Breakdown of the Landau-Ginzburg-Wilson paradigm at quantum phase transitions
Correlated 2D Electron Aspects of the Quantum Hall Effect · 2019-12-18 · ?integer quantum Hall...
Transcript of Correlated 2D Electron Aspects of the Quantum Hall Effect · 2019-12-18 · ?integer quantum Hall...
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Correlated 2D Electron Aspects of the Quantum
Hall Effect
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0 20 40 60 80 100 1200
5
10 ? = 2 ? = 4
compositefermions
"mixed?""stripes"
Res
ista
nce
(arb
. uni
ts)
magnetic field (kG)
Magnetic field spectrum of the correlated 2D electron system:Electron interactions lead to a range of manifestations
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Lectures Outline:
I. Introduction: materials, transport, Hall effects
II. Composite particles – FQHE, statistical transformations
III. Quasiparticle charge and statistics
IV. Higher Landau levels
V. Other parts of spectrum: non-equilibrium effects, electron solid?
VI. Multicomponent systems: Bilayers
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Outline:
I. Introduction: materials, transport, Hall effects
II. Composite particles – composite fermions
III. Quasiparticle charge and statistics
IV. Higher Landau levels
V. Other parts of spectrum: non-equilibrium effects, electron solid?
VI. Multicomponent systems: Bilayers
A. General 2D physics B. Materials – MBEC. Measurements – quantum Hall effectD. CorrelationsE. Fractional quantum Hall effect
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A. General 2D physics
I. Introduction: materials, transport, Hall effects
ky
kx
kF= (2?n)1/2
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A. General 2D physics
I. Introduction: materials, transport, Hall effects
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A. General 2D physics
I. Introduction: materials, transport, Hall effects
Higher Landau levels have more nodes
Magnetic length l0
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A. General 2D physics
I. Introduction: materials, transport, Hall effects
1
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A. General 2D physics
I. Introduction: materials, transport, Hall effects
What are the sources of scattering in a real 2D
electron system?
How do you make a real 2D electron system?
Molecular beam epitaxy
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Heated substrate
Ga AsAl Si
B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
In ultra-high vacuum, sources provide material that is evaporated onto a heated substrate
The material is deposited at ~ monolayers / second
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Loren Pfeiffer Ken West
2D electrons in high purity AlGaAs/GaAs interface
GaAs
AlGaAs
2D electron gas forms at interface of AlGaAs/GaAs in MBE grown crystal
Si doping
B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
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B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
The material is deposited at ~ monolayers / second
Shuttering different sources layers the materials
AlGaAs
AlGaAs
AlGaAs
AlGaAs
GaAs
GaAs
GaAs
15 monolayers
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B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
a) layering: electrons from Si layer reside at AlGaAs/GaAsinterface – ionized dopants isolated from electron layer
b) Energy level diagram: electron wavefunction traverses interface plane, has finite z-extent – only lowest bound state used
Doping modulation
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B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
(<1nm in normal metal)
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Temperature (K)0.1 1 10 100
104
103
106
105
107
Ele
ctro
n M
ob
ility
(cm
2 /V
sec)
1998
1988
1986
1982
1981
1980
1979
1978
Bulk
31 million cm2/Vsec
Si-modulation-doping Stormer-Gossard-Dingle
Undoped setback
Single interface
Sample loadlock
LN2 Shielded Sources
Al, Ga, As SourcePurity
UHV cryopump bake
Sample structure2000
Historical landmarks of 2DEG mobility
in GaAs.
Annotated with the specific
MBE innovation that
caused the mobility
improvement.
B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
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Scattering mechanisms:
? interface roughness
? alloy scattering
? ionized impurities
? residual disorder
? “systematic” disorder
B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
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B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
Numerous “tricks” used to provide clean layer interfaces to reduce the scattering probabilities
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Multiple uses for MBE samples:
Electronic and structural
B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
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C. Measurements – Hall effect
I. Introduction: materials, transport, Hall effects
Cool down:? He4? He3? Dilution process
Apply B-field orthogonal to sample
Diffuse contacts into wafer pieceCleave piece of wafer
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current
Voltage R
Piece of MBE wafer
Metal contacts to 2D electrons
direct current from one contact to another with magnetic field applied perpendicular to layers
Measure scattering length (mean-free-path)
Scattering length is curved path length
characterizing the electron system
300 ? m mean-free-path in best samples:<1nm in normal metal
B. Materials – molecular beam epitaxy
I. Introduction: materials, transport, Hall effects
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Rxy
RxxIxx
B-field
B-field
Rx
y
C. Measurements – Hall effect
I. Introduction: materials, transport, Hall effects
12
3
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Rxy
RxxIxx
B-
field
B-fieldR
xy
C. Measurements – Hall effect
I. Introduction: materials, transport, Hall effects
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Shubnikov-deHaas oscillations
C. Measurements – Hall effect
I. Introduction: materials, transport, Hall effects
With increasing B, degeneracy of LL increases and Fermi level is swept through spectrum (constant density n)
Landau levels resolved when ? c?>>1
B
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Localization of single electrons between extended states produces plateaus in Hall resistance
C. Measurements – quantum Hall effect
I. Introduction: materials, transport, Hall effects
At extended states, the Hall voltage increases
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C. Measurements – quantum Hall effect
I. Introduction: materials, transport, Hall effects
RH = (1/?)(h/e2)
(Spin gaps at filling factors 1,3,5,…..)
Minima at n = 2, 4, 6,.. show activated transport
R = R0 e(-? /kT)
? = cyclotron gap
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C. Measurements – quantum Hall effect
I. Introduction: materials, transport, Hall effects
RH = (1/?)(h/e2)
Integral quantum Hall effect represents single particle localization process
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Edge conduction
C. Measurements – quantum Hall effect
I. Introduction: materials, transport, Hall effects
No backscattering
along same edge
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C. Measurements – quantum Hall effect
I. Introduction: materials, transport, Hall effects
RH = (1/?)(h/e2)
- samples must have sufficiently low disorder that the Landau levels can be resolved (? c?>>1)
- decreasing disorder further will unveil correlations
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Correlations
D. Correlations
I. Introduction: materials, transport, Hall effects
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D. Correlations
I. Introduction: materials, transport, Hall effects
Magnetic field quenches kinetic energy:If low intrinsic disorder, correlations manifest
At high magnetic fields, electron orbits smaller than electron separation
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Potential Energy
x
Electron gas(or liquid)
Fluctuations in potential
Correlation effects may be seen IF:1) Temperature is low enough2) Disorder is low enough
D. Correlations
I. Introduction: materials, transport, Hall effects
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Potential Energy
x
Electron gas
Fluctuations in potential
Lower density = Larger influence of disorder on electron gas
Correlation effects may be seen IF:1) Temperature is low enough2) Disorder is low enough
D. Correlations
I. Introduction: materials, transport, Hall effects
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Potential Energy
x
Electron gas
Fluctuations in potential
Disorder can destroy correlations
Correlation effects may be seen IF:1) Temperature is low enough2) Disorder is low enough
D. Correlations
I. Introduction: materials, transport, Hall effects
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Potential Energy
Electron gas
x
Fluctuations in potential
Correlation effects may be seen IF:1) Temperature is low enough2) Disorder is low enough
D. Correlations
I. Introduction: materials, transport, Hall effects
MINIMIZE DISORDER and USE HIGH ELECTRON DENSITY
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Potential Energy
x
Electron gas
Fluctuations in potential
MINIMIZE DISORDER and USE HIGH ELECTRON DENSITY
Correlation effects may be seen IF:1) Temperature is low enough2) Disorder is low enough
D. Correlations
I. Introduction: materials, transport, Hall effects
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D. Correlations
I. Introduction: materials, transport, Hall effects
Back to transport measurements:
Higher mobility (lower disorder) samples produced –AlGaAs/GaAs heterostructures, modulation doped
new quantum Hall state found at fractional filling factor 1/3
(note: high densities, high B – fields)
1 ½ 1/3
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
Higher mobility (lower disorder) samples produced –new quantum Hall state found at fractional filling factor: shouldn’t be there
? = 1 ? = 1/3Energy
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1) a hierarchy of fractions observed:
New “quantum numbers” at 1/3, 2/5, 3/7, 4/9,….
Filling factor ? = p / (2p+1)
E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx
(ar
b. u
nits
)
magnetic field (kG)
2/5
1/3
3/7
Higher mobility samples show more FQHE states
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1) a hierarchy of fractions observed:
New “quantum numbers” at 1/3, 2/5, 3/7, 4/9,….
Filling factor ? = p / (2p+1)
2) The minima display activated transport:
R = R0 e(-? /kT)
? here should reflect the Coulomb energy
e2/?l0
E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx
(ar
b. u
nits
)
magnetic field (kG)
2/5
1/3
3/7
Higher mobility samples show more FQHE states
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
How can this all be explained?
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
The Laughlin wave function
Describes an incompressible quantum liquid at ?=1/3
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E. The Fractional quantum Hall effect - pictures
I. Introduction: materials, transport, Hall effects
Single electron in the lowest Landau level
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E. The Fractional quantum Hall effect - pictures
I. Introduction: materials, transport, Hall effects
Single electron in the lowest Landau level
Filled lowest Landau level
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E. The Fractional quantum Hall effect - pictures
I. Introduction: materials, transport, Hall effects
Uncorrelated ? = 1/3 state
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E. The Fractional quantum Hall effect - pictures
I. Introduction: materials, transport, Hall effects
Uncorrelated ? = 1/3 state Correlated ? = 1/3 state
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
The Laughlin wave function and its excitations
Add one flux quantum
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
The Laughlin liquid and its excitations
??= 1/3 + Badd one flux quantum
??= 1/3 - Bsubstract one flux quantum
?= 1/3 quantum liquiduniform density
Non-uniform charge densities
Added charges +, - 1/3e
Energy required to change charge is ? ?~ e2/?l0l0 the magnetic length
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
Laughlin state describes:
1) New incompressible liquid state
2) Excitations of the liquid, charge 1/m
3) Consistency with experimental results at 1/3, 1/5 (found later)
Fractionally charged excitations
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
Higher mobilities result in more fractional quantum Hall states
0 20 40 60 80 100 1200
5
10
Res
ista
nce
(arb
. uni
ts)
magnetic field (kG)
? = 2 ? = 1
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E. The Fractional quantum Hall effect
I. Introduction: materials, transport, Hall effects
Even higher mobilities result in even more fractional quantum Hall states
Pan,et al. PRL 04
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Summary:
?2D electron samples show 2D physics in transport: Shubnikov-deHaas oscillations
?integer quantum Hall effect: resolved Landau levels with localization between centers of Landau levels
?low disorder 2D electron systems show fractional quantum Hall effect – correlations of electrons as described by the Laughlin wave function
?what about manyfractional quantum Hall states?
I. Introduction: materials, transport, Hall effects
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Outline:
I. Introduction: materials, transport, Hall effects
II. Composite particles – composite fermions
III. Quasiparticle charge and statistics
IV. Higher Landau levels
V. Other parts of spectrum: non-equilibrium effects, electron solid?
VI. Multicomponent systems: Bilayers
A. Experiments - hierarchy of fractionsB. Composite fermions and their Landau levelsC. Composite fermions and experimentsD. Fermi surface picture - SAWE. Other Fermi surface experiments F. Composite fermion effective massG. Other composite fermions
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A. Experiments - hierarchy of fractions
II. Composite particles – composite fermions
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx (
arb.
uni
ts)
magnetic field (kG)
2/5
1/3
3/7With lower disorder samples, more fractional states observed
Better samples, larger activation energies
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1/3 filling factor understood from Laughlin state: what are the others?
FQHE states found at filling factors ??= p/(2p+1), p=1, 2, 3...
Or more generally, at filling factors ??= p/(2np ± 1) and at ?= 1 - p/(2np ± 1)
This includes series of 2/3, 3/5, 4,7… and the series around filling factor 1/4
A. Experiments – hierarchy of fractions
II. Composite particles – composite fermions
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx
(arb
. uni
ts)
magnetic field (kG)
2/5
1/3
3/7
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
magnetic field
electrons
From previous description of FQHE liquid we saw that a “correlation hole”is energetically favorable spot for electron to reside: this “associates”flux line(s) to the electrons - example 1/3
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
magnetic field
electrons
Any number of magnetic flux may be associated with charge to produce a quasiparticle of the flux/charge composite
Filling factor 0 1 1/2 1/3
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
magnetic field
electrons
Given that flux may be associated with charge, now examine the statistics of these quasipartles:An electron wave function upon particle exchange gains phase change
FERMIONS
e-i?
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
magnetic field
electrons
Given that flux may be associated with charge, now examine the statistics of these quasipartles:An electron with one associated flux quantum obeys bosonic statistics
FERMIONS
e-i?
BOSONS
e-i2?
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
magnetic field
electrons
Given that flux may be associated with charge, now examine the statistics of these quasipartles:An electron with two associated flux quanta obeys fermionic statistics
FERMIONS
e-i?
COMPOSITE FERMIONS
e-i?
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
magnetic field
electrons
J. Jain examined the correlated 2DES using the quasiparticle, the composite fermion, with the rational that the FQHE states are due to Landau levels of this quasiparticle
COMPOSITE FERMIONS
e-i?
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
Composite particles of charge and magnetic flux:
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx
(arb
. uni
ts)
magnetic field (kG)
2/5
1/3
3/7
Composite fermion at its filling factor of 1
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx
(ar
b. u
nits
)
magnetic field (kG)
1/2
1/3
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B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
0 20 40 60 80 100 1200
1
2
3
4
5
Rxx
(ar
b. u
nits
)
magnetic field (kG)
+B(?=1/2)
1/2
1/3
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By enumeration, the hierarchy of observed fractions now become integer Landau levels for this quasiparticle
true composite fermionfilling factor filling factor
1/3 12/5 23/7 34/9 4
6 8 1 0 1 2 1 4
0
Rxx
M a g n e t i c f i e l d i n T e s l a
1
5/9
4/72/5
6/11
7/13
6/13
2/3 3/5
9/17
8/15
5/114/9
3/7
7/15
9/19
8/17
1/3
B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
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While this picture developed, new findings at an “odd” location –
Filling factor 1/2 : should be the center of the Landau level –non-localized electrons following the classical Hall trace – metallic?
1/23/2
5/2
B. Composite fermions and their Landau levels
II. Composite particles – composite fermions
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Surface acoustic wave experiments:Measure conductivity over short distances
C. Composite fermions and experiments
II. Composite particles – composite fermions
? sound
0.2 – 30 ? m
Propagating sound wave applies electric field: electrons respond to this field
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? SAW
SAW measures conductivity of the 2DES at the wavelength and
frequency of the SAW
? xx(q,? ) <=> ? v/v
SAW device launches longitudinal wave with E-field in direction of
propagation: conducting layer can short this piezoelectric field, changing
the propagation properties
C. Composite fermions and experiments
II. Composite particles – composite fermions
SAW ? down to 0.2? m
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Results: At low frequencies, large wavelengths see all the features of a standard transport measurement
C. Composite fermions and experiments
II. Composite particles – composite fermions
SAW measures conductivity of the 2DES at the wavelength and
frequency of the SAW
? xx(q,? ) <=> ? v/v
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Results:
At higher frequencies, smaller wavelengths (<3? m),
see new features at ½ filling factor
Marks a new quantum number
C. Composite fermions and experiments
II. Composite particles – composite fermions
? = 1/2
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Results:
The smaller the wavelength, the larger the feature at 1/2
Feature corresponds to enhanced conductivity
C. Composite fermions and experiments
II. Composite particles – composite fermions
? = 1/2
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Results:
At 3GHz, 1? m ? , dominant feature is enhanced conductivity at ½
C. Composite fermions and experiments
II. Composite particles – composite fermions
? = 1/2
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C. Composite fermions and experiments
II. Composite particles – composite fermions
What is causing this?
For higher frequencies, smaller wavelengths, the enhanced conductivity grows
1/2
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
Halperin, Lee, and Read (1993):
Quasiparticle composite fermions produce not only FQHE by filling Landau levels, they also form true filled Fermi sea at filling factor ½
ky
kx
kF= (2)1/2 kF electrons
at ? = 1/2
Near ½, quasiparticles move in effective magnetic field Beffective = Bapplied - B (1/2)
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
Halperin, Lee, and Read (1993):
Quasiparticle composite fermions produce not only FQHE by filling Landau levels, they also form true filled Fermi sea at filling factor ½
ky
kx
kF= (2)1/2 kF electrons
at ? = 1/2
Near ½, quasiparticles move in effective magnetic field Beffective = Bapplied - B (1/2)
Away from ½ the quasiparticles move in cyclotron orbits with radiusRc = h kF / 2?e Beffective
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Halperin, Lee, and Read (1993):
Quasiparticle composite fermions produce not only FQHE by filling Landau levels, they also form true filled Fermi sea at filling factor ½
D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
Near ½, quasiparticles move in effective magnetic field
Beffective = Bapplied - B (1/2)
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
For SAW wavelength less than the composite fermion mean-free-path, enhanced conductivity observed
Wavevector dependence of conductivity derived in HLR
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
Width of enhanced conductivity at ½ used to extract kF of composite fermions
FWHM
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
H.L.R. :
Commensurability of composite fermion cyclotron orbit and potential (SAW or lithographically defined) should be observed as has been done for electrons
Need composite fermion mean-free-path > 2?Rc
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
H.L.R. :Explicit predictions for SAW results if commensurability present –Use large SAW q and large composite fermion m.f.p
1/2
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
For large SAW q, large composite particle m.f.p.must also consider denstiy inhomogeneities
1/2
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
Commensurability experimentally observed
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
10 GHz SAW
secondary resonance
primary resonance
SAW ? ?
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D. Fermi surface picture: composite fermions form Fermi surface at filling factor 1/2
II. Composite particles – composite fermions
Experimental magnetic field positions of resonances for different SAW wavevectors can measure kF.
? B ~ kF qSAW
kF= (2)1/2 kF electrons
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E. More experiments on Fermi surfaces: focusing
II. Composite particles – composite fermions
direct current from one contact to another with magnetic field applied perpendicular to layers
Smet: PRL 94
Use composite fermion cyclotron radius to focus into contacts
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E. More experiments on Fermi surfaces: antidots
II. Composite particles – composite fermions
Encircle holes made in 2D gas with cyclotron orbits and resistance increases as with electrons
Kang, et al. PRL 93
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E. More experiments on Fermi surfaces: ballistic shorting
II. Composite particles – composite fermions
As nanostructure channel is defined, the Beffective ballistic charge transport is enhanced for both electrons and composite fermions
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F. Composite fermion effective mass
II. Composite particles – composite fermions
H.L.R.:Cyclotron energy gaps of the composite fermions use the effective mass of the quasiparticle
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F. Composite fermion effective mass
II. Composite particles – composite fermions
in transport measurements the activation energies of the series of fractions (4/9, 3/7, 2/5, 1/3) corresponding to composite fermion Landau levels 4,3,2,1 indeed increase linearly withBeffective.
The effective mass derived from this is ~ 0.8me, almost a factor of 10 larger than the free GaAs mass.
A mass divergence toward ½ is expected
Du, et al. PRL 93
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F. Composite fermion effective mass
II. Composite particles – composite fermions
Further transport measurements support this
Du, et al. PRL 95
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F. Composite fermion effective mass
II. Composite particles – composite fermions
This effective mass picture is compared with the results from SAW measurements:
The quasiparticle cyclotron orbit frequency must be greater than the SAW frequency to observe resonances
As effective mass increases, the cyclotron frequency will drop
10 GHz SAW
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10 GHz SAW
F. Composite fermion effective mass
II. Composite particles – composite fermions
The observation of SAW resonances is not consistent with a diverging composite fermion effective mass
See theory of effective mass, Simon et al 96.
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G. Other composite fermions
II. Composite particles – composite fermions
Composite fermions and their Fermi surfaces expected at other even denominator filling factors (1/4, 3/4, 3/2, 3/8, …)
Features observed in transport
Resonances in SAW observed, positions in Beffective must be adjusted for the active composite particle number.
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G. Other composite fermions
II. Composite particles – composite fermions
Composite fermions and their Fermi surfaces expected at other even denominator filling factors (1/4, 3/4, 3/2, 3/8, …)
Presumably observed in transport
Resonances in SAW observed, positions in Beffective must be adjusted for the active composite particle number.
3/2
3/4
1/4
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G. Statistical transformations and vortex picture:
6 8 1 0 1 2 1 4
0
Rxx
M a g n e t i c f i e l d i n T e s l a
1
5/9
4/72/5
6/11
7/13
6/13
2/3 3/5
9/17
8/15
5/114/9
3/7
7/15
9/19
8/17
1/3
Composite fermions
Composite bosons
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Summary:
?2D electron samples show 2D physics: shubnikov-deHaas oscillations
?integer quantum Hall effect: resolved Landau levels with localization between centers of Landau levels
?low disorder 2D electron systems show fractional quantum Hall effect – correlations of electrons as described by the Laughlin wave function
?composite fermions explain series of fractional quantum Hall states
?statistical transformations an important part of the magnetic field spectrum in 2D