Circularity Assessment of Water and Waste in Cities

88
Circularity Assessment of Water and Waste in Cities A Proposed Framework for Sustainable Performance Evaluation using LCA and LCC Kavitha Shanmugam Department Of Chemistry Umeå 2021

Transcript of Circularity Assessment of Water and Waste in Cities

Page 1: Circularity Assessment of Water and Waste in Cities

Circularity Assessment of Water and

Waste in Cities

A Proposed Framework for Sustainable Performance

Evaluation using LCA and LCC

Kavitha Shanmugam

Department Of Chemistry

Umeå 2021

Page 2: Circularity Assessment of Water and Waste in Cities

This work is protected by the Swedish Copyright Legislation (Act 1960:729) Dissertation for PhD ISBN: 978-91-7855-527-7 (print) ISBN: 978-91-7855-528-4 (pdf) Cover Art: Harish Kumar with Kavitha Shanmugam Electronic version available at: http://umu.diva-portal.org/ Printed by: VMC-KBC,Umeå University Umeå, Sweden 2021

Page 3: Circularity Assessment of Water and Waste in Cities

To my Dad and Mom

I love you both a lot, appreciate your effort, and love in bringing me up

to be a better individual

Page 4: Circularity Assessment of Water and Waste in Cities

1

Table of Contents

Abstract ............................................................................................. 3

Abbreviations .................................................................................... 5

Definitions ........................................................................................ 8

Sammanfattning på svenska ............................................................. 9

List of Publications .......................................................................... 11

Authors Contributions ..................................................................... 12

1. Introduction ................................................................................. 13

2. Objective of this Thesis ................................................................. 17

3. Urban System ............................................................................... 19 3.1 Elements of an Urban System .................................................................................. 19 3.2 Essential Municipal Services ................................................................................... 20

3.2.1 Wastewater Treatment Service ...................................................................... 21 3.2.2 Municipal Solid Waste (MSW) Treatment Service ...................................... 23

3.3 Management of Essential Municipal Services in Cities Complying with Circular

Economy Principles ........................................................................................................ 27

4. Tool & Methodology ..................................................................... 31 4.1 Life Cycle Assessment ............................................................................................... 31

4.1.1 Goal & Scope Definition .................................................................................. 33 4.1.2 Life Cycle Inventory (LCI) Analysis ...............................................................35 4.1.3 Life Cycle Impact Assessment ........................................................................ 36 4.1.4 Interpretation of Results ................................................................................ 39 4.1.5 Uncertainty Analysis ....................................................................................... 41 4.1.6 Scenario Analysis ........................................................................................... 42 4.1.7 Limitations of LCA .......................................................................................... 43

4.2 Life Cycle Costing (LCC) ......................................................................................... 44 4.3 Environmental Externalities Cost ........................................................................... 45

5. Contribution of Papers to the Development of the Framework ....47

6. Assessment Framework for Treatment of Municipal Services in

Cities ............................................................................................... 50 6.1 Proposed Assessment Framework ........................................................................... 51 6.2 Attributes of the Framework .................................................................................... 55

6.2.1 Assessment Framework - Data Requirements .............................................. 55 6.2.2 Assessment Framework – Stage-wise Technology Options for carrying out

LCAs ......................................................................................................................... 58 6.2.3 Total Cost Calculation .................................................................................... 60 6.2.4 Future Work to Develop the Framework ...................................................... 61 6.2.5 Unique Features of the Model........................................................................ 62

6.3 Case Study of a Wastewater Treatment Plant ........................................................ 62

7. Conclusion & Future work ............................................................67

Page 5: Circularity Assessment of Water and Waste in Cities

2

8. Acknowledgements ..................................................................... 69

References ....................................................................................... 71

Appendix ............................................................................................ 1

Papers I-V ......................................................................................... 5

Page 6: Circularity Assessment of Water and Waste in Cities

3

Abstract

Urbanization is a global phenomenon, happening on a massive scale and at a

rapid rate, with 68% of the planet’s population predicted to be living in cities by

2050 (UN-DESA, 2018). The sustainability of a city (Goal 11 of UN SDGs)

undergoing rapid urbanization depends on its ability to maintain a low

consumption of resources and materials at any given time (referred to as the

urban metabolic rate), whilst simultaneously providing essential municipal

services to its inhabitants, such as a water supply, wastewater treatment and solid

waste management. The latter must comply with circular economy principles,

meaning recovery of byproducts, prevention of discharge of toxic pollutants, and

avoidance of landfill usage. The appended papers in the thesis (Papers I–V)

describe sustainable assessments of wastewater and waste services to increase

their degree of circularity, using tools such as Life Cycle Assessment (LCA) and

Life Cycle Costing (LCC). Paper I describes the environmental performance of

using the biogas from a Wastewater Treatment Plant (WWTP) and converting it

to Liquefied Biomethane (LBM), which can used as fuel in Tractor-Trailers (TT).

Overall, the study suggests that changing from diesel to LBM fuel improves the

environmental performance of TT. However, the magnitude of environmental

benefit depends on an alternate source of electricity required for operation of the

WWTP. Paper II evaluates the Social Cost-Benefit Analysis (SCBA) of

Compressed Biomethane (CBM) obtained from a food waste digestion plant in

Mumbai, India for use as a fuel in transit buses. SCBA results indicate that the

food waste-based CBM model can save 6.86 billion Indian rupees (99.4 million

USD) annually for Mumbai. Paper III describes the Sustainable Return on

Investment (SROI) of lightweight Advanced High Strength Steel (AHSS) and

Carbon Fiber Reinforced Polymer (CFRP) intensive multi-material Body in White

(BIW) for automobiles. The SROI of CFRP BIWs is maximized when carbon fiber

production uses energy from a low carbon-intensity electric grid or decentralized

sources such as waste-to-energy incineration plants. Paper IV assesses the

ecoefficiency of a thermal insulation panel that consists of a Polyurethane (PU)

foam core sandwiched between two epoxy composite skins, prepared by

reinforcing Glass Fibers (GF) and SFA (Silanized Fly Ash) in epoxy resin. The

results revealed that the ecoefficiency of the composite panels is positive (47%)

and superior to that of market incumbent alternatives with PU foam or rockwool

cores and steel skins. Paper V quantifies the Total Cost to Society (TCS) (sum of

private cost and environmental externalities cost) of a centralized urban WWTP,

including the operation as well as byproduct utilization stream. The

environmental performance and circular compliance are both factored in, when

determining the TCS of a WWTP. The results revealed savings of 1.064 million

USD, which include direct and indirect revenues to the plant, as well as avoidance

costs attributed to environmental externalities. Based on the studies described in

Page 7: Circularity Assessment of Water and Waste in Cities

4

these papers, a five-stage assessment framework for determining the overall

sustainability performance of essential treatment services in a city is proposed in

this thesis. The framework considers the combined effect of urban metabolic

features and initiatives aimed at improving circular compliance of essential

services.

Page 8: Circularity Assessment of Water and Waste in Cities

5

Abbreviations

AD Anaerobic Digestion

AHSS Advanced High Strength Steel

AP Acidification Potential

BAU Business as Usual

CBM Compressed Biomethane

CED Cumulative Energy Demand

CF Characterization Factor

CFRP Carbon Fiber Reinforced Polymer

CNG Compressed Natural Gas

EEC Environmental Externalities Cost

EU European Union

FDP Fossil Depletion Potential

FEP Freshwater Eutrophication Potential

FETP Freshwater Ecotoxicity Potential

FU Functional Unit

GDP Gross Domestic Product

GF Glass Fibers

GWP Global Warming Potential

HH-CP Human Health-Cancer Potential

HH-NCP Human Health-Non-Cancer Potential

Page 9: Circularity Assessment of Water and Waste in Cities

6

HTP Human Toxicity Potential

IFA Incineration Fly Ash

ISO International Standard Organization

LCA Life Cycle Assessment

LCC Life Cycle Costing

LCEE Life Cycle Environmental Externalities

LCI Life Cycle Inventory

LCIA Life Cycle Impact Assessment

LUP Land Use Potential

MCDA Multi Criteria Decision Analysis

MFDP Mineral Fossil Depletion Potential

MSW Municipal Solid Waste

OD Ozone Depletion

OFW Organic Food Waste

PMFP Particulate Matter Formation Potential

POFP Photochemical Ozone Formation Potential

PU Polyurethane

SCBA Social Cost Benefit Analyses

SDGs Sustainable Development Goals

SFA Silanized Fly Ash

SROI Sustainable Rate of Returns

SRR Sustainable Rate of Returns

Page 10: Circularity Assessment of Water and Waste in Cities

7

TCMS Total Cost of Municipal Services

TCS Total Cost to Society

TCUMR Total Cost of Urban Metabolic Rate

TEP Terrestrial Ecotoxicity Potential

TPC Total Private Cost

TT Tractor-Trailers

UMR Urban Metabolic Rate

UN United Nations

WtE Waste-to-Energy

WWTP Waste Water Treatment Plant

Page 11: Circularity Assessment of Water and Waste in Cities

8

Definitions

Urbanization is defined as an increase (population shift) in the proportion of

people living in urban areas compared to rural areas. An urban area is a built-up

area such as a town or city.

Sustainability is defined as meeting our own needs without compromising the

ability of future generations to meet their own needs (the ability to exist

constantly).

Ecological Footprint measures how fast human activities consume resources

and generate waste compared to how fast nature can absorb that waste, and

regenerate.

Total Cost is defined as the sum of private costs plus environmental externality

costs associated with the system studied.

Urban system refers to the area around a city.

Circular Economy or Circularity is an economic system aimed at

minimizing waste with the continual use of resources (contrast to linear economy

– take, make, dispose).

Framework is defined as a basic structure underlying a system, concept or text.

Municipality is an urban administrative division having corporate status that is

connected to other municipalities, regions, states and international communities

through resource areas, financial systems, social influences and transnational

paradigms.

Essential Municipal Services, in this thesis, are considered to be wastewater

treatment, waste services including organic waste management, and residual

waste management provided by the municipality.

Page 12: Circularity Assessment of Water and Waste in Cities

9

Sammanfattning på svenska

Urbanisering är ett globalt fenomen som sker i stor skala och i snabb takt, där

68% av jordens befolkning förutspås bo i städer år 2050 (UN-DESA, 2018).

Hållbarheten för en stad (UN SDG, Mål 11) som genomgår en snabb urbanisering

beror på dess förmåga att upprätthålla en låg förbrukning av resurser och

material vid varje given tidpunkt (kallas urban metabolic rate), samtidigt som den

tillhandahåller viktiga kommunala tjänster till dess invånare, såsom

vattenförsörjning, avloppsvattenrening och hantering av fast avfall. De senare

måste följa principerna för cirkulär ekonomi, vilket innebär återvinning av

biprodukter, förebyggande av utsläpp av giftiga föroreningar och undvika

material på deponi. Artiklarna i avhandlingen (Papers I – V) beskriver

hållbarhetsbedömningar av avloppsvattenrening och avfallstjänster för att öka

deras grad av cirkularitet med hjälp av verktyg som Life Cycle Assessment (LCA)

och Life Cycle Costing (LCC). I Paper I beskrivs miljöprestandan för att använda

biogasen från ett reningsverk (ARV) och omvandla den till flytande biometan

(LBM), som kan användas som bränsle i tyngre fordon. Sammantaget föreslår

studien att byte från diesel till LBM-bränsle förbättrar miljöprestandan.

Storleken på miljöfördelarna beror dock på vilken alternativ el som krävs för drift

av reningsverket. Paper II utförs en sociala kostnadsnyttoanalysen (SCBA) av

komprimerad biometan (CBM) som producerasvid en matavfallsanläggning i

Mumbai, Indien för användning som bränsle i bussar. SCBA-resultaten tyder på

att den livsmedelsbaserade CBM-modellen kan spara 6,86 miljarder indiska

rupier (99,4 miljoner USD) årligen för Mumbai. Paper III beskriver hållbar

avkastning på investeringar (SROI) av avancerat lättvikts höghållfast stål (AHSS)

och kolfiberförstärkt polymer (CFRP) som komponeneter i materialstommen i

bilar. SROI maximeras när kolfiberproduktion använder elenergi med låg

koldioxidintensitet eller från decentraliserade källor, såsom

avfallsförbränningsanläggningar. I Paper IV bedöms ekoeffektiviteten för en

värmeisoleringspanel som består av en polyuretanskumkärna (PU) som lager

mellan två epoxikompositsidor, och med förstärkning av glasfibrer (GF) och SFA

(Silanized Fly Ash) i epoxiharts. Resultaten visar att ekoeffektiviteten hos

kompositpanelerna är positiv (47%) och överlägsen den för de befintliga

alternativen på marknaden med PU-skums- eller stenullskärnor och ståls. Paper

V kvantifierar den totala kostnaden för samhället (TCS) (summan av privata

kostnader och miljökostnader) för ett centraliserat stadsnätverk, inklusive drift

och biproduktanvändning. Miljöprestanda och graden av cirkularitet inkluderas

vid bestämning av TCS för ett avloppsreningsverk. Resultaten visar på stora

besparingar (1.064 miljoner USD i exemplet), som inkluderar direkta och

indirekta intäkter till anläggningen, samt undvikande av kostnader som

hänförstill externa miljöeffekter.

Page 13: Circularity Assessment of Water and Waste in Cities

10

Baserat på studierna som beskrivs i dessa artiklar föreslås i avhandlingen en fem-

stegs utvärderingsram för bestämning av den övergripande

hållbarhetsprestandan för viktiga behandlingstjänster i en stad.

Bedömningsramverket tar hänsyn till den kombinerade effekten av

stadsmetaboliska funktioner och initiativ som syftar till att förbättra

cirkulariteten hos viktiga tjänster.

Page 14: Circularity Assessment of Water and Waste in Cities

11

List of Publications

All the following papers are provided as appendices.

I. Shanmugam, K., Tysklind, M. and Upadhyayula. V.K.K. (2018) Use of

Liquefied Biomethane (LBM) as a Vehicle Fuel for Road Freight

Transportation: A Case Study Evaluating Environmental Performance of

Using LBM for Operation of Tractor Trailers. Life Cycle Engineering

Procedia CIRP 69 ,517 – 522

II. Shanmugam, K., Baroth, A., Nande, S., Yacout, D.M.M., Tysklind, M. and

Upadhyayula, V.K.K. (2019) Social Cost Benefit Analysis of Operating

Compressed Biomethane (CBM) Transit Buses in Cities of Developing

Nations: A Case Study. MDPI Sustainability August 2019,11,4190

III. Shanmugam, K., Gadhamshetty, V., Yadav, P., Athanassiadis, D.,

Tysklind, M. and Upadhyayula, V.K.K. (2019) Advanced high strength

steel and carbon fiber reinforced polymer composite body in white for

passenger cars: Environmental performance and sustainable return on

investment under different propulsion modes. ACS Sustainable

Chemistry and Engineering January 2019, 7, 4951-4963

IV. Shanmugam, K., Jansson, S., Gadhamshetty, V., Matsakas, L., Rova, U.,

Tysklind, M., Christakopoulos, P. and Upadhyayula, V.K.K. (2019)

Ecoefficiency of Thermal Insulation Sandwich Panels Based on Fly Ash

modified With Colloidal Mesoporous Silica. ACS Sustainable Chemistry

& Engineering November 2019, 7, 20000-20012

V. Shanmugam, K., Gadhamshetty, V., Tysklind, M., and Upadhyayula,

V.K.K. (2021) Total Cost Assessment Framework for Sustainable and

Circular Management of Activated Sludge Based Centralized Wastewater

Treatment Plants. Submitted Manuscript.

Page 15: Circularity Assessment of Water and Waste in Cities

12

Authors Contributions

Paper I

The author was involved in planning the scope of the study, modeling parameters,

processing data and writing the manuscript.

Paper II

The author was involved in planning the goal and scope of the study, modeling,

collecting data and writing the manuscript.

Paper III

The author was involved in designing the scope of the study, modeling the scope,

reporting results and drafting the manuscript.

Paper IV

The author was involved in partly planning the scope of the study, designing the

scope, data processing, modeling and reporting the results.

Paper V

The author was involved in planning the scope, calculation of design parameters,

modeling the study and co-writing the manuscript.

Page 16: Circularity Assessment of Water and Waste in Cities

13

1. Introduction

In the 21st century, urbanization is one of the five signature megatrends that will

permanently change the definition of human sustenance (approach to

sustainability) on this planet [1]. The concept of urbanization can be described as

the migration of people to urban settlements i.e. cities, in anticipation of better

opportunities for employment, and thereby enjoyment of the benefits of

improved living standards [2]. Historically, urbanization has been associated

with significant economic and social transformations (urban living is linked to

higher levels of literacy and education, better health, longer life expectancy) [3].

While this contribution to socio-economic development is true, an accelerated

urbanization also brings a multitude of challenges that a nation must deal with in

order to avoid any dire sustainability consequences [2]. The world population is

projected to reach 9.7 billion by 2050 and, by then, around 68% of the people will

reside in urban areas [4]. Urbanization occurring at such unprecedented rates

presents numerous sustainability challenges to policy makers and governing

authorities. In particular, it exerts tremendous pressure on cities and towns [4,

5]. Cities are responsible for provision of three essential municipal services to the

residents: (a) supply of water for potable and non-potable needs, (b) treatment of

wastewater, and (c) management of solid waste (including organic waste)

generated by the inhabitants [6]. Ensuring sustainability of these essential

services becomes increasingly difficult for city authorities with increases in the

inflow of population. Figure 1 shows the various environmental implications

resulting from rapid urbanization [7] [8] [9].

Figure 1. A simplified illustration of various environmental implications

resulting from rapid urbanization

Due to rapid urbanization, many cities around the world are experiencing

difficulties due to inefficiencies (lack of financial resources, proper organization,

Page 17: Circularity Assessment of Water and Waste in Cities

14

complexity and system multi-dimensionality) associated with the management of

essential services [8]. For instance, some cities are resource constrained in

relation to the supply of drinking water. Recently (in 2018), the city of Cape Town

in South Africa ran out of water (high per capita water consumption) [10]. Ten

other major cities, including London and Tokyo, are predicted to follow the same

path and will be facing severe drinking water shortages by 2040 [10]. For other

cities, especially in developing countries, lack of adequate treatment of

wastewater is one of the major causes of public health concern [11]. It is estimated

that, globally, 80% of wastewater resulting from human activities is discharged

into fresh and marine water bodies without undergoing any treatment for

removal of chemical and biological pollutants [11]. Discharge of untreated or

partially treated municipal wastewater into natural waters exacerbates

eutrophication and ecotoxicity impacts [9], and endangers numerous aquatic

species [12]. Also, given the shortage of freshwater, reuse of wastewater for

agricultural purposes is practiced in some regions [4] [13]. However, reusing

untreated and partially treated wastewater for irrigation has been shown to have

a direct link with food-borne disease outbreaks [4] [13]. Even the use of treated

wastewater from crop cultivation can have public health repercussions that may

vary from season to season [13] [14]. Lastly, management of municipal solid

waste (MSW) has also emerged as a serious issue. The global production of MSW

is expected to reach 3.4 billion tonnes by 2025 [15] and its disposal without

causing social externalities will be an uphill task for cities worldwide [14]. The

problem is more pronounced for many cities in developing nations, where MSW

is predominantly landfilled [1] [8].

In this thesis, Sweden is used as an exemplar country (data for modeling comes

from a Swedish city) and the findings can be applied to countries with similar

practices. Sweden is not an exception for urbanization challenges, but Swedish

cities are different from many other parts of the world for two reasons. First,

Sweden was mentioned in the World Wide Fund for Nature Living Planet Report

(2016) for its high import-oriented resource (material and food) consumption

pattern, which means transferring environmental impacts elsewhere in the world

[16] [17] [18]. Second, a large proportion of the population (87% as of 2018) in

Sweden already resides in urban areas. Over recent decades, there has been a shift

of largest population increase in the large urban areas [19]. However, all major

Swedish cities have efficient essential municipal service operations in place. They

fulfill at least one of the three major criteria for circular compliance in waste

management: (a) byproduct utilization, (b) minimization of residual waste to

landfill, and (c) prevention of the leakage of nutrients and emerging

contaminants (e.g. pharmaceutical residues) into the biosphere [20]. Over the

years, municipalities in Sweden have mastered the ability to recover byproducts

with energy value (e.g. biogas from wastewater treatment plants (WWTPs) and

organic waste bio-digestion plants, and energy from MSW incineration plants)

Page 18: Circularity Assessment of Water and Waste in Cities

15

and put them to beneficial use in the society. [21] In addition, some Swedish cities

have already begun to treat their emerging contaminants from wastewater while

others are expected to acquire this ability shortly [22]. Also, rigorous efforts are

underway to ban the landfilling of residual waste streams and increase their use

in the technosphere. EU legislation and waste hierarchy have played a key role in

improving the sustainable performance of the municipal services in Sweden [23].

However, the problem for Swedish city municipalities still lies with the disposal

of residual waste streams (sludge and ashes) and removal of emerging

contaminants from wastewater [24].

From the above perspective, it would be of great scientific and societal value to

develop a methodology that combines the urban metabolic rates of cities with

their current and future initiatives, with the aim of achieving circular compliance

of their essential municipal service operations. The urban metabolism (UM) is a

model that facilitates the description and analysis of energy and material flow

within cities. UM involves the study of the interaction of natural and human

systems in specific regions [25]. There are several urban metabolism models

described in literature [25–29]. They are designed to measure the resources

flowing within, and waste streams flowing out of, a city, understand how different

forces (e.g. social and cultural aspects) influence a city’s metabolic rate, and can

be well integrated with urban planning efforts towards building sustainable cities

[30]. However, assessment models also exist that quantify sustainability aspects

of municipal service operations and develop indicators reflecting their

performance [16, 27, 31–33]. A combined effort to assess the sustainable

implications of the urban metabolic rate and circularity of essential treatment

services in cities is yet to be undertaken.

In this thesis, the recess is addressed by proposing an assessment methodology

designed to understand the sustainable implications of cities, by taking their

urban metabolic rates and performance of essential municipal services into

consideration. The integrated model proposed in this thesis is potentially more

helpful for cities to deduce strategies and make decisions related to sustainable

urbanization (focusing on water-waste-energy). Papers I–IV of this thesis served

as a basis for evolving such a conceptual framework. The work in these papers

was formulated to evaluate the sustainable performance of municipal treatment

services (wastewater and solid waste) to comply with circularity at the treatment

plant level. These papers showed the way to identify the different stages of the

proposed framework. Paper V describes the evaluation of the stages of the

framework applied to the wastewater treatment service. A structured five-stage

framework for evaluation of sustainable operation of essential municipal services

of a city using the supporting logic i.e. an assessment based on application of life

cycle assessment (LCA) [34] and life cycle costing (LCC) tools, is presented in this

Page 19: Circularity Assessment of Water and Waste in Cities

16

thesis. Other environmental assessment tools, such as Environment Impact

Assessment (EIA), Ecological Risk Assessment (ERA) and Material Flow Analysis

(MFA), along with those based on economic metrics such as Cost Benefit Analysis

(CBA), can also be used for such an evaluation [35]. These tools can be used

depending on the objectives to be fulfilled, and address other aspects of

sustainability. For the purpose of this thesis, LCA is used as it quantifies the

environmental effects and implications of essential services at various levels of

adherence to circular economy compliance [34]. Second, it quantifies the

environmental performance contribution made by the essential service systems

in improving sustainability of cities.

The data used for modeling in this thesis were obtained from Umeå city

stakeholder companies (Papers I, II and IV). The assessment of the essential

services (wastewater and solid waste) carried out for the papers/modeling

approach can be applied to cities with a similar population (approx. 130,000

inhabitants as of 2020, similar to most European medium-sized cities [36]) and

technology practices. The population of the city is predicted to reach 200,000 (an

increase of 60,000 houses by 2050 in order to meet the growing population) by

2050, meaning there is a greater demand for housing, transport and other

services likely to produce more waste [36]. Transition in cities (to sustainable

technologies to meet the requirements of the population) of the above nature can

be handled by our unique modeling approach, where combining urban

metabolism and circular economy concepts, while measuring the sustainable

performance of a city or an urban community, is essential.

The framework can serve as a basis for development of a decision support system

that cities can apply to evaluate iteratively and improve their sustainability

performance. Finally, the framework allows for the establishment of grounds for

comparison between cities, based on how environmentally - friendly the essential

services are run in each city and the extent to which they contribute to the

sustainable performance of that city. The structure of the five-stage LCA

framework is clearly explained in subsequent chapters of the thesis.

Page 20: Circularity Assessment of Water and Waste in Cities

17

2. Objective of this Thesis

The goal of this thesis is to describe a systems-oriented modeling framework for

comprehensively evaluating the sustainable performance of essential services

(wastewater and solid waste) in cities. The modeling framework is designed to

consider collectively the concepts of urban metabolism and circular economy

while evaluating the sustainable performance of the city. A city (municipality,

society) must provide essential municipal services to its residents, including the

crucial services treatment of wastewater, and municipal solid waste management

(MSW) (e.g. disposal in landfills and prevention of leakage of toxic contaminants

into the biosphere). Umeå city (data and treatment techniques for modeling) was

used as a test case to develop the framework, with real-time data (obtained from

Umeå Energi, Vakin) being used in the modeling approach of the papers in order

to reduce data uncertainty and make better decisions. Papers I–V, appended to

this thesis, form part of this objective of evaluating the environmental

performance of the essential services in the city using sustainable assessment

tools such as LCA and LCC. Figure 2 shows how these papers describe the

different stages of the proposed framework.

Figure 2. The stages of the assessment framework with the current and future

scenarios of essential treatment services, as described in Papers I–V

Page 21: Circularity Assessment of Water and Waste in Cities

18

The following objectives are discussed in this thesis:

1. Gather and outline the wastewater and household waste treatment

technologies in the city. Assess the environmental performance of the current

treatment processes using LCA. (Papers I, II, IV and V)

2. Collect site-specific information on treatment processes, byproduct

utilization, residual stream disposal and advanced treatment techniques

planned for a future sustainable scenario. Evaluate the environmental

performance of the future scenario. (Papers I–V)

3. Amalgamate the different LCA studies, allowing for the development of an

assessment framework, which can analyze the overall environmental

performance of essential municipal services in cities and its contribution to

the utility needs of the city, along with the urban metabolic rate of the city.

4. Based on the results obtained from these three objectives, calculate the total

cost for essential services and urban metabolic rate of cities (part of Paper V).

Page 22: Circularity Assessment of Water and Waste in Cities

19

3. Urban System

This chapter describes the major essential municipal services considered in the

thesis. The wastewater treatment service and the municipal solid waste

(household waste, recyclables, organic food waste) service are both included.

In this thesis, a city [37] is considered to be an urban system and is viewed as a

combination of five elements. Figure 3 shows these elements.

Figure 3. Five elements that determine the sustainable performance of an urban

system, with systemic features focusing on infrastructure, material flows,

cultural dimensions, essential ecosystem services and utilities

3.1 Elements of an Urban System

The elements of an urban system are described as follows [38]:

Physical Element: Denotes physical infrastructure e.g. individual houses,

apartment buildings, industrial buildings, offices, commercial complexes etc.

Human Element: The actual people (residents, employees etc.) of an urban

system.

Services Element: Represents three essential municipal services i.e. water

supply, wastewater treatment and management of MSW. A city might be

Page 23: Circularity Assessment of Water and Waste in Cities

20

comprised of other essential (e.g. fire station, healthcare) services. However,

these and other services are not in the scope of the present work.

Utility Element: Two critical utilities i.e. energy (electricity and heat) and

public transportation. The city municipalities are either direct service

providers of these utilities or contract them to third party companies.

Materials Element: This includes a wide range of materials, either those

directly consumed by the city residents or those that the city is indirectly

responsible for the production and utilization of elsewhere. Direct material

consumption includes products such as cosmetics, pharmaceuticals, metals,

plastics wood etc., which can have a profound influence on the operational

efficiency of the services element. Indirect consumption refers to materials

such as fertilizers and pesticides used for local food production (i.e. food

produced and consumed in cities in the same country) and exported from

elsewhere (i.e. food produced in one country and consumed in another

country).

All five elements collectively determine the sustainable performance of an urban

system. The sustainability performance of the physical element is related to

physical infrastructure i.e. materials used in construction and land use, and

affected by several other criteria such as energy and water efficiency etc., as

stipulated by green building standards for individual buildings [39]. The

sustainable performance of the human element depends on a wide range of

factors such as socio-economic conditions, ethnographic influences, awareness of

people and their sense of responsibility towards sustainability challenges faced

by urban systems. The services, utility and material elements collectively

determine the operational sustainability performance of urban systems (urban

metabolic rate). Furthermore, essential municipal services, depending on how

they are managed, can positively influence the sustainable performance of the

material and utility elements. Therefore, a comprehensive understanding and

application of a systems approach is critical in managing the services element.

3.2 Essential Municipal Services

The major essential municipal services investigated in this thesis are the

treatment of wastewater and the management of solid waste (including organic

waste) generated by the residents. The treatment practices discussed are the most

commonly used practices by Swedish municipalities. The treatment services in

Sweden are managed by waste companies (stakeholder companies) that are

responsible, or have been hired by the municipality, for these services and have

signed contracts to supply treatment and management services [23]. Figure 4

shows the wastewater/waste/recyclables treatment service in Umeå (Umeå data

were used for modeling purposes) [40]. Umeå is situated in northern Sweden and

has a population of 130,000 inhabitants (similar to most European medium-sized

Page 24: Circularity Assessment of Water and Waste in Cities

21

cities) as of 2020. It is well connected to municipal services [36] [41]. Umeå is

one of the fastest growing European cities and is the center of growth in northern

Sweden, which has a great effect on the use of natural resources and its

infrastructure [36]. In Sweden, a symbiotic city network (a mutually beneficial

arrangement between cities to ensure environmental sustainability) between

municipalities exists to ensure the sustainable treatment of waste. Here, for

example, waste from different municipalities is transported between cities

depending on where the treatment plant is located [40]. These treatment steps

can vary for cities in Sweden; only the most common treatment practices (as used

in Umeå in this case) are considered in this thesis.

Figure 4. A simplified illustration of wastewater, organic waste, residual

combustible waste and recyclables waste treatment services in Umeå [40]

3.2.1 Wastewater Treatment Service

Umeå’s WWTP is designed for 166,000 inhabitants (included industrial loads)

and can purify a maximum 8100 cubic meters of wastewater per hour [42].

Depending on its physical area, population, and sewer network connectivity, a

city will require one or more centralized WWTPs. According to Statistics Sweden

(2018), more than 8.5 million people in Sweden (total population 9.7 million) had

access to municipal wastewater treatment in 2015 [43]. Figure 5 shows the

schematic view of Umeå’s WWTP. The wastewater in Umeå is treated aerobically

Page 25: Circularity Assessment of Water and Waste in Cities

22

(i.e. using a biologically activated sludge process) in combination with anaerobic

digestion of sewage sludge generated during the treatment as an additional

optional step. The effluent treatment train involves a primary step, meant for grit

removal and suspended solids separation in a primary clarifier using FeCl3

coagulant, and a secondary step involving an activated sludge process. This

process microbiologically metabolizes organic compounds present in the primary

treated wastewater under aerobic conditions, followed by settling of the

biologically active sludge in the secondary clarifier.

Figure 5. Workflow of the wastewater treatment process in Umeå including the

effluent treatment, sludge management and byproduct processing

The sludge from the secondary clarification unit is recycled to the aeration tank

to maintain a desired concentration of mixed liquor suspended solids (MLSS),

with excess sludge removed periodically through the sludge drain line. This

clarified effluent is sent for further treatment where phosphorus is removed

through precipitation by addition of FeCl3. Finally, this wastewater effluent is

pumped to the receiving body (in this case, the Ume river) [43–45].

In the sludge streams (raw sludge from the primary clarifier, excess secondary

sludge, and polymer thickened tertiary sludge), the sludge is anaerobically

digested, thereby generating biogas and dried digestate as byproducts. Biogas

(containing 50–70% CH4, 30–40% CO2 and other trace elements) is used to

produce heat and electricity, with a certain amount being flared. The heat

produced is used within the plant and seasonal excess heat is sold to the

municipality. Paper I describes an investigation into diverting the biogas from

WWTP and treating it so that it can be used as a Liquefied Biomethane (LBM)

Page 26: Circularity Assessment of Water and Waste in Cities

23

fuel to operate heavy-duty trucks. The environmental performance of the

consequential use of biogas as a fuel was assessed in this paper.

The dried sewage sludge is used as a soil conditioner for agricultural use (it was

converted into pellets but this was stopped due to lack of demand), but only when

the concentration of heavy metals and emerging contaminants is lower than the

criteria established by regulations. It is also used for capping of landfills and the

remaining sludge is disposed of in landfill [44]. The current ban on landfilling

sludge in Sweden has triggered incineration of the sewage sludge [24].

Incineration of sludge results in the destruction of harmful substances such as

pharmaceutical residues, multi-resistant bacteria, micro plastics and harmful

organic substances. The possibility of eliminating the undesired substances found

in sewage sludge that have detrimental effects on the ecosystem, along with the

potential for recovery of phosphorus, makes incineration one possible circular

option [24]. In Paper V, a scenario analysis described, which evaluated the

environmental performance of WWTP where the sewage sludge had been

incinerated for energy recovery.

3.2.2 Municipal Solid Waste (MSW) Treatment Service

MSW management in Swedish cities involves actors having a clear division of

responsibilities. Municipalities are obliged to have a waste management plan and

bear the responsibility of collecting and disposing of household waste, except for

the product categories covered by the so-called producer responsibility [46].

Waste minimization is the top priority according to the EU Waste Framework

Directive (2008/98/EC)[47]. Households in Sweden generated an average of

466kg/ year / person as of 2018. According to Avfall Sverige report in 2018, the

quantity of Swedish household waste treated was 4,583,000 tonnes. The

proportion of household waste taken for biological treatment was 15.5%, while

50% was used for waste-to-energy recovery and 33.8% was recycled (0.5%

landfilled) [48].

Combustible domestic waste and food waste are collected using a curbside

system, with a “green bin” for combustible waste and a “brown bin” for organic

food waste (see Figure 4). Packaging materials, such as glass, paper/cardboard,

plastic, metal packages and newspapers, are collected in recycling stations

around the municipality. In addition to the recycling stations, a majority of the

apartment buildings have recycling rooms where tenants can sort their packaging

waste into separate bins. Bulky waste, waste for reuse and garden waste are

collected at recycling centers normally run by the municipalities [40, 48].

Page 27: Circularity Assessment of Water and Waste in Cities

24

(a) Organic Food Waste Treatment

Organic food waste (OFW) in Umeå is transported to the Skellefteå biogas plant.

Figure 6 illustrates the workflow of an OFW treatment plant in Skellefteå. The

plant receives organic waste from households and local slaughterhouse waste

daily. The waste first undergoes a pre-treatment process (a sand trap to remove

unwanted materials). The mass is diluted with water (36–40ºC), with the larger

particles bigger than 6mm being removed, dewatered and sent to the incineration

plant. The remaining organic matter and the blood and slaughter waste are sent

directly to the grinding unit to provide an optimal digestion process [48, 49].

Figure 6. Organic food waste treatment process at the Skellefteå biogas plant

with anaerobic digestion of waste to produce biogas, which is converted to CBM

for use as fuel in buses, and sludge for use as soil conditioner

The organic slurry is sanitized (at 70ºC to kill pathogenic bacteria and then cooled

to 55ºC in a heat exchanger) before being pumped into the digestion chamber.

Anaerobic digestion can be achieved over different temperature ranges including

mesophilic digestion at temperatures of 35–40ºC and thermophilic digestion at

temperatures between 50–60ºC (which is faster and produces more gas). The

residence time in the digester is about 18 to 20 days and produces biogas.

Specifically in certain cities like Skellefteå, the biogas is then sent to an

upgradation unit (for removal of CO2, H2S from biogas, either to meet the vehicle

fuel standard or to meet the required natural gas quality for use in the natural gas

grid) [50]. The upgradation unit consists of a water scrubber, carbon molecular

sieves, and selexol scrubbing to obtain Biomethane (99% CH4) which is then sent

to a storage tank. This is known as Compressed Bio Methane (CBM) when used

in vehicles [50] [51]. In Skellefteå, pipelines were recently built to transport the

gas to the town center. The buses (short distance and selected long distance) in

the city and municipal passenger cars run on CBM. The sludge obtained from the

digestion process is dewatered and thickened (by adding cationic polyacrylamide

Page 28: Circularity Assessment of Water and Waste in Cities

25

polymer), then used as soil conditioner on grasslands and forestry. Paper II

describes a study of the transfer of technology for treating organic food waste

from developed nations to developing nations, where a significant amount of food

waste is routinely open dumped. The societal cost benefits of using CBM as a fuel

for buses and cars in Mumbai, India was evaluated in this paper.

(b) Waste-to-Energy Plants

The fraction of combustible domestic waste not extracted for recycling at source

or separated out in Sweden is used in Waste-to-Energy (WtE) plants for energy

generation [52]. The thermal process converts waste to generate fly ash, bottom

ash, emissions to the air, and process water. Of the total waste stated above that

goes into the MSW treatment service, almost 50% of household waste in Sweden

is used for energy generation [36]. Incineration is a waste treatment process that

involves the combustion of organic substances contained in waste materials, and

is one of the most robust ways to replace fossil fuels and reduce CO2 emissions.

The emissions from these plants are treated (flue gas treatment) to meet the

stringent regulations, and hence provide improved air quality in many cities [53].

A typical waste incineration facility includes the following operations [54]:

Waste storage and feed preparation

Combustion in a furnace, producing hot gases and a bottom ash residue

for disposal

Gas temperature reduction, frequently involving heat recovery using

steam generation

Treatment of the flue gas (cleaning using filters, scrubbers, sieves) to

remove air pollutants, and disposal of fly ash obtained from this

treatment process

Dispersion of the treated gas to the atmosphere using draft fans or stacks

Depending on the capacity and type of waste, there are different types of

incinerator technologies used e.g. Rotary kiln Incineration, Grate incineration

and Liquid, Gases and fumes incineration [54].

Figure 7 shows the workflow of a WtE plant such as the one in Umeå. The

incineration process (fluid bed boiler) is fed with oxygen (O2) so that the waste

has enough caloric value to burn without support fuel; fuel oil is only used to start

the combustion process. The working temperature in the boiler is approximately

950ºC and the residence time of the waste in the furnace varies from 45 to 90

minutes. After the combustion step, there remains heavier bottom ash,

accounting for around 10% of the original volume of waste (97000 tonnes of

household waste in 2018), and high temperature flue gases.

Page 29: Circularity Assessment of Water and Waste in Cities

26

Figure 7. Workflow of a WtE Plant in Umeå with fluid bed boiler that produces

heat and electricity for households, flue gas purified to 99.7% and ash used in

the construction industry (Umeå Energi)

The bottom ash is cooled and particles bigger than 40mm are separated (sieving).

An electromagnet is used to separate the metals from the ashes; the ash is stored

in an ash bunker. The semiconductors and some toxic substances (e.g. As, Cd, Cr

and Zn) are separated from the ashes. After this treatment, the bottom ash

contains fewer toxic compounds and can be used in construction materials. The

main part of the WtE plant cleans the flue gas before releasing it into the

atmosphere. The European directives for emissions specify important

restrictions on using an incinerator plant [52]. The residue from the flue gas

treatment (fabric filters, an acid scrubber, and an SO2 scrubber are all used to

purify the gases to 99.7%) is fly ash which contains hazardous substances such as

dioxins, furans, chlorine, bromine etc. The fly ash is transported to landfills

specializing in hazardous waste storage. Energy recovery from these plants can

produce heat in combination with electricity used in households (district heating

network) [52] [55]. Paper IV describes an evaluation of the environmental

performance of using fly ash from WtE plants (currently landfilled) as a filler

(after immobilizing the heavy metal content in the fly ash) in epoxy composite

panels with a PU foam core for use in the building industry. The ecoefficiency of

silanized fly ash epoxy composite sandwich panels compared to the steel-skinned

incumbent market sandwich panels was calculated in that work.

(c) Recyclables

According to the EU waste hierarchy, recycling is the most preferred option after

prevention (non-waste) and preparation for reuse [56]. In Sweden, the

Page 30: Circularity Assessment of Water and Waste in Cities

27

recyclables sorted from households are transported to recycling stations/centers

at different locations within cities. In addition, there are several unmanned

container-based sorting options that are covered by Producer Responsibility

Obligations Regulations for packaging, newspapers, tires, and cars along with

electrical and electronic products, whose producers are responsible for dealing

with end-of-life processing [21, 40].

The common items collected from recycling stations/waste rooms in Umeå as of

2019 (Avfall-Web) are glass packaging (3156 tonnes), cardboard (443 tonnes),

metals (1643 tonnes), plastic packaging (1276 tones), paper (4055 tonnes), paper

packaging (2960 tonnes) textiles (117 tonnes), wood (3764 tonnes), lightbulbs,

batteries (portable-22 tonnes, car batteries-84 tonnes), and electronic waste

(1604 tonnes). The data above are expressed in tonnes/year (2019). The possible

amount of recyclables collected was 27% in the year 2018. The remaining fraction

that cannot be reused or recycled were transported to WtE plants[36].

3.3 Management of Essential Municipal Services in Cities

Complying with Circular Economy Principles

In general, managing essential municipal services in an urban system has

undergone a major transformational change over recent years [4, 12]. Over the

last few years in Sweden, essential services in a city only needed to undertake

basic functions. This meant that the wastewater and MSW were treated and

managed to reduce health and ecological threats otherwise posed by these

streams when untreated or mismanaged. The influent wastewater from the city

was treated in centralized WWTP using secondary methods such as an activated

(aerobic) sludge process. Further, the residual waste, such as undigested sewage

sludge from WWTPs, was disposed of in landfills [45, 57]. MSW from cities was

collected and treated in a waste-to-energy plant (with the ashes disposed of in

landfills), organic material was composted or anaerobically digested, with the rest

sent to landfill [57, 58, 59]. These were considered to be common practices by

cities [60].

At present, cities are expected to fulfil their functional requirements and to

achieve a greater degree of conformity to circular economy compliance (EU

legislation) [61–63]. Figure 8 shows the energy, material and resource values

potentially recoverable and extractable that are generated by essential municipal

services management [36]. To meet these criteria, essential municipal services

have to satisfy two requirements. First, leakage of hazardous contaminants (e.g.

release of heavy metals from waste incineration fly ash into landfill or

micropollutants entering natural water streams from wastewater treatment

discharge) into the biosphere must be prevented. Second, operation of essential

municipal services will generate byproducts and residual waste streams. These

Page 31: Circularity Assessment of Water and Waste in Cities

28

residual streams must be further processed, if needed, and their economic value

must be extracted and put to beneficial use within the technosphere [36, 64].

Figure 8. Essential municipal services management that complies with

circularity in order to produce energy value, material value, and fuel value in

cities

Generally, cities having a WtE plant incinerate the refuse fraction of MSW and

generate high-pressure steam and electricity. The cities in cold climate regions,

such as Umeå, use a large proportion of the steam to meet the heating and hot

water needs of buildings, converting a relatively smaller proportion into

electricity [54]. Cities with smaller district heating demands prefer to operate

their WtE plants maximized for electricity production. The electricity generated

by a WtE plant can also be used to support electric transportation in a city

(electric cars, city buses etc.) [65].

Biogas can be generated from three sources within municipal service operations:

(a) the WWTPs that have the infrastructure and capability to anaerobically digest

their sewage sludge, (b) cities treating their organic fraction of MSW in anaerobic

digestion facilities, and/or (c) cities landfilling MSW-generated organic material

and equipped with a biogas collection system [66]. Biogas sourced from these

sites can be used either to produce heat and electricity, or converted to

biomethane and used as a fuel for public and private transportation vehicles in a

city [50, 51]. Papers I and II describe an investigation and assessment of the

Page 32: Circularity Assessment of Water and Waste in Cities

29

environmental impacts of diverting the biogas from wastewater and organic food

waste treatment for use as fuel in heavy-duty trucks, buses and cars. The societal

benefits of using such renewable fuel compared to a baseline using diesel or

gasoline are expressed in terms of cost equations.

The output in terms of material value resulting from a city’s essential municipal

service operations can include secondary materials and materials obtained from

the residual waste streams [67] [68]. The secondary materials, such as metals,

plastic, wood, glass etc., are produced from a city’s MSW recyclable waste fraction

by using reuse, recycling and recovery techniques in that order of hierarchy [21].

The principal reason why a city separates and processes its MSW recyclable

fraction is to increase the circularity of existing materials and minimize the

dependency on natural sources to provide virgin materials. Residual waste

streams can potentially be a cheaper raw material source for generation of value-

added materials.

Nutrients, such as phosphorus, can be extracted from digested sewage sludge

generated by WWTPs [24]. Alternatively, it can be used to produce biochar, which

serves as a cheaper raw material in a variety of industrial applications [68]. The

digestate from MSW organic digestion facilities has significant nutrient value and

can be directly applied as a conditioner to agricultural land [49]. In addition,

some cities treat their food waste in composting facilities and the compost thus

generated is used as an organic fertilizer [23]. Multiple industrial pathways have

been established for recycling and upcycling the bottom and fly ash from a WtE

plant (discussed in detail in Paper IV) [69]. Paper IV describes the upcycling of

fly ash (using silanization to immobilize the heavy metals) as a filler in composite

panels, and stated the ecoefficiency of the silanized fly ash composite panel.

Finally, tertiary treated wastewater is a resource value that can be assigned to

WWTPs. This may not be of concern to cities where freshwater (surface or

ground) is available in abundance. However, for cities facing extreme water

stress, tertiary treated wastewater is of great value and reduces freshwater

withdrawal rates [13]. In 2018, the summer was very dry in Sweden, causing a

drought in some regions. Wastewater reuse, unlike in other water stress regions,

is not common in Sweden and there is no legislation specifically regulating this

[67, 70]. Thus, environmental regulations and policies play a significant role in

implementing a circular economy. Paper V describes a review of the overall

circular performance of WWTP. The total cost (environmental cost and operating

cost) related to achieve the circularity of such plants operating in cities was also

determined.

Page 33: Circularity Assessment of Water and Waste in Cities

30

Thus, achieving circular compliance with respect to operation of essential

municipal services is important, owing to its valuable contribution in improving

the services’ overall environmental performance [67].

Page 34: Circularity Assessment of Water and Waste in Cities

31

4. Tool & Methodology

4.1 Life Cycle Assessment

Life Cycle Assessment (LCA) is a methodology used to evaluate the environmental

impacts associated with a product or service from cradle to grave. LCA studies

can explore large industrial systems by collecting and analyzing large amounts of

environmental information [71]. In order to know which action is the most

environmentally preferable and avoid the causes of major emissions (hotspots)

in a product/service, a structured assessment tool is needed. One such tool used

in the thesis is LCA. The LCA procedure has four steps according to ISO 14040

and 14044 [71], as shown in Figure 9.

Figure 9. Steps for carrying out an LCA as described in ISO (14040) [72, 73] and

followed in all the papers appended to the thesis

First, the product studied is described and the purpose of the LCA is specified by

the goal and scope definition, including system boundaries and functional unit.

The LCI step involves the construction of the life cycle model and a calculation of

the emissions produced and resources used during the life cycle of the

product/process. The emissions and resources are related to various

environmental problems through classification and characterization weighting.

These are calculated in the LCIA step. Finally, the results are interpreted to the

Page 35: Circularity Assessment of Water and Waste in Cities

32

target group and can be used for direct applications in product development and

improvement, strategic planning, public policy making etc. [72].

Many research groups have set up their own software to handle environmental

impacts, using packages such as Microsoft Excel. In addition, there are a number

of LCA software packages commercially available [71]. The software has been

developed for any type of LCA and some are designed for particular LCA

applications or specific industry sectors (all comply with ISO 14040 standards).

This classification is based on the computational capacity of the tool and the

extent to which quality of data used in calculations can be reviewed [74]. Some

commonly used LCA software includes GABI, Simapro, OpenLCA, and Umberto

[74]. Data collection is also time-consuming when carrying out LCA calculations,

especially for complex activities. The foreground data are specified by the

supplier/industry; the background data are obtained from a set of representatives

who build local, national and international databases in coordinated efforts from

several countries [75, 76]. In addition, industries have taken initiatives to set up

public LCA databases as a way of maintaining control over the data used in LCA

studies. The databases are maintained and combined by public authorities,

(national and international levels), industry sector organizations, consultants and

research institutes [71].

The LCA studies carried out in this thesis were modeled using the Simapro PhD

8.2.0 software - Pre 2017. SimaPro is a professional tool for collecting, analyzing

and monitoring the sustainability performance data of products and services. It

enables a student or a researcher to examine an entire life cycle thoroughly with

a set of powerful and unique features [77]. The ecoinvent database (v. 3.2) was

used for background LCI datasets [78]. It provides well-documented process data

for thousands of products and is the best source in terms of transparency and

consistency [78]. The foreground data for modelling (Papers I–V) were obtained

from industry, literature and treatment plants (Umeå Energi, Dåva DAC, Vakin,

Skellefteå biogas plant). Data obtained from supplier or site-specific data were

preferred for LCAs (reduced uncertainty, data regionalized) over predicted or

generic datasets [79]. Real-time data from sites can provide environmental

information for better process understanding and improved decision-making. It

can assist stakeholders in making more effective and efficient decisions (timely

and more accurate).

There are three types of LCA [71]:

Attributional LCA: inputs and outputs are attributed to the functional

unit of a product system. They are used for comparison of existing

products.

Page 36: Circularity Assessment of Water and Waste in Cities

33

Consequential LCA: product system are linked in modelling such that

activities are included that are expected to change as a result of differing

demand for the functional unit. They are used in comparison, product

development, building design and process choice decisions, such as waste

management options or recycling schemes. The work described in Papers

I–V uses consequential modeling approach.

Standalone LCA: describes a single product and some important

environmental characteristics (identify hotspots) of that product.

4.1.1 Goal & Scope Definition

The initial goal and scope definition in an LCA establishes the purpose of the

assessment and determines decisions made about the details of the product

system being studied before any data are collected. The transformation of the

general goal to a more specific purpose to make relevant methodological choices

in modeling is necessary [72]. The goal and scope definition needs to answer the

following questions [80]:

What is the main application and who are the target groups of the study?

What would the environmental consequences of changing a certain process

be?

What kind of data and quality of input data are required and which

assumptions need to be made based on the level of detail in the study?

What type of environmental impacts are being considered (a default list of

impacts is considered in most LCAs), and what are the limitations based on

the study?

This is a very important phase of LCA methodology because this is where the

exact approach to be followed is determined. The goal and scope definition

phase includes determining the functional unit, system boundaries, data

reflecting process-specificity or genericness (i.e. foreground or background)

data.*

Functional Unit & System Boundary

The functional unit (FU) and system boundary are specified in the goal scope

definition. LCA relates environmental impacts to a product, specifically to the

functional unit of the product system. Thus, there is a need to express the FU in

quantitative terms such as passenger transportation in person kms, or amount of

waste incinerated per year. The FU corresponds to a reference flow to which all

other modeled flows of the system are related. Products or processes often fulfill

more than one function, therefore, depending on the goal of the study, one of the

functions must be chosen that is related to one reference flow. The amount of

product needed to fulfill the FU is the reference flow [71].

Page 37: Circularity Assessment of Water and Waste in Cities

34

The system boundary describes (flow model) which process to include, based on

the choices made in the goal and scope definition. According to Tillman et al.

(1994) [81], system boundaries need to specified in several dimensions:

Geographical boundaries i.e. electricity production, waste management,

transport from one region to another

Boundaries related to natural systems i.e. where is a product’s cradle

(beginning) and grave (end)

Time boundaries i.e. number of years considered in the study

Boundaries within the technical system i.e. capital goods, personnel,

allocation to be included in the product/process studied.

Figure 10 shows examples of the different system boundaries which can be

considered in an LCA.

Figure 10. System boundary examples considered in an LCA, shown as a

conceptual line that divides the system being studied from 'everything else' that

is not a part of the system

The most commonly used system boundaries are [82]:

Cradle to Grave LCAs are the most comprehensive and commonly used

to compare products and generate Environmental Product Declarations

(EPD) etc.

Cradle to Gate LCAs are used when product functionality remains the

same but the changes occur in raw materials and manufacturing.

Gate to Gate LCAs are carried out when a specific stage of the product

changes.

Page 38: Circularity Assessment of Water and Waste in Cities

35

For example, for Paper II, a cradle to grave LCA was carried out to investigate the

possible benefits of using CBM as a fuel to operate buses in Mumbai, India. The

food waste from the city is transported to a biogas plant where it is processed by

anaerobic digestion (AD). Compressed biomethane (CBM) is obtained by

converting (water scrubbing) the biogas produced as a byproduct and is then used

to fuel buses within the city. In this case, the functional unit chosen was the total

distance driven in bus-kilometers (bus-km) in a year by buses operating on CBM

fuel produced from a biomethane-producing plant treating food waste generated

by Mumbai residents. The environmental performance results were compared to

an equivalent distance driven in a baseline scenario using a diesel and

compressed natural gas (CNG) bus.

4.1.2 Life Cycle Inventory (LCI) Analysis

The Inventory analysis step (Step 2 in Figure 9) builds a systems model according

to the requirements of the goal and scope definition. The resulting mass and

energy balance is incomplete in the sense that only relevant environmental flows

(emissions, use of resources) are considered [72]. LCI models are normally

created to be static and linear, so time is not used as a variable and all

relationships are simplified to be linear [83]. Consequently, efforts to build

dynamic LCI models have explicitly incorporated dynamic process modeling in

the context of temporal and spatial variations [84]. The LCI analysis includes:

Flowchart construction according to the determined system boundaries

Data collection for all activities in the product system (raw materials,

emission to air, water and solid waste) followed by documentation of data

Calculation of environmental load (amount of resource use and pollutant

emission) with respect to the FU

The LCI analysis is complex since many technical processes produce more than

one product. The environmental load for such processes are allocated, that is

partitioned, between different products within the system [85]. Table 1 shows the

typical parameters of an LCI, illustrated with data from Paper I where the

conversion (amine scrubbing and liquefaction) of biogas from a WWTP is used as

an LBM fuel in tractor-trailers (TT). The inventory for the LBM lifecycle for the

FU of 16,000,000 ton-km of a TT transporting products and goods is also shown.

Table 1. Life cycle inventory of LBM-TT life cycle (Paper I)

Inputs

Outputs/

FU

Unit Paper I (Input

/Output)

Quantity

Page 39: Circularity Assessment of Water and Waste in Cities

36

Input

Raw

Materials

Mass/Volume

Clean biogas (after amine

scrubbing)

364,000 Nm3

Utilities

Heat

Electricity

Fuel

Joules

KWh

Liters

Electricity from Swedish

grid

Electricity credit from

biogas

1745 MWh

- 1184 MWh

Output

End

products

Waste

disposal

Mass/Volume

Liquefied Biomethane

(LBM)

Fuel consumption LBM

TT

280,000 kg

28 kg/100 km

0.0175 kg/tonne-

km.

Emission

Air

Water

Soil

Mass

Biogenic CO2

CH4

NOx

PM

798 tonnes

14 tonnes

420 tonnes

2.4 kg

4.1.3 Life Cycle Impact Assessment

Life Cycle Impact Assessment (LCIA) (Step 3, Figure 9) aims to highlight the

impacts and environmental consequences of the environmental load quantified

in the LCI. It transforms the inventory results into more environmentally relevant

information (acidification, ozone depletion etc.) [86]. The ISO standard (14042)

for LCIA contains the following sub-phases [72, 87, 88]:

Impact category definition is the specification of environmental

impacts relevant to the goal and scope definition. The decision to include

these categories is based on completeness, practicality, relevance,

scientific method. i.e. midpoint indicators and endpoint indicators

Classification is used to sort the inventory parameters according to

the environmental impact they contribute to i.e. the cause-effect

pathway.

Characterization is the relative contribution of the emissions and

resource consumption to each type of impact calculated e.g. total

emissions of greenhouse gases are combined into one indicator for global

warming.

Normalization relates the characterization results to a reference value.

The main aim is to gain a better understanding of the magnitude of the

environmental impacts caused e.g. relating the impacts of the studied

product to the impacts of the total amount of pollutants in a region.

Grouping means to sort and possibly rank the indicators

Page 40: Circularity Assessment of Water and Waste in Cities

37

Weighting means to combine the characterization results across impact

categories

Data quality analysis means to carry out a sensitivity analysis to

obtain a better understanding of the reliability of the LCIA results e.g. the

most polluting activities, the most crucial inventory data, and the

significance of alternative methodological choices.

Not all sub-phases in the LCIA have the same level of importance. An LCA study

typically includes core phases such as classification, characterization and

normalization.

The most commonly used LCIA methods in this thesis were RECIPE Europe (H)

(Paper I), RECIPE World (H) (Paper II), and ILCD 2011 (Papers III and IV) [75,

88, 89]. These methods were used based on their goal and scope, which

determines the region (Europe, World) over which the study was carried out,

important environmental impacts to be included in the study, and environmental

costs available for the LCIA methods. The commonly used midpoint indicators

(Papers I–V) are listed in Table 2.

Table 2. Midpoint indicators/impact categories considered in LCIA

Midpoint Impact

Category

Unit Cause Effect Pathway

Global Warming Potential

(GWP)

kg CO2 eq. Greenhouse gas impacts

depend on changes in

radiative forcing

(expressed as W/m2)

Ozone Depletion Potential

(ODP)

kg CFF-11 eq. A number of persistent

gaseous compounds

released to the air may

result in an increase of

chlorine and bromine

concentrations in the

stratosphere, causing a

reduction in the

stratospheric ozone

concentration.

Acidification Potential

(AP)

kg SO2 eq./mole

H+ eq.

Substances causing

acidification, such as sulfur

dioxide and nitrogen

oxides, are diffused while

carried in an air stream.

These substances will be

Page 41: Circularity Assessment of Water and Waste in Cities

38

transformed to acidifying

substances such as sulfuric

acid or nitric acid through

oxidization and

photochemical reactions.

Freshwater

Eutrophication Potential

(FEP)

kg P eq. Airborne substances

involving nitrogen and

waterborne substances

containing nitrogen and

phosphorus may promote

eutrophication on land and

in water areas (surface

water/freshwater).

Human Toxicity Potential

(HTP)

kg 1–4 DB

eq./CTUh

Available characterization

factors for toxicological

impacts on human health

in LCA that account for

chemical fate, human

exposure, and toxicological

effects.

Photochemical Ozone

Formation Potential

(POFP)

kg NMVOC eq. Photochemical smog is

caused by the creation of

ground level (tropospheric)

ozone from the interactions

of volatile organic

substances (VOCs) and

oxides of nitrogen.

Particulate Matter

Formation Potential

(PMFP)

kg PM10 eq. The change in ambient

concentration of PM2.5 after

the emission of a precursor

i.e. NH3, NOx, SO2 and

primary PM2.5, was

predicted using the

emission-concentration

sensitivities matrices for

emitted precursors.

Terrestrial Ecotoxicity

Potential (TEP)

kg 1,4 DB eq.

/CTUe

Ecotoxicity is treated in a

similar way to human

toxicity including both fate

and effect; exposure is

generally implicitly taken

Freshwater Ecotoxicity

(FETP)

kg 1,4 DB

eq./CTUe

Page 42: Circularity Assessment of Water and Waste in Cities

39

into account in the effect

factor.

The LCIA methods normally assign a factor to each elementary flow in an

inventory table [75]. For example, to measure the GWP as carbon dioxide

equivalent, the following factors are considered: releasing 1 kg of CH4 into the

atmosphere is roughly equivalent to releasing 84 kg of CO2. Similarly, releasing 1

kg of N2O into the atmosphere is roughly equivalent to releasing about 298 kg

of CO2 [90]. For all the appended papers, these midpoint impact categories were

investigated in order to evaluate the overall environmental performance of the

process studied with the tradeoffs between the impacts explained using

supporting (substances/process causing the impact) information.

4.1.4 Interpretation of Results

According to ISO 14040, Life Cycle Interpretation (LCI) (Step 4, Figure 9) is a

systematic technique to identify, quantify, check, and evaluate information from

the results of the LCI and/or the LCIA [86, 91]. The large number of parameters

generated in the calculation of the quantitative LCA must be processed before

interpretation and visualization of results. Using a city as an example, the

municipal stakeholders are the target audience and hence the results must be

presented as an overview of the system studied, as well as identify the hotspots

which cause specific environmental impacts. However, researchers and scientists

who understand chemistry, the behavior of chemical compounds in the

environment and their transformation in air, water and soil need detailed

inventory results to examine the processes that cause such compounds. The

advantage of an LCA is that it not only illustrates the whole life cycle, but also

makes it possible to delve inside the different parts of the life cycle. A contribution

analysis can be carried out to interpret the critical contributions from the life cycle

stages (individual unit processes or groups of processes). A contribution analysis

was carried out in the study described in Paper II in order to identify which

environmental loads (activities) contributed to the total environmental impact of

various life cycle stages in the conversion of food waste to CBM fuel. This

contribution analysis is shown in Figure 11 below.

Page 43: Circularity Assessment of Water and Waste in Cities

40

Figure 11. Contribution analysis of the environmental impacts (Table 2) of life

cycle stages in the conversion of food waste to CBM fuel. The stages include the

anaerobic digestion plant, cogeneration unit, sludge and waste management,

conversion of biogas to biomethane, CBM service station, use of CBM as fuel in

buses

As can be seen in Figure 11, the biogas plant (which includes the pretreatment of

food waste and production of raw biogas by AD) contributed 57–86% of the total

impact in the GWP, ODP, FEP, HTP, TEP and FETP categories. GWP was mainly

driven by methane slip emissions (2%) from the AD plant whereas the other five

impacts are caused by addition of FeCl3 in the digester to inhibit high

concentrations of gases such as H2S and NH3. The use stage contributed to high

AP, POFP and PMFP impacts (80–89% of total impact). Release of NOx

emissions due to combustion of CBM fuel is responsible for AP and POFP impacts

whereas particulate matter emissions increase PMFP. However, the absolute

scores of these impact categories for CBM buses are much lower than CNG or

diesel buses.

The sludge and waste management stage (i.e. sludge thickening and drying, and

disposal of non-biodegradable waste in open dumps) contributes to a reduction

in ODP, HTP, FEP and FETP impacts by 28–42% and completely negates (100%)

the TEP burden imposed by other stages of the life cycle. This is attributed to

environmental credits associated with the application of digested sludge as bio

fertilizer. However, open dumping of non-biodegradable waste reduces the

Page 44: Circularity Assessment of Water and Waste in Cities

41

benefits, particularly in the GWP and FEP impact categories. The results of this

type of analysis are important for comparing resource use, and emissions at the

characterization level. One can also see the dominance of different stages of the

life cycle (raw material, manufacturing, use, end of life) and their contribution to

the environmental impacts. These analyses allow identification of improvements

(processes, chemicals, energy) that are most wanted or needed. The quality of

results must be transparent and also, according to ISO14040/44, the reporting of

LCA results must contain in-depth information along with robustness checks of

results that include [80]:

Completeness check – Data gaps in inventory

Consistency check – Within the defined goal and scope, check for

appropriateness of life cycle modeling and methodological choices

Uncertainty analyses - Effect of uncertain data

Sensitivity analyses – Identify and check effect of critical data

Variation analyses – Effect of alternative scenarios and life cycle models

Data quality assessments - The background data use the unit process

from the ecoinvent database with a specified uncertainty. The foreground

data use the pedigree matrix. The pedigree matrix (PM) is a post-normal

approach to assigning uncertainty. It is a framework, that measures data

quality based on the indicators’ reliabilities, completeness, temporal

correlation, geographical correlation, and technology correlation.

In the final step of an LCA, all conclusions based on the previous steps of the

interpretation, should be qualified in terms of their robustness, and

4.1.5 Uncertainty Analysis

The imprecision of data used for LCA can be evaluated by using uncertainty

analysis. The range of possible values over an interval for a particular material

introduces variability. The information obtained from different suppliers and

production processes under different conditions can affect the environmental

performance of the product [84]. There are also other different sources of data

uncertainty [92]:

Uncertainty in measurements and estimates

Uncertainty in consumer behavior in the use and disposal phases

Uncertainty in future disposal scenarios

Uncertainty in impact assessment factors

The interval over which the data can range can be an important piece of

information for comparison (e.g. minimum and maximum values). It is of crucial

importance to collect all variability in the data used for the LCI so that the interval

Page 45: Circularity Assessment of Water and Waste in Cities

42

and distribution can be established. Table 3 shows, as an example, the variation

in fuel economy, methane slip and tail pipe emissions of different fuels (CBM,

diesel, CNG used in buses) used for calculating uncertainties in the study

described in Paper II, and investigate how these uncertainties influenced the

environmental impacts.

Table 3. Variation of key modeling processing parameters for

uncertainty analysis (Paper II)

Parameter Range Varied Notes

Methane slip

emissions 2–4% of CBM produced

Based on minimum and

maximum slip emissions

for AD and conversion

units. This results in

variation in bus-km from

1,213,297 to 1,257,997 bus-

km (same range considered

for CNG and diesel buses).

Fuel economy 0.48–0.6 Nm3/km

Baseline considered 0.57

Nm3/km of CBM and CNG

buses

Tailpipe emissions

CO 0.36–3.00g/km

(Diesel);

0.4–1.5 g/km (CNG)

Based on driving cycle and

actual emission studies

CO2 700–1200 g/km

(Diesel and CNG buses)

NOx 6–11 g/km (Diesel)

0.5–6.5g/km(CNG

and CBM)

PM 0.1–0.5 g/km (Diesel)

0–0.03 g/km (CBM

and CNG)

4.1.6 Scenario Analysis

Scenario analysis is a strategic process for analyzing decisions by considering

alternative possible outcomes. It provides a basis for further analyses, discussions

and developments to gain greater knowledge of various scenarios in LCA. It is

seen as an investigation of the effects of changing parts of the life cycle model or

changing life cycle processes in the system studied [85, 93]. The results of the

scenario analyses make it possible to see which changes would lead to substantial

reductions in environmental load and which would lead only to marginal changes.

Page 46: Circularity Assessment of Water and Waste in Cities

43

Paper II describes the scenario analysis of the influence of using an external

energy supply (Indian electricity mix) in biomethane plants on the overall

environmental performance of using buses fueled with CBM. Significant tradeoffs

were seen when the electricity powering the biomethane plant was supplied from

an external source i.e. Indian electrical grid mix [94](coal 75%, gas & oil 8%,

renewables 17%, nuclear 3% as of 2019) and when all the biogas produced was

converted and used to fuel buses. CBM buses still performed better than CNG and

diesel buses in most impact categories (ODP, FDP, TEP) and marginally better

with respect to reduction in GWP.

From an environmental perspective, coal is the worst source of fuel for electricity

production since it increases environmental problems such as acidification

eutrophication, human and freshwater ecotoxicities [95]. Combustion of coal to

produce electricity also increases particulate matter emissions. However, since

the emission comes from stationery (power plants) sources, the environmental

externalities attributed to damage caused to a society are lower than tailpipe

emissions resulting from diesel combustion in vehicles.

Interestingly, in spite of methane losses and use of electricity from the high

carbon intensity electrical grid, CBM buses reduce GHG emissions marginally by

8–10% but can decrease FDP by 46–56% compared to diesel and CNG buses. This

can significantly reduce crude oil imports to India. The scenario analysis results

suggest that the monetary valuation of environmental externalities caused by a

trio of impacts (GWP, PMFP and FDP) can still be lower than the status quo,

considering that traffic-related particulate matter emissions have higher damage

costs than power plant emissions [96]. Further, converting all the biogas to CBM

may be reasonable from a perspective of reducing capital expenditure for a

biomethane plant that is self-sufficient in energy i.e. installation of a CHP unit

and biogas conversion plant can be extremely capital intensive [96].

4.1.7 Limitations of LCA

LCA studies are based on assumptions and scenarios because they assess the real

world using a simplified model. The LCA methodology has its own limitations

that can lead to doubt about the results. The main problem lies in the idea that

methodological choices, such as system boundaries and functional units, tend to

be inconsistent which means that it is very challenging to compare different

studies [84]. Although there have been increasing concerns about the use of LCAs

for marketing claims, the concept of life cycle studies has developed over the

years. A whole series of LCA standards has been published as a code of practice,

providing a rigid methodology applicable to a large range of products used in

different contexts for different purposes [97]. Another critical issue debated is the

Page 47: Circularity Assessment of Water and Waste in Cities

44

impacts associated, are if the outcome from the LCA should be considered

potential or real impacts. The difference between a potential and real impact

depends on the location of the impact (e.g. acidification depends on the buffering

capacity of lakes and soil). To quantify real impacts, more data (data on locations,

receiving bodies, background concentrations of pollutants) and work are

required. It is important to emphasize that the potential impacts reported by an

LCA will be the greatest possible for that scenario, and so are not underestimated

[84, 97].

Allocation is another major issue that has been discussed frequently in LCA

forums (e.g. Forum for sustainability through Life Cycle Initiative, Nordic

Dialogue Forum for LCA). The problem of how the environmental loads of a

process are shared among themselves as well as among different products has

been debated. The recent guidelines (ISO 14044:2006) [80] have a way to deal

with allocation (types of allocation), but the issue has not been completely

resolved. These are general limitations and not all are necessarily applicable to

the context of the study carried out in this thesis.

4.2 Life Cycle Costing (LCC)

LCC is a tool similar to LCA that includes all costs over a product life cycle [98].

LCC or Whole Life Costing (WLC) determines the most cost-effective option from

different competing alternatives (e.g. disposal of an object, or process alternatives

for maintenance, operation) [99]. Figure 12 shows the flowchart for WLC. The

strengths of carrying out an LCC are that it can accurately identify cost hotspots

over a product/process life cycle [99]. This can be essential and valuable

information (municipality, stakeholder companies) for selecting the most cost-

efficient alternatives. Papers II, III, IV, and V in this thesis describe LCC

calculations for their respective scopes.

Page 48: Circularity Assessment of Water and Waste in Cities

45

Figure 12. Flowchart to evaluate the whole life cycle costs including the financial

(planning, design, construction and acquisition, operations, maintenance,

renewal and rehabilitation, depreciation) cost which is relatively simple to

calculate and also the environmental and social costs, which are more difficult

to quantify and assign numerical values to [99]

4.3 Environmental Externalities Cost

The environmental impacts obtained from the life cycle analysis of the

product/process can be monetized as the Environmental Externalities Cost

(EEC). The consequence of an action by any agent affecting the environment for

which the agent does not pay compensation or is penalized is defined as

environmental externalities [89]. These externalities arise when the agent

responsible (individual, country) for the activity does not bear all the costs

(negative externalities) or benefits (positive externalities) of that activity. The

environmental pricing used in this thesis is based on damage costs. These

damages are based on the environmental pollution with respect to a range of

midpoints; a value is assigned to the additional overall damage caused by an

additional kilogram of a given emission [100]. Environmental prices are thus

rough-and-ready estimates that are not necessarily valid in specific situations. In

practice, environmental prices can support decision making in two ways [100]:

Page 49: Circularity Assessment of Water and Waste in Cities

46

In environmental analyses such as LCA and EIA, these prices can be used

to weight the various impacts identified. Weighting the impacts is used

in LCA to express the results as a single score indicator.

In Social Cost Benefit Analyses (SCBA), environmental prices are used

primarily for valuation, providing a means of comparing environmental

impacts with financial items to arrive at integral consideration* of all the

impacts associated with an (investment) decision.

The values for the environmental prices of midpoints indicators in this thesis are

mostly unit environmental externality prices published in the literature [89]. In

addition, regional environmental prices were also considered from the literature

to obtain specific cost values [101]. The Life Cycle Environmental Externalities

(LCEE) cost can be calculated using the formula [100]:

LCEE = ∑ (Unit Externality Price in €

Impact) (Env. Impact from LCA Results)

For Paper IV, the ecoefficiency of using fly ash from WtE plants as a filler in epoxy

composite PU panels compared to that of incumbent steel skin sandwich panels

used in the building industry was calculated using:

Ecoefficiency = [1 − (LCEE costs

LCC Private Actors)] × 100

By monetizing the adverse environmental impacts identified in the LCA, the

environmental externalities resulting from the product’s use that are imposed on

society as well as the private costs incurred by stakeholders are measured.

Ecoefficiency was widely used by large chemical companies (e.g. BASF and

AkzoNobel) [102] to evaluate the potential societal environmental gains

achievable by using their products (which may result from, for example, reducing

negative environmental externalities) as well as their own private costs [103].

Similar cost indicators, such as Sustainability Return on Investment (SROI) and

Social Cost Benefit Analysis (SCBA) are calculated in Papers II and III, and can

be used in making investment decisions, product development and in mapping

value chain related environmental and energy risks.

Page 50: Circularity Assessment of Water and Waste in Cities

47

5. Contribution of Papers to the

Development of the Framework

Papers I–V presented in this thesis describe the assessment of different

technology levels within wastewater and MSW treatment plants, including a

system expansion of the boundary studied. System expansion is part of the

consequential LCA method where a consequence of a certain activity is used to

capture changes in environmental impact and obtain information on the

consequences of certain actions [34, 79]. The papers were aligned to different

services of the city i.e. WWTP, OFW Plant, and WtE plant. A framework was

proposed that evaluated the sustainability of the essential municipal services of

an urban system in fulfilling their functional duties and achieving a greater degree

of circular economy compliance (see Figure 7). Figure 13 shows the contributions

of the papers in this thesis to the creation of the proposed framework.

Figure 13. Different stages of circularity in wastewater and waste treatment

plants identified in Papers I–V included in this thesis that led to development of

the five-stage framework

The different stages of the framework identified in these papers are described

below:

Business as usual (BAU) and future alternative scenario. In Paper I,

the objective was to compare the environmental performances of

Liquefied Biomethane (LBM) and Diesel as a fuel to operate Tractor-

Page 51: Circularity Assessment of Water and Waste in Cities

48

Trailers (TTs). The LBM was obtained by converting biogas from WWTP

(Biogas from OFW digestion and landfills can also be a potential source).

Currently, based on the Umeå study, the WWTP uses biogas, produced

onsite for co-generation of heat and electricity, thereby meeting its

energy needs. A system expansion approach was applied where the

electricity and heat equivalents to the amount of biogas used for LBM

production are supplied from the Swedish grid (SE) mix (65% hydro and

nuclear power, 20% wind power and others 15%) and incineration of

wood chips respectively. The plant has currently no liquefaction

technology (converting biogas to LBM).

Additional processing of byproducts. In Paper II, the sustainable

performance of producing CBM from an Organic Food Waste (OFW)

treatment plant to be employed as a fuel in transit buses was evaluated.

In developing countries, the transportation sector is excessively

dependent on conventional fuels such as diesel and petrol, which has

resulted in severe reduction in the urban air quality in their cities.

Therefore, adopting a strategy to connect food waste management and

the operation of transit buses can positively improve the sustainable

performance of cities in developing nations. The sludge obtained after

digestion is used as a fertilizer or soil conditioner and hence the residual

stream is handled by returning nutrients to the biosphere.

Future alternative scenario. In Sweden, the energy obtained from

WtE plants is typically used for meeting the district heating needs of a

city. However, in some countries, such as South Korea, WtE plants are

an integral part of eco industrial parks, where the energy obtained by

combusting MSW is used to meet the needs of an industrial

manufacturing unit (used for electricity and a heat source for

industries) [104, 105]. Thus, in Paper III, a similar scenario was

considered where the energy from a WtE plant was used to power the

carbonization step in carbon fiber (CF) production. This study

evaluated the Sustainable Return on Investment (SROI) of lightweight

Advanced High Strength Steel (AHSS) and Carbon Fiber Reinforced

Polymer (CFRP)-intensive multi-material Body in White (BIW) for

automobiles. The SROI depends on the lightweight BIW

manufacturing cost and the difference in sustainable cost between a

baseline (mild steel) BIW and the lightweight alternative (AHSS,

CFRP). The SROI of CFRP BIWs was maximized when CF was

produced using energy from a low carbon intensive electric grid or

decentralized sources such as waste-to-energy incineration plants. This

scenario of using energy from WtE plants for industrial manufacturing

Page 52: Circularity Assessment of Water and Waste in Cities

49

describes the concept of industrial symbiosis and contributes to

creation of a circular economy.

Handling of residual streams. The incineration of MSW results in

the formation of bottom ash and fly ash, two undesirable forms of

residual byproducts. Bottom ash is a non-hazardous material which can

be easily recycled as a material in road pavements and concrete. Fly ash,

on the other hand, contains toxic components including heavy metals

(e.g., Pb, Cd, Zn, etc.) and dioxins. Thus, incineration plants permanently

dispose of the fly ash in hazardous waste landfills as enforced by the

environmental regulations in many nations. In Paper IV, an evaluation

of the environmental performance of upcycling the fly ash is described. A

thermal insulation panel that consisted of a Polyurethane (PU) foam core

sandwiched between two epoxy composite skins prepared with

reinforcing Glass Gibers (GF) and Silanized Fly Ash (SFA) in epoxy resin

was considered.

Circular compliance. In Paper V, a holistic systems level assessment

decision-making framework that allows urban municipalities (in

collaboration with other key stakeholders) to prepare a long-term

sustainable wastewater management strategy for their cities was

described. From a city perspective, the framework encapsulates two

ideas. First, the sustainable performance of centralized urban WWTPs

will improve with increased circular economy compliance. Second, the

sustainability benefits of a circular compliant urban WWTP will extend

beyond its boundary (application of byproducts and residual stream) and

can be realized at a city, or even at a national, level.

In summary, Papers I to V describe the different layers (BAU, byproducts

processing, residual treatment, advance treatment) within the modeling of a

circular compliant treatment plant for essential municipal services. Thus, the

framework was created (using LCA and LCC tools) from a city perspective to

increase the circularity of these treatment services and included the urban

metabolic rate in order to give a holistic view of the utilization of resources within

an urban system.

Page 53: Circularity Assessment of Water and Waste in Cities

50

6. Assessment Framework for Treatment

of Municipal Services in Cities

As described previously, municipalities currently include sustainability at the top

of their agendas with their ambitions aligned to the sustainability goals of their

respective nations [106]. Sustainable city-centric techno-entrepreneurial

concepts, such as development of low cost and modular technologies for removal

of micropollutants from treated wastewater [107], conversion of MSW to biofuels,

recovery of phosphorus from sewage sludge, and implementation of

decentralized treatment methods etc. have gained significant traction over recent

years [8, 22, 24, 66, 67, 108, 109]. The proposed assessment framework in this

thesis is designed to evaluate the essential services provided by municipalities,

along with the urban metabolic rate of the city, to optimize the overall resource

use. This also helps us understand the relationship between human activities and

the natural environment.

Several quantifiable approaches to measure the sustainable performance of

essential services of a city are available. Sustainable method indicators [110] [111],

the green city index indicators [112], biophysical metrics [113], urban

environment and social inclusion index [114] etc. have been developed. For

instance, the green city index proposed by ESPON, 2015 [112] uses metrics to

measure the ecological footprint in a particular city. The index also includes

indicators related to management of essential services in a city [112]. Assessment

models also exist to quantify sustainability aspects of municipal service

operations and develop indicators reflecting their performance [115]. For

instance, an approach for assessing municipal level sustainability indicators in

Sweden, proposed by Anderson (2013), was developed for Falun Municipality in

Dalarna County, Sweden [33]. There have been individual studies that have

investigated model-based decision support for measuring sustainable water

services combining numerous aspects using tools such as multi-criteria decision

analysis (MCDA) [116].

There are also urban metabolism models described in the literature [29, 117, 118].

They are designed to measure the resources flowing into, and waste streams

flowing out of, a city, and to help understand how different forces (e.g. social and

cultural aspects) influence a city’s metabolic rate [119]. They can be integrated

well with urban planning efforts to build sustainable cities [120]. For example,

Goldstein (2016) addressed the environmental sustainability of food systems in

an urban setting by analyzing their resource flows. This Danish approach is a

hybrid LCA (economic input output/LCA) urban metabolism model looking at

developing the overall material and energy flows in urban agriculture in Denmark

Page 54: Circularity Assessment of Water and Waste in Cities

51

[121]. The metabolism of cities is another open source data hub of data about

resources flowing within different cities around the globe [120]. In addition,

urban metabolism models for use within local authorities for furniture, have also

been assessed [30]. There are also projects such as NEOM 2030 in Saudi Arabia,

which is run by the crown prince and is a sustainable ecosystem generating new

ideas and solutions focused on setting new standards for community health,

environmental protection and the effective and productive use of new technology

[122].

The intention of the framework was to combine both aspects of essential

treatment services of a city (including their contribution in value-added streams

such as ash and biogas) and the urban metabolic rate of the city to evaluate their

sustainable performance. Several frameworks already exist for providing a

comparative analysis of how urban metabolism can be integrated into planning

of cities in different locales [27, 31, 123–125]. These frameworks describe the

capacity, demand, and flow of urban regulating ecosystem services, and related

benefits (the location, typology, and size of urban green infrastructure) controlled

by urban planning. However, a comprehensive understanding of how the

environmental performance of an urban system, such as a city, will be affected

when (a) new technologies are implemented, (b) essential services are

decentralized, and (c) policy-related changes take place with respect to essential

services management, is yet to be achieved.

Thus, it is important to create a strategic framework that encompasses short and

long-term developments within the domain of three essential municipal services

i.e. water supply (potable and non-potable needs), wastewater treatment and

MSW management, and link the framework to the ecological footprint of a city.

This would help to enhance the understanding of the forces (material, energy)

that shape urban metabolism and how these forces affect urban living and

environment. Once validated, the modeling framework proposed in this thesis

can serve as a basis for development of a decision support system (e.g. software)

that will enable authorities to plan strategies for sustainable cities. In addition,

using sustainable assessment tools such as LCA and LCC provides an insight for

emerging technologies in a market that might prove to be innovative.

6.1 Proposed Assessment Framework

The suggested framework assists the evaluation of a comprehensive sustainability

performance of essential municipal service operations within an urban system,

by using a combination of Life Cycle Assessment (LCA) and Life Cycle Costing

(LCC) approaches. The proposed five-stage assessment framework is shown in

Figure 14. The left side of the figure represents essential municipal service

operations structured in five stages. The right side represents total demand of an

Page 55: Circularity Assessment of Water and Waste in Cities

52

urban system including the contribution of energy, material and fuel, obtained

from treating residual wastes generated by essential municipal service

operations. The stages are briefly described as follows.

Stage 1. Business as Usual (BAU) Scenario. Includes current best available

treatment and management practices followed by a city with respect to operation

of their essential municipal services. Papers I–V assessed the BAU scenario in

order to evaluate the environmental impacts of the current practices followed and

to track the tradeoffs in the environmental performance when new treatment

steps are added.

Stage 2. Byproduct Processing. In this stage, the sustainable performance of

additional processing (e.g. converting biogas from the bio digester of the WWTP)

of byproducts (if needed) obtained from Stage 1 is quantified. Papers I, II, III

describe the processing/alternative use of byproducts i.e. Paper I describes the

evaluation of the alternative use of biogas as LBM fuel for heavy-duty trucks

instead of used as energy within the WWTP (current practice). Paper II describes

how biogas obtained from AD of organic food waste was converted to CBM fuel

to be used in buses in Mumbai, India. The alternative use of electricity from a

WtE plant utilized in the manufacturing sector (Carbon fiber) was described in

Paper III.

Stage 3. Treatment of Residual Waste Streams. This stage measures the

sustainable performance of residual waste streams generated from BAU

operations (Stage 1). The residual waste streams include sewage sludge from

WWTP, and bottom and fly ash from a WtE plant. The main intention here is to

optimize the final amount of waste materials disposed of in landfill. Papers IV

and V describe the detailed investigation into the treatment of the residual waste

streams. Paper IV describes the environmental performance of using fly ash

(residue) from WtE plants to be used as filler in epoxy composite panels (building

industry). The environment and cost performances of nutrient recovery, energy

recovery options of sewage sludge from WWTP are discussed in Paper V.

Stage 4. Advanced Treatment Techniques. Determines the sustainable

performance of treatment options that address inefficiencies of BAU operational

practices followed in Stage 1. Treatment of secondary wastewater for removal of

emerging micropollutants is an example of a Stage 4 operation. In Paper V,

ozonation was considered as an advanced treatment option to remove/reduce the

micropollutants load from wastewater and to reuse the effluent water (industry,

farming) from WWTP.

Stage 5. Game-changing Concepts. This refers to entirely different methods

of essential municipal service operations. Treating wastewater using microbial

fuel cells [126] instead of the conventional activated sludge process, or utilizing

the MSW-refuse fraction for biofuel [61] instead of incineration, are both

examples of game-changing concepts. For a city, the sustainable implications of

Page 56: Circularity Assessment of Water and Waste in Cities

53

replacing conventional technologies with novel technologies must be understood

holistically i.e. how replacement affects urban metabolic rates etc.

The Urban Metabolic Rate (UMR) [118] of a city is illustrated to the right in

Figure 14. The UMR is defined as the rate at which resources (water, energy, food,

materials) are consumed by the inhabitants of a city over a given time period.

Using the UMR will enable cities to have a summative picture of all value streams

generated from their services to utilize them effectively towards meeting the

energy, fuel, material, nutrients and water demand of the entire urban system.

Page 57: Circularity Assessment of Water and Waste in Cities

54

Fig

ure

14

. P

rop

ose

d f

ive-

sta

ge

ass

essm

ent

fra

mew

ork

to

ev

alu

ate

th

e su

sta

ina

ble

per

form

an

ce o

f ci

ties

. T

he

left

pa

ne

con

sist

s o

f th

e fi

ve

sta

ges

to

be

eva

lua

ted

in

ord

er t

o c

om

ply

wit

h c

ircu

lari

ty o

f th

e es

sen

tia

l se

rvic

es

trea

tmen

t p

lan

ts.

Th

e ri

gh

t p

an

e co

nsi

sts

of

the

tota

l re

sou

rce

dem

an

d (

wa

ter,

en

erg

y,

fuel

, m

ate

ria

l) o

f th

e

urb

an

po

pu

lati

on

met

by

mu

nic

ipa

l se

rvic

es a

nd

oth

er s

ou

rces

– t

he

urb

an

met

ab

oli

c ra

te.

Page 58: Circularity Assessment of Water and Waste in Cities

55

6.2 Attributes of the Framework

Figure 15 is a flowchart of a systematic evaluation of the essential municipal

services and urban metabolic rate as proposed by the framework. The total cost

(private cost + environmental externalities cost) of operating essential municipal

services (A) in a city is calculated in the left pane. The right pane is the flowchart

for obtaining total cost of urban metabolic rate (B+C) of the city.

6.2.1 Assessment Framework - Data Requirements

Collection of aggregate data from relevant sources is a key component in

evaluating the proposed assessment framework. Various data collection methods

such as interviews, surveys, documents, and focus groups can be implemented

from a city perspective [118]. These data collected are of crucial importance to

describe, and draw insights on, the performance of the essential municipal

services and also the urban metabolic rate of the city. The following data should

be collected:

Data on Essential Municipal Services Operations of Cities

Business as Usual (BAU) scenario of municipal service operations

Population served by centralized water, wastewater and MSW (all fractions)

treatment plants and treatment cost

Amount of residual waste generated from municipal service operations

Future plans of the city to improve circular compliance of existing treatment

trains (Stages 3 and 4) or adopting game-changing concepts (Stage 5)

Some treatment plants meet their energy needs from byproducts generated

internally, with the surplus sold to the city, whereas others sell everything and

meet their energy needs from external sources (e.g. Swedish grid). This

information should also be collected.

A sample data - collection sheet is shown in Appendix A1.

Data on Urban Metabolic Rate of Cities

The data on total urban metabolic rate, including the contribution from essential

municipal service operations and from other sources, should be established. Data

on the following should be collected:

Water demand of a city

Residential energy demand of a city

Fuel demand based on transportation characteristics (i.e. use of public and

private transport), types of transport fuels used

Material (glass, paper, plastic and metals) consumption of a city, and the

distribution of primary or secondary (recycled) materials

A sample data - collection sheet is shown in Appendix A2.

Page 59: Circularity Assessment of Water and Waste in Cities

56

In Sweden, these data can be obtained in collaboration with city municipalities,

site visits, and by reference to open literature sources such as Waste Management

Reports and other sources (e.g. SCB, Avfalls-Web) [47]. For Umeå, the data were

obtained from municipal stakeholder companies (Vakin, Umeå Energi, Skellefteå

biogas plant) as a collaborative effort, and from open literature (Umeå EGCA

report). The data sources can vary in different countries.

Page 60: Circularity Assessment of Water and Waste in Cities

57

Fig

ure

15

. F

low

cha

rt t

o e

va

lua

te t

he

esse

nti

al

mu

nic

ipa

l se

rvic

es a

nd

urb

an

met

ab

oli

c ra

te a

s p

rop

ose

d b

y t

he

fra

mew

ork

. T

he

wo

rkfl

ow

in

clu

des

d

ata

co

llec

tio

n,

carr

yin

g

ou

t L

CA

a

nd

L

CC

o

n

the

esse

nti

al

serv

ices

trea

tmen

t p

lan

t, m

ak

ing

im

pro

ved

dec

isio

ns

ba

sed

on

th

e in

dic

ato

rs,

ad

din

g t

he

va

lue

stre

am

s fr

om

th

e

mu

nic

ipa

l se

rvic

es t

o t

he

urb

an

met

ab

oli

c ra

te o

f th

e ci

ty,

mo

net

izin

g t

he

imp

act

s a

nd

ca

lcu

lati

ng

th

e to

tal

cost

(pri

va

te c

ost

+L

CE

E)

Page 61: Circularity Assessment of Water and Waste in Cities

58

6.2.2 Assessment Framework – Stage-wise Technology Options for

carrying out LCAs

The BAU treatment techniques related to operation of three essential municipal

services (Stage 1), technology options available to achieve a greater degree of

circular compliance of approaches (Stages 2 through 4), and the game-changing

technology concepts (Stage 5) used to provide municipal services (i.e. Wastewater

and MSW fractions) are summarized in Tables 4–6.

Table 4. Technology options for water treatment service

Water Treatment Service [108, 127, 128]

BAU Scenario (Stage 1) Conventional water treatment train

involving coagulation, flocculation and

sedimentation followed by sand filtration

and disinfection using chlorine-based

chemicals (sodium hypochlorite, UV light

or ozone)

Byproducts Processing (Stage

2)

Not applicable

Residual Waste Treatment

(Stage 3)

Not applicable

Advanced Treatment

Technologies (Stage 4)

Treatment for removal of micropollutants

(associated with conventional water

treatment)

Membrane or thermal desalination

techniques (Alternative treatment

technologies)

Game-changing Concepts

(Stage 5)

Not applicable

Table 5. Technology options for WWT service

Wastewater Treatment Service [22, 24, 62, 63, 68, 126, 129, 130]

BAU Scenario (Stage 1) Includes primary, biological secondary and

tertiary treatment steps as well as sludge

management with, or without, anaerobic

digestion (AD) process.

Byproduct Processing (Stage

2)

Conversion of biogas

Residual Waste Treatment

Pathways (Stage 3)

Direct nutrient recovery from digested

sewage sludge

Upcycling as secondary raw material for

industries

Page 62: Circularity Assessment of Water and Waste in Cities

59

Advanced Treatment Steps

(Stage 4)

Removal of micropollutants

Game-changing Concepts

(Stage 5)

Microbial fuel cell or algae-based

wastewater treatment

Table 6. Technology options for MSW service

Treatment of Municipal Solid Waste Service

MSW-Refuse [21,

52, 54, 61, 65, 66,

69] [53, 131, 132]

MSW-Organics

[49, 133-136]

MSW-

Recyclables

[23, 40, 52, 57,

137]

BAU

Scenario

(Stage 1)

Incineration with

energy recovery

Organic waste

pretreated followed

by AD. Biogas and

digestate obtained

as byproducts.

Biogas used as

energy or fuel

source. Sludge

digestate sold as

organic compost.

Glass, paper,

metal, plastic

are recycled.

Electronics,

batteries etc.

are producer’s

responsibility.

Byproduct

Processing

(Stage 2)

Conversion of

biogas

Residual

Waste

Treatment

(Stage 3)

Fly ash

utilization

pathways

Nutrient recovery

from dried sludge

digestate.

Integrated process

based on

combination of AD

& other

thermochemical

processes [138].

Residues that

cannot be

recycled are

sent to WtE

plants for

energy

recovery.

Advanced

Technology

Initiatives

(Stage 4)

Address problems

of incomplete

combustion

Carbon capture

and storage

Improving district

heating efficiency

Hydrogen

Separation from

biogas produced by

AD units

Converting

plastics to

fuel

(pyrolysis)

Page 63: Circularity Assessment of Water and Waste in Cities

60

Game-

changing

Concepts

(Stage 5)

Gasification or

pyrolysis for

biofuel

production

Recycling,

selective sorting

and production of

fuel

Gasification and

pyrolysis of waste

Fermentation of

food waste

Once the system boundary for the treatment services has been decided, LCAs are

carried out to calculate the environmental impacts of the process. The functional

unit (FU) of the LCA and LCC studies is “Providing essential municipal services

to residents of the city for one year”. A sample system boundary is shown in

Appendix A3.

Similarly, the functional unit for carrying out LCA and LCC studies on the UMR

is “Urban metabolic rate met by a city per year”. The system boundary is shown

in Appendix A4.

Monetization of Environmental Impacts. The midpoint environmental impacts

(shown in Table 2) determined by the LCA study are subsequently monetized by

multiplying the impact score with unit environmental externality prices specified

by literature (see Chapter 4) [89] [101].

In this framework, LCC is applied to determine private costs incurred by the city

to operate its essential municipal services and for meeting its urban metabolic

rate (Chapter 4) [98]. The cost sector is added to the framework to translate the

LCA results to the societal value (environmental effects of production and

consumption that affect consumer utility) of reducing impacts on the

environment.

6.2.3 Total Cost Calculation

Total Cost of Municipal Services TC (MS)

The sustainable value of essential municipal service operations is determined

for cities considering two scenarios: (a) BAU and (b) future initiatives scenarios

(e.g. phosphorus recovery from sludge).

The TCMS (measured in Swedish Krona (SEK)) is determined as follows,

𝐓𝐂(𝐌𝐒) = [(𝐓𝐏𝐂) + (𝐄𝐄𝐂)] 𝐌𝐮𝐧𝐢𝐜𝐢𝐩𝐚𝐥 𝐒𝐞𝐫𝐯𝐢𝐜𝐞𝐬

where

Page 64: Circularity Assessment of Water and Waste in Cities

61

TPC = Total Private Costs incurred by a city to provide essential municipal

services to its residents. This includes costs of basic treatment and byproduct

processing (Stages 1 and 2) + cost of treating/disposal of residual streams (Stage

3) + cost of advanced treatment costs (Stage 4).

EEC = Environmental Externality Costs. The LCA results are monetized and,

ultimately, the EEC is determined as the sum of the monetized values of

individual impacts. It also includes credits from the secondary material obtained

from residual waste (Stage 3).

Total Cost of Urban Metabolic Rate TC (UMR)

The TC (UMR) (in SEK)) is determined as follows:

𝐓𝐂 (𝐔𝐌𝐑) =

{[(𝐓𝐏𝐂) + (𝐄𝐄𝐂)]𝐎𝐭𝐡𝐞𝐫 𝑺𝒐𝒖𝒓𝒄𝒆𝒔 + [(𝐓𝐏𝐂) + (𝐄𝐄𝐂)]𝐕𝐚𝐥𝐮𝐞 𝐚𝐝𝐝𝐞𝐝 𝐬𝐭𝐫𝐞𝐚𝐦𝐬 𝐟𝐫𝐨𝐦 𝐌𝐒 }

where

Total Private Costs (TPC) = Sum of cost of water, energy, fuel, and material

consumption costs of a city per year i.e. other sources (electricity from solar,

hydro, wind, imports, bioenergy, fuel demand met by diesel, gasoline, biofuels

etc.) and municipal service value streams.

Environmental Externality Costs (EEC). LCA is carried out to quantify

environmental impacts corresponding to urban metabolic rate with the results

monetized.

6.2.4 Future Work to Develop the Framework

The framework could be developed further to produce information about cities

such as a qualitative rating (circular compliance) developed for municipal

services, and environmental indicators measuring the sustainable performance

of a city.

A qualitative rating indicating the circularity of essential municipal service

operations can be developed for each city. The qualitative scale could be

developed based on predefined criteria such as: (a) population connected to

centralized WWTP, (b) MSW recycling rate, (c) planned initiatives to manage

residual waste, and (d) use of advanced treatment technologies to remove

emerging trace contaminants from wastewater or reduce inefficiencies in the

district heating network etc.

In addition, environmental performance indicators such as waste

generated/capita, CO2 emissions/capita, air pollution, energy consumption/

Page 65: Circularity Assessment of Water and Waste in Cities

62

capita etc. could be developed based on the output of the framework to optimize

the utilization of resources within a city. These indicators should have scientific

validity, sensitivity, responsiveness and use data available about past situations

[139]. They should reflect a city’s sustainable performance in its present form and

could identify hotspots for future improvement. For example, based on these

performance indicators, a city may choose to use byproducts from essential

municipal service operations differently (e.g. use biogas for cars and trucks

instead of buses) or consider game-changing concepts e.g. production of biofuels

from MSW refuse might be undertaken instead of incineration when the future

fuel demands of the city increased. Stakeholder groups might use these results to

make sustainable decisions.

6.2.5 Unique Features of the Model

The framework has three unique features.

1. The framework is designed to capture all (current and future) activities

associated with essential municipal service operations of a city that are either

targeted at addressing circular compliance (Stages 2 to 4) established for

existing technologies or consider entirely new technology (Stage 5) as a

potentially sustainable alternative.

2. All resources flowing into (from external sources), generated and used within

(energy and fuel from essential municipal service operations), and moving out

of the city (material credits from municipal services) are grouped in the urban

metabolic rate. This allows for greater accountability of resources and

provides an opportunity to improve their usage. For example, a city may

choose to use biogas/biomethane fuel for cars and trucks instead buses. In

addition, the structuring framework supports the intention of developing

decision support software that can be applied to develop strategies for

sustainable urbanization.

6.3 Case Study of a Wastewater Treatment Plant

The challenges associated with treating wastewater as a part of urban sanitation

service are both complex and diverse in nature. In the developing world, where

urbanization is accelerating, inadequate treatment of wastewater has become a

major concern [9,10,64,140,141]. For a specified level of circular compliance

(effluent reuse, energy recovery, nutrient recovery), the proposed assessment

framework quantifies the sustainability performance of a centralized WWTP of a

city. By applying the model, total costs can be calculated, with private costs of

treatment and residual waste management calculated using life cycle costing

(LCC) and the related environmental externality costs calculated using life cycle

assessment (LCA) approaches (stage-wise technology options). Figure 16 shows

Page 66: Circularity Assessment of Water and Waste in Cities

63

the use of the assessment framework for a particular municipal service, treating

wastewater in a city.

Figure 16. Illustration of the framework applied to a case study of a WWTP to

evaluate the sustainable performance of operating a circular compliant WWTP

in a city (based on Paper V)

The five stages included in the operation of a WWTP in a city are:

Stage 1. Business as Usual (BAU) Scenario Includes the conventional WWTP

where the water is treated aerobically (i.e. biologically activated sludge process)

in combination with anaerobic digestion of sewage sludge generated during the

treatment as an additional optional step. The dried sewage sludge is landfilled in

this scenario.

Stage 2. Byproducts Processing In this stage, the biogas (66% methane and

remaining CO2) obtained from AD unit is treated (amine scrubbing) to remove

CO2 and other trace elements (H2S, water), and used as Compressed Biomethane

(CBM) to fuel vehicles.

Stage 3. Treatment of Residual Waste Streams This stage includes the

treatment of sewage sludge from WWTP. The sludge is incinerated for energy

recovery (heat and electricity for the city) and phosphorous is recovered from the

ash using chemical treatments.

Stage 4. Advanced Treatment Techniques includes the treatment of

secondary wastewater to remove emerging micropollutants. An ozonation unit is

added as an advanced treatment option in the WWTP to remove/reduce the

Page 67: Circularity Assessment of Water and Waste in Cities

64

micropollutants load from wastewater and to reuse the effluent water (industry,

farming).

Stage 5. Game-changing Concepts refers to an entirely different method of

treating wastewater in a city. Microbial fuel cell systems have the potential to

enhance energy, water and nutrient resource recovery from a WWTP.

The Urban Metabolic Rate (UMR) includes resources flowing into a city from

other sources, and the contribution of value-added streams from operation of a

WWTP. The water, heat, electricity and fuel demands of the city, and the extent

to which operating a circular compliant WWTP with the previously mentioned

technologies contributes to these resources, are calculated.

LCAs are carried out utilizing the information from different stages, with the

functional unit “operating a WWTP in a city for one year”.

A detailed discussion of the possible technology levels to be used in a WWTP

within the internal boundary of treating wastewater and the external boundary of

possible utilization pathways of biogas and sewage sludge is given in Paper V.

Figure 17 shows the schematic for calculating the total cost to a society of

operating a centralized WWTP by obtaining data from LCAs carried out with the

different technology levels (Stages 1 to 5).

Page 68: Circularity Assessment of Water and Waste in Cities

65

Fig

ure

17

. S

chem

ati

c fo

r ca

lcu

lati

ng

th

e to

tal

cost

to

so

ciet

y o

f o

per

ati

ng

a c

entr

ali

zed

WW

TP

in

clu

din

g t

he

effl

uen

t

trea

tmen

t tr

ain

BA

U a

s th

e in

tern

al

bo

un

da

ry a

nd

ass

essm

ent

of

dif

fere

nt

step

s o

f ci

rcu

lari

ty i

n W

WT

P (

effl

uen

t

reu

se,

ener

gy

rec

ov

ery

, re

sid

ua

l m

an

ag

emen

t) c

on

sid

ered

as

the

exte

rna

l b

ou

nd

ary

Page 69: Circularity Assessment of Water and Waste in Cities

66

The internal boundary cost for a WWTP refers to the total cost of wastewater

treatment operations i.e. the sum of treatment (capital and operational

expenditures) and environmental externality costs (LCAs) incurred by the

WWTP. This includes gathering details about the treatment capacity of the plant,

percentage of the population of the city connected to the central WWTP,

wastewater influent and effluent quality parameters, along with operational data

from within the plant boundary (inventory data e.g. chemicals and electricity

consumed during wastewater treatment). The total external boundary cost is the

cost of byproduct management outside the physical boundary of a WWTP. This

means that data on the utilization of three WWTP byproducts (treated effluent,

biogas (if produced)) and sludge) within the external boundary have to be

consolidated.

Both the BAU scenario (Stage 1 of the assessment framework), and any future,

potentially improved, circular compliance scenarios (Stages 2 to 4 of the

assessment framework) that are under consideration by city authorities (and

other stakeholders) are included in this phase. Additional information on

regional factors such as the water stress index of the city, public and private

transportation within the city (e.g. fuels used, annual distance covered by buses

and cars in a city etc.) will be needed. These data can be factored into the total

cost assessment process reflecting sustainability performance of choices made by

stakeholders with respect to utilization of WWTP byproducts in the external

boundary. The Total Cost is the sum of private and environmental externality

costs associated with wastewater treatment operations and byproduct

management within the internal and external boundaries of a centralized WWTP

respectively.

A life cycle costing (LCC) approach is used to carry out stage-wise quantification

of private costs of all activities related to internal and external boundaries of the

WWTP. The corresponding environmental externality costs are obtained by

monetizing life cycle impact assessment results obtained from the LCA study. The

calculation of such costs comprehensively accounts for the operation of a

centralized urban WWTP, reflecting sustainability performance and different

levels of circular compliance (indicators can also be developed at this point).

Based on the results obtained from the assessment framework in terms of

sustainable value/sustainable cost, stakeholders can establish how operating

such services in a city perform environmentally, and to what extent they

contribute to the sustainability of the city. Paper V describes in detail the

application of the framework to wastewater treatment services of a city in order

to quantify the overall ecoefficiency scope of operating a centralized urban

WWTP.

Page 70: Circularity Assessment of Water and Waste in Cities

67

7. Conclusion & Future work

The world’s population is predicted to grow by 2.5 billion by 2050. Rapid

urbanization without proper planning can lead to a potential environmental

disaster. For city municipalities who play a critical role in planning

implementation, this challenge (proper management of resources) has become

the objective of running the city (i.e. provision of essential services such as heat,

power, water, waste management etc.) with low ecological footprints.

This thesis proposes a strategic assessment framework to guide the assessment

of essential municipal service operations at different technology levels and the

calculation of the urban metabolic rate of a city, using LCA and LCC tools. The

framework was developed with the intention of significantly reducing the

environmental burdens caused by municipal treatment services. From this

perspective, this thesis is most relevant to Sustainable Development Goal (SDG)

11 – Sustainable Cities and Communities that aims to make our cities sustainable

by 2030 [142].

The intention of this systems-oriented assessment framework is to assist city

authorities in developing strategies for sustainable urbanization, implement

them and monitor their progress. The integrated modeling approach (essential

municipal service operations and urban metabolic rate) shows how increased

contributions from byproducts (Stage 2) of municipal services reduce the

dependency on primary energy/fuel sources and, therefore, make a city cleaner

and more resource efficient. However, these byproduct flows must be correlated

to the total urban metabolic rate of a city to plan their utilization wisely (urban

planning target indicator of SDG 11). Stage 3 analyzes the sustainability potential

of emerging technologies for treating residual wastes e.g. phosphorus from

sludge, and heavy metals from fly ash (SDGs 9 and 12). Stage 4 measures the

efficacy of methods for the removal of micropollutants from wastewater

(prevention of leakage of toxic materials into environmental systems (SDG 6 and

9)). These stages address the main criteria for circular compliance. The urban

metabolic rate includes imports, and determines the environmental tradeoffs

occurring elsewhere in the world due to imported food products to Swedish cities

(SDG 12) [106].

The framework needs to be developed further to ensure validation (using data for

all services of a city) of a city’s sustainable performance. The qualitative rating for

circular compliance of municipal services has to be developed, along with the

definition of environmental performance indicators for the urban metabolic rate

(based on LCA and LCC results). The indicators will be qualitative and

quantitative in nature, and reflect multiple factors (technical feasibility,

Page 71: Circularity Assessment of Water and Waste in Cities

68

consumption of resources) that affect the sustainability of a city. The framework

is well suited for medium-sized cities (such as Umeå with 130,000 inhabitants)

[64], where limited number of treatment plants exist, to manage the essential

municipal services. For megacities (over 10 million inhabitants) [143], quite

extensive data collection and technology validation is needed for the framework.

In cities with a greater number of treatment plants that follow different treatment

technology pathways, the complexity of modeling will increase dramatically.

Nevertheless, if the framework can be converted into software, with the

comprehensive modeling approach integrating other sustainability assessment

tools (ecosystem services, social LCA to identify waste behavioral patterns,

consumption patterns), it might then be feasible to use extensive data and

calculate the sustainable performance of operating essential services in

megacities. The framework also does not take into consideration informal waste

management practices that are commonly followed in many developing nations

[144].

The framework itself will be of great value to academic researchers who are

working on projects related to circular transition of municipal service operations

and urban metabolism. In addition, there are three main groups that may have

interest in this thesis: (a) the scientific community, (b) targeted stakeholders, and

(c) non-targeted readers. The targeted stakeholder group includes actors at a city

level as well as municipality companies responsible for crucial municipality

services (e.g. wastewater treatment plants, waste-to-energy plants etc.). Other

important stakeholders include state-funded circular economy platforms that

promote circular economy initiatives, such as Smart City Sweden [145]. The

results of the framework generated in the form of sustainability indicators will

allow a comparison between cities and provides a basis for ranking them. This

would be of general interest for different actors in society, including public actors

as well as private companies.

Page 72: Circularity Assessment of Water and Waste in Cities

69

8. Acknowledgements

Thanks to almighty God for all the blessings upon me. Among many people who

contributed to this thesis, I would like to start by thanking my supervisor Venkata

Krishna Upadhyayula for your guidance, advice, discussion and help in

developing ideas during my PhD. It has been a pleasure to work under your

supervision. I have learnt a lot from you. Thank you for your support and inputs

for the Papers appended to the thesis.

I would like to extend my gratitude to my co-supervisor Mats Tysklind for giving

me the opportunity to work on the Green Technology and Environmental

Economics project. Thank you for all the interesting discussions and support

provided during my PhD. Thank you to my other co-supervisor Runar Brännlund

for lending a helping hand during my PhD. I am thankful to Patrik Andersson and

Dimitris Athanassiadis for their work as committee members and guidance

throughout my PhD.

I would like to extend my thanks to the Umeå municipality companies VAKIN,

Umeå Energi, and Dåva DAC for our fruitful collaboration and also for arranging

site visits, providing data and answering emails and questionnaires whenever

requested. It was very helpful to gather data, which was used in Papers I and IV.

Thanks to Skellefteå Biogas plant at Tuvan for arranging site visits and providing

data for modeling in Paper II. Thanks to the Bio4Energy systems analysis group

and Anna Ström for insightful meetings and discussions.

I am thankful for the Wallenberg Travel grant, AFORSK travel grant received

during my PhD. Thanks to ARCUM Artic Research Centre at Umeå University for

selecting and supporting me in my attendance at the Summer Barents School,

Archangelsk, Russia, in 2017. Special thanks go to the International Office Umeå

University for the short project grant provided for me to carry out research in

India.

Thanks to my co-authors, Stina Jansson, Venkataramana Gadhamshetty, Dalia

Abdelfattah, Leonidas Matsakas, Paul Christakopoulos and Ulrika Rova for

contributions to the papers.

A special thanks to Harish Kumar for drawing the cover of my thesis book. Thanks

to Majid Mustafa for discussions on wastewater treatment.

I want to thank Laxmi Mishra, Alexandra Charlson, Pierre Oesterle, Ioana

Cheicea, and Piotr Jablonski for their interactions during the PhD Council and

after parties. I would like to extend my thanks to Dalia Abdelfattah and Pooja

Page 73: Circularity Assessment of Water and Waste in Cities

70

Yadav for interesting discussions about LCA and for the fun involved. I would also

like to thank the PhD council and Journal Club groups for all our fun-filled

discussions. Thanks to Veronica Benavente and Elena Dracheva for making it

very comfortable to share the same room for work. I want to thank Josef Meens

Eriksson (Sef) at CERE for LCA and costing-related discussions.

I would like to thank Venkata Krishna Kumar Upadhyayula and Mats Tysklind

for allowing me to take different courses during my PhD, which allowed me to

have a broader perspective of modeling. I want to thank Maria Jansson and

Birgitta Berglund for all their help with administrative processes throughout my

PhD.

Finally, I want to thank my family and friends for their support at all times.

Thanks to my dad Shanmugam and mom Vijayatharani for their love and care

and for always looking out for me. A special mention of the support, love and care

from my husband during my PhD, a big hug to you Suresh Kumar, you made it

easier for me. It would have been hard to achieve this without you. Also my son

Dhruv Adhiran, who is a bundle of joy and kept me going through all the hard

times. I want to extend my gratitude to my in-laws Siva Ragunath and

Prabhavathy, my sister Jayalakshmi Shanmugam and brother-in-law Yuvaraj

Sekar, for all their support.

Page 74: Circularity Assessment of Water and Waste in Cities

71

References

1. PWC, Five megatrends and their implications for global defense and security. 2016, PricewaterhouseCoopers: London, UK. p. 1-32.

2. Arouri M E H, Y.A.B., Nguyen-Viet C,Soucat A, Effects of urbanization on economic growth and human capital formation in Africa. 2014, Harvard University: Boston, MA, USA. p. 1-23.

3. UNDESA-2014. Urbanization Trends. 2014 [cited 2021; Available from: https://www.un.org/en/desa.

4. Hu B, C.C., New urbanization under globalization and the social implications in China. Asia & The Pacific Policy Studies, 2015. 2(1): p. 34-43.

5. McDonald R I, G.P., Balk D,Fekete B M, Revenga C,Todd M, Montgomery M, Urban growth, cimate change and freshwater availability. PNAS 2011. 108(15): p. 6312-6317.

6. IVL Sweden, National Waste Management Review. 2012. 7. Hubacek K, G.D., Barrett J,Wiedmann T, Environmental implications of

urbanization and lifestyle change in China: Ecological and Water Footprints. Journal of Cleaner Production, 2009. 17(14).

8. GunnartzK, Drivers and consequences of urban development, G. K, Editor. 2017, The Royal Swedish Academy Of Engineering Sciences (Iva).

9. UnitedNations, Health risks associated with wastewater use. 2017. 10. ChapmaW. 10 Cities Most At Risk of Running Out of Water. 2019 [cited

2021; Available from: https://www.usnews.com/news/cities/slideshows/10-cities-most-at-risk-of-running-out-of-water?slide=2.

11. Chen H, L., Y, Li Z, Xue D, Urbanization, economic development and health: evidence from China's labor force dynamic survey. International Journal of Equity in Health, 2017. 16(207): p. 1-8.

12. Cui L, S.J., Urbanization and its environmental effects in Shanghai, China. Urban Climate 2012, 2012(2): p. 1-15.

13. UnitedNations. Exploring the use of wastewater in agriculture. 2017; Available from: http://www.fao.org/news/story/en/item/463433/icode/.

14. Li S, M.Y., Urbanization, economic development and environmental change. Sustanability, 2014. 6: p. 5143-5161.

15. TiseoI. Global municipal solid waste generation projection 2016-2050. 2018 [cited 2021; Available from: https://www.statista.com/statistics/916625/global-generation-of-municipal-solid-waste-forecast/.

16. Liljefors P, Social sustainability in Swedish urban development– what does it mean?, in Sustainable development, environmental science and engineering. 2016, KTH Royal Institute of Technology: Sweden.

17. The Local. Sweden's consumption footprint among the worst. 2016 [cited 2020 April 12 2020]; Available from: https://www.thelocal.se/20161027/swedens-consumption-footprint-among-the-worst.

Page 75: Circularity Assessment of Water and Waste in Cities

72

18. UnitedNations, Swedish National Reporting to the UN Commission on Sustainable Development CSD18‐19 in Chemicals, Waste management, Sustainable consumption and production, Transport and Mining.

19. StatisticsSweden. There are 8.9 million inhabitants in urban areas. Localities and urban areas 2018 2019 [cited 2021; Available from: https://www.scb.se/en/finding-statistics/statistics-by-subject-area/environment/land-use/localities-and-urban-areas/pong/statistical-news/localities-and-urban-areas-2018/.

20. Authorities, N., Competition In The Waste Management Sector – Preparing For A Circular Economy. 2016.

21. SwedishWasteManagement, Avfall Sverige. 2017. 22. Swedish EPA, Advanced wastewater treatment for separation and

removal of pharmaceutical residues and other hazardous substances 2017.

23. Avfall Sverige. The Swedish Waste Management 2020; Available from: https://www.avfallsverige.se/in-english/.

24. Dagerskog L, O.O., Swedish sludge management at the crossroads. 2020, Stockholm Environmental Institute: Stockholm, Sweden. p. 1-8.

25. United Nations., Urban metabolism for resource-efficient cities: From theory to implementation. 2017, United Nations Environment.

26. Dijst M, W.E., Bocker L,Brunner P,Davoudi S,Geertman S,Harmsen R,Helbich M,Holtslag A A M,Lenz B,Lyons G,Mokhtarian P L,Newman P,Perrels A,Ribeiro A P,Carreon J R,Thomson G,Zeyringer M, Exploring urban metabolism: Towards interdisciplinary perspective. Resources, Conservation and Recycling, 2018. 132: p. 190-203.

27. Newman, P.W.G., Sustainability and cities: extending the metabolism model. Landscape and Urban Planning, 1999. 44: p. 219-226.

28. United Nations: New York, U., 2014, UNWorld urbanization prospects: The 2014 revision highlights. 2014: p. pp 1-32.

29. WenyHan W, G.Y., Lu Y,Wilson J,Sun L,Satoshi O,Geldron A,Qiana Y, Urban metabolism of megacities: A comparative analysis of Shanghai, Tokyo, London and Paris to inform low carbon and sustainable development pathways. Energy, 2018. 155: p. 887-898.

30. Russo T, B.E., Franzese P P, The urban metabolism of the city of Uppsala (Sweden). Journal of Environmental Accounting and Management 2014. 2(1).

31. Magrini C, E.D.A., Marco D E,Bonoli A, A framework for sustainability assessment and prioritisation of urban waste prevention measures. Science of the Total Environment, 2021.

32. Martínez F P, Castro-Pardo M, Barroso M V, Azevedo C J, Assessing Sustainable Rural Development Based on Ecosystem Services Vulnerability. MDPI Land, 2020. 9(7).

33. AndersonL, Measuring Sustainable Cities:An approach for assessing municipal-level sustainability indicator systems in Sweden. 2013, Uppsala University: Uppsala.

34. Claudia Peña, B.C.A.G.-S., Angela Druckman, Armando Caldeira- Pires, Bo Weidema, Eric Mieras, Feng Wang, Jim Fava, Llorenç Milà i Canals, Mauro Cordella, Peter Arbuckle, Sonia Valdivia, Sophie Fallaha, Wladmir Motta, Using Life Cycle Assessment to achieve a circular economy, in

Page 76: Circularity Assessment of Water and Waste in Cities

73

Position Paper of the Life Cycle Initiative, July 2020. 2020, Life Cycle Initiative.

35. Harsimran K, G.P., Urban Sustainability Assessment Tools: A Review. Journal of Cleaner Production, 2018.

36. OECD, The circular cconomy in Umeå, Sweden 2020, Organization for Economic Development and Cooperation: Paris, France. p. 1-90.

37. United Nations SDG, Goal 11: Make cities inclusive, safe, resilient and sustainable. [cited 2021; Available from: https://www.un.org/sustainabledevelopment/cities/.

38. Cristiano S, Z.A., Liu G, Ulgiati S,o Gonella F, On the Systemic Features of Urban Systems. A Look at Material Flows and Cultural Dimensions to Address Post-Growth Resilience and Sustainability. Urban Resource Management, 2020.

39. USEPA. Comparison of Green Building Standards. 2020 2020 [cited 2021; Available from: https://www.epa.gov/smartgrowth/comparison-green-building-standards.

40. EGCA 2018, U., Sweden Waste Production and Management. 2018. 41. Umeåkommun. Umeå in brief. Available from:

http://www.umea.se/mer/otherlanguages/inenglish/umeainbrief.4.1255481e123d7d67aaa800010679.html.

42. Cleantech, N. Umeå Wastewater Treatment Plant. Available from: https://www.northswedencleantech.se/en/technical-and-business-visits/umea-wastewater-treatment-plant/.

43. SEPA, Wastewater treatment in Sweden 2016. 2016, Swedish Environmental Protection Agency: Stockholm, Sweden. p. 1-32.

44. Vakin. Sewage 2017; Available from: https://www.vakin.se/tjansterochabonnemang/avloppsvatten.4.30ef415915f7bdea1ee24f03.html.

45. Swedish EPA, Wastewater treatment in Sweden. 2014, Swedish Environmental Protection Agency.

46. Umeå Kommun, Avfallsplan för umeåregionen - Resurshushållning för ett cirkulärt samhälle 2020.

47. Avfall, Annual report 2018. 2018, Avfall Scerige: Stockholm, Sweden. p. 1-23.

48. Avfall Sverige, Avfall i Sverige 2018 – Uppkomst och behandling –. 2018.

49. Kommun, S., The Skellefteå Biogas Plant. 50. Kommun, S. Skellefteå biogas plant. 2019 [cited 2021; Available from:

https://www.skelleftea.se/boende/avfall-och-atervinning/biogas. 51. TrendsetterReport, Biogas as Vehicle Fuel, in A European Overview.

2003: Stockholm. 52. Folk E. Waste Management in Sweden: Perspectives. 2020 [cited 2020

24.01.2020]; Available from: https://www.bioenergyconsult.com/waste-management-sweden/.

53. EllenP, Emissions Trading for Waste Incineration Plants with Energy Recovery in Sweden, in Institutionen för ekonomisk och industriell utveckling, Energisystem. 2020, Lund University.

Page 77: Circularity Assessment of Water and Waste in Cities

74

54. Makarichi L, J.W., Techato K, The evolution of waste-to-energy incineration: A review. Renewable and Sustainable Energy Reviews, 2018. 91.

55. Umea Energi. The combined heat and power plants Dåva 1 and 2. [cited 2021 24.01.2021]; Available from: https://www.umeaenergi.se/.

56. European Union. Directive 2008/98/EC on waste (Waste Framework Directive). [cited 2021.

57. Milios L, Municipal waste management in Sweden. 2013, European Environmental Agency.

58. Shahivand R, R.A.M., Environmental assessment of different municipal waste management methods with approach to life cycle assessment (Case study: Yazd, Iran). Nature, Science and Technology, 2021.

59. Ekwall K, Waste incineration in sweden - past and future in Waste Management And The Environment. 1997.

60. Lindqvist K. Hybrid Governance: The case of household solid waste management in Sweden. in t IRSPM Annual Conference - XVI - University of Rome Tor Vergata 2012. 2012.

61. European Parliamentary Research Service, Towards a circular economy – Waste management in the EU. 2017.

62. Nordic Investment Bank. Sweden is growing and so is the need for wastewater treatment. 2017 [cited 2021; Available from: https://www.nib.int/who_we_are/news_and_media/articles/2073/sweden_is_growing_and_so_is_the_need_for_wastewater_treatment.

63. BjörkmanA. Towards more efficient wastewater treatment. 2017 2017 [cited 2021; Available from: https://www.uu.se/en/news/article/?id=8006&typ=artikel.

64. OECD. National urban policy in OECD countries. OECD publishing Paris 2017; 1-133].

65. O, S., Energy from waste in Sweden: State of the art and possibilities for the future. 2017, IVL Swedish Environmental Institute Stockholm, Sweden. p. 1-23.

66. Gustavsson M, S.E., Stigson P,Zetterberg L, Energy Scenario for Sweden 2050. 2011: Sweden.

67. European Comission, Eco innovation in Sweden. 2015, European Commission: Brussels, Belgium. p. 1-39.

68. Rasheed A, S.S., Kashif S, Umer Z and Khatoon M, To Evaluate the Efficiency of Char and Biochar for Waste Water Treatment. Resources,Recycling and Waste management, 2017.

69. Shamnugam K, Jansson S., Gadhamshetty V,Matsakas L,Rova U,Christakopoulos P,Tysklind M,Upadhyayula V K K, Ecoefficiency of thermal insulation sandwich panels based on fly ash modified with colloidal mesoporous silica. ACS Sustainable Chemistry and Engineering, 2019. 7: p. 20000-20012.

70. Takman M. Opportunities for wastewater giants in Sweden. 2019; Available from: https://www.tidskriftenvatten.se/tsv-artikel/opportunities-for-wastewater-reuse-in-sweden/.

71. LiebschT. Life Cycle Assessment (LCA) – Complete Beginner's Guide. [cited 2020 24.01.2020]; Available from: https://ecochain.com/knowledge/life-cycle-assessment-lca-guide/.

Page 78: Circularity Assessment of Water and Waste in Cities

75

72. BritishStandards, Environmentalmanagement —Life cycle assessment —Principles and framework. 2006.

73. ISO. Environmental management -- Life cycle assessment -- Principles and framework. ISO14040:2006 2006-07.

74. Ecochain. Life Cycle Assessment Software Tools – Overview. 2020; Available from: https://ecochain.com/knowledge/life-cycle-assessment-software-overview-comparison/.

75. European Union, Analysis of Environmental Impact Assessment Methodologies for use in Life CycleAssessment, in ILCD Handbook. 2010.

76. Althaus H J, B.C., Doka G, Dones R, Frischknecht R, Hellweg S, Humbert S, Jungbluth N, Köllner T, Loerincik Y, Margni M, Nemecek T, Implementation of Life Cycle Impact Assessment Methods, W.B. Hischier R, Editor. 2010: St. Gallen.

77. Pre. SimaPro PhD. 2017 [cited 2018 Feb 06 2018]; Available from: https://simapro.com/licences/phd/.

78. Ecoinvent. Introduction to ecoinvent Version 3. [cited 2021; Available from: https://www.ecoinvent.org/.

79. J, S.O., Life cycles assessments and solid waste – Guidelines for solid waste treatment and disposal in LCA. 1999, IVL, Swedish Environmental Research Institute.

80. ISO. ISO 14040: 2006 Environmental management: Life cycle assessment principles and framework. 2006 [cited 2020 April 5 2020]; Available from: https://www.iso.org/standard/37456.html.

81. TillmanM A, E.T., Baumann H,Rydberg T, Choice Of System Boundaries In Life Cycle Assessment. Journal of Cleaner Production, 1994. 2(1).

82. EuropeanUnion, Life Cycle Assessment (LCA). 83. Rebitzer G, E.T., Frischknecht R, Hunkeler D, Norris G,Rydberg

T,Schmidt W P, Suh S, Weidema B P, Pennington D W, a, and Li, Life cycle assessment: Part 1: Framework, goal and scope definition, inventory analysis, and applications. Environmental International, 2004. 30(5): p. 701-7220.

84. Guinée J B, H.R., Huppes G, Zamagni A, Masoni P, Buonamici R, Ekvall T and Rydberg T, Life Cycle Assessment: Past, Present, and Future. Environmental Science and Technology, 2010. 45(1): p. 90-96.

85. Guinée B J, H.R., Life Cycle Assessment. 2005. 86. Horne R, G.T., Verghese K, Life Cycle Assessment- Principles,Practice

and Prospects. 2009. 87. Muralikrishna V I, M.V., Life Cycle Assessment. Environmental

Management, 2017. 88. RIVM. LCIA: the ReCiPe model. 2018 [cited 2020 April 5 2020];

Available from: https://www.rivm.nl/en/life-cycle-assessment-lca/recipe.

89. Bruyn S, B.M., deGraaff L,Schep E,Schroten A,Vergeer R,Ahdour S, Environmental prices handbook EU 28 version: Methods and numbers for valuation of environmental impacts. 2018, CE Delft University of Technology: Delft, Netherlands. p. 1-175.

90. Climatechange Connection, CO2 Equivalents. 2020.

Page 79: Circularity Assessment of Water and Waste in Cities

76

91. Life Cycle Initiative, Life Cycle Impact Assessment definition study: Background document III.

92. Igos E, B.E., Meyer R, Baustert P,Othoniel B, How to treat uncertainties in life cycle assessment studies. International Journal of LCA, 2019.

93. Curran M A., Life Cycle Assessment: a review of the methodology and its application to sustainability. Current Opinion in Chemical Engineering, 2013. 2(3): p. 273-277.

94. GOI, Ministry of Power.,Power Sector at a Glance All India. 2021; Available from: https://powermin.nic.in/en/content/power-sector-glance-all-india.

95. EbnesajjadS. Why is coal the worst fossil fuel – emissions, climate, health, smog…? 2017 [cited 2021; Available from: https://chemical-materials.elsevier.com/chemical-rd/coal-worst-fossil-fuel-emissions-climate-health-smog/.

96. Kavitha S, Baroth A., Nande S, Yacout D M M, Tysklind M, Upadhyayula V K K, Social cost benefit analysis of operating compressed biomethane (CBM) transit buses in cities of developing nations: A case study. Sustanability, 2019. 11(4190): p. 1-22.

97. Fibre Net. Life Cycle Assessment: Benefits and limitations. Available from: http://fibrenet.eu/index.php?id=blog-post-eleven#:~:text=LCA%20also%20has%20limitations%20that,that%20another%20study%20has%20included.

98. Norman G, Life Cycle Costing. 2018. 99. David G W., Life cycle costing--theory,information acquisition and

application International Journal of Project Management, 1997. 15(6): p. 335-344.

100. Bruyun S, A.S., Bijleveld M,DeGraff L,Schep E,Schorten A,Vergeer R, Environmental prices handbook: Methods and numbers for valuation of environmental impacts. 2017, Delft, Netherlands: CE Delft. 1-377.

101. Karkour S, I.Y., Abeynayaka A, Itsubo N, External-Cost Estimation of Electricity Generation inG20 Countries: Case Study Using a Global Life-Cycle Impact-Assessment Method. MDPI Sustainability, 2020.

102. BASF. Eco-Efficiency Analysis. [cited 2021; Available from: https://www.basf.com/se/en/who-we-are/sustainability/we-drive-sustainable-solutions/quantifying-sustainability/eco-efficiency-analysis.html.

103. Sustainability Concepts, Eco-efficiency. 2015. 104. GlobalGreenGrowthInstitute, Greening Industrial Parks —A Case Study

on South Korea’s EcoIndustrial Park Program. 2017, Global Green Growth Institute.

105. Kim J., Case Study Greening Industrial Parks A Case Study on South Korea’s EcoIndustrial Park Program. 2017, Global Green Growth Institute.

106. United Nations: New York, U., 2014, Suatainble Development Goals. 2018.

107. Rodríguez S G, O.P., Rodríguez E, Singh D N,Chueca Towards the Implementation of Circular Economy in the Wastewater Sector: Challenges and Opportunities. MDPI Water, 2020.

108. SillanpääM, Advanced Water Treatment, ed. S. M. 2020.

Page 80: Circularity Assessment of Water and Waste in Cities

77

109. Gil-Garcia R, P.A.T., Nam T, What makes a city smart? Identifying core components and proposing an integrative and comprehensive conceptualization. Information Policy, 2015. 20: p. 61-87.

110. María Yetano Roche, S.L., Manfred Fischedick, Marie-Christine Gröne, Chun Xia, and Carmen Dienst, Concepts and Methodologies for Measuring the Sustainability of Cities. Annual Review of Environment and Resources, 2014. 39: p. 519-547.

111. EuropeanCommission, Indicators for Sustainabiltiy cities, in Science for Environmental Policy. 2015.

112. ESPON. Siemens' Green Cities Index 2014 [cited 2021; Available from: https://apps.espon.eu/etms/index.php/this-big-city/qr/534-siemens-green-cities-index.

113. Cochran F V, B.N.A., Biophysical metrics for detecting more sustainable urban forms at the global scale. International Journal of Sustainable Built Environment, 2017. 6(2).

114. UESI, Metrics For Sustainable And Inclusive Cities. 2018. 115. Georgia, E. Municipal Service Quality Assessment Toolkit (MUSQAT).

2020; Available from: www.ctc.org.ge. 116. Schuwirth N, H.M., Logar I,Stamm C, Multi-criteria decision analysis

for integrated water quality assessment and management support. Water Research X, 2018. 1.

117. Musango K J, C.P., Robinson B, Urban Metabolism For Resource-Efficient Cities: From Theory To Implementation. 2017.

118. Sanche L T, B.N.V.S., Urban Metabolism: A Tool to Accelerate the Transition to a Circular Economy. Sustainable Cities and Communities, 2020.

119. Swedish EPA, Transition to sustainable consumption patterns: 6746. 2015, Swedish EPA: Stockholm, Sweden. p. 1-108.

120. HoekmanP. Metabolism of Cities Data Hub. 2020 [cited 2020 24.01.2020]; Available from: https://data.metabolismofcities.org/dashboards/.

121. GoldsteinB, Hybrid life-cycle-assessment-urbanmetabolism model as a framework for quantifying the contributions of urban agriculture to the sustainability of urban food systems. 2016, Technical University of Denmark.

122. NEOM. The Race To A New Future Is On. 2020 [cited 2021; Available from: https://www.neom.com/index.html#vision-2030.

123. BanchevaS, Integrating the concept of urban metabolism into planning of sustainable cities: Analysis of the Eco2 cities initiative: No. 168. 2014, University of Central London: London, UK. p. 1-37.

124. Ramaswami A, W.C., Main D, Heikkila T, Siddiki S, Duvall A, Pattison A , Bernard M, A Social‐Ecological‐Infrastructural Systems Framework for Interdisciplinary Study of Sustainable City Systems. Journal of Industrial Ecology, 2012.

125. Cortinovis C, G.D., A framework to explore the effects of urban planning decisions on regulating ecosystem services in cities. Ecosystem Services, 2019. 38.

Page 81: Circularity Assessment of Water and Waste in Cities

78

126. Gude V G., Microbial fuel cells for wastewater treatment and energy generation, in Microbial Electrochemical and Fuel Cells - Fundamentals and Applications 2016. p. 247-285.

127. Safe Drinking Water Foundation. Conventional water treatment: Coagulation and filtration fact sheet. [cited 2021; Available from: https://www.safewater.org/fact-sheets-1/2017/1/23/conventional-water-treatment.

128. Frenkel V S., Planning and design of membrane systems for water treatment. Materials, Processes and Applications, 2015.

129. Yadav G, D.B.K., Sena R, A comparative life cycle assessment of microalgae production by CO2 sequestration from flue gas in outdoor raceway ponds under batch and semi-continuous regime. Journal of Cleaner Production, 2020. 258.

130. .Lindberg R H, N.S., Lage S,Östman M,Gojkovic Z,Funk C,Gentili F G,Tysklind M, Fate of active pharmaceutical ingredients in a northern high-rate algal pond fed with municipal wastewater. Chemosphere, 2021.

131. Izaharuddina A N, P.M.C., Theppitakb S,Daib X,Yoshikawab K, Food Waste Gasification through Hydrothermal Carbonization Pre-treatment. 2018, Joint meeting the german and italian sections of the combustion institute: Italy.

132. Klinghoffer N B, C.M.J., Gasification and pyrolysis of municipal solid waste (MSW), in Waste to energy conversion technology, N.B. Klnghoffer and M.J. Castaldi, Editors. 2013, Woodhead Publishing: Cambridge, UK. p. 146-176.

133. Protection, N.S.f.C.A.a.E., Biogas as Road Transport, in An assessment on the potential role of biogas aa a renewable transport fuel. 2006: England.

134. Marcoberardino G D*, V.D., Spinelli F, Binotti M , Manzolini G, Green Hydrogen Production from Raw Biogas. MDPI Processes, 2018. 6(19).

135. Marlies Hrad, M.P., Marion Huber-Humer, Monitoring of fugitive methane emissions at Austrian biogas plants - a case study. 2nd IBBA workshop on methane emissions in Kiel, 2014.

136. Grycová B, K.I., Pryszcz A, Pyrolysis process for the treatment of food waste. Bioresource Technology, 2016.

137. Kunwara B, C.H.N., Chandrashekaran R S,Sharmaa K B, Plastics to fuel: a review. Renewable and Sustainable Energy Reviews, 2016. 54: p. 421-428.

138. Saur G , M.A., Renewable Hydrogen Potential from Biogas in the United States. 2014, National Renewable Energy Laboratory.

139. SegnestamL, Environmental Performance Indicators. 1999, The World Bank Environment Department.

140. UnitedNations, 2017 UN World Water Development Report, Wastewater: The Untapped Resource. 2017.

141. Memon A, M., Wastewater Management in Developing Countries. 2011, UNEP.

142. UnitedNations, Transforming our world: The 2030 agenda for sustainable development. 2015: New York, USA. p. 1-41.

Page 82: Circularity Assessment of Water and Waste in Cities

79

143. Iberdrola. Megacities', a future challenge. Environment 2021 [cited 2021; Available from: https://www.iberdrola.com/environment/megacities-urban-area.

144. Wilson D C, V.C., Cheeseman C, Role of informal sector recycling in waste management in developing countries. Habitat International, 2006. 30(4).

145. Explore smart & sustainable city solutions from Sweden. [cited 2021; Available from: https://smartcitysweden.com/.

Page 83: Circularity Assessment of Water and Waste in Cities
Page 84: Circularity Assessment of Water and Waste in Cities

Appendix

Ap

pen

dix

A1

sho

ws

a s

am

ple

da

ta c

oll

ecti

on

sh

eet

for

esse

nti

al

mu

nic

ipa

l se

rvic

es i

n a

cit

y,

as

men

tio

ned

in

th

e

att

rib

ute

s o

f th

e fr

am

ewo

rk s

ecti

on

. T

his

sh

eet

can

be

use

d t

o g

ath

er i

nfo

rma

tio

n a

bo

ut

Um

eå,

for

exa

mp

le.

case

.

Page 85: Circularity Assessment of Water and Waste in Cities

2

Ap

pen

dix

A2

Sa

mp

le d

ata

sh

eet

sho

win

g t

he

pa

ram

eter

s re

qu

ired

to

ca

lcu

late

th

e u

rba

n m

eta

bo

lic

rate

(w

ate

r, e

ner

gy

, fu

el m

ate

ria

ls)

of

the

city

. T

his

sh

eet

can

be

use

d t

o c

oll

ect

da

ta f

or

Um

eå,

for

exa

mp

le.

Page 86: Circularity Assessment of Water and Waste in Cities

Ap

pen

dix

A3

Sa

mp

le S

yst

em b

ou

nd

ary

fo

r ca

lcu

lati

ng

th

e to

tal

cost

of

esse

nti

al

mu

nic

ipa

l se

rvic

es.

Th

is c

an

be

use

d i

n c

alc

ula

tin

g t

he

tota

l co

st o

f o

per

ati

ng

tre

atm

ent

serv

ices

in

Um

eå.

Page 87: Circularity Assessment of Water and Waste in Cities

4

Ap

pe

nd

ix A

4 S

am

ple

sy

ste

m b

ou

nd

ary

fo

r d

eter

min

ing

th

e en

vir

on

men

tal

imp

act

s a

sso

cia

ted

wit

h t

he

urb

an

met

ab

oli

c ra

te.

Th

e fo

od

se

cto

r is

in

clu

ded

to

det

erm

ine

the

ov

era

ll u

rba

n m

eta

bo

lic

rate

of

the

city

.

Page 88: Circularity Assessment of Water and Waste in Cities

Papers I-V