Cloud screening and aerosol retrievals from MAX-DOAS measurements at Ukkel Clio Gielen Michel Van...
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Transcript of Cloud screening and aerosol retrievals from MAX-DOAS measurements at Ukkel Clio Gielen Michel Van...
Cloud screening and aerosol retrievals from MAX-DOAS measurements at Ukkel
Clio GielenMichel Van Roozendael, Francois Hendrick, Caroline Fayt,
Christian Hermans, Gaia Pinardi, Didier Gilllotay, and Tim Vlemmix
+ Hugo De Backer, Veerle De Bock, and Quentin Laffineur from RMI
BIRA contribution to WP3:
Goals
Qualify sky and cloud conditionsfrom MAX-DOAS data
Apply to Ukkel station to improve aerosol retrievals
Tasks 3.1 (algorithm improvements) and 3.2 (operating a MAX-DOAS instrument at Ukkel)
Sky conditions: the colour index
Trace gas and aerosol retrievals affected by clouds
→ introduce: additional photon absorption multiple scattering strong temporal variation Degenerate problem: thin/thick clouds, broken clouds, fog, haze, white clouds, grey clouds, high/low aerosol load, ....
Use observed colour of the sky for characterisation
→ Colour Index = ratio of intensities
Colour Index characteristics
Investigation of the colour index shows that:
- the CI = high for clear skies
- the CI < in the presence of clouds, aerosols,
fog,...
- the CI = a constant value over time in the
presence of
optically thick clouds
- the CI = highly variable in the presence of
broken/scattered clouds
Cloud-Screening flags
Using the colour index we define two flags:
- a flag to describe the general sky condition (clear/polluted/full-cloud cover)
→ Colour-Index flag
- a flag to note the presence of scattered clouds
→ Broken-Cloud flag
Broken-Cloud flag
Temporal variation to determine presence of scattered clouds
→ model observations with double-sine function and detect outliers→ no information on presence of full-cloud cover!
Colour-Index flag: sky condition
Good
Mediocre
Bad
By combining measurements and simulations we define 3 sky-condition regions
Good= clear sky
Med= thin clouds/ low
aerosols
Bad= thick clouds/ high
aerosols
Impact on aerosol retrievals
+ no cloud screening
+ CI-flag=good/med
+ CI-flag=good/med and no broken clouds
◊ AOD measurements (Aeronet + Brewer)
+ AOD retrievals (MAX-DOAS + bePRO profiling
code)
Impact on aerosol retrievals
+ no cloud screening
+ CI-flag=good/med
+ CI-flag=good/med and no broken clouds
Interpretation of aerosol data at Ukkel
Exploiting the ensemble of data at BIRA-RMI (task 3.3):
- BIRA: Aerosol AOD and extinction profiles (MAX-
DOAS) Aerosol AOD (CIMEL) Cloud screening (MAX-DOAS) Cloud-cover fraction (thermic infrared)
- RMI: Aerosol AOD (Brewer) Backscatter profiles/mixing-layer height
(lidar) Cloud screening (lidar/Brewer)+ Aethalometer in the future
Vertical Profiles: BIRA-RMI
Aerosol AOD (BIRA/RMI)
Backscatter/ cloud/MLH
(RMI)
Aerosol vert.prof+
cloudscreening(BIRA)
Aerosol vert.prof(BIRA)
Status
- Operational cloud-screening method for MAX-DOAS measurements
- Aerosol retrievals for full Ukkel dataset (2011-2013): AOD and extinction profiles
- Applying cloud screening strongly improves aerosol retrievals
- Good agreement between BIRA cloud screening and RMI data
- Good agreement between MAX-DOAS cloud screening and thermal infrared cloud-cover data
Future tasks for the last part of the project
- Further improvement of cloud-screening method: Include O4 DSCDs → distinguish
clouds/aerosols/fog... + cloud bottom height
- Detailed study of aerosol retrievals at Ukkel (BIRA + RMI):
Trends (seasonal/daily/weekly) Correlation with meteorology
- Estimation of the radiative forcing effect at Ukkel (task 3.3)