiltonian pro-duces an ellipsoidal isosurface that encloses the Weyl point. Theisosurface shrinks to a point at the Weyl frequency ฯWeyl. Scat-tering properties associated with the DC point are carried to highfrequencies within Weyl medium, resulting in exceptionallystrong resonant scattering. As illustrated in Fig. 1b, the averagecross section scales as ฯ $ 1
ฯ0%ฯWeylรฐ ร2 around the Weyl point. This
allows high frequency resonant scatterers, such as atoms andquantum dots, to attain large cross sections, potentially at amacroscopic scale.
We now demonstrate a specific example of resonant scatteringin a Weyl photonic crystal22. We consider a localized resonantscatterer in an infinitely large photonic crystal. The simulationsare performed in two steps. First, we numerically calculate theeigenmodes of the resonant frequency in the Brillouin zone byusing MIT photonic bands32 (MPB). Next, we use eacheigenmode as excitation and numerically calculate the scatteringcross section by using the quantum scattering theory wedeveloped recently33, which is described in detail in Supplemen-tary Note 2.
The structure of the Weyl photonic crystal consists of twogyroids, as shown in Fig. 3a. The magenta gyroid is defined by theequation f rรฐ ร>1:1, where f rรฐ ร ยผ sinรฐ2ฯx=aร cosรฐ2ฯy=aร รพsinรฐ2ฯy=aร cosรฐ2ฯz=aร รพ sinรฐ2ฯz=aร cosรฐ2ฯx=aร and a is thelattice constant. The yellow gyroid is the spatial inversion of themagenta one. The two gyroids are filled with a material with adielectric constant of ฯต ยผ 13. To obtain Weyl points, we add fourair spheres to the gyroids to break the inversion symmetry(Fig. 3a). These spheres are related by an S4รฐzร transformation.The resulting band structure has four isolated Weyl points at thesame frequency of ฯWeyl ยผ 0:5645 รฐ2ฯc=aร. Figure 3b illustratesconical dispersion in the 2kz ยผ %kx % ky plane.
The resonant scatterer is a quantum two-level system (TLS)embedded in the above photonic crystal. We numerically solvethe scattering problem using quantum electrodynamics33, 34. TheHamiltonian is ยผ Hpc รพ HTLS รพHI. The first two terms, Hpc ยผP
q !hฯqcyqcq and HTLS ยผ !hฯ0byb, are the Hamiltonian of thephotons and the TLS, respectively35. Here, !h is the reducedPlanck constant, bโ and b are the raising and lowering operatorsfor the quantum dot, respectively, and cyqand cq are the bosoniccreation and annihilation operators of the photons, respectively.The Lamb shift35 is incorporated into the resonant frequency ฯ0.The third term, HI ยผ i!h
Pq gqรฐcyqb% cqbyร, is the interaction
between the TLS and the radiation. The coupling coefficient isgq ยผ d ( Eq
ffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiฯ0=2!hฯต0L3
p, where d is the dipole moment, ฯต0 is
vacuum permittivity, Eq is the unit polarization vector of thephotons and L3 is the quantization volume.
Scattering inside photonic crystals is much more complex thanthat in free space. The continuum is highly dispersive, anisotropicand non-uniform, and thus the scattering cross section dependsstrongly on the location of the scatterer and orientation withinthe photonic crystal.
As an example, we consider a TLS with a transition frequencyฯ0 slightly below the Weyl frequency:ฯ0 % ฯWeyl ยผ %0:0005 รฐ2ฯc=aร. The calculated cross sectionฯ qรฐ ร (see Supplementary Note 2 for derivation) is plotted onthe isosurface as shown by Fig. 3e, f. As expected, it stronglydepends on the incident wavevector q. In addition, ฯ qรฐ ร variesgreatly at different locations, as shown by comparing Fig. 3e andFig. 3f. Despite all these differences, when integrated over theisosurface, โฌ ฯ qรฐ รds always results in the same constant: 16ฯ2. Weperform the integration for a TLS at 20 different locations, allwith the same constant, as shown in Fig. 3d.
As the transition frequency of the TLS approaches the Weylpoint, i.e., ฯ0 ! ฯWeyl, the isosurface shrinks in size, as illustratedby the insets of Fig. 4a. The conservation law leads to anincreasing ฯรฐqร, as shown by stronger colours. Near the Weylfrequency (black dashed line), the average cross sections ฯ isenhanced by three orders of magnitude compared to that in freespace, eventually diverging at the Weyl point (Fig. 4a). Theanalytical prediction from Eq. 2 and the area of the isosurfaceagree very well with predictions from numerical simulation(circles in Fig. 4a).
Frequency dependence of resonant scattering. A Weyl pointgreatly enhances the cross section at the resonant frequency.However, it comes at the price of suppressed cross section awayfrom the resonant frequency. Next, we discuss the spectral featureof the average cross section ฯรฐฯร for a given TLS. The spectraldependence is shown in Supplementary Note 3 as
ฯ ฯรฐ ร $ฯ0 % ฯWeyl! "2
}
ฯ0 % ฯรฐ ร2รพ}2 ฯ0%ฯWeylรฐ ร44
รฐ4ร
Here, } is a constant that depends on the local electric field at theposition of the TLS, but does not vary significantly with frequency.In order to derive Eq. 4, we use the fact that the spontaneous decayrate is proportional to ฯ0 % ฯWeyl
! "2 (Supplementary Eq. 32). Atthe resonance when ฯ0 % ฯ ยผ 0; the average cross section scales as1= ฯ0 % ฯWeyl! "2, which increases as the resonant frequency moves
closer to the Weyl point. However, away from the resonancewhen jฯ0 % ฯj ) jฯ0 % ฯWeylj, Eq. 4 reduces toฯ ฯ0รฐ ร $ ฯ0 % ฯWeyl
! "2= ฯ0 % ฯรฐ ร2, which shows that being close
to the Weyl point suppresses the cross section. In Fig. 4b, we cal-culate the spectra for three different TLSs with their transitionfrequencies approaching the Weyl point (black dashed line). Whilethe peak value of the cross section grows, the full width at halfmaximum of the spectrum decreases. The spectral integration of thecross section remains around a constant (Supplementary Note 3).
Rayleigh or non-resonant scattering. The non-resonant scat-tering of electrically small objects in free space follows the Ray-leigh scattering law. In great contrast to resonant scattering, thecross section of Rayleigh scattering scales as ฯ $ ฯ4, anddiminishes at the DC frequency, as shown in Fig. 5a. Thisproperty is also closely related to the isosurface and can be carriedto high frequency at the Weyl point (see proof in SupplementaryNote 5). While the resonant cross section diverges, the non-resonant cross section diminishes at Weyl points, as illustrated inFig. 5b.
Using perturbation theory and the first-order Born approx-imation36, the Rayleigh scattering cross section can be shown as(details in Supplementary Note 5):
ฯ ฯ; kincรฐ ร ยผ ฯ2 โฌS:ฯ ksรฐ รยผฯ
d2ks uks r0รฐ รVukinc r0รฐ รj j2/ ฯ2S รฐ5ร
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Here, ukรฐrร is the eigenmode of the Weyl photonic crystalassociated with wavevector k. ks and kinc are the wavevectors ofthe scattered and incident eigenmodes, respectively. V is a tensorfor the scattering potential of the Rayleigh scatterer. The integralis proportional to the area of the isosurface S. At the DC point,the isosurface shrinks to a point with S ยผ 0, and the cross sectionof Rayleigh scattering is zero. Similarly, around the Weyl point,the area of the isosurface S $ ฮฯ2 ยผ ฯ% ฯWeyl
! "2. The cross
section scales as ฯ $ ฯ2ฮฯ2, and is zero at the Weyl point(Fig. 5b).
To validate our theoretical prediction above, we numericallycalculate the Rayleigh scattering cross section of a small dielectricsphere embedded in the same Weyl photonic crystal. We useMPB32 to obtain the eigenmode of the Weyl photonic crystal,then numerically calculate the Rayleigh scattering cross sectionusing the normal-mode expansion37โ39 (see more details in
x
y
z
!/ (
2%c/a)
kx /(2%/a) k y/(2%
/a)
a
c
b
d
"(q)/&2
16%2
A' (
B
C
0
500
250
00.005
โ0.005
โ0.005
0.005
0
0
0.005
11.0
0.57
0.568
0.566
0.564
0.562
0.56โ0.2 โ0.1 0 0.1 0.2 โ0.2
0
0.2
Ez
0.5
โ0.5
โ1.0A B C A
0.00z
/a
x /a
โ1
โ1 0 1
โ0.005
q z/(
2%/a)
q z/(
2%/a)
qx /(2%/a)
qx /(2%/a)q y
/(2%/a
)
q y/(2
%/a)
fe
00.005
โ0.005
โ0.005
0.005
0
0
0.005
โ0.005
!!"(k)ds
Fig. 3 Simulation of resonant scattering in Weyl point photonic crystals. a The unit cell of the photonic crystal that supports Weyl points. Four air sphereswith a radius of 0.07a, where a is the lattice constant, are added to the gyroids to break the inversion symmetry. The positions of the air spheres are givenby รฐ 14 ; %
18 ;
12รa,
14 ;
18 ; 0
! "a, รฐ58 ; 0;
14รa and รฐ38 ;
12 ;
14รa. b Band structure of the photonic crystal close to the Weyl points. The band structure is plotted on the
plane 2kz ยผ %kx % ky . Four Weyl points are created with conical dispersion relation. c The normalized electric-field distribution of one eigenmode of thephotonic crystal on the xโz plane. We plot the z-component of the electric field as an example. d The resonant cross sections of the two-level system (TLS)for different locations. The integration in the momentum space always leads to the same constant. The dipole moment of the TLS is in the x direction.Positions A-B-C-A are also labelled in c. e, f Examples of ฯรฐqร at two different positions ฮฑ (e) and ฮฒ (f) are plotted on the isosurfaces as colour intensity.The positions ฮฑ and ฮฒ are labelled in c. Both e and f use the same colour map so that the cross sections can be directly compared
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Supplementary Note 6). The calculated Rayleigh scattering crosssections around the Weyl point are obtained by averaging100 scatterers at random locations within one unit cell of thephotonic crystal, and are plotted in Fig. 5c as red circles. They arenormalized by ฯR, the scattering cross section of the samescatterer in free space. The blue dashed line indicates the scalinglaw ฯ $ ฯ2ฮฯ2. The calculated Rayleigh scattering cross sectionagrees with the theoretical prediction well, with a vanishing crosssection observed at the Weyl point. For high-frequency devices,such as integrated waveguides and laser cavities, Rayleighscattering caused by interface roughness degrades performanceand increases noise. The combination of suppressed Rayleighscattering and enhanced resonant scattering could make Weylmedia attractive for these optoelectronic applications.
DiscussionMoreover, the conservation law of resonant scattering can also beextended to lower-dimensional space. In two-dimensional pho-tonic crystals, diverging cross sections can be realized at Diracpoints; an example is provided in Supplementary Note 4. Tofurther generalize the findings in this paper, we may not neces-sarily need conical dispersion. Quadratic dispersion found aroundthe band edges of photonic crystals also provides shrinking iso-surfaces. However, this is less useful in practice because the zerogroup velocity at the band edge makes it difficult to obtain pro-pagating waves40 in the presence of disorders. In addition, cou-pling into such media is difficult due to the large impedancemismatch.
As a final remark, the transport properties of electrons aroundDirac and Weyl points has also been studied in the past fewyears15โ17. Some of the observations are consistent with thephysics of photon scattering shown in this paper. Here, weexplicitly show the general conservation law of cross section andits connection to the dispersion relation. We expect that similarconclusions can be drawn for both electrons and phonons. Itprovides useful insight to understand general scattering physicsbeyond Dirac and Weyl systems.
In conclusion, large resonant cross sections are of great prac-tical importance. They are only achievable with long resonantwavelengths when the frequency approaches the DC point. Asshown in this work, the dispersion, rather than the wavelength, is
responsible for the cross section. As a result, Weyl points, whichcan achieve similar conic dispersion as that around the DC point,lead to the diverging resonant cross section at any desired fre-quency. The exceptionally strong resonant scattering is also
SimulationAnalytical
!0/(2ฯc/a)
!0= 0.562 (2ฯc/a)
!0= 0.563 (2ฯc/a)
!0= 0.564 (2ฯc/a)"(q)/&2
a
Res
onan
t ave
rage
cro
ss s
ectio
n
b
Aver
age
cros
s se
ctio
n
104"0โ
103"0โ
103"0โ
102"0โ
10โ1"0โ
10โ2"0โ
10โ3"0โ
10โ4"0โ
10โ5"0โ
10โ6"0
10"0โ
"0โ
102"0โ
10"0โ
"0โ
0.560 0.562 0.564 0.566 0.568
500
400
300
200
100
0
0.570!0/(2ฯc/a)
0.559 0.560 0.561 0.562 0.563 0.564 0.565
Fig. 4 Resonant scattering cross section in Weyl photonic crystal. a Diverging resonant scattering cross section is realized around the Weyl frequency.Isosurfaces have an ellipsoidal shape (insets) with its colour indicating the value of the cross section; the shrinking isosurface leads to increasing crosssections around the Weyl frequency, which is indicated by the black dashed line. The results from quantum scattering simulation (red circles) agree wellwith the prediction based on the band structure (blue dashed line). The cross section is normalized by the average cross section in free space ฯ0 ยผ ฮป2=ฯ. Itscales as ฯ $ 1=ฮฯ2. b Spectra of average scattering cross sections for TLSs with different transition frequencies. For simplicity, the spontaneous emissionrates of the TLSs in vacuum are chosen to be 10%4ฯ0. We also assume the dipole moments and locations of the TLSs are the same. The black dashed linealso indicates the Weyl frequency
k kฯ=ck
Weyl point
Rayleighscattering
Weyl pointDC
a b
c
0.4"R
0.2"R
0
0.6"R
Aver
age
cros
s se
ctio
n
!/(2ฯc/a)0.560 0.562 0.564 0.566 0.568 0.570
!
!4!2โ!2
!
! !
" "
โ!
Fig. 5 Rayleigh scattering in free space and Weyl systems. a In free space, theRayleigh scattering cross section scales as ฯ $ ฯ4 and vanishes at the DCfrequency. b In Weyl systems, the Rayleigh scattering cross section scales asฯ $ ฯ2ฮฯ2 and vanishes at the Weyl frequency, which is indicated by theblack dashed line. In both a and b, regions with stronger red colours indicatesmaller Rayleigh scattering cross section. c Numerical calculation of Rayleighscattering in a Weyl photonic crystal. The Rayleigh scatterer is a dielectricsphere with a radius of 0.01a and a dielectric constant of 2. The numericalresults (red circles) are normalized by the Rayleigh scattering cross section infree space ฯR , and fit well the predictedฯ $ ฯ2ฮฯ2scaling (blue dashed line).The black dashed line also indicates the Weyl frequency
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accompanied by diminishing non-resonant scattering, which isalso similar to that around the DC point. Since Weyl points canbe realized at any frequency, we can effectively decouple the crosssection and the wavelength. It opens up possibilities for tailoringwaveโmatter interaction with extraordinary flexibility, which alsocan be extended to acoustic and electronic wave scattering.
Data availability. The data that support the finding of this studyare available from the corresponding author upon reasonablerequest.
Received: 25 May 2017 Accepted: 25 September 2017
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AcknowledgementsM.Z., L.Y. and Z.Y. acknowledge the finanical support of DARPA (YFA17 N66001-17-1-4049 and DETECT program). L.L. was supported by the National key R\&D Progam ofChina under Grant No. 2017YFA0303800, 2016YFA0302400 and supported by theNational Natural Science fundation of China (NSFC) under Project No. 11721404. L.S.and J.Z. were supported by 973 Program (2015CB659400), China National Key BasicResearch Program (2016YFA0301100) and NSFC (11404064).
Author contributionsM.Z. developed the theoretical formalism, performed the analytic calculations and per-formed the numerical simulations. All authors contributed to the final versions of themanuscript. Z.Y. supervised the project.
Additional informationSupplementary Information accompanies this paper at doi:10.1038/s41467-017-01533-0.
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ยฉ The Author(s) 2017
NATURE COMMUNICATIONS | DOI: 10.1038/s41467-017-01533-0 ARTICLE
NATURE COMMUNICATIONS |8: ๏ฟฝ1388๏ฟฝ |DOI: 10.1038/s41467-017-01533-0 |www.nature.com/naturecommunications 7
Supplementary Note 1: Conservation law of resonant scattering
As we discussed in the main text, the conservation law of resonant scattering applies to both classical and quantum resonances in any continuum with a well-defined dispersion relation. Here in this section, we will derive the conservation law using quantum electrodynamics.
To simplify the discussion, we consider a non-degenerate resonance embedded in a medium. The resonance frequency of the resonance is ๐๐0 . We also incorporate the Lamb shift into the resonance frequency to simplify the discussion1. The dispersion relation of the medium is defined by ๐๐(๐ค๐ค), where ๐ค๐ค is the wave vector. The interaction between the resonance and the propagating waves in the medium is described by the interaction Hamiltonian ๐ป๐ปI. The exact expression of ๐ป๐ปI is not required to derive the conservation law as we will demonstrate below.
We consider the incident photon is in an eigenmode of the medium with a momentum of ๐ค๐คi. The resonance is initially in its ground state |gโฉ. The incident photon is scattered by the resonance to all the eigenmodes of the medium. For a final state with a momentum of ๐ค๐คf, the transition probability is given by2
โ๐๐๐๐ =โจg,๐ค๐ค๐๐|๐ป๐ปI|๐๐, 0โฉโจ๐๐, 0|๐ป๐ปI|g,๐ค๐คiโฉ
โ๐๐ โ โ๐๐0 + ๐๐๐๐ โ |โจ๐๐,๐ค๐ค๐๐|๐ป๐ปI|๐๐, 0โฉ|2๐ฟ๐ฟ๏ฟฝโ๐๐๐ค๐ค๐๐ โ โ๐๐0๏ฟฝ๐ค๐คf (1)
where โ is the reduced Planck constant and |๐๐, 0โฉ indicates that the resonance is in its excited state and there is no photon in the medium. Using Fermiโs golden rule, we can obtain the optical cross section of the resonance as
๐๐(๐ค๐ค๐๐,๐๐) =1
๐ฃ๐ฃ๐ค๐ค๐๐ ๐ฟ๐ฟ3โ ๏ฟฝ2ฯโ
|โ๐๐๐๐|2๐ฟ๐ฟ๏ฟฝโ๐๐๐ค๐คf โ โ๐๐๐ค๐คi๏ฟฝ๐ค๐ค๐๐
(2)
The normalization factor ๐ฃ๐ฃ๐ค๐ค๐๐ ๐ฟ๐ฟ3โ is the power flux of a single incident photon, where ๐ฃ๐ฃ๐ค๐ค๐๐ is the group
velocity of the incident photon and ๐ฟ๐ฟ3 is the quantization volume.
We focus on the resonant cross section at the resonant frequency ๐๐๐ค๐คf = ๐๐๐ค๐คi = ๐๐0. The summation in the momentum space then can be converted to an integration over the iso-surface S defined by ๐๐(๐ค๐ค) = ๐๐0 as
๏ฟฝ๐ฟ๐ฟ๏ฟฝโ๐๐๐ค๐คf โ โ๐๐0๏ฟฝ๐ค๐ค๐๐
= ๏ฟฝ๐ฟ๐ฟ
2๐๐๏ฟฝ3๏ฟฝ
๐๐๐๐โ๐ฃ๐ฃ๐ค๐ค๐๐๐๐
(3)
The resonant cross section at ๐๐๐ค๐คf = ๐๐๐ค๐คi = ๐๐0 then can be further calculated as
๐๐(๐ค๐ค๐๐,๐๐0) =2ฯโ
|โจ๐๐, 0|๐ป๐ปI|๐๐,๐ค๐คiโฉ|2
๐ฃ๐ฃ๐ค๐ค๐๐ ๐ฟ๐ฟ3โ1
๐๐2 ๏ฟฝ ๐ฟ๐ฟ2๐๐๏ฟฝ3โฌ ๐๐๐๐
โ๐ฃ๐ฃ๐ค๐ค๐๐|โจ๐๐,๐ค๐ค๐๐|๐ป๐ปI|๐๐, 0โฉ|2๐๐
= 16๐๐2|โจ๐๐, 0|๐ป๐ปI|๐๐,๐ค๐คiโฉ|2
โ๐ฃ๐ฃ๐ค๐ค๐๐โฌ ๐๐๐๐
โ๐ฃ๐ฃ๐ค๐ค๐๐|โจ๐๐,๐ค๐ค๐๐|๐ป๐ปI|๐๐, 0โฉ|2๐๐
(4)
Next, we integrate the resonant cross section ๐๐(๐ค๐ค๐๐,๐๐0) over the iso-surface S and immediately obtain the conservation law
๏ฟฝ๐๐(๐ค๐ค๐๐,๐๐0)๐๐๐๐๐๐
= 16๐๐2โฌ ๐๐๐๐
โ๐ฃ๐ฃ๐ค๐ค๐๐|โจ๐๐, 0|๐ป๐ป๐ผ๐ผ|๐๐,๐ค๐คiโฉ|2๐๐
โฌ ๐๐๐๐โ๐ฃ๐ฃ๐๐๐๐
|โจ๐๐,๐ค๐ค๐๐|๐ป๐ปI|๐๐, 0โฉ|2๐๐
= 16๐๐2 (5)
Supplementary Note 2: Quantum scattering theory
The resonant scattering cross section of a single two-level system (TLS) can be calculated using many approaches2,3. Here in our work, we calculated the scattering cross section and further numerically verified the conservation law by using the quantum scattering theory we recently developed4. In this section, we will describe our quantum scattering theory in detail.
As we described in the main text, the general Hamiltonian governing the interaction between photons and a single TLS is given by5
๐ป๐ป = โ๐๐0๐๐โ ๐๐ +๏ฟฝโ๐๐๐ค๐ค๐๐๐ค๐คโ ๐๐๐ค๐ค
๐ค๐ค
+ ๐๐โ๏ฟฝ๐๐๐ค๐ค๏ฟฝ๐๐๐ค๐คโ ๐๐ โ ๐๐๐ค๐ค๐๐โ ๏ฟฝ
๐ค๐ค
(6)
Here ๐๐โ (๐๐) is the raising (lowering) atomic operator of the TLS. The transition frequency of the TLS is ๐๐0. The creation (annihilation) operator for photons with angular frequency ๐๐๐ค๐ค is ๐๐๐ค๐ค
โ (๐๐๐ค๐ค), with ๐ค๐ค being the momentum. The coupling strength between the TLS and the photon with momentum ๐ค๐ค is given by ๐๐๐ค๐ค = ๐๐ โ ๐๐๏ฟฝ๐ค๐ค๏ฟฝ๐๐0/2โ๐๐0๐ฟ๐ฟ3, where ๐๐ is the dipole moment of the TLS, ๐๐๏ฟฝ๐ค๐ค is the unit polarization vector of the photons at the location of the TLS and ๐๐0 is the vacuum permittivity.
Supplementary Figure 1: Quantum scattering theory. a Schematic of a two-level system in a continuum. Periodic boundary conditions with periodicity L are applied in both x and y directions. Because of the periodicity, incident photons can only be scattered to a set of discretized directions. b The ๐ช๐ช๐๐,๐๐๐๐ space is discretized by โ๐๐ = 2ฯ/๐ฟ๐ฟ, and represents a set of eigenmode channels (grey dots). c Real space bosonic creation operators. The real-space operators ๐๐F,๐๐,๐๐
โ (๐๐) and ๐๐B,๐๐,๐๐โ (๐๐) create a forward
and backward propagating single photon at position ๐๐ in the nth channel of the mth Weyl point, respectively. d Spatial single-photon wavefunctions ๐๐F,๐๐,๐๐(๐๐) and ๐๐B,๐๐,๐๐(๐๐) in the nth channel of the mth Weyl point. The coefficients ๐๐๐๐,๐๐ and ๐ก๐ก๐๐,๐๐ are the amplitudes of reflected and transmitted photons in the nth channel of the mth Weyl point, respectively.
The second term โ โ๐๐๐ค๐ค๐๐๐ค๐คโ ๐๐๐ค๐ค๐ค๐ค describes the propagating photons in the photonic crystals. Here we focus
on the Weyl-point photonic crystal. As we described in the main text, the dispersion is governed by the Weyl Hamiltonian โ(๐ช๐ช) = ๐ฃ๐ฃ๐ฅ๐ฅ๐๐๐ฅ๐ฅ๐๐๐ฅ๐ฅ + ๐ฃ๐ฃ๐ฆ๐ฆ๐๐๐ฆ๐ฆ๐๐๐ฆ๐ฆ + ๐ฃ๐ฃ๐ง๐ง๐๐๐ง๐ง๐๐๐ง๐ง, where ๐๐๐ฅ๐ฅ,๐ฆ๐ฆ,๐ง๐ง are Pauli matrices. The momentum ๐ช๐ช๏ฟฝ๐๐๐ฅ๐ฅ, ๐๐๐ฆ๐ฆ, ๐๐๐ง๐ง๏ฟฝ = ๐ค๐ค โ ๐ค๐คWeyl defines the distance to the Weyl point in the momentum space. Diagonalization of the Weyl Hamiltonian yields a three-dimensional (3D) conical dispersion around the frequency of the Weyl point ๐๐Weyl. To simplify the discussion, we consider isotropic Weyl points where ๐ฃ๐ฃ๐ฅ๐ฅ = ๐ฃ๐ฃ๐ฆ๐ฆ = ๐ฃ๐ฃ๐ง๐ง = ๐ฃ๐ฃ. The dispersion around the Weyl point then can be simplified to ๐๐๏ฟฝ๐ช๐ช = ๐๐๐ค๐ค โ ๐๐Weyl =ยฑ๐ฃ๐ฃ|๐ช๐ช|. Note Weyl points typically appear in pairs and the minimum number of Weyl points is two. Here we assume the number of Weyl points is M and the position of mth Weyl point in the momentum space is
๐ค๐คWeyl,๐๐ . By defining ๐ช๐ช๐๐ = ๐ค๐ค โ ๐ค๐คWeyl,๐๐ , the Hamiltonian in Supplementary Equation (1) can be rewritten as
๐ป๐ป = โ๐๐0๐๐โ ๐๐ + ๏ฟฝ๏ฟฝโ๐๐๏ฟฝ๐ช๐ช๐๐๐๐๐ช๐ช๐๐โ ๐๐๐ช๐ช๐๐
๐ช๐ช๐๐
๐๐
๐๐=1
+ ๐๐โ ๏ฟฝ๏ฟฝ๐๐๐ช๐ช๐๐๏ฟฝ๐๐๐ช๐ช๐๐โ ๐๐ โ ๐๐๐ช๐ช๐๐๐๐
โ ๏ฟฝ๐ช๐ช๐๐
๐๐
๐๐=1
(7)
The key idea of our quantum scattering theory is to convert the summation over ๐ช๐ช๐๐ to a summation over a set of 1-dimension (1D) channels, or waveguides, where solutions have been successfully obtained6. Each channel carries a eigenmode of the photonic crystal with a distinct momentum ๐ช๐ช๐๐. They can be illustrated in the ๐ช๐ช๐๐-space as shown in Supplementary Figures 1a-b. Here, we use box quantization for the ๐ช๐ช๐๐ -space by setting up a periodic boundary condition in both x and y directions. At the end of derivation, we will take the periodicity L to โ to effectively remove the impact of this artificial periodic boundary condition. Because of the periodicity, incident photons can only be scattered to a set of discretized channels. These channels are defined by the in-plane wave vectors ๐ช๐ช๐๐,๐ฅ๐ฅ๐ฆ๐ฆ of the wave, which are discretized by โ๐๐ = 2๐๐/๐ฟ๐ฟ (Supplementary Figure 1b). For a given frequency ๐๐๐ช๐ช๐๐, the channels are located on a sphere of radius |๐ช๐ช๐๐| = ๐๐๐ช๐ช๐๐/๐ฃ๐ฃ. Thereby, the total number of channels N is given by ๐๐ =โฏ cos ๐๐๐ช๐ช๐๐ ๐๐
2๐ช๐ช๐๐/(โ๐๐)2 /2 = ๐๐(๐๐๏ฟฝ๐ช๐ช๐๐/๐ฃ๐ฃโ๐๐)2. We can then convert the summation over ๐ช๐ช๐๐ to
๏ฟฝโ๐๐๏ฟฝ๐ช๐ช๐๐๐๐๐ช๐ช๐๐โ ๐๐๐ช๐ช๐๐
๐ช๐ช๐๐
= ๏ฟฝ ๏ฟฝ โ๐๐๏ฟฝ๐๐๐๐,๐๐๐๐๐๐๐๐,๐๐โ ๐๐๐๐๐๐,๐๐
๐๐๐๐,๐๐
๐๐
๐๐=1
(8)
๏ฟฝ๐๐๐ช๐ช๐๐๏ฟฝ๐๐๐ช๐ช๐๐โ ๐๐ โ ๐๐๐ช๐ช๐๐๐๐
โ ๏ฟฝ๐ช๐ช๐๐
= ๏ฟฝ ๏ฟฝ๐๐๐๐๐๐,๐๐๏ฟฝ๐๐๐๐๐๐,๐๐โ ๐๐ โ ๐๐๐๐๐๐,๐๐๐๐
โ ๏ฟฝ๐๐๐๐,๐๐
๐๐
๐๐=1
(9)
Note the wave number ๐๐๐๐,๐๐ is a scalar. Itโs also useful to differentiate waves with opposite group velocities as their dispersions are governed by two different branches. We define two scalar wave numbers ๐๐๐๐,๐๐F and ๐๐๐๐,๐๐
B for forward and backward propagating waves, respectively. The summations over ๐ช๐ช๐๐ then become
๏ฟฝโ๐๐๏ฟฝ๐ช๐ช๐๐๐๐๐ช๐ช๐๐โ ๐๐๐ช๐ช๐๐
๐ช๐ช๐๐
= ๏ฟฝ(๏ฟฝ โ๐๐๏ฟฝ๐๐๐๐,๐๐F ๐๐๐๐๐๐,๐๐Fโ ๐๐๐๐๐๐,๐๐F
๐๐๐๐,๐๐F
+ ๏ฟฝโ๐๐๏ฟฝ๐๐๐๐,๐๐B ๐๐๐๐๐๐,๐๐Bโ ๐๐๐๐๐๐,๐๐B
๐๐๐๐,๐๐B
)๐๐
๐๐=1
(10)
๏ฟฝ๐๐๐ช๐ช๐๐๏ฟฝ๐๐๐ช๐ช๐๐โ ๐๐ โ ๐๐๐ช๐ช๐๐๐๐
โ ๏ฟฝ๐ช๐ช๐๐
= ๏ฟฝ ๏ฟฝ๐๐๐๐๐๐,๐๐F ๏ฟฝ๐๐๐๐๐๐,๐๐Fโ ๐๐ โ ๐๐๐๐๐๐,๐๐F ๐๐โ ๏ฟฝ
๐๐๐๐,๐๐F
๐๐
๐๐=1
+๏ฟฝ ๏ฟฝ๐๐๐๐๐๐,๐๐B ๏ฟฝ๐๐๐๐๐๐,๐๐Bโ ๐๐ โ ๐๐๐๐๐๐,๐๐B ๐๐โ ๏ฟฝ
๐๐๐๐,๐๐B
๐๐
๐๐=1
(11)
where ๐๐๏ฟฝ๐๐๐๐,๐๐F = ๐ฃ๐ฃ๐๐๐๐,๐๐F and ๐๐๏ฟฝ๐๐๐๐,๐๐B = โ๐ฃ๐ฃ๐๐๐๐,๐๐B are the dispersion relationships for forward and backward propagating photons in each channel, respectively. Note ๐๐๐๐,๐๐F and ๐๐๐๐,๐๐B are scalars with opposite signs.
Our next step is to convert the ๐ช๐ช๐๐ -space operators ๐๐๐๐๐๐,๐๐Fโ and ๐๐๐๐๐๐,๐๐B
โ to real-space operators. It can be
realized by defining the following Fourier transformation
๐๐๐๐๐๐,๐๐Fโ = ๏ฟฝ1
๐ฟ๐ฟ๏ฟฝ ๐๐๐๐๐๐F,๐๐,๐๐โ (๐๐)๐๐๐๐๐๐๐๐F ๐๐
๐ฟ๐ฟ
โ๐ฟ๐ฟ(12)
๐๐๐๐๐๐,๐๐Bโ = ๏ฟฝ1
๐ฟ๐ฟ๏ฟฝ ๐๐๐๐๐๐B,๐๐,๐๐โ (๐๐)๐๐๐๐๐๐๐๐B ๐๐
๐ฟ๐ฟ
โ๐ฟ๐ฟ(13)
where operators ๐๐F,๐๐,๐๐โ (๐๐) and ๐๐B,๐๐,๐๐
โ (๐๐) create a forward and a backward propagating photon at position ๐๐ in the nth channel, respectively (Supplementary Figure 1c). By using rotating wave approximation, the summations over ๐๐๐๐,๐๐F further become
๏ฟฝโ๐๐๏ฟฝ๐๐๐๐,๐๐F ๐๐๐๐๐๐,๐๐Fโ ๐๐๐๐๐๐,๐๐F
๐๐๐๐,๐๐F
= ๏ฟฝโ๐ฃ๐ฃ๐๐๐๐,๐๐F
๐ฟ๐ฟ ๏ฟฝ ๏ฟฝ ๐๐๐๐๐๐๐๐โฒโ
โโ
โ
โโ๐๐F,๐๐,๐๐โ (๐๐)๐๐F,๐๐,๐๐(๐๐โฒ)๐๐๐๐๐๐๐๐
F ๏ฟฝ๐๐โ๐๐โฒ๏ฟฝ
๐๐๐๐,๐๐F
=โ๐ฃ๐ฃโ๐๐๐ฟ๐ฟ๏ฟฝ ๏ฟฝ ๐๐๐๐๐๐๐๐โฒ
โ
โโ
โ
โโ๐๐F,๐๐,๐๐โ (๐๐)๐๐F,๐๐,๐๐(๐๐โฒ)๏ฟฝ ๐๐๐๐,๐๐F ๐๐๐๐๐๐๐๐F ๏ฟฝ๐๐โ๐๐โฒ๏ฟฝ ๐๐๐๐๐๐,๐๐F
โ
โโ
= ๐๐โ๐ฃ๐ฃ ๏ฟฝ ๏ฟฝ ๐๐๐๐๐๐๐๐โฒโ
โโ
โ
โโ๐๐F,๐๐,๐๐โ (๐๐)(โ
๐๐๐๐๐๐)๐๐F,๐๐,๐๐
(๐๐โฒ)๐ฟ๐ฟ(๐๐ โ ๐๐โฒ)
= ๐๐โ๐ฃ๐ฃ ๏ฟฝ ๐๐๐๐๐๐F,๐๐,๐๐โ (๐๐) ๏ฟฝโ
๐๐๐๐๐๐๏ฟฝ ๐๐F,๐๐,๐๐
(๐๐)โ
โโ(14)
and
๏ฟฝ๐๐๐๐๐๐,๐๐F ๏ฟฝ๐๐๐๐๐๐,๐๐Fโ ๐๐ โ ๐๐๐๐๐๐,๐๐F ๐๐โ ๏ฟฝ
๐๐๐๐,๐๐F
= ๏ฟฝ๐๐๐๐๐๐,๐๐F ๏ฟฝ1๐ฟ๐ฟ ๏ฟฝ๏ฟฝ ๐๐๐๐๐๐F,๐๐,๐๐
โ (๐๐)๐๐๐๐๐๐๐๐,๐๐F ๐๐๐๐โ
โโโ ๏ฟฝ ๐๐๐๐๐๐F,๐๐,๐๐(๐๐)๐๐โ๐๐๐๐๐๐,๐๐F ๐๐๐๐โ
โ
โโ๏ฟฝ
๐๐๐๐,๐๐F
=๐๐๐๐๐๐,๐๐F
โ๐๐๏ฟฝ1๐ฟ๐ฟ ๏ฟฝ๏ฟฝ ๐๐๐๐๐๐F,๐๐,๐๐
โ (๐๐)๐๐โ
โโ๏ฟฝ ๐๐๐๐๐๐,๐๐F ๐๐๐๐๐๐๐๐,๐๐F ๐๐โ
โโโ ๏ฟฝ ๐๐๐๐๐๐F,๐๐,๐๐(๐๐)๐๐โ
โ
โโ๏ฟฝ ๐๐๐๐๐๐,๐๐F ๐๐โ๐๐๐๐๐๐,๐๐F ๐๐โ
โโ๏ฟฝ
= ๐๐๐๐,๐๐โ๐ฟ๐ฟ๏ฟฝ ๐๐๐๐๐ฟ๐ฟ(๐๐)๏ฟฝ๐๐F,๐๐,๐๐โ (๐๐)๐๐ โ ๐๐F,๐๐,๐๐(๐๐)๐๐โ ๏ฟฝ
โ
โโ(15)
Similarly, the summations over ๐๐๐๐B further become
๏ฟฝ โ๐๐๏ฟฝ๐๐๐๐,๐๐B ๐๐๐๐๐๐,๐๐Bโ ๐๐๐๐๐๐,๐๐B
๐๐๐๐,๐๐B
= ๐๐โ๐ฃ๐ฃ ๏ฟฝ ๐๐๐๐๐๐B,๐๐,๐๐โ (๐๐) ๏ฟฝโ
๐๐๐๐๐๐๏ฟฝ ๐๐B,๐๐,๐๐(๐๐)
โ
โโ(16)
and
๏ฟฝ๐๐๐๐๐๐,๐๐B ๏ฟฝ๐๐๐๐๐๐,๐๐Bโ ๐๐ โ ๐๐๐๐๐๐,๐๐B ๐๐โ ๏ฟฝ
๐๐๐๐,๐๐B
= ๐๐๐๐,๐๐โ๐ฟ๐ฟ๏ฟฝ ๐๐๐๐๐ฟ๐ฟ(๐๐)๏ฟฝ๐๐B,๐๐,๐๐โ (๐๐)๐๐ โ ๐๐B,๐๐,๐๐(๐๐)๐๐โ ๏ฟฝ
โ
โโ(17)
By substituting Supplementary Equations (8) โ (17) into Supplementary Equation (7) we obtain the real-space Hamiltonian as
๐ป๐ป = โ๐๐0๐๐โ ๐๐ + ๐๐โ๐ฃ๐ฃ๐ฟ๐ฟ ๏ฟฝ ๏ฟฝ๏ฟฝ ๐๐๐๐ ๏ฟฝ๐๐F,๐๐,๐๐โ (๐๐) ๏ฟฝโ
๐๐๐๐๐๐๏ฟฝ ๐๐F,๐๐,๐๐ + ๐๐B,๐๐,๐๐
โ (๐๐)(๐๐๐๐๐๐)๐๐B,๐๐,๐๐(๐๐)๏ฟฝ
โ
โโ
๐๐
๐๐=1
๐๐
๐๐=1
+ ๐๐โ ๏ฟฝ ๏ฟฝ๏ฟฝ ๐๐๐๐๐๐๐๐,๐๐๐ฟ๐ฟ๐ฟ๐ฟ(๐๐) ๏ฟฝ๏ฟฝ๐๐F,๐๐,๐๐โ (๐๐) + ๐๐B,๐๐,๐๐
โ (๐๐)๏ฟฝ ๐๐ โ ๏ฟฝ๐๐F,๐๐,๐๐(๐๐) + ๐๐B,๐๐,๐๐(๐๐)๏ฟฝ ๐๐โ ๏ฟฝโ
โโ
๐๐
๐๐=1
๐๐
๐๐=1
(18)
Given the real-space Hamiltonian, our next step is to solve the time-independent Schrodinger equation ๐ป๐ป|๐๐โฉ = โ๐๐๐ช๐ช|๐๐โฉ, where |๐๐โฉ is the eigenstate. The most general eigenstate can be written in terms of the eigenmodes of the photonic crystal as
|๐๐โฉ = ๏ฟฝ ๏ฟฝ๏ฟฝ๐๐๐๐๏ฟฝ๐๐F,๐๐,๐๐(๐๐)๐๐F,๐๐,๐๐โ (๐๐) + ๐๐B,๐๐,๐๐(๐๐)๐๐B,๐๐,๐๐
โ (๐๐)๏ฟฝ |0, gโฉ๐๐
๐๐=1
๐๐
๐๐=1
+ ๐ธ๐ธ๐๐โ |0, gโฉ (19)
where |0, gโฉ indicates that the TLS is in the ground state and ๐ธ๐ธ is the excitation amplitude of the TLS. The single-photon wavefunctions ๐๐F,๐๐,๐๐(๐๐) and ๐๐B,๐๐,๐๐(๐๐) in the nth channel of the mth Weyl point are given by
๐๐F,๐๐,๐๐(๐๐) = ๐ข๐ข(๐๐)๐๐๐๐๐๐๐๐,๐๐๐๐๏ฟฝ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐๐๐(โ๐๐) + ๐ก๐ก๐๐.๐๐๐๐(๐๐)๏ฟฝ (20)
๐๐B,๐๐,๐๐(๐๐) = ๐ข๐ข(๐๐)๐๐โ๐๐๐๐๐๐,๐๐๐๐๏ฟฝ๐๐๐๐,๐๐๐๐(โ๐๐)๏ฟฝ (21)
where ๐ข๐ข(๐๐)๐๐๐๐๐๐๐๐๐๐ is the eigenmode associated with wave number ๐๐๐๐,๐๐ and ๐๐(๐๐) is the Heaviside step function. The Kronecker delta ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐ indicates that single photons are incident from the in the pth channel of the lth Weyl point. The coefficients ๐๐๐๐,๐๐ and ๐ก๐ก๐๐,๐๐ are the amplitudes of the reflected and transmitted photons in the nth channel of the mth Weyl point, respectively. We schematically plot the wavefunctions in Supplementary Figure 1d for clear visualization.
By substituting the eigenstate into the real-space Hamiltonian, we obtain the following set of equations for each channel
โ๐๐๐ฃ๐ฃ๐๐๐๐๐๐ ๏ฟฝ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐๐ข๐ข(๐๐)๐๐(โ๐๐) + ๐ก๐ก๐๐,๐๐๐ข๐ข(๐๐)๐๐(๐๐)๏ฟฝ + ๐๐๐๐๐๐,๐๐โ๐ฟ๐ฟ๐๐โ๐๐๐๐๐๐,๐๐๐๐๐ธ๐ธ = 0 (22)
๐๐๐ฃ๐ฃ๐๐๐๐๐๐๐๐,๐๐๐๐๐๐๐๐๐๐ ๐๐๐๐,๐๐๐ข๐ข(๐๐)๐๐(โ๐๐) + ๐๐๐๐๐๐,๐๐โ๐ฟ๐ฟ๐๐๐๐๐๐๐๐,๐๐๐๐๐ธ๐ธ = 0 (23)
and the following equation for the interaction between the TLS and the propagating waves
๐๐0๐ธ๐ธ โ ๐๐ ๏ฟฝ ๏ฟฝ๐๐๐๐,๐๐โ๐ฟ๐ฟ ๏ฟฝ๐ข๐ข(0)๏ฟฝ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐ + ๐ก๐ก๐๐,๐๐๏ฟฝ
2 +๐ข๐ข(0)๐๐๐๐,๐๐
2 ๏ฟฝ๐๐
๐๐=1
๐๐
๐๐=1
= ๐๐๐ช๐ช๐ธ๐ธ (24)
By solving Supplementary Equation (22) and Supplementary Equation (23) we can obtain the coefficients ๐ก๐ก๐๐ and ๐๐๐๐ as
๐ก๐ก๐๐,๐๐ =๐๐๐๐,๐๐โ๐ฟ๐ฟ๐ฃ๐ฃ๐ข๐ข(0) ๐ธ๐ธ + ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐ (25)
๐๐๐๐,๐๐ =๐๐๐๐,๐๐โ๐ฟ๐ฟ๐ฃ๐ฃ๐ข๐ข(0) ๐ธ๐ธ (26)
By substituting Supplementary Equations (25) โ (26) into Supplementary Equation (24), we obtain a simple equation of the excitation amplitude E as
๏ฟฝ๐๐๐ช๐ช โ ๐๐0 + ๐๐ ๏ฟฝ ๏ฟฝ๏ฟฝ๐๐๐๐,๐๐๏ฟฝ
2๐ฟ๐ฟ๐ฃ๐ฃ
๐๐
๐๐=1
๐๐
๐๐=1
๏ฟฝ๐ธ๐ธ = โ๐๐๐๐๐๐,๐๐โ๐ฟ๐ฟ๐ข๐ข(0) (27)
We can then obtain the transmission coefficient ๐ก๐ก๐๐,๐๐ and reflection coefficient ๐ก๐ก๐๐,๐๐ in the nth channel of the mth Weyl point as
๐ก๐ก๐๐,๐๐ = โ๐๐๐๐๐๐,๐๐๐๐๐๐,๐๐๐ฟ๐ฟ
๐ฃ๐ฃ1
๐๐๐ช๐ช โ ๐๐0 + ๐๐ ฮ2+ ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐ (28)
๐๐๐๐,๐๐ = โ๐๐๐๐๐๐,๐๐๐๐๐๐,๐๐๐ฟ๐ฟ
๐ฃ๐ฃ1
๐๐๐ช๐ช โ ๐๐0 + ๐๐ ฮ2(29)
where ฮ = 2โ โ ๏ฟฝ๐๐๐๐,๐๐๏ฟฝ2๐ฟ๐ฟ/๐ฃ๐ฃ ๐๐
๐๐=1๐๐๐๐=1 is the spontaneous emission rate of the TLS and the factor of 2
results from the forward and backward propagating waves.
Thus, the scattering cross section can be calculated as
๐๐๏ฟฝ๐๐๐ช๐ช, ๐๐๐๐,๐๐๏ฟฝ =โ โ ๏ฟฝ|๐ก๐ก๐๐,๐๐ โ ๐ฟ๐ฟ๐๐๐๐๐ฟ๐ฟ๐๐๐๐|2 + |๐๐๐๐,๐๐|2๏ฟฝ๐๐
๐๐=1๐๐๐๐=1
1/๐ฟ๐ฟ2
=2๏ฟฝ๐๐๐๐,๐๐๏ฟฝ
2๐ฟ๐ฟ3
๐ฃ๐ฃโ โ ๏ฟฝ๐๐๐๐,๐๐๏ฟฝ
2๐ฟ๐ฟ/๐ฃ๐ฃ๐๐๐๐=1
๐๐๐๐=1
(๐๐0 โ ๐๐๐ช๐ช)2 + ฮ24
= ๏ฟฝ๐๐๐๐,๐๐๏ฟฝ
2๐ฟ๐ฟ3
๐ฃ๐ฃฮ
๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ2 + ฮ2
4
(30)
We can further normalize the coupling coefficient ๏ฟฝ๐๐๐๐,๐๐๏ฟฝ2๐ฟ๐ฟ/๐ฃ๐ฃ by its maximum (๐๐0)2๐ฟ๐ฟ/๐ฃ๐ฃ, and define an
angular factor ๐๐๐๐,๐๐ = ๏ฟฝ๐๐๐๐,๐๐/๐๐0๏ฟฝ2. Supplementary Equation (30) then can be rewritten to an expression
similar to the well-known Breit-Wigner formula as
๐๐๏ฟฝ๐๐๐ช๐ช, ๐๐๐๐,๐๐๏ฟฝ =2๐๐๐๐,๐๐๐ฟ๐ฟ2
โ โ ๐๐๐๐,๐๐ ๐๐๐๐=1
๐๐๐๐=1
ฮ24
๏ฟฝ๐๐0 โ ๐๐๐๐๏ฟฝ2 + ฮ2
4
=4๐๐๐๐,๐๐๐ฟ๐ฟ2(โ๐๐)2
|๐๐๐๐.๐๐|2 โ โฎ cos๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐๐๐๐๐=1
ฮ24
๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ2 + ฮ2
4
=๐๐๐๐,๐๐โฑ
16๐๐2๐ฃ๐ฃ2
(๐๐0 โ ๐๐๐๐๐๐๐ฆ๐ฆ๐๐)2
ฮ24
๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ2 + ฮ2
4
(31)
where ฮฉ๐๐,๐๐ is the solid angle associated with ๐๐๐๐,๐๐, โฑ = โ โฎ cos ๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐๐๐๐๐=1 and ๐๐๐๐,๐๐/โฑ indicates
the angular distribution of the scattering cross section. The prefactor 16๐ฃ๐ฃ2/(๐๐0 โ ๐๐Weyl)2 ultimately determines the maximum cross section, which agrees with the conclusion in the main text. Note we have assumed that the isosurface around each Weyl point is isotropic throughout the derivation, i.e. |๐๐๐๐.๐๐| =๏ฟฝ๐๐๐๐๐๐.๐๐ โ ๐๐Weyl๏ฟฝ/๐ฃ๐ฃ. For anisotropic Weyl point, the scattering cross section has the same form and only differs from the isotropic case by a constant.
Supplementary Note 3: Frequency dependence of the spectrum of the average cross section
In the main text, we focus on the maximum of the average cross section when ๐๐๐ช๐ช = ๐๐0 and briefly discuss the spectrum of the average cross section in Fig. 4. Here we will discuss more details about the frequency dependence of the spectrum of the average cross section.
The average cross section can be directly calculated by using Supplementary Equation (30). To simplify the discussion, here we will also assume that the isosurface around each Weyl point is identical and isotropic, i.e., |๐๐๐๐.๐๐| = ๏ฟฝ๐๐๐๐๐๐.๐๐ โ ๐๐Weyl๏ฟฝ/๐ฃ๐ฃ . Recall that (๐๐0)2 = ๐๐2๐๐0/2โ๐๐0๐ฟ๐ฟ3 and ๐๐ is the dipole moment of the TLS. Thereby, the spontaneous emission rate ฮ can also be calculated as
ฮ = 2 ๏ฟฝ ๏ฟฝ๏ฟฝ๐๐๐๐,๐๐๏ฟฝ
2๐ฟ๐ฟ๐ฃ๐ฃ
๐๐
๐๐=1
๐๐
๐๐=1
=(๐๐0)2๐ฟ๐ฟ3๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ
2
4๐๐2๐ฃ๐ฃ3 ๏ฟฝ ๏ฟฝ cos๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐
๐๐
๐๐=1
๐๐2๐๐0๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ2
8โ๐๐0๐๐2๐ฃ๐ฃ3๏ฟฝ ๏ฟฝ cos๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐
๐๐
๐๐=1
= ๐ ๐ ๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ2 (32)
where ฮฉ๐๐,๐๐ is the solid angle associated with wave number ๐๐๐๐,๐๐ . For simplification, we define a coefficient ๐ ๐ = ๐๐2๐๐0 โ โฎ cos ๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐
๐๐๐๐=1 /8โ๐๐0๐๐2๐ฃ๐ฃ3. Around the Weyl point, the coefficient ๐ ๐
does not vary significantly with the frequency. As a result, the spontaneous emission rate ฮ scales as
๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ2.
Next, we calculate the average cross section by integrating the cross section on the isosurfaces and then dividing the integration by the area of the isosurfaces. The spectrum of the average cross section then is given by
๐๐๏ฟฝ๏ฟฝ๐๐๐ช๐ช๏ฟฝ =(๐๐0)2๐ฟ๐ฟ3
๐ฃ๐ฃโ โฎ cos ๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐๐๐๐๐=1
โ โฎ๐๐ฮฉ๐๐,๐๐๐๐๐๐=1
ฮ
๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ2 + ฮ2
4
= ๐๐2๐๐0
8๐๐โ๐๐0๐๐๐ฃ๐ฃ๏ฟฝ ๏ฟฝ cos ๐๐๐๐.๐๐ ๐๐๐๐,๐๐๐๐ฮฉ๐๐,๐๐
๐๐
๐๐=1
ฮ
๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ2 + ฮ2
4
= ๐๐๐ ๐ 2๐ฃ๐ฃ2
๐๐๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ
2
๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ2 +
๐ ๐ 2๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ4
4
(33)
Note the prefactor ๐๐๐ ๐ 2๐ฃ๐ฃ2/๐๐ does not vary significantly with the frequency around the Weyl point. On
resonance, i.e., ๐๐๐ช๐ช = ๐๐0, the resonant average cross section scales as 1/๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ2 and increases
drastically as ๐๐0 โ ๐๐Weyl . In great contrast, the cross section of off-resonance frequencies scales as
๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ2/๏ฟฝ๐๐0 โ ๐๐๐ช๐ช๏ฟฝ
2 and is strongly suppressed around the Weyl point.
Meanwhile, itโs clear to see that the integration of the average cross section โซ ๐๐๏ฟฝ๏ฟฝ๐๐๐ช๐ช๏ฟฝ๐๐๐๐๐ช๐ชโโโ is roughly a
constant, which can be shown as
๏ฟฝ ๐๐๏ฟฝ๏ฟฝ๐๐๐๐๏ฟฝ๐๐๐๐๐๐โ
โโ= ๏ฟฝ ๐๐๐๐๐๐
โ
โโ
๐๐๐ ๐ 2๐ฃ๐ฃ2
๐๐๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ
2
๏ฟฝ๐๐๐๐ โ ๐๐0๏ฟฝ2 +
๐ ๐ 2๏ฟฝ๐๐0 โ ๐๐Weyl๏ฟฝ4
4
=2๐ ๐ ๐๐2๐ฃ๐ฃ2
๐๐(34)
where 2๐ ๐ ๐๐2๐ฃ๐ฃ2/๐๐ remains around the same around the Weyl point.
Supplementary Note 4: Resonant scattering in Dirac systems
The conservation law of resonant scattering can be also extended to two-dimensional (2D) space. In 2D space, the conical dispersion forms a Dirac point, which is the 2D analogy of the Weyl point. In this section, we will use a 2D Dirac photonic crystal as an example and demonstrate the diverging resonant scattering cross section around the Dirac point.
We consider a triangular lattice of dielectric rods (grey circle in Supplementary Figure 2a), which has a dielectric constant of ๐๐ = 12. The radius of the rods is 0.3๐๐, where a is the lattice constant. We then solve the band structure of this Dirac photonic crystal by using MPB7. We obtain 6 Dirac points in the band structure for the transverse electric (TE) bands at ๐๐ = 0.462 (2๐๐๐๐/๐๐). To visualize the momentum space in 2D space, we plot the isofrequency contour for ๐๐ = 0.461 (2๐๐๐๐/๐๐) in Supplementary Figure 2b. For each Dirac point, the isofrequency contour is almost a circle.
Supplementary Figure 2: Resonant scattering in Dirac systems. a Schematic of the 2D Dirac photonic crystal. b Isofrequency contour of the Dirac photonic crystal at ๐๐ = 0.461 (2๐๐๐๐/๐๐). 6 Dirac points are obtained at ๐๐ = 0.462 (2๐๐๐๐/๐๐) for the TE bands. The isofrequency contour is almost a circle. c The resonant cross section of the TLS for different locations. The resonant frequency of the TLS is ๐๐0 = 0.461 (2๐๐๐๐/๐๐). The integration in momentum space always leads to the same constant. Positions A-B-C-A are labelled in a. Examples of ๐๐(๐ช๐ช) at two different positions are plotted as insets. d Diverging
average resonant cross section is realized around the Dirac frequency. The results from quantum scattering simulation (red circles) agree well with the prediction based on the band structure (blue dashed line). The cross section is normalized by the average cross section in free space ๐๐๏ฟฝ0 = 2๐๐/๐๐. The black dashed line indicates the Dirac frequency.
Next, we numerically verify the conservation law of resonant scattering in Dirac systems. As an example, we consider a TLS with a transition frequency of ๐๐0 = 0.461 (2๐๐๐๐/๐๐). The dipole moment of the TLS is in the x direction. The calculated cross sections ๐๐(๐ช๐ช) of the TLS at two different positions are plotted as insets of Supplementary Figure 2c. Similar to the cross section in Weyl photonic crystals, it also strongly depends on the incident wavevector ๐ช๐ช = ๐ค๐ค โ ๐ค๐คDirac and varies significantly at different locations.
The conversation law of resonant cross section in 2D space is slightly different from that in 3D space. Instead of integrating over the isosurface, we now integrate the resonant cross section over the isofrequency contour and the conservation law becomes
๏ฟฝ๐๐(๐ช๐ช)๐๐๐๐ = 8๐๐ (35)
To confirm the above conservation law, we integrate the resonant cross section for a TLS at 16 different locations and plot the results in Supplementary Figure 2c. As expected, the integration โซ๐๐(๐ช๐ช)๐๐๐๐ always results in the same constant of 8๐๐.
We then sweep the transition frequency of the TLS to across the Dirac point, which is indicated by black dashed line in Supplementary Figure 2d. To better demonstrate the enhancement, we also define an average cross section ๐๐๏ฟฝ = โซ๐๐(๐ช๐ช)๐๐๐๐ /๐ถ๐ถ, where C is the total circumference of the isofrequency contours. The calculated average cross section is plotted as red circles in Supplementary Figure 2d. Itโs enhanced by almost three orders of magnitude compared to ๐๐๏ฟฝ0 = 2๐๐/๐๐, the average cross section in free space. At the Dirac frequency, the resonant cross section diverges.
Supplementary Note 5. Proof of suppressed Rayleigh (non-resonant) scattering in Weyl systems
The suppressed Rayleigh scattering in Weyl system can be directly proved by using perturbation theory and Born approximation. In this section, we will describe the mathematical proof in detail.
Under the framework of the first-order Born approximation8, the scattering amplitude ๐๐(๐ค๐คs,๐ค๐คinc)for a Rayleigh scatterer with a weak scattering potential ๐๐(๐ซ๐ซ) is given by
๐๐(๐ค๐คs,๐ค๐คinc) = ๏ฟฝ๐๐3๐ซ๐ซโฒ๐ฎ๐ฎ๐ค๐คs ๏ฟฝ๐ซ๐ซโฒ๏ฟฝ๐๐ ๏ฟฝ๐ซ๐ซโฒ๏ฟฝ๐ฎ๐ฎ๐ค๐คinc ๏ฟฝ๐ซ๐ซ
โฒ๏ฟฝ ๐๐๐๐(๐ค๐คincโ๐ค๐คs)โ๐ซ๐ซโฒ (36)
Here ๐ฎ๐ฎ๐ค๐ค๐๐๐๐๐ค๐คโ๐ซ๐ซ is the eigenmode of the surrounding medium associated with wave vector ๐ค๐ค. ๐ค๐คs and ๐ค๐คinc are the wave vectors of the scattered and incident eigenmodes, respectively. For simplicity, we assume the scatterer is very small compared to the incident wavelength and can be considered as a point scatterer located at ๐ซ๐ซ0. The scattering potential then can be written as ๐๐(๐ซ๐ซ) = ๐๐๐๐๐ฟ๐ฟ(๐ซ๐ซ โ ๐ซ๐ซ0). Note here ๐๐ is a tensor containing the dielectric constant of the scatterer. Thus, the scattering amplitude becomes
๐๐(๐ค๐คs,๐ค๐คinc) = ๐๐๐ฎ๐ฎ๐ค๐คs(๐ซ๐ซ0)๐๐๐ฎ๐ฎ๐ค๐คinc(๐ซ๐ซ0)๐๐๐๐(๐ค๐คincโ๐ค๐คs)โ๐ซ๐ซ0 (37)
The total scattering cross section then can be calculated as
๐๐(๐๐,๐ค๐คinc) = ๏ฟฝ|๐๐(๐ค๐คs,๐ค๐คinc)|2๐ค๐คs
= ๐๐2๏ฟฝ๏ฟฝ๐ฎ๐ฎ๐ค๐คs(๐ซ๐ซ0)๐๐๐ฎ๐ฎ๐ค๐คinc(๐ซ๐ซ0)๏ฟฝ2
๐ค๐คs
(38)
The summation over ๐ค๐คs can be readily converted to a surface integral over the isosurface given by ๐๐(๐ค๐คs) = ๐๐, and Supplementary Equation (38) further becomes
๐๐(๐๐,๐ค๐คinc) = ๐๐2 ๏ฟฝ ๐๐2๐ค๐คs ๐๐:๐๐(๐ค๐ค๐ฌ๐ฌ)=๐๐
๏ฟฝ๐ฎ๐ฎ๐ค๐คs(๐ซ๐ซ0)๐๐๐ฎ๐ฎ๐ค๐คinc(๐ซ๐ซ0)๏ฟฝ2 โ ๐๐2๐๐ (39)
where ๐๐ is the area of the isosurface. In free space, the area of the isosurface S scales ๐๐~๐๐2. Consequently, the Rayleigh scattering cross section scales as ๐๐(๐๐,๐ค๐คinc)~๐๐4. In great contrast, the area of the isosurface S scales ๐๐~โ๐๐2 = (๐๐ โ ๐๐Weyl)2 and thus the Rayleigh scattering cross section scales as ๐๐(๐๐,๐ค๐คinc)~๐๐2(๐๐ โ ๐๐Weyl)2 in Weyl systems.
Supplementary Note 6. Numerical calculation of Rayleigh (non-resonant) scattering in Weyl systems
The Rayleigh scattering cross section can be rigorously calculated by using the normal-mode expansion of the dipole field9โ11 that radiated by the scatterer. In this section, we will briefly describe the normal-mode expansion method that we implemented to numerically calculate the Rayleigh scattering cross section.
In a nonmagnetic medium with a dielectric constant of ๐๐(๐ซ๐ซ), the Maxwellโs equations are given by
โ ร ๐๐ = โ๐๐0๐๐๐๐๐๐๐ก๐ก
(40a)
โ ร ๐๐ = โ๐๐(๐ซ๐ซ)๐๐0๐๐๐๐๐๐๐ก๐ก + ๐๐ (40b)
โ โ (๐๐(๐ซ๐ซ)๐๐0๐๐) = 0 (40c)
โ โ ๐๐ = 0 (40d)
where ๐๐0 is vacuum permeability. The electric (magnetic) field is denoted by ๐๐ (๐๐). An electromagnetic field is produced by a current density ๐๐. Since the charge density is zero, the scalar potential is zero. The electric and magnetic fields can be written in terms of vector potential ๐๐ as
๐๐ = โโ๐๐โ๐ก๐ก
(41a)
๐๐ =1๐๐0โ ร ๐๐ (41b)
Thus, the wave equation for the vector potential ๐๐ is given by
โ ร โ ร ๐๐ +๐๐(๐ซ๐ซ)๐๐2
โ2๐๐โ2๐ก๐ก = ๐๐0๐๐ (42)
where ๐๐ is the speed of light.
The homogeneous solutions to the above wave equation can be written as a superposition of the eigenmodes ๐๐๐ค๐ค(๐ซ๐ซ) = ๐ฎ๐ฎ๐ค๐ค(๐ซ๐ซ)๐๐๐๐๐ค๐คโ๐ซ๐ซ of the photonic crystal, which satisfy the homogenous wave equation
โ ร โ ร ๐๐๐ค๐ค(๐ซ๐ซ) +๐๐๐ค๐ค2
๐๐2 ๐๐(๐ซ๐ซ)๐๐๐ค๐ค(๐ซ๐ซ) = 0 (43)
The eigenmodes ๐๐๐ค๐ค(๐ซ๐ซ) also have to satisfy the orthogonalization, normalization and closure conditions given by
๏ฟฝ๐๐3๐ซ๐ซ ๐๐(๐ซ๐ซ)๐๐๐ค๐ค(๐ซ๐ซ)๐๐๐ค๐คโฒโ (๐ซ๐ซ) = (2๐๐)3๐ฟ๐ฟ3๐ฟ๐ฟ(๐ค๐ค โ ๐ค๐คโฒ) (44)
Here ๐ฟ๐ฟ3 is the normalization volume.
We then consider a generic Rayleigh scatterer embedded in such a medium. During the Rayleigh scattering process, the incident wave induces an oscillating dipole moment ๐๐ = ๐ผ๐ผ๐๐inc(๐ซ๐ซ0) in the scatterer. Here ๐ผ๐ผ is the polarizability of the scatterer, and ๐๐inc(๐ซ๐ซ0) is the local incident electric field at the position of the scatterer. Since the scatterer is quite small compared to the wavelength, the external current source ๐๐ can be written as
๐๐(๐ซ๐ซ, ๐ก๐ก) = โ๐๐๐๐0๐๐๐ฟ๐ฟ(๐ซ๐ซ โ ๐ซ๐ซ0)๐๐โ๐๐๐๐0๐ก๐ก (45)
where ๐ซ๐ซ0 is the position of the scatterer. The vector potential ๐๐(๐ซ๐ซ, t) then can be obtained by solving Supplementary Equation (42) in terms of ๐๐ via the dyadic Greenโs function ๐๐ as
๐๐(๐ซ๐ซ, ๐ก๐ก) = ๏ฟฝ ๐๐๐ก๐กโฒโ
โโ๏ฟฝ๐๐3๐ซ๐ซโฒ ๐๐ ๏ฟฝ๐ซ๐ซโฒ, ๐ก๐ก๏ฟฝ๐๐ ๏ฟฝ๐ซ๐ซ, ๐ก๐ก; ๐ซ๐ซโฒ, ๐ก๐กโฒ๏ฟฝ (46)
The exact expression of the dyadic Greenโs function ๐๐ can be found in Supplementary Reference [8] and we will not discuss the technical details here. Given the vector potential ๐๐(๐ซ๐ซ, ๐ก๐ก), one can show that the time-average radiation power from the induced dipole moment ๐๐ is given by11
๐๐(๐๐) =๐๐๐๐2
4๐๐0๏ฟฝ ๐๐2๐ค๐ค
๐๐(๐ค๐ค)=๐๐
|๐ฎ๐ฎ๐ค๐ค(๐ซ๐ซ0) โ ๐๐|2
๐ฃ๐ฃ๐๐,๐ค๐ค(47)
Here ๐ฃ๐ฃ๐๐,๐ค๐ค is the group velocity associated with wave vector ๐ค๐ค. Then the Rayleigh scattering cross section can be calculated as
๐๐(๐๐,๐ค๐คinc) =๐๐(๐๐)
12๐๐0
๐ฎ๐ฎ๐ค๐คinc(๐ซ๐ซ0) ร ๏ฟฝโ ร ๐ฎ๐ฎ๐ค๐คincโ (๐ซ๐ซ0)๏ฟฝ
(48)
Here we assume the incident wave is one of the eigenmodes associated with wave vector ๐ค๐คinc . The denominator in Supplementary Equation (48) indicates the Poynting vector of the incident wave at the location of the scatterer, which usually does not vary much with the frequency. On the other hand, Supplementary Equation (47) clearly indicates that the radiation power ๐๐(๐๐) is proportional to the area of the isosurface S as ๐๐(๐๐) ~๐๐2๐๐ . Consequently, the Rayleigh scattering cross scales as ๐๐~๐๐2๐๐, which is consistent with Supplementary Equation (39) that we derived by using perturbation theory.
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