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ANNUAL REPORT Max-Planck-Institut für Festkörperforschung Centre National de la Recherche Scientifique G. Chouteau - G. Rikken N. Samba R. Graziotti http://ghmfl.polycnrs-gre.fr 2OO1

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  • ANNUALREPORT

    Max-Planck-Institut für Festkörperforschung

    Centre National de laRecherche Scientifique

    G. Chouteau - G. RikkenN. SambaR. Graziotti

    http://ghmfl.polycnrs-gre.fr

    2OO1

  • Grenoble High Magnetic Field Laboratory • Annual Report 20013

    This report intends to provide a rathercomplete overview of the in-house andcollaborative scientific and technicalactivities of the Grenoble High MagneticField Laboratory (GHMFL), in the year2001. The laboratory is a joint operation ofthe Max-Planck-Institut fürFestkörperforschung (Germany) andthe Centre National de la RechercheScientifique (France), originally establishedin 1971 and renewed and extended after1.1.1992.

    The existing 24 MW power supply allows tooperate simultaneously two resistive 10 MWmagnets. Magnets with a powerconsumption of 20 MW can reach routinelyd.c. fields up to 30 T. These two high-powermagnets allow to respond very effectively tothe increasing demand of magnet time inthis range. With the forthcoming installationof a new hybrid system (in operation in2003) we aim to reach continuous magneticfields above 40 T. This will guarantee thatthe GHMFL can keep up with the rapiddevelopments in high magnetic fieldfacilities worldwide and can continue to playa leading role in the research in these fields.

    This report and the list of publications showthat important and interesting results can beobtained in magnetic fields, either on thebasis of in-house research or very often as aresult of a close collaboration betweenseveral research groups from many differentcountries. In addition, the GHMFL is proudto contribute to the training of many youngscientists by giving them the opportunity tobe part of such research activities andperforming their work for a PhD.

    Finally, we wish to thank most cordially thescientific and technical staff of thelaboratory (over 80 people) and thenumerous visitors for their contribution tothe successful operation and the quality ofthe scientific work.

    P. Wyder - G. MartinezJanuary 2002

  • Grenoble High Magnetic Field Laboratory • Annual Report 20014

    1. LOW DIMENSIONAL ELECTRON SYSTEMS .............................................................................71.1. Electron-phonon interaction in the intrinsic magneto-photoluminescence of a two dimensional electron gas ..................91.2. Small ring interferometer on the basis of a GaAs quantum well with a high density 2D electron gas.............................101.3. Magneto-optical studies of exciton-electron scattering processes in Cd0.998Mn0.002Te/Cd0.8Mg0.2Te quantum wells..............101.4. Multi spin-flip Raman scattering in CdMnTe quantum wells............................................................................................121.5. Resistively detected EPR of Mn2+ ions coupled to a 2DEG in quantum Hall regime ......................................................131.6. Quantum Hall effect under conditions of vanishing Zeeman energy.................................................................................131.7. Electron-hole coupling in InAs/GaSb bilayers studied by cyclotron resonance................................................................141.8. Single-dot-like emission induced by high magnetic fields ................................................................................................151.9. Insulating states and the breakdown of the quantum Hall effect in an electron-hole system............................................161.10. Anomalous resistively detected NMR lineshape around ν = 1..........................................................................................171.11. Magnetic channelling in tilted magnetic fields ..................................................................................................................181.12. Magnetic field induced metal-to-insulator transition in PbTe wide quantum wells ..........................................................191.13. Transport of two-dimensional electrons in the lattice of diffusive and thermalizing scatterers ........................................201.14. Single-electron conductance oscillations of small open quantum dot ...............................................................................201.15. Gated wires and interferometers based on a Si / SiGe heterostructure..............................................................................211.16. Coexistence of a two-dimensional and three-dimensional Landau states in a wide parabolic quantum well...................221.17. New phase transition of the quantum Hall state at ν = 2/3................................................................................................231.18. Observation of a new scaling behavior of the ν = 1/3 state...............................................................................................241.19. Magnetic field induced linear Coulomb gap in tunnelling between disordered two-dimensional electron systems ........251.20. Probing the electronic properties of disordered two-dimensional systems by resonant magneto-tunnelling....................261.21. Polaron coupling in high electron density GaAs Quantum Well (QW).............................................................................271.22. Many body effects revealed in Cyclotron Resonance (CR) spectra ..................................................................................281.23. Electronic transport through nuclear-spin-polarization-induced quantum wire.................................................................291.24. Luminescence of a dense two-dimensional electron gas involving free- and bound holes in a

    GaAs/InGaAs/AlGaAs quantum well.................................................................................................................................301.25. Magneto-tunnelling spectroscopy of Si donor states in (AlGa)As/GaAs/(AlGa)As quantum wells.................................311.26. Semi-circle relation between Gxx and Gxy in the flow diagram of the integer quantum Hall effect .................................311.27. Negative magnetoresistance due to ballistic weak localization in a dense hexagonal lattice of antidots .........................321.28. Magnetotransport of a strongly correlated 2D electron system .........................................................................................33

    2. BULK SEMICONDUCTORS...................................................................................................352.1. Angle resolved magneto-luminescence of neutral acceptor bound excitons in Gallium Nitride ......................................372.2. Magneto-spectroscopy of two-electron transitions in homoepitaxial GaN........................................................................372.3. Spin excitations of donor-acceptor pairs in GaAs..............................................................................................................382.4. Hall effect measurements in ferromagnetic GaMnAs.......................................................................................................392.5. Paramagnetic to ferromagnetic phase transition in GaMnAs.............................................................................................402.6. Coupled plasmon-LO phonon modes at very high magnetic fields...................................................................................412.7. Motional narrowing effectively reduces the electron spin relaxation in wide gap semiconductors ..................................42

    3. SUPERCONDUCTORS .........................................................................................................453.1. Impurities in high-Tc superconductors: an NMR study of YBa2(Cu0.995Zn0.005)4O8 ......................................................473.2. Two-gap superconductivity in MgB2 .................................................................................................................................473.3. Electronic structure of MgB2: pressure behaviour .............................................................................................................483.4. Memory effects in the vortex matter of type II super- conductors investigated using the magnetostriction technique ...........493.5. Resonant Cooper pair tunneling through a double-island qubit.........................................................................................503.6. Spontaneous emission transition in a superconducting nanocircuit...................................................................................513.7. Evidence of superconductivity in magnetic compound YFe4Al8 ......................................................................................523.8. Interlayer transport in the misfit-layer superconductor (LaSe)1.14(NbSe2) ........................................................................533.9. Evidence for a 3D behaviour of the vortices at low temperature and high magnetic field ...............................................543.10. Deviations from Lifshitz-Kosevich-behaviour in κ-(BEDT-TTF)Cu(NCS)2 ....................................................................553.11. Characterization of transport properties variations with magnetic field and temperature of

    ITER-candidate NbTi strands .............................................................................................................................................55

  • Grenoble High Magnetic Field Laboratory • Annual Report 20015

    4. MAGNETISM - MOLECULAR MAGNETISM............................................................................574.1. Magnetic hardening induced by antiferromagnetic-ferromagnetic exchange interactions ................................................594.2. Low-temperature field induced spin reorientation in Gd5(SixGe1-x)4 ................................................................................604.3. Phase separation in Pr0.5Ca0.5MnO3 thin films ..................................................................................................................604.4. Transport measurements in charge-ordered Pr0.5Ca0.5MnO3 thin films .............................................................................614.5. Controversial origin of the magnetic behaviour in LiNiO2 ...............................................................................................624.6. Magnetic properties of the delafossite compound LaCuO2.66: a study by high-frequency/high-field ESR ......................634.7. ESR spectroscopy of the frustrated ising pyrochlore Ho2Ti2O7 ........................................................................................644.8. Short range order in the frustrated pyrochlore Gd2Ti2O7 ..................................................................................................654.9. Quantum topological excitations: from the sawtooth lattice to the Heisenberg chain.......................................................664.10. Condon domains .................................................................................................................................................................674.11. High field and high frequency ESR of the one dimensional magnetic system (TMMC)..................................................684.12. Very high frequency and very high field EPR on the Mn2+ metalloprotein D-xylose isomerase......................................684.13. HF-EPR study of a spin model for the g = 4.1 S-2 state of PhotoSystem II .....................................................................694.14. HF-EPR single crystal study of [Mn12O12(CH3COO)16(H2O)4] ........................................................................................704.15. High field EPR study on three different glycyl radical enzymes.......................................................................................714.16. Structural and electronic properties of mononuclear manganese (III) complexes, models of metalloproteins.................724.17. Determination of the zero-field splitting in myoglobin .....................................................................................................734.18. Low temperature and high-frequency EPR of a giant keplerate magnetic molecule ........................................................744.19. NMR evidence for a magnetic superstructure in the 1/8 magnetisation plateau of 2D spin system SrCu2(BO3)2 ...........744.20. NMR in the field-induced phase of deuterated CuHpCl ....................................................................................................75

    5. ATOMIC AND OPTICAL PHYSICS ........................................................................................775.1. Free electron on a helix model for magneto-chiral anisotropy ..........................................................................................795.2. Magnetochiral anisotropy in cholesterics ...........................................................................................................................795.3. Magnetotransverse scattering of surface plasmon polaritons.............................................................................................805.4. Faraday effect of photonic crystals.....................................................................................................................................815.5. Chiral symmetry breaking in photo crystallization ............................................................................................................825.6. Magneto-transverse thermal conductivity ..........................................................................................................................835.7. Magneto-electric linear birefringence.................................................................................................................................845.8. Electrical magneto-chiral anisotropy in carbon nanotubes ................................................................................................855.9. Magneto-chiral deflection of light ......................................................................................................................................865.10. Modulation of the Yb3+ to Er3+ energy transfer in LiNbO3 crystals by applying magnetic field......................................86

    6. MAGNETS & INSTRUMENTATION .......................................................................................896.1. Magnets and performances .................................................................................................................................................916.2. Instrumentation and techniques available to users .............................................................................................................916.3. Measurement of forced convection heat tranfer coefficients in mini-channels .................................................................936.4. Nanomechanical resonators in silicon-on-insulator ...........................................................................................................936.5. ESR multifrequency spectrometer ......................................................................................................................................946.6. Implementation of a Quasi-Optical bridge on the HF-EPR spectrometer .........................................................................956.7. Quasi-stationary magnetic fields of 60 T using inductive energy storage .........................................................................966.8. Generation of coherent sub-THz acoustic phonons ...........................................................................................................976.9. Very low temperature, high-frequency, high-field ESR spectroscopy ...............................................................................98

    7. MAGNETOHYDRODYNAMICS...........................................................................................1017.1. Liquid metal jet into a high magnetic field ......................................................................................................................1037.2. Magnetohydrodynamics: transition of Hartmann layers between laminar and turbulent states ......................................1047.3. Anisotropic effect of magnetic field during copper electrodeposition onto an oxidized titanium electrode...................104

    ANNEXES...............................................................................................................................107List of publications 2001 ............................................................................................................................................................109List of Ph.D Theses 2001............................................................................................................................................................119Scientific Staff of the Grenoble High Magnetic Field Laboratory during 2001........................................................................120Collaborating External Laboratories...........................................................................................................................................121Proposals for magnet time carried out in 2001 ..........................................................................................................................122

  • Grenoble High Magnetic Field Laboratory • Annual Report 20017

  • Grenoble High Magnetic Field Laboratory • Annual Report 20019

    1.1. Electron-phonon interaction in theintrinsic magneto-photoluminescence ofa two dimensional electron gas

    Low temperature magneto-photoluminescence (MPL) hasproved to be an interesting tool to investigate the propertiesof two-dimensional electron gas (2DEG) under strongperpendicular high magnetic fields. Up to now, most ofinvestigations were focused on the effects of electron-electron and electron-impurity interaction. Here, we reportthe observation of pronounced effects induced by electron-phonon Frölich interaction but correlated with filling factor.

    In undoped polar semiconductors, such as GaAs, themotion of free charges is affected by their coupling to thepolarization field of longitudinal-optical (LO) phonons. Indoped semiconductors however this field is coupled tointer-subband excitations giving rise to a mixedlongitudinal mode -hωLi- below -hωLO. Recent progress inthe crystal growth of high quality (mobility > 106 cm2/Vs)GaAs QWs with high electron concentration (EF > -hωLi-)makes it possible to observe strong interaction betweenelectrons and such a mixed mode.

    Representative experimental spectra obtained for such asystem (a symmetric QW with thickness 10 nm,EF = 43 meV) are shown in figure 1.1. The correspondingfan chart of luminescence transitions is presentedin figure 1.2. The emission lines Lnp correspond torecombination processes involving electrons and holes

    from nth conduction band Landau level (LL) and pth-valence band LL respectively. The low energy tailLET below the main recombination line L00 is a knownfeature originating from manybody interaction in the2DEG. These spectra show two original features:(i) associated with all Lnn lines (allowed transitions) weobserve Ln0 lines (forbidden transitions in symmetricQW) and (ii) their phonon like replica appearing as a redshifted satellite (RSS in figure 1.2) below the L00 line.

    The RSS transition has an energy dependence onmagnetic field which roughly follows the Ln0 dependenceminus -hωLi- where nth is the highest occupied LL. At evenfilling factor (crossover of the Fermi level from n + 1th tonth LL) the Lnn and Ln0 transitions show a discontinuityin their energy variation. We tentatively explain thisnew features as due to a resonant interaction betweenthe lowest LL and the highest occupied LL coupled with-hωLi- excitation. This process can be understood asequivalent in luminescence of the well known resonantmagneto-polaron effect in cyclotron resonance. Furtherwork is in progress in Raman spectroscopy to quantifythis interaction.

    Reference and authors:

    C.Bardot et al., Physica E, in press

    C.Bardot, M.Potemski, G.MartinezA.Riedel, R.Hey, K.J.Friedland (Paul Drude Institute,Berlin, Germany)

    Figure 1.1: Magneto-photoluminescence spectra of highquality and high density GaAs quantum well structure at1.7 K. The transition labelled RSS is attributed to theeffect of electron-phonon interaction.

    Figure 2.1: “Landau fan chart” of luminescencetransitions. RSS is the line of main interest (starsymbols), it stands for red-shifted satellite of thecorresponding Ln0 line where n is the index of highestoccupied Landau level.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200110

    1.2. Small ring interferometer on thebasis of a GaAs quantum well with ahigh density 2D electron gas

    Magneto-transport properties of small ringinterferometers with narrow electronic channels made onthe basis of a 2D electron gas in a GaAs quantum wellwith AlAs/GaAs superlattice barriers are studied. It wasfound that the amplitude of the h/e-oscillations arecorrelated with the Shubnikov-de Haas oscillations in thearea where the 2D electron gas is connected to the ring.

    The original semiconductor structure has been grown bymolecular beam epitaxy on a (100) GaAs substrate. Thequantum well was formed by a 10 nm thick GaAs layer. AtT = 4.2 K, the equilibrium parameters of the 2DEG wereas follows: concentration ns = 1.8.1012 cm-2 and mobilityµ = 3.5.105 cm2/V.s. The Hall bars were fabricated byoptical lithography with wet chemical etching, and therings were formed by electron beam lithography and dryetching. The effective geometrical radius of the ringsdetermined from the period of h/e-oscillations wasreff ~ 0.13 µm.

    Figure 1.3a shows that the magnetoresistance of the ring(R23) exhibits large-scale fluctuations and small-scaleoscillations. The small-scale oscillations have a periodcorresponding to the threading of one additional fluxquantum h/e through the area of the ring. It can be seen(figure 1.3b) that at B > 4 T, the amplitude of the h/e-oscillations is correlated with the resistance of the 2DEGconnected to the ring. The h/e-oscillations are suppressed atfilling factors νc = i, their amplitude is maximal at νc = i + 1/2.

    The R23(B) and R34(B) curves show that for the ringsstudied in the experiment, the quantized Hall regimearises only in the macroscopic parts of the sample. Onesees from figure 1.3a that the two-terminal resistanceR23(B) does not exhibit quantum plateaus. Thecomparison of the width of the electronic channelscalculated from the width of the Fourier spectrum with thedouble magnetic length 2.rc shows that, at 15 T, ωe < 2.rc:it means that the edge states in the rings were notseparated up to 15 T. In this case the suppression theAharonov-Bohm effect at νc = i is not due to the absenceof backscattering in the channels of the rings. A possiblemechanism for this suppression is a change of theconfining potential that forms the geometry of the regionsadjoining the input and output of the ring, in the quantizedHall regime. It is well known that the screening in a2DEG is essentially different if the highest Landau levelis half-filled or completely filled [1]: for this reason, theedge channel structure is different in these two cases.Namely, in the case where the highest Landau level ishalf-filled, edge current channels are narrower andtherefore penetrate more effectively into the ring. It leadsto an increase of the amplitude of the Aharonov-Bohmoscillations. When the ring is almost closed, the sameeffect could be connected with an increase of thetunneling current proportional to the density of states inthe source/drain regions.

    Figure 1.3: a) Magnetoresistance of the small ringinterferometer and 2DEG at T = 1.7 K. b) Aharonov-Bohm oscillations in magnetic field up to15 T at T = 1.7 K.

    Reference and authors:

    [1] D.B.Chklovskii et al., Phys. Rev. B 46, 4026 (1992)

    A.A.Bykov et al., Physica E, in press

    O.Estibals, J.C.PortalA.A.Bykov, I.V.Marchishin, L.V.Litvin, A.K.Bakarov,A.I.Toropov (Institute of Semiconductor Physics,Novosibirsk, Russia)

    1.3. Magneto-optical studies of exciton-electron scattering processes inCd0.998Mn0.002Te/Cd0.8Mg0.2Te quantumwells

    Whereas two-particle excitonic effects dominate theoptical response of undoped semiconductor structures,negatively charged excitons and exciton-electronscattering processes appear in the optical spectra ofquantum wells with increasing electron concentration. Inthis report we focus our attention on the polarization rulesfor negatively charged excitons and the so-called

    LOW DIMENSIONAL ELECTRON SYSTEMS

  • Grenoble High Magnetic Field Laboratory • Annual Report 200111

    combined exciton-cyclotron resonanceabsorption processes. Our experiments(polarization resolved luminescenceand luminescence excitationmeasurements in magnetic fields up to14 T) have been performed onmodulation doped CdMnTe quantumwell structures. The representativephotoluminescence excitations spectraat different magnetic fields and fordifferent circular polarization of theabsorbed light are shown in figure 1.4for two different samples with electron concentrations of~ 1010 cm-2 (sample S1) and ~ 1.2 x 1011 cm-2 (sampleS2). The magnetic field evolution of the absorption andthe emission peaks observed in the configuration of σ+circularly polarized light are shown in figure 1.5. As canbe seen in these figures both samples show clearabsorption peaks related to negatively charged excitons(X–) and the combined exciton-cyclotron resonanceprocesses (ExCR), in addition to the usual strong exciton(X) absorption lines. The absorptions peaks observed athigher energies are identified with the ground state of thelight hole exciton and the 3d– state of the heavy holeexciton (surprisingly enough the 2s heavy hole state is notvisible in our spectra). It is very characteristic that at lowmagnetic fields the X– absorption is σ+ polarized whereasthe ExCR absorption is observed mostly in σ–polarization. The σ– absorption of the X– and similarly theσ+ absorption of the ExCR appears at fields above ~ 10 T.In CdMnTe, the total Zeeman splitting is determined bythe sum of the external magnetic field and the effectivemagnetic field induced by the spin polarization of Mn2+ions. The two terms are of opposite sign. The Mn2+polarization field dominates at low magnetic fields but theintrinsic Zeeman terms dominate at high fields resultingin the change of the sign (expected around 12 T in oursamples) of the effective Zeeman splitting for electrons.Our results show the sensitivity of both X– and ExCR tothe spin polarization of the 2DEG confined in a quantumwell. Our observations might be helpful for a betterunderstanding the nature of exciton-electron scatteringprocesses (ExCR) which can be surprisingly strong inoptical spectra of lightly modulation doped quantumwells. The coexistance of excitonic like transitionstogether with inter Landau level band-to-band transitions(LL0) clearly visible for the sample with higher electronconcentration is a surprising effect which requires furtherinvestigations.

    Authors:

    Ye Chen, F.J.Teran, M.PotemskiG.Karczewski, T.Wojtowicz (Institute of Physics,PAS, Warsaw, Poland)

    Figure 1.4: Magnetic field evolution of thePLE spectra for two CdMnTe quantum well

    structures (samples S1 and S2) measured forσ+ and σ– polarization of the absorbed light.

    Figure 1.5: Magnetic field dependence of the energypositions of the transitions observed in PLE (solidsymbols) and PL (open circles) for two CdMnTe quantumwells. X, X–, and ExCR denote absorption lines due toexcitons, charged excitons and combined exciton-cyclotron resonance processes.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200112

    1.4. Multi spin-flip Raman scattering inCdMnTe quantum wells

    The unique properties of bulk dilute magneticsemiconductors (DMS) have been investigated using thespin flip Raman scattering technique for many years.Using this method the magnetic transitions of thelocalized spins of magnetic ions (Mn2+ in our case) and ofthe free carriers can be probed.

    We report here new and detailed Raman measurements ona system with a reduced dimensionality. The sampleswere Cd1-xMnxTe quantum wells with low Mnconcentration, x = 0.0054. The measurements wereperformed at 1.7 Kelvin in the Faraday configurationusing circularly cross polarization. An important featureof our measurements was that specific illumination laserfrequencies were searched for and found where theRaman peaks of each subsystem (i.e. electron and Mn2+)were observable alone and could therefore be studiedindependently.

    Figure 1.6 shows results from such a sample. The Ramanpeak shift for the free carrier electrons is plotted togetherwith seven lines related to spin transitions within theMn2+ subsystem. Also included in the figure is the resultof a detailed fit to the electron peak shift. The agreementof the fit with experiment is excellent. A large effectivemagnetic field due to the Mn2+ is experienced by the

    electrons (analogous to the Overhauser field). Thissaturates around 2 T. The initial electron Raman peak shiftat low fields is due to this effective field. At fields beyondthe Mn2+ saturation field the peak shift slowly decreasesreflecting the Zeeman spin splitting associated with theapplied external magnetic field and the negative g factor.In the theoretical fit the Overhauser field was assumed tobe proportional to the magnetization of the Mn subsystem.The fitted value of the electron g factor was -1.7 (ascompared to previously measured values of -1.6).

    The longer term focus of this study revolves around threespecific magnetic field regions where novel many bodyeffects have been predicted. These regimes are (i) close tozero magnetic field where the electron Raman peak shiftmay not extrapolate to zero due to the effect of magneticpolarons, (ii) the Raman peak crossing regions i.e.magnetic fields at which the same energy is required for aMn and electron spin flip, where anticrossing behaviourmay occur between the two peaks and (iii) the zeroeffective magnetic field regime experienced by theelectron spin system at higher magnetic fields whereinteraction effects may in fact prevent the observation ofa linear crossing through zero. Understanding theseregimes would resolve several outstanding issues relatedto DMS and their phase diagrams.

    However, figure 1.6 also raises a more fundamentalquestion which must first be understood, namely theorigin of the multiple Mn related lines. The peaks arewithin experimental error exactly equally spaced at fixedmagnetic fields. The line with the lowest slopecorresponds to a g factor close to 1.95. The differencefrom the g = 2 standard value is well outside ofexperimental error and is thought to be due to a Knightshift originating from the exitonic holes. The maximumnumber of peaks observed was seven. This number (>5)rules out mechanisms based on single Mn2+ localizedspins (spin 5/2). It is also important to note that similarmultiple peak cascades for low Mn concentrations (i.e.where the physics is governed by isolated Mn ions) haveonly been reported in samples with a reduceddimensionality. Previous explanations based specificallyon the Voigt geometry [1] can be ruled out in our casesince these new measurements were made in the Faradayconfiguration. We believe that, as a candidate for theorigin of the multiple lines, an interaction which makesthe forbidden multiple spin flip transition allowed andwhich is dramatically more significant in devices withreduced dimensionality is the asymmetric Dzialoshynski-Moriya interaction. Further investigations to confirm thisare being pursued.

    Reference and authors:

    [1] J.Stülher et al., Phys. Rev. Lett. 74, 2567 (1995)

    D.Plantier, F.J.Teran, M.Potemski A.Sachrajda (Institute for Microstructural Sciences,NRC, Ottawa, Canada)Z.Wilamowski, G.Karczewski (Institute of Physics,PAS, Warsaw, Poland)

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.6: Magnetic field dependence of Raman shift.Symbols denote experimental data and the solid line isthe best fit to the electron peak.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200113

    1.5. Resistively detected EPR of Mn2+ions coupled to a 2DEG in quantumHall regime

    The sp-d exchange interaction between the delocalizedband electrons and the 3d electrons of the localizedmagnetic ions is responsible for many unique propertiesobserved in diluted magnetic semiconductors (DMS) suchas CdMnTe. Most attention has been focused on the effectof such coupling on the behavior of the band electrons. Inthe mean field approximation, an additional magneticfield proportional to the average Mn2+ magnetization actson the band states and induces a giant enhancement of theZeeman splitting of the electronic states. Due to thereciprocal coupling between the electronic and magneticsystem, the inverse phenomena is also expected. Theamplitude of the spin splitting of Mn2+ should be sensitiveto the nature and the spin polarization of free carriers. Thefree carrier induced shift, similar to the well knownKnight shift for nuclear spins, has been observed in theEPR spectra of Mn2+ in 3D DMS lead compounds.

    We report here on the influence of the carrier presence onthe magnetic properties of Mn2+ ions embedded in a10 nm-thick CdMnTe modulation doped quantum wellstructure with a carrier concentration of ne = 5.9 x 1011 cm-2and a mobility µ = 60000 cm2/Vs. The average Mn2+concentration in the QW was ~ 0.3 %. In order to studythe magnetic subsystem, we have measured the changes inthe longitudinal resistance of the 2DEG induced bymicrowave irradiation under electron paramagneticresonance (EPR) conditions for the Mn2+ ions. Since Rxxis sensitive to changes of the electronic Zeeman energy,any alteration of the Mn2+ magnetization induced bymicrowave irradiation, will affect the transport properties.

    This technique allows us to selectively probe the very fewMn2+ ions embedded in our quantum well in contrast tostandard EPR and/or magnetization techniques which arenot sufficiently selective to detect only the magneticmoments in the QW layer. Rxx has been measured using a0.5 x 1 mm Hall bar, with and without continuousmicrowave illumination at liquid helium temperatures.The microwave frequencies used are in the range 68.4-230 GHz and the power, at the sample position, wasa few mW. Close to the sample a DPPH g-factor markerwas placed and its EPR spectrum has been measured witha carbon bolometer mounted below the sample. Using thisexperimental arrangement we have been able to measurethe Mn2+ resonance in our sample in the vicinity of fillingfactor ν = 10, 9, 7 and 3 (B ~ 2.4, 2.7, 3.5 and 8.1 T).

    As can be seen in figure 1.7, a resonant increase of theRxx is observed when the sample is illuminated withmicrowaves (∆Rxx corresponds to the change in resistanceunder microwave illumination). Our study reveals adifferent influence of the carrier presence in low and highmagnetic field regions. Whereas the mean-field theoryreasonably describes the observed carrier effects on theMn properties at low magnetic fields, it is not sufficient toaccount for the observations around 8 T. In this latter case

    the resonance position is very sensitive to thetemperature: a shift of 250 G is observed when varyingthe temperature between 4.2 and 1.6 K indicating anincrease of the Mn2+ spin splitting. In this magnetic fieldrange, the electronic and magnetic excitations havecomparable energy. A model based on a resonantinteraction between electronic and magnetic spinexcitations can successfully describe our experimentalfindings.

    Reference and authors:

    F.J.Teran et al., Physica E, in press

    F.J.Teran, M.Potemski, D.K.Maude, A.K.Hassan T.Andrearczyk, J.Jaroszynski, Z.Wilamowski,G.Karczewski (Institute of Physics, PAS, Warsaw,Poland)

    1.6. Quantum Hall effect underconditions of vanishing Zeeman energy

    The possibility of tuning the effective electron Zeemansplitting via the s-d exchange interaction betweenelectronic states and localized magnetic moments in dilutemagnetic semiconductors has been used to probe thequantum Hall effect under conditions of vanishingZeeman energy. Magneto-transport has been used toinvestigate a two dimensional electron gas (2DEG)confined in a modulation doped, Cd0.995Mn0.005Te 10 nmQW structure with ne = 5.9 x 1011 cm-2 andµ = 60000 cm2/Vs. The effective Zeeman energy of the

    Figure 1.7: ∆Rxx / Rxx for a microwave illumination at230 GHz, at two different temperatures, in the vicinity offilling factor ν = 3. Inset: Left axis, Knight shift as afunction of magnetic field (triangles) at T = 1.6 K. Rightaxis, the temperature dependence of the Knight shift(circles) in the vicinity of ν = 3 (B ~ 8.1 T).

  • Grenoble High Magnetic Field Laboratory • Annual Report 200114

    electrons in the 2DEG results from the competitionbetween the external and the exchange magnetic fieldswhich have different signs. To a good approximation forexternal magnetic fields B > 2 T and at low temperatures(T < 4 K) the Zeeman energy decreases linearly passingthrough zero for a total magnetic field ~ 18.5 T [1].Whereas the effective Zeeman gap is defined by the totalmagnetic field, the filling factor is determined by themagnetic field component which is perpendicular to the2D plane. Rotating the sample in magnetic field thereforeallows to tune the effective Zeeman energy independentlyof filling factor.

    We concentrate on the quantum Hall state at filling factorν = 3. Tilting the magnetic field with respect to the 2Dplane we can investigate the ν = 3 minimum for Zeemanenergies in the range EZ ≈ -1 up to +1 meV. From theactivated behavior of the temperature dependence of theresistance Rxx for a tilt angle θ = 64° (BT = 18.5 T), forwhich the Zeeman energy is expected to vanish, wemeasure a spin gap ∆S = 0.3 ± 0.03 meV. The observationof a nonzero spin gap at EZ = 0 for the case of a quantumHall state at odd filling factor is not surprising. The keypoint for understanding the physics of the quantum Hallregime at odd filling factors is electron-electron exchangeinteraction which forces the spin gap to remain open evenif the bare Zeeman gap is zero.

    We assume an activated behavior for the longitudinalresistance at ν = 3: Rxx(EZ, kT) = R0 x exp(-∆S(EZ)/kT),with R0 = 27.1 kΩ determined from the thermal activationat θ = 64°. Rotating the sample at a fixed temperature weuse the measured value of Rxx at ν = 3 to plot thedependence of ∆S on EZ as shown in figure 1.8. Asexpected the spin gap has a minimum for the tilt angleθ = 64°, for which the Zeeman energy is expected tovanish. Either side of EZ = 0, ∆S increases approximately

    linearly, in spite of some asymmetry observed fornegative EZ (large tilt angles). The values of ∆S obtainedfor different temperatures all collapse onto the same ∆S vsEZ dependence, which validates the assumption ofthermally activated behavior.

    We would expect that in a first approximation thedependence of the spin gap on the Zeeman gap is ∆S = Ee-e + EZ (see dashed lines in figure 1.8) where Ee-e is independent on EZ. We notice, however, that suchan interpretation does not fully agree with our data. Infact, on both sides of the minimum, the spin gap has avalue equal to EZ, but when EZ is close to zero, the spingap takes a non-zero constant value. Such ∆S vs EZdependence can be interpreted as the result of a simpleanti-crossing between the spin up and spin down Landaulevels. More work is needed to clarify the origin of theopening of the spin gap under conditions of vanishingeffective Zeeman splitting observed in our samples.

    Reference and authors:

    [1] F.J.Teran et al., Physica E, in press

    F.J.Teran, M.Potemski, D.K.MaudeT.Andrearczyk, J.Jaroszynski, G.Karczewski(Institute of Physics, PAS, Warsaw, Poland)

    1.7. Electron-hole coupling inInAs/GaSb bilayers studied bycyclotron resonance

    There is a controversy on the nature of the electron-holeinteraction observed experimentally in coupled e-hInAs/GaSb bilayers. The valence band (VB) of GaSb lies15 meV above the conduction band (CB) of InAs resultingin the system being two spatially separated twodimensional electron and hole gases. The electron andhole states can be coupled through tunnelling, whichresults in hybridisation of their wave functions [1] or canbe coupled, by Coulomb interactions [2].

    We have studied cyclotron resonance (CR) in high-mobility 2D structures and the influence of the spatialseparation of the electron and hole gases. FIR CRspectroscopy is used to study the effective mass of thecarriers involved in the transitions. CR behaviour isstrongly influenced by tunnelling, however our resultsalso show that Coulomb interactions can be important.

    The samples studied consist of a single narrow InAs well,sandwiched between thick layers of GaSb close to the samplesurface resulting in only one layer of GaSb being populatedby holes. The mean e/h separation (∆eh) is controlled both byvarying the thickness of the InAs well, and by the

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.8: Evolution of the spin gap as a function of EZat integer filling factor ν = 3 measured at severaldifferent temperatures.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200115

    introduction of short-period superlattices (SL) at theinterfaces. The structures are grown on GaAs substrates byMOVPE with a thick GaSb buffer layer of 2 µm, followed by9-40 nm of InAs, and 120 nm of GaSb. Typical values of thecarrier densities in these samples are ne ~ 6.5 x 1015 m–2 andnh ≈ 5 x 1015 m–2. These figures fall rapidly as the InAs widthapproaches 9 nm, which is where the InAs CB re-crosses theVB of the GaSb due to the electron confinement increase. CRwas measured with an FIR Fourier Transform spectrometerup to 27 T and the transmission spectra (TB) were normalisedby dividing by a reference spectrum (T0) at zero magneticfield, and a relative spectrum TB/T0 was recorded. Thespectra are fitted with Lorentzian line shapes and the effectivemass (m*) is deduced from the cyclotron energy ωc.

    When narrowing the well width and decreasing ∆eh thespectra show a large and systematic increase of m* at lowfield. We observe that at 3 T the CR mass is enhanced as ∆ehis increased from 10.5 nm to 61.5 nm. The smallest ∆eh,corresponding to a narrow well width of 9 nm shows a heavymass of m* = 0.054 m0, while the addition of 10 periodsuperlattice induces a decrease of the mass to m* = 0.028 m0,which is only slightly higher than the bulk InAs band edgemass. We explain this behaviour as due to resonant interbandtunnelling and more strongly coupled e/h states as they arebrought more closely together. At higher fields narrowerlayers show a series of oscillations of the CR linewidth andamplitude as well as the observation of multiple transitionswith very different magnetic field dependence. Thesephenomena resemble previous observations [1] but are muchmore pronounced due to the narrower well widths studied.The splitting of resonances, which are due to interbandcoupling as the e/h Laudau levels anticross, increases rapidlyin magnitude when the ∆eh is decreased.

    In the quantum limit at high magnetic fields in the region14-27 T the resonances are found to show a further series ofcouplings which shift in magnetic field as ∆eh increases.Figure 1.9 illustrates a plot of such spectra at 20 T. Multipletransitions are split from the main resonance by 10-50 cm–1and the size of these splittings is found to be stronglydependent on ∆eh and densities. We attribute the resonancesplitting observed in this regime to the spin splitting of thee/h states which is enhanced for narrow well.

    References and authors:

    [1] Yu.B.Vasilvey et al., Phys Rev. B 60, 10636 (1999)[2] J.Kono et al., Phys Rev. B 55, 1617 (1997)

    C.Petchsingh et al., Physica E, in press

    J.ZemanC.Petchsingh, R.J.Nicholas (Clarendon Laboratory,University of Oxford, U.K.)

    1.8. Single-dot-like emission induced byhigh magnetic fields

    The quest for the possibility to optically generate a cold,tunable-density, two-dimensional electron-hole gas hasstimulated investigations of double quantum wellstructures such as, for example, GaAs/AlAs hetero-wellswith a built in type II interface. Luminescence spectra ofsuch systems are known to exhibit a number of intriguingproperties which have been interpreted as the observationof a precursor of a Bose condensate of excitons oralternatively are assigned to effects of trapping ofphotoexcited carriers in naturally occuring quantum-dot-like objects formed from potential fluctuations induced bythe interface roughness.

    In this report we present a new set of experimental factsregarding luminescence properties of GaAs/AlAs hetero-well structure (figure 1.10). Our structure shows well-defined spectra at low excitation powers (figure 1.10), butcuriously enough, the appearance of a "broad band" ofsharp emission lines in macro-luminescence experimentsat higher laser excitations. These lines are clearly resolvedwhen high magnetic fields are applied in the directionperpendicular to the quantum well plane (figure 1.11).The appearance of these lines is not well understoodalthough they are tentatively attributed to laterally type IIquantum-dot-like objects. This is thought to be related to

    Figure 1.9: Plot of CR spectra at high field (20 T) ofsamples with varied mean separation between e and h(as indicated). Multiple splitting is observed in samplewith large ∆eh.

    Figure 1.10: Schematic diagram of the investigatedstructure and typical PL spectra measured using lowexcitation power.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200116

    the combined effect of the interface roughness and thepresence of a large number of electron-hole pairs. Wespeculate that the specific character of the GaAs/AlAsinterface favors the formation of lateral type II quantumdots for X electrons in the AlAs well and Γ holes in theGaAs well. We further speculate that the emission fromsuch type II dots is suppressed by the magnetic field ifthey are of low symmetry. On the other hand, those ofcircular symmetry resembling ring like structure remainradiatively active even in high magnetic fields. Indeed,the appearance and disappearance or even thecharacteristic interplay between the intensities of theneighboring lines observed as a function of magnetic field(figure 1.11) support this suggestion.

    Authors:

    A.Wysmolek, M.PotemskiV.Thierry-Mieg (L2M, Bagneux, France)

    1.9. Insulating states and thebreakdown of the quantum Hall effectin an electron-hole system

    We have studied the in-plane transport properties of anInAs/GaSb based electron-hole bi-layer system grown byMOCVD at the University of Oxford. InAs/GaSb is acrossed gap system giving it the ability to possess both

    electrons and holes in equilibrium through charge transferwithout doping or the application of an electrical bias.Here, we study a double heterostructure with a two-dimensional electron layer adjacent to a two-dimensionalhole layer. Previous studies of this system have shownthat in magnetic field, compensated quantum Hallplateaux appear at the value of the Hall resistance Rxycorresponding to the net occupancy given by νeff = νh – νeand Rxy = h/e2νeff.

    The figure 1.12 shows magneto-resistivity measurementstaken on a series of samples where the hole concentrationwas varied while the electron concentration remainedrelatively constant. The graphs on the left show thelongitudinal resistivity while those on the right show theHall resistivity. The lowest graphs show data from asample with electron to hole ratio of approximately 2 : 1,while the uppermost graphs show data from a sample withne : nh of approximately 4 : 3.

    Simple considerations of the electrical current flow in thequantised Hall regime reveal drastic differences betweenthis system and a single carrier type system, both in termsof bulk local conduction and edge states. In terms of edge-states, if both the electron and hole layers are individuallyin quantized Hall states, both layers must contribute edgestates at a given edge in opposite directions. In terms oflocal conduction, the currents in the two layers must beantiparallel and can be greater in magnitude than theapplied current.

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.11: The intensity changes of theneighboring lines as a function of magnetic field in therange 18-28 T.

    Figure 1.12: Left: Longitudinal resistivity at basetemperature for a series of samples with differing holeconcentrations. Right: Hall resistivity of the samesamples (R(–B) – R(+B))/2. (a): ne = 7.9, nh = 6.1(b): ne = 8.0, nh = 5.2 (c): ne = 7.8, nh = 3.7 x 1015 m–2.An insulating state forms with increasing holeconcentration at high field.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200117

    A special case of the quantum Hall effect can be achieved[1] when the quantised occupancies of the two layers areequal. i.e. νeff = νh – νe = 0. We have found that such astate exhibits novel insulating behaviour. The longitudinaland Hall resistance show reproducible fluctuations andthe Hall resistance becomes completely symmetric underfield reversal (the antisymmetric part shown in the figurebecomes zero). We have performed a series ofexperiments which have shown conclusively that theconduction in Hall bars in this state is dominated by themesa edges. Measurements on Corbino discs have shownmuch stronger insulating behaviour.

    We have also studied the current driven breakdownproperties of the quantum Hall states where νe – νh isfinite, and have shown that the critical currents in thissystem can be disproportionately smaller compared withsingle carrier type systems. Experiments on thedependence on the channel width have revealed tworegimes of behaviour: a linear width dependence at largercritical current (> 5 µA) and a superlinear dependence forsmaller critical currents.

    References and authors:

    [1] R.J.Nicholas et al., Phys. Rev. Lett. 85, 2364-2367(2000)

    K.Takashina et al., Physica B 298/1-4, 8-12 (2001)

    D.K.Maude, J.C.PortalK.Takashina, R.J.Nicholas, B.Kardynal, N.J.Mason(University of Oxford, UK)

    1.10. Anomalous resistively detectedNMR lineshape around ν = 1

    We have performed resistively detected nuclear magneticresonance (NMR) on a high-mobility AlGaAs/GaAsheterojunction in the quantum Hall regime [1]. Applyinga radio frequency field with a coil wound around thesample it is possible to detect the nuclear resonances ofthe GaAs isotopes which are present in the 2-DEG. Thelongitudinal resistance Rxx exhibits the resonances of the75As, 69Ga and 71Ga nuclei at both integer (ν = 1,2,3,…)and fractional filling factors (ν = 4/3,2/3,…). Theresistance variation ∆Rxx occurs via a modification of theelectronic Zeeman energy due to the hyperfine couplingbetween the electronic and nuclear spins. This experimentis performed under thermal equilibrium conditions atmillikelvin temperatures (T = 50 mK) without recourse todynamic nuclear polarization.

    A typical resonance line obtained at B = 5.76 T is shownin the inset of figure 1.13. When approaching theresonance frequency (41.8 MHz), Rxx suddenly decreasesbefore relaxing back exponentially with a time constant

    controlled by the nuclear spin lattice relaxation time T1.This behavior which is typical of a fast adiabatic passageis globally observed for all the filling factors withresonance amplitudes in the range 0.1-1 %. However,either side of filling factor ν = 1 an anomalous lineshapeis observed as shown in figure 1.14. This has beendetected for the 75As nuclei at B = 7.4 T corresponding tothe filling factor ν = 0.89. Its lineshape is similar to thederivative of a common NMR absorption signal.

    Steady-state measurements have been performed (opencircles) and are superimposed on the dynamic curverecorded at an rf sweep rate of 4 kHz/s (figure 1.14). Thesystem is therefore under equilibrium (slow passage)conditions indicating that the nuclear spin relaxation timeT1 is short. Another striking feature of this lineshape is itshuge amplitude which can be as large as 50 %, i.e. twoorders of magnitude larger than at other filling factors (seefigure 1.13).

    Figure 1.13: Magnetic field dependence of theresonance amplitude ∆Rxx/Rxx. The inset represents a75As resonance line at B = 5.76 T.The magnetoresistance Rxx is shown for reference (rightaxis).

    Figure 1.14: Resonance line measured at B = 7.4 T(ν = 0.89) for the 75As nuclei. Both the upsweep (solidline) and the downsweep (dashed line) have beenrecorded at 4 kHz/s. The open circles are the saturationvalues obtained under static conditions.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200118

    An enhanced coupling between the electrons and thenuclear spins due to the formation of spin textures(Skyrmions) has recently been invoked by Melinte et al.[2] in order to explain the anomalously large heat capacityat ν = 1. Theoretically, it has been shown that a couplingto a gapless spin wave excitation of the Skyrme crystalcould be at the origin of the dramatic enhancement of thenuclear spin relaxation rate 1/T1 [3]. In our sample atν = 1 the dimensionless Zeeman energy η = gµBB/(e2/εlB)~ 0.015 is favorable for the formation of Skyrmions. Wetherefore speculate that the coupling of the nuclear spinsto the gapless spin-wave excitations of the Skyrme crystalis responsible for the observed large amplitude andanomalous lineshape of the resistively detected NMRaround ν = 1.

    References and authors:

    [1] W.Desrat et al., Proc. ICPS, Osaka, Japan (2000)[2] S.Melinte et al., Physica E 6, 52 (2000)[3] R.Côté et al., Phys. Rev. Lett. 78, 4825 (1997)

    W.Desrat, D.K.Maude, M.Potemski, J.C.PortalZ.R.Wasilewski (IMS/NRC, Ottawa, Canada)G.Hill (University of Sheffield, UK)

    1.11. Magnetic channelling in tiltedmagnetic fields

    Recent work has demonstrated electron channelling inmicroscopically inhomogeneous magnetic fields [1,2].The stray fields of Dysprosium micromagnets fabricatedat the surface of a 2D electron gas are used to deflect andredirect ballistic electrons underneath. A positivemagnetoresistance was ascribed to the progressivequenching of snake orbit channelling by an externalmagnetic field. This picture however requires asufficiently hard ferromagnet so that the stray fields arestronger than the applied magnetic field to allow snakeorbits to form at H = 0. It has been proposed [3] that apositive magnetoresistance may arise from a softferromagnet in the absence of magnetic channelling. Theproblem is further complicated are the many stablemagnetic configurations arising as the magnet sizedecreases and the polycrystalline nature of Dy films onGaAs.

    Figure 1.15 shows the magnetoresistance peak plottedagainst H when the field is tilted from the normal to thein-plane direction. A soft ferromagnet would have itsmagnetization depending on the total magnetic field, H,whereas the suppression of snake states would give amagnetoresistance peak occurring at a constant value ofits normal field component, Hz = Hcos(θ). Thedependence of the magnetoresistance on the tilt angleshown in the inset of figure 1.15 therefore provides ameans of distinguishing between both mechanisms.

    Figure 1.16 shows that the peak position scalesremarkably well with Hz ~ 1.4 KOe while shifting overtwo orders of magnitude with H in figure 1.15. Asimilarly invariant peak is reported in the Hall quantityRxy/Rxy0 where Rxy0 is the asymptotic Hall dependence.The field value at the resistance peaks is shown in theinset to figure 1.16 for different tilt angles. Its invarianceforces the conclusion that the Hall voltage measures thevariation in the number of magnetic edge states ratherthan the average magnetic field in the Hall junction. Thehard ferromagnetic behavior of Dy is consistent with twofurther observations. Firstly, the structure at H ~ 28 KOein the 89° trace, labelled (a) in figure 1.15, is understoodto be the onset of the coherent rotation of themagnetization from the hard in-plane to the easy normalaxis. Its position is comparable to the anisotropy field ofthe Stoner-Wohlfarth picture and the structure vanishes

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.15: The magnetoresistance peak shifts over twoorders of magnitude when the applied field is tilted fromnormal to in-plane. The exp(αH2) background arisesfrom a small hopping component in our δ-dopedquantum well.

    Figure 1.16: Magnetoresistance, re-plotted as a functionof the normal component of magnetic field, showsremarkably little variation with angle. Inset summarizespeak position for both Rxx and normalized Rxy againstangle.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200119

    when the field is tilted only a few degrees from the hardaxis. Secondly, Dysprosium films grow with the easy axisnormal to the surface [1]. These observations concurtowards the hard magnetization picture of channelling.

    References and authors:

    [1] D.N.Lawton et al., Phys. Rev. B 64, 2231 (2001)[2] A.Nogaret et al., Phys. Rev. Lett. 84, 2231 (2000)[3] J.Reijniers et al., Phys. Rev. B 63, 165317 (2001)

    D.K.Maude, J.C.PortalA.Nogaret, D.Lawton (University of Bath, UK)M.Henini (University of Nottingham, UK)

    1.12. Magnetic field induced metal-to-insulator transition in PbTe widequantum wells

    Transport experiments in high magnetic fields reveal alarge variety of interesting and fundamental questions likethe transition between quantum Hall (QH) liquid and Hallinsulator (HI) in 2D-systems and the magnetic fieldinduced metal-to-insulator transition (MIT) in 3D-systems. In this context the investigation of electronicsystems in the intermediate regime between 2D and 3D isof special importance. Our samples are grown on the basisof the n-i-p-i concept with Lead Telluride (PbTe) andcover a wide range of electron concentration, mobility andelectron channel width. We have demonstrated, that themagnetic field driven transition to an insulator regime isdetermined by a parallel contribution of overlappingLandau-subband levels (LSLs), which are individually inthe regime of the Hall insulator [1,2], like known from 2Dsystems. On this basis also the temperature dependence ofthe insulator regime is investigated. Our data show a wellpronounced low temperature saturation behavior andtherefore a scaling function different from the Tκ-scalingknown from 2D-systems has to be used. In subsequent

    experiments we aimed at higher magnetic fields in orderto get a more accurate determination of the insulatorbehavior. Figure 1.17 shows an example where we get atransition to the insulating regime at about 12.5 T.However, instead of a further exponential increase athighest fields a recovery of the metallic regime appearsabove about 25 T. This behavior has been reproduced infurther experiments. Understanding the insulator - likebehavior results from pushing down the Fermi level intothe tails of the lowest overlapping LSLs by the high fields,the re - appearance of the metallic - like behavior shouldmean that the Fermi level stops to move further into thetails of the lowest LSLs with further increasing magneticfield. Numerical studies show that at highest fields theFermi energy can be pushed to the band edge alreadycloser than 1 meV. This is much less than the estimatedamplitude of native potential fluctuations. Consequently astrong redistribution of carriers must occur, which leads toa screening of the disorder potential and thus favors themetallic regime [3]. We made also numerical simulationsand figure 1.18 shows the results of our transportmodel [3] by using a magnetic field depended LL-broadening [4]. As can be seen, the MIT occurs at aboutB = 17 T, which is at a somewhat higher field than in theexperiment shown in figure 1.17. But the most importantresult is that this model indeed predicts a re-appearance ofthe metallic behavior at about B = 25 T like observedexperimentally.

    References and authors:

    [1] P.Ganitzer et al., Physica B 256-258, 600 (1998)[2] J.Oswald et al., Proc. 9th Int. Conf. on Narrow GapSemiconductors, Berlin 1999, Magnetotransport -Humboldt University at Berlin, 134 (2000)[3] A.Homer et al., Superlattices and Microstruct. 25,191 (1999)[4] D.Braun et al., Proc. 10th Int. Conf. on Narrow GapSemiconductors, Ishikawa, Japan 2001 (in print)

    D.K.Maude, J.C.PortalD.Braun, J.Oswald (University of Leoben, Austria)

    Figure 1.17: Rxx of one of the samples which exhibit therecovery of the metallic behavior above 25 T.

    Figure 1.18: Results of our transport model by using amagnetic field dependent LL-broadening.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200120

    1.13. Transport of two-dimensionalelectrons in the lattice of diffusive andthermalizing scatterers

    In this work we report the results of the experimentalstudy of a new kind of electron system with artificialscatterers: a two-dimensional electron gas (2DEG) with alattice of diffusive and thermalizing scatterers. Thissystem, based on a high-mobility 2DEG in aAlGaAs/GaAs heterostructure with an electron mean freepath l ≈ 5 µm, was fabricated in the following way: first,a square lattice of holes was made by means of electronlithography in the electron resist PMMA. The period ofthe lattice was d = 0.7 µm, and the hole diametera = 0.2 µm. Secondly, the GeAuNi alloy usually used forthe preparation of ohmic contacts to a 2DEG wasevaporated on this structure. Then, the electron resist wasremoved, and the lattice of GeAuNi dots remained on thesurface of the structure. Finally, an ordinary annealing ofthe alloy was performed. Thus after all the technologicalprocedures we have obtained a 2DEG in a square latticeof dirty metallic (GeAuNi alloy) dots (see the insert offigure 1.19).

    Figure 1.19 shows the magnetoresistance (rxx(B)) tracesof the 2DEG with a lattice of scatterers and of theunpatterned 2DEG at 1.5 K in magnetic field up toB = 4 T. One can see that at B = 0.32 T acommensurability peak (CP) corresponding the condition2Rc = d is observed. At larger magnetic field, there is alarge negative magnetoresistance. This behavior of theMR is similar to that observed in the antidot lattice. Itmeans that the introduction of the dirty metallic dots doesnot break the ballistic electron motion between scatterers.

    Now let's consider the results of the weak localizationstudy of our samples. Figure 1.20a shows the dependenceof the array conductivity as a function of lnT.

    One can see a small decrease of σ in the temperaturerange 5 K – 1 K and a saturation below 1 K. Theestimation of the conductivity variation gives the value of

    ∆σ ~ e2/h that is to say close to the value of the weaklocalization correction to the conductivity. However fromfigure 1.20a it is also clearly seen that the resistance riseis badly described by a logarithmic temperaturedependence. Figure 1.20b shows the conductivity as afunction of T. This figure clearly demonstrates that ∆σ(T)is described much better by a linear temperaturedependence. Recently this dependence has been predictedin the new version of weak localization theory as reportedin [1].

    Reference and authors:

    [1] G.Zala et al., cond-mat/0105406

    O.Estibals, J.C.PortalZ.D.Kvon, A.Y.Plotnikov, A.I.Toropov (Institute ofSemiconductor Physics, Novosibirsk, Russia)

    1.14. Single-electron conductanceoscillations of small open quantum dot

    In this work we report the observation of single-spinoscillations in the conductance of a small open lateralquantum dots fabricated on the basis of a high mobility

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.19: rxx(B) dependences of the 2DEG in latticeof GeAuNi dots (solid) and of the unpatterned 2DEG(dashed) at T = 1.5 K.

    Figure 1.20: Temperature dependence of theconductivity: ∆σ(lnT) – a; ∆δ(T) – b.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200121

    two-dimensional (2D) electron gas in an AlGaAs/GaAsheterostructure. This observation suggests the existence ofspin-charge separation in these dots as predicted in [1].Small open quantum dots have been fabricated on thebasis of a high mobility 2D electron gas (electronconcentration Ns = 3 . 1011 cm-2 and mobilityµ = 3 . 105 cm2/V . s at T = 1,7 K) located 100 nm belowthe surface. The technological procedure was thefollowing. Three antidots located at the vertexes of anequilateral triangle have been made by means of electronlithography and consequent plasma etching. The distancebetween the antidots centers was d = 0.4 µm, and theirsize a = 0.2 µm. Then a metallic Ti/Au gate has beenevaporated on the top of the experimental structure.Figure 1.21 shows the scanning electron micrograph andschematic view of the sample.

    Figure 1.21: SEM micrograph of the structure andschematic view of triangular-shape three leads quantumdot inside an Hall bar.

    The area of this dot is S ≈ d2(√3/4 – π/8) if the antidot sizea ≈ d. It corresponds to S ≈ 6.1 . 10-11 cm-2 for d = 0.4 µm.So the quantum dot studied in this paper has the same areathan the smallest laterally defined quantum dotsfabricated recently by means of split-gate technology. Butin other respects our dot differs quite significantly fromthe split-gate dots. First, it has three leads while most ofthe dots studied earlier have two ones; secondly, it has acontinuous metallic gate and correspondingly no middlemetallic gate as split gate fabricated dots.

    Figure 1.22 shows the results of the measurements of thetwo-terminal conductances as a function of the voltage

    applied to the top continuous metallic gate Vg atT = 50 mK. One can see very large conductanceoscillations at Vg < –20 mV which become weaker atVg > 0. The period of these oscillations is ∆Vg ≈ 20 mV.Figure 1.22 also shows that at Vg > –30 mV G2323becomes larger than 2e2/h. Actually at these gate voltagesthe first plateau of the ballistic quantization is observedfor this conductance configuration if one exclude theoscillations. It means that the large G1212 and G1313oscillations are observed in the open regime. For an otherconductance configuration, in the closed regime, we havemeasured Coulomb blockade oscillations which periodcoincides with the one measured in the open regime. Thisis the important signature of the existence of spin-chargeseparation in these dots as predicted in [1].

    Reference and authors:

    [1] L.I.Glazman et al., Phys. Rev. Lett. 83, 1830 (1999)

    O.Estibals, J.C.PortalZ.D.Kvon, A.Y.Plotnikov, A.I.Toropov (Institute ofSemiconductor Physics, Novosibirsk, Russia)J.L.Gauffier (INSA Toulouse)

    1.15. Gated wires and interferometersbased on a Si / SiGe heterostructure

    We report the fabrication and study of gated Si/SiGequantum wires and interferometers: our samples werefabricated on a high mobility n-type modulation dopedSi/Si1-xGex heterostructure using electron lithography andanisotropic ion etching. Finally a TiAu metal gate wasevaporated on the top part of the structures.

    Negative magnetoresistance (NMR) or positivemagnetoconductivity (PMC) connected with weaklocalisation effects in the wires and Aharonov-Bohmoscillations in the ring were investigated in thetemperature range 30 mK – 5 K.

    The lithographic length of the wire was L = 5 mm and itswidth W = 0.5 mm. A rough estimation of the effectivewidth from the wire resistance gives W = 0.1 – 0.2 mm. Itis less than the electronic mean free path l = 0.5 mm – 1 mm,thus we have quasiballistic wires where l > W and l

  • Grenoble High Magnetic Field Laboratory • Annual Report 200122

    different from the predictions of the theory in the quasi-one-dimensional case and also from that obtained inGaAlAs/GaAs wires. Indeed, the ordinary observedsaturation occurs at much lower temperatures, close to

    0.1 K. For this reason we are forced to suggest that thissaturation has some technological origin rather than anyother one, connected with possible fundamental orexternal factors. At so high temperature, the only non-temperature dependant source of decoherence can only bemagnetic impurities, which may be introducedaccidentally during the fabrication process of our Si/SiGeheterostructures.

    Figure 1.24a shows Aharonov-Bohm oscillationsmeasured at weak magnetic field, in a Si/SiGe ring withan inner diameter din = 0.3 mm and outer dout = 0.8 mm.Their period, ∆B = 0.016 T, corresponds to the averageeffective diameter of the ring deff = 0.6 mm. In agreementwith what has been obtained in [1], the amplitude of theseoscillations proved to be small in comparison withAlGaAs/GaAs rings, even at T = 30 mK. One of thereasons of this situation can be an insufficiently largephase coherence time at low temperatures because of theabove discussed saturation in Si/SiGe wires.

    In a smaller ring, (din = 0.2 mm and dout = 0.6 mm), wehave observed for the first time in Si/SiGe ringsAharonov-Bohm oscillations in high magnetic fieldcorresponding to edge current transport (figure 1.24b).The Fourier power spectrum of these oscillations showstwo close peaks: under the conditions of edge currenttransport, two frequencies are observed, ∆B = 0.035 T and∆B = 0.042 T. We believe that they correspond to theinterference of the edge current trajectories around theinner and outer boundary of the ring.

    References and authors:

    [1] W.X.Gao et al., Appl. Phys. Lett. 65, 3114 (1994)

    O.Estibals et al., Physica E, in press

    O.Estibals, Z.D.Kvon, J.C.PortalA.Y.Plotnikov (Institute of Semiconductor Physics,Novosibirsk, Russia)N.J.Woods (Imperial College, London, UK)J.Zhang, J.J.Harris (University College, London, UK)

    1.16. Coexistence of a two-dimensionaland three-dimensional Landau states ina wide parabolic quantum well

    The existence of the energy gap in the electron spectrumof the two-dimensional electron gas in a strong magneticfield is the crucial point for the explanation of theQuantum Hall effect (QHE) [1]. It demonstrates why theQHE is a property of a two-dimensional system and is notobserved in a three dimensional case, where the electronspectrum is continuous.

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.23: Temperature dependence of the phasecoherence time in the Si/SiGe wire.

    Figure 1.24: Aharonov - Bohm oscillations and theirFourier power spectrum for Si/SiGe rings in weakmagnetic field - a and in high magnetic field - b.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200123

    The remarkable example of the quasi-three-dimensionalsystem is a parabolic quantum well (PQW) [2]. The basicidea behind these structures is to create a conduction bandprofile in the growth direction of GaAs/AlGaAsheterostructures by properly varying Al mole fractionsuch that it mimics the parabolic potential of a uniformlydistributed slab of positive charge. It allows to form awide layer of highly mobile carriers with uniform density.Considerably larger mobility in comparison with heavilydoped GaAs epitaxial layers has been achieved byremoving the dopant atoms from the quantum well.

    In the present work we study 2000 Å and 4000 Åparabolic wells with narrow (100 Å) spacer and 5-8occupied subbands. Our samples are overfilled, and thewidth of the electron slab is almost coincident with thegeometrical width. We realize the system with 2D andquasi 3D electron gas coexisting in the same quantumwell. We measured the Shubnikov-de Haas oscillations inwide parabolic quantum wells with 5-8 subbands in tiltedmagnetic field. We found two types of oscillations(figure 1.25). The oscillations at low magnetic fields areshifted toward higher field with the tilt angle increasingand can be attributed to the two-dimensional Landaustates. The position of the oscillations of the second typedoes not change with the tilt angle increasing whichpoints out to a three-dimensional character of theseLandau states. We calculated the level broadening due to

    the elastic scattering rate Γ = -h/2τ, where τ is the quantumtime, and energy separation between two-dimensionalsubbands ∆ij = Ej – Ei in parabolic well. For all the levelswe obtained Γj ~ ∆ij, which means that the levels overlap,supporting the observation of the three-dimensionalLandau states. Surprisingly, we found that the lowestsubband, which has a smaller energy separation from thehigher level, does not overlap with these subbands andforms a two-dimensional state. Therefore we produce asystem containing 2D and 3D electron gas with almost thesame Fermi energy.

    References and authors:

    [1] See for review, R.E.Prange, S.M.Girvin eds., TheQuantum Hall effect, second edition (Springer-Verlag,New York, 1990)[2] M.Shayegan et al., Appl. Phys. Lett. 53, 791 (1988)

    C.S.Sergio et al., Phys. Rev. B 64, 115314 (2001)

    O.Estibals, D.K.Maude, J.C.PortalC.S.Sergio, G.M.Gusev, J.R.Leite (Instituto de Físicada Universidade de São Paulo, SP, Brazil)E.B.Olshanetskii, A.A.Bykov, N.T.Moshegov, A.K.Bakarov, A.I.Toropov (Institute ofSemiconductor Physics, Novosibirsk, Russia)

    1.17. New phase transition of thequantum Hall state at ν = 2/3

    The electron spin-polarization P of a two-dimensionalelectron gas confined in two different GaAs/GaAlAsmultiple quantum-well (QW) samples M280 and M242,previously used in other studies [1,2], was measured bynuclear magnetic resonance (NMR). At the fractionalquantum Hall (FQH) state with filling factor ν = 2/3, aphase transition from a partially polarized (P ≈ 3/4) to afully polarized (P = 1) ground-state can be driven byincreasing the ratio between the Zeeman and the Coulombenergy above a critical value ηc = ∆Z/∆C = 0.0185.

    NMR is a very sensitive direct measurement of thespin polarization of 2D-electrons in the QWs, since theFermi contact interaction H = 8π/3|γe|γn-h2∑ijSi . Ijδ(

    →ri –

    →Rj)

    (γ is the gyromagnetic ratio) between itinerant electronspins Si at position

    →ri and nuclear spins Ij at →Rj shifts the

    resonance frequency of 71Ga nuclei in the QWs by amagnetic hyperfine shift KS proportional to P [1,2]. TheNMR signal from barriers, where the conduction band isempty, is used as a zero-shift reference. The spinpolarization is inferred from the hyperfine shift asP(ν, T, θ) = KS(ν, T, θ) / KS(P = 1), where KS(P = 1) is themaximum shift measured for high Zeeman energy.

    The dependence of the electron spin polarization onη = ∆Z/∆C at the exact filling factor ν = 2/3 is shown in

    Figure 1.25: Two-dimensional Shubnikov de-Haasoscillations (2D SdH) as a function of the magnetic fieldat T = 50 mK, W = 2000 Å. Solid lines - experimentalcurves, dashes - theory. (b) Three-dimensional Shubnikovde Haas (3D SdH) oscillations obtained by subtractionof the 2D SdH oscillations from the experimental curvein perpendicular magnetic field at T = 50 mK. Dashes -theory.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200124

    figure 1.26 for both samples M280 and M242, as obtainedfrom the low temperature saturation values of P at varioustilt angles θ. We observe a Zeeman energy induced phasetransition from a partially polarized ground-state (GS)with an average P ≈ 3/4 to a fully polarized GS above thesame critical value ηc ≈ 0.018 for both samples (the totalmagnetic fields at this critical point are BcM280 = 6.7 T andBcM242 = 8.9 T). The transition from one GS to the otheris very sharp, within a change of η of about 3%. Such asharp jump in spin-polarization suggests a first-orderphase transition. The precision of this measurement canbe seen from the inset to figure 1.26, where the spectra forM280 are plotted. The error on the line's position is lessthan 0.1 kHz.

    Within the composite fermion (CF) model at ν = 2/3 onlyP = 0 and P = 1 are possible. The ν = 2/3 state is built outof the fully polarized or unpolarized ν = 2 state byattaching two flux quanta, pointing anti-parallel to theexternal magnetic field, to each electron and projectingthe wavefunction on the lowest Landau level (LL). Withinthis picture a partial polarization P ≈ 3/4 cannot beconstructed from filled CF-LL's, but have to beconsidered as an inhomogeneous mixture of P = 1 andP = 0 states.

    There is no satisfactory understanding of the FQH effectin the low magnetic field limit. In particular, since filledCF-Landau levels can only produce fully polarized orunpolarized states at ν = 2/3, the nature of a partiallypolarized state at this filling factor is open. Among thepossible states, it is natural to consider some of the otherknown spin-liquid states which have been considered inthe literature such as the valence-bond GS of the 2DShastry-Sutherland model. Other well-known spin-gapped states are commensurate spin-density waves.

    An alternative viewpoint is to consider partially polarizedstates as inhomogeneous mixture of fully polarized andunpolarized regions. The GS could also be described asisolated singlets forming a commensurate modulatedstructure through the sample, in many ways similar tovalence-bond commensurate spin-liquid GSs. Naturally,the real challenge is to determine among all the possibleGSs, which one has the lowest energy.

    References and authors:

    [1] S.Melinte et al., Phys. Rev. Lett. 84, 354 (2000)[2] N.Freytag, Ph.D thesis, Université de Grenoble 1(2001)

    N.Freytag et al., Phys. Rev. Lett. 87, 136801 (2001)

    N.Freytag, Y.Tokunaga, M.Horvatić, C.Berthier, L.P.LévyM.Shayegan (Princeton University, USA)

    1.18. Observation of a new scalingbehavior of the ν = 1/3 state

    The temperature dependence of the electron spin-polarization P of a two-dimensional electron gas at fillingfactor ν = 1/3, was determined from NMR measurementsof the Knight shift. The data presented here was obtainedusing the multiple quantum-well sample M280,introduced in the previous report. The thermal activationof P probes the chargeless excitations of a quantum Hallstate and gives valuable information for the understandingof strongly interacting many-body systems. Especially inthe case of ν = 1/3, where the ground-state is very wellknown and given by the Laughlin wave-function, thedetermination of the excitation spectrum can be used totest the different theoretical approaches.

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.26: The phase transition of the ν = 2/3 state asrevealed by the dependence of the spin polarization onthe ratio of Zeeman and Coulomb energies η = ∆Z/∆Cfor sample M280 (•) and M242 (❒) at temperaturesbelow 100 mK. η was varied by changing the angle θbetween the magnetic field direction and the normal tothe 2D plane. The inset shows the NMR spectracorresponding to the points for M280, where the QWssignal amplitude is renormalized.

    Figure 1.27: The temperature dependence of the spinpolarization P at ν = 1/3 is shown for four different tiltangles θ = 0°, 30°, 37°, and 45°. The lines are theprediction of a free particle model using Eq.1.1.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200125

    In figure 1.27 we show the temperature dependence ofP(ν = 1/3) for four different tilt angles θ = 0°, 30°, 37°,and 45°. The corresponding magnetic fields are 10.65 T,12.3 T, 13.34 T, and 15.06 T.

    A simple model of P(T) assumes that the partitionfunction factorizes into a spin-independent and a spin-dependent part, i.e. the broadening of the energy levels issmall compared to the spin splitting ∆(B). Under theseconditions, the electrons can be treated as free particlesobeying Fermi-Dirac statistics, and the temperaturedependence of the polarization is given by:

    P(B, T) = tanh (∆(B) / 4kBT). (1.1)

    This model predicts the temperature dependence of thespin polarization quite accurately, if one accounts for anincreased spin-flip gap ∆ > ∆Z, where ∆Z has beendetermined using the g-factor of electrons in bulkGaAs g = 0.44. From the fits to Eq. 1.1 for the fourdifferent tilt angles (see figure 1.27), we deduce that theeffective spin-flip gap ∆ ≈ 1.27 ∆Z is an enhanced Zeemangap, i.e. the enhancement by 27% does not depend on themagnetic field.

    Since the Zeeman energy appears to be the uniqueparameter to determine P(T), we can attempt to scale thedata presented in figure 1.27: figure 1.28 shows P versusthe effective temperature T* = T/∆Z. Indeed, the datacorresponding to four different total magnetic field valuesfall on a unique curve.

    Physically, the spin excitations at ν = 1/3 are magnons ofa quantum Hall ferromagnet: a quasi-electron with spin-up is destroyed and created with spin-down at somedistance. If the distance separating this quasi-particle/holepair is large, the excitonic Coulomb interaction betweenquasi-particle and hole is small and the excitation energyis mostly the Zeeman energy associated with the spin-flip.In general, however, spin-waves are thermally excitedwith arbitrary wave-vectors k and their dispersion has tobe taken into account, from which follows that this type of

    experiment is a measure of the integral of the spin-wavedispersion. Therefore, the exchange enhancement of thespin-flip gap is expected to be rather ∆ = ∆Z + c . ∆X,where ∆X ∝ √ B⊥ is a constant for every filling factor andelectron density, and not ∆ = c . ∆Z as is experimentallyobserved. The accurate scaling with the Zeeman energysuggests a mechanism that “cuts” the integration forq

  • Grenoble High Magnetic Field Laboratory • Annual Report 200126

    The existence of a "soft" linear gap in the density of statesnear the Fermi level, due to the Coulomb interaction oflocalised electrons, was predicted many years ago. Sincelocalisation increases with increasing B, it is notsurprising that the dip in the tunnel conductance due to thegap in the density of states appears only in a magneticfield, when most of the states along the 2DEG becomelocalised. However, the behaviour of the gap withmagnetic field has not previously been measured. Weargue that the narrow conductance peak at zero bias in lowB is related to tunnelling from strongly localised electronpuddles in the emitter into 2D extended states in thecollector. This is the well known Fermi-edge singularity,which was first observed in tunnelling between a 2Dcontinuum and zero-dimensional impurity states. In ourstructure, the donor concentration fluctuates in the planeof the 2DES. Therefore, it is possible that there areregions with low electron concentration, which havestrongly localised states, and regions of higherconcentration with extended 2D electron states. Since thepotential fluctuations in the electron systems on differentsides of the barrier are independent, there should existregions where electrons tunnel from localised to extendedstates, giving rise to the conductance peak. The magneticfield tends to induce localisation and the Fermi edgesingularity is no longer visible in the tunnel conductance.

    Authors:

    D.K.Maude, J.C.PortalYu.V.Dubrovskii, V.G.Popov, E.E.Vdovin,D.Yu.Ivanov (Institute of MicroelectronicsTechnology RAS, Chernogolovka, Russia)R.Hill, P.C.Main, L.Eaves, M.Henini (University ofNottingham, UK)V.A.Volkov (Institute of Radioengineering andElectronics RAS, Moscow, Russia)G.Hill (University of Sheffield, UK)

    1.20. Probing the electronic propertiesof disordered two-dimensional systemsby resonant magneto-tunnelling

    A thin pseudomorphic InAs layer (wetting layer-WL)incorporated in the central plane of an(AlGa)As/GaAs/(AlGa)As quantum well (QW) leads to asignificant lowering of the energy of the quasi-twodimensional (2D) ground state subband of the QW. Abovea critical wetting layer thickness, self-assembled InAsquantum dots (SAQDs) are formed. This modifies furtherthe electronic states of the system: firstly, the dots giverise to discrete zero-dimensional bound states and,secondly, they create a considerable amount of disorder,which influences the properties of the continuum ofwetting layer subband states. In this paper, we study theeffect of disorder on the electronic properties of thecontinuum states in the well using magneto-tunnellingspectroscopy (figure 1.30).

    Sample studied qd comprised a 1.8 monolayer (ML) InAswith growth rate 0.13 ML/s to form InAs QD in the centreof the well. For the sample in which the dots are formed,a wetting layer is still present. It is easy to show that theresonance condition between the 3D electrons in thedoped contact layers and WL subband is possible at zerobias, or shifts to higher bias, depending on the QD densityin the layer, and one would expect to see a resonanttunnelling feature through the ground state in the I(V)plot. In contrast to this expectation, the I(V) curve ofsample qd shows only a monotonic exponential increaseof the current with bias at low voltage with no currentpeaks or negative differential conductance regions whichusually characterise resonant tunnelling. We argue that theexponential increase of the current at low bias simplyreflects tunnelling with no momentum conservationthrough two-dimensional states in the well stronglylocalised by the fluctuating random potential arising fromlocal strains and charging of the quantum dots. The

    LOW DIMENSIONAL ELECTRON SYSTEMS

    Figure 1.29: (a) The slope of the linear variation of thegap with energy in arbitrary units; (b) the depth of thelinear gap in arbitrary units; (c) the width of the gap inmV, all versus magnetic field applied normal to the2DES.

    Figure 1.30: Differential conductance of sample qdversus voltage at different magnetic fields. The magneticfield, B, is perpendicular to the current direction. In thepresence of high magnetic fields (> 6 T), a new peakwith associated NDC region appears, which shifts tohigher voltages with increasing B as in conventionalresonant tunnelling double barrier structures.

  • Grenoble High Magnetic Field Laboratory • Annual Report 200127

    exponential current-voltage dependence changesexponent at around V*b1 ≈ 110 mV. Above this criticalvalue V*b1 a 2D accumulation layer is formed near theemitter barrier, which we confirm by analysis of magneto-oscillations in the tunnelling current.

    Two sets of magneto-oscillations, each periodic in 1/B,appear simultaneously at bias voltage V*b2 ≈ 140 mV. Thelow B oscillations (below 4 T) are due to the formation ofoccupied Landau levels in the accumulation layer. Theoscillations at higher B reflect tunnelling through emptyLandau states in the quantum well. We interpret thisbehaviour in terms of a threshold energy, E*, in the qdsample. Only for energies above E* it is possible forLandau levels to form. This apparent threshold betweenlocalised and delocalised states can be understood interms of the screening of the random potential in the wellby electrons in the accumulation layer. Estimates showthat, for our structure, dispersion of the random potentialin the well is reduced by three times after the formation ofthe accumulation layer. This model also explains ourmagneto-tunnelling data for magnetic field appliedperpendicular to the current direction. In the presence ofhigh magnetic fields (> 6 T), a new peak with associatedNDC region appears, which shifts to higher voltages withincreasing B as in conventional resonant tunnellingdouble barrier structures.

    Authors:

    D.K.Maude, J.C.PortalYu.V.Dubrovskii, E.E.Vdovin, D.Yu.Ivanov,Yu.N.Khanin (Institute of MicroelectronicsTechnology RAS, Chernogolovka, Russia)A.Patane, L.Eaves, P.C.Main, A.Levin, and M.Henini(University of Nottingham, UK)P.N.Brounkov (A.F.Ioffe Physico-Technical Institute,St.-Petersburg, Russia)I.A.Larkin, G.Hill (University of Sheffield, UK)

    1.21. Polaron coupling in high electrondensity GaAs Quantum Well (QW)

    In polar materials, the longitudinal optical phonon (LO)mode leads to a macroscopic polarisation. Thispolarisation can influence the electronic motion via theFrölich interaction which is the main contribution to theelectron-phonon interaction. Its most spectacularmanifestation is the resonant magneto-polaron coupling(RMPC), i.e. an anticrossing behaviour between the|n = 0 + 1LOphonon〉 and the |n = 1〉 states, n being theLandau level (LL) index, when the cyclotron frequencyωc = eB/m* equals the LO phonon frequency ωLO (B isthe magnetic field and m* is the electron effective mass).

    We have performed experiments on 3 different QW ofwidth 10 nm for sample 1038 (ns = 1