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    Journal of Advanced Mechanical Design,Systems, andManufacturing

    Vol. 1, No. 3, 2007

    358

    A Study of Self-Loosening of Bolted Joints Due

    to Repetition of Small Amount of Slippage at

    Bearing Surface*

    Shinji KASEI**

    **Shinshu University,

    4-17-1, Wakasato, Nagano, 380-8553 JAPAN

    E-mail: [email protected]

    Abstract

    This paper deals with the mechanism and relating matters on self-loosening rotation

    of bolted joints in the cases when very small slippages occur repeatedly at bearing

    surfaces under transverse loads. It can be supposed that accumulation of this kind

    of loosening finally produces serious states for bolted joints. Based on an

    assumption that a restoring force caused by an elastic torsion of a bolt shank which

    arises from a relative displacement between bolt and nut threads drives loosening

    rotation, a theoretical explanation is presented about how loosening rotation occurs

    and grows larger. Experiments in quasi-static states show results which agree with

    the theory of this paper. Additionally, consumption of transverse work and

    anti-loosening performance being taken up as relating subjects, more information

    about self-loosening is shown through examinations on some kinds of test samples.

    Key words: Bolted Joint, Transverse Load, Loosening Rotation, Minute Slippage,

    Bolt-Shank Torsion, Loosening Mechanism, Consumed Work,

    Anti-Loosening Performance

    1. Introduction

    Self-loosening of screw threads is one of major subjects relating directly to reliability of

    bolted joints. Accordingly, many efforts have been made to understand this phenomenon

    and prevent its occurrence. It is well known that there exist two kinds of self-loosening, the

    one due to rotation of a bolt or a nut and the other not due to it. Their respective features

    and mechanisms have been known gradually(1)~(4)

    . Especially, many researchers have

    exerted themselves for self-loosening due to rotation since it has a dangerous inclination to

    bring greater loss of a fastening force than the case not due to rotation. G.H.Junker

    (5)

    pointedout clearly that loosening rotation occurs easily under repetition of transverse loads and thus

    we should take notice of this case. A.Yamamoto and S.Kasei(6),(7)

    presented a hypothesis of

    the loosening mechanism, in which behavior of an elastic torsion of a bolt shank performs

    an important role, and verified it experimentally. As recent achievements, many papers have

    been published by R.I.Zadoks & X.Yu(8)

    , P.Wolfsteiner & F.Pfeiffer(9)

    , N.G.Pai &

    Hess(10),(11)

    , Y.Jiang, et al.(12),(13)

    , S.Izumi, et al.(14),(15)

    and so on. Each paper has respectively

    contributed to explication of the self-loosening problems. It is noticeable that three

    dimensional FEM was used as a tool of analyses in some papers(10)~(12),(14),(15)

    . This fact

    makes us feel that an era in which problems like self-loosening can be numerically analyzed

    has come. Among them, S.Izumi, et al.(14)

    showed the analytical results supporting the

    results by the author, et al.

    (6),(7)

    .The author, et al.

    (16),(17)pointed out that loosening rotation can be induced even when*Received 24 Jan., 2007 (No. 07-0054)

    [DOI: 10.1299/jamdsm.1.358]

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    slippages at bearing surfaces are very small and its situation should be considered as a sign

    capable to connect to a serious state. And a theoretical consideration about the loosening

    mechanism was developed by basing on the hypothesis(6),(7)

    mentioned above. Subsequently,

    several researches intending to this case were performed(10)~(13),(15)

    . In particular, S.Izumi, et

    al. classified contacting situations of a mating surface on threads and a bearing surface with

    nine kinds of combinations and explained loosening behavior in each combination.

    This study was planned to follow up the previous report (16)

    , especially about

    experimental considerations which have been remained not enough. So, it is the main

    purpose to prove the theory experimentally by using an improved experiment apparatus and

    consequently contribute explication of the self-loosening mechanism. In addition, to present

    more information about self-loosening of bolted joints, consumptions of transverse work

    and anti-loosening performances are examined about some test bolt-nut samples.

    2. Theory

    Along the hypothesis of the previous report(16)

    , a theoretical approach will be promoted.

    Basically, the author considers that loosening rotation is caused by a restoring action of an

    elastic torsion of a bolt shank which is due to a relative motion at a mating surface on

    threads. Figure 1 shows an explanatory illustration about this relation in the case of

    right-hand threads. Speaking relatively, it can be said that whichever side is fixed between a

    bolt and a nut, it does not make an essential difference.

    2.1 Behavior of elastic torsion of bolt shank

    Figure 2 illustrates slide loci(6)

    at the mating surface on threads under the transverse

    load. The side of bolt-threads is replaced with a concentrated point and the slide loci which

    the point draws on a thread surface of the nut are expressed schematically in processes of

    sliding-up and -down (the nut side is fixed). Where, : a half angle of thread, : a lead angle

    of a helix, r: a radial position from the bolt axis, u: a circumferential displacement

    (corresponding to the torsion), Rr: a force which moves the bolt-threads up or down along

    the thread surface of the nut,Fa: a force which moves the bolt-threads down along the helix,

    andFt: a restoring force due to the torsion along the helix. The direction of a resultant force

    ofRr,FaandFtis considered to coincide with the tangential direction of the loci and to be

    opposite to the direction of a frictional force on the thread surface. In the mating surface on

    threads, parts of sliding-up and sliding-down coexist and the slide brings the torsion angle

    T. By taking a pitch diameter of thread dpinto account, an equation pT du2= is obtained.

    If the nut side is fixed throughout the processes, ucan reach to a critical value ucr(or Tcr, a

    critical value of T) in a critical condition ta FF = . However, once the nut slides at the

    bearing surface, the torsion is released by a rotation of a unified body composed of the boltand the nut

    (6),(16). Since the bolt-threads descend along the helix of the nut-threads with

    FtFa

    Rr

    A

    B

    aFriction force

    Screw surface

    of nut

    Circumfer-

    ential dir.

    Axial dir.

    Radial dir.

    u

    r

    In sliding-up

    Slide locus

    a u

    r

    A'

    B'

    Slide locus

    In sliding- down

    Fig.2 Slide loci on mating surface on threads

    Fixed plate

    Movable plate

    Bolt shank

    TorsionRestoring

    force

    Fig.1 Transverse displacementand torsion of bolt-shank

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    360

    increasing of u and thus an axial tension Ff reduces by a quantity corresponding to a

    deformation of tanu , the above rotation becomes a loosening one in the result.

    The slide locus is formulated by the following equation(6),(7)

    .

    coscos

    cos

    d

    d

    ta

    r

    FF

    R

    u

    r

    = (1)

    Denoting a part ofFfasFf', a coefficient of friction assand a part of a spring constant

    of the boltKuasKu', the following relations are induced for Eq.(1)(6)

    .

    ( ) ( )2''

    '

    ,

    '

    )cos4(,sin

    costan1costandown)(slidingup)(sliding

    putfa

    s

    fs

    r

    s

    fs

    r

    duKFFF

    FR

    FR

    ==

    +

    ==

    Consequently, the critical torsion angle Tcr is

    known as

    tan2

    tan2 '

    '

    u

    fp

    u

    fp

    TcrK

    Fd

    K

    Fd== (2)

    whereKuandKu'are quantities with the unit of

    [Nm/rad].

    2.2 Progress of loosening rotation

    Typically, the case where an initial torsion

    u0due to a bolt clamping is greater than ucr is

    discussed. Figure 3 conceptually illustrates two

    typical relations between the number ofloading cycle n and a behavior of u. The one

    denoted as (a) is in a state where the nut does

    not slide and conversely the other (b) is in a

    state where the slide of the nut exists at the

    bearing surface little by little. In the case (a), u

    approaches gradually to ucrfrom an upper side

    because of a gradual release of uat the mating

    surface on threads, but no loosening rotation

    occurs. In the case (b), at an initial stage of the

    transversely repeated loading u goes down

    beneath ucrdue to a slide at the mating surface on threads and/or the bearing surface of thenut. Afterward, u increases toward ucrwhen no slippage occurs at the bearing surface and

    conversely decreases when the slippage occurs. In Fig.3, a zigzag line expresses a process

    of progress of the loosening conceptually and means that the loosening rotation occurs

    cyclically in sections from uun to uln. It is considered that uun and uln depend on the axial

    tension, the transverse load, frictional conditions, etc. Moreover, the difference between uun

    and ulnis considered to have a close relation with the magnitude of loosening rotation.

    2.3 Relation between transverse load and transverse displacement

    Figure 4 shows two basic models expressing the relation between the transverse load W

    and the transverse displacement x. The models correspond to cases with some losses of

    energy at the mating surface on threads and/or the bearing surface. S 0is a starting point ofthe loading. In the case (a), the slippage at the mating surface on threads only exists (S4'S5'

    Number of cycle n

    Tors

    ion

    ofbo

    lt-s

    han

    k

    u

    looseningOccurrence oflooseningOccurrence of

    uln

    uun

    ucr

    (a)

    u0

    (b)

    Fig.3 Explanatory figure of relation between

    torsion and number of loading cycle

    W

    S3

    S5

    S0

    S1

    S2

    S4

    S5

    S6

    S7 xS7

    S2

    S4

    W

    xS0

    S1

    (a) (b)

    Fig.4 Two basic models between

    transverse load and displacement

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    and S7'S2'), but there is no

    slippage at the bearing

    surface. The case (b) has, in

    addition to the part of the

    slippage at the mating surface

    on threads (S4S5 and S7S2),the part of the slippage at the

    mating surface on threads

    plus at the bearing surface

    (S2S3 and S5S6). The case (a)

    corresponds to the one of

    Fig.3(a) and the case (b) to

    the one of Fig.3(b).

    Incidentally, sections of S0S1, S2'S4' and S5'S7' in the former and sections of S0S1, S3S4and

    S6S7 in the latter express processes in which the bolt and the nut displace together like a

    unified body.

    3. Experiment apparatus and experimentalconditions

    Fig.5 shows an outline of the experiment

    apparatus. Roughly speaking, it consists of a main

    body, a driving part and a system for measurement

    and control. In the main part, many steel balls being

    inserted in-between, a movable plate is clamped to a

    fixed plate by a test bolt and a test nut under a

    required force. In the driving part, through a

    differential screw mechanism a servomotor gives

    the movable plate a transverse alternatingdisplacement. The servomotor has a reduction gear

    drive and a rotational encoder, and its rated output

    performances are 111W and 30rpm. In addition, the

    differential screw mechanism in which a

    combination of pitch of 1.5 and 1.25mm is

    employed is used to convert a rotational motion to a

    translational one and make a small and smooth

    quasi-static transverse displacement. A motion

    control is performed for the amplitude of the

    transverse displacement of the movable plate.

    Figure 6(a) shows a detailed drawing of the sideview of the main body. Parts numbered are: the

    test bolt, the test nut, a attachment for

    measuring the bolt shank's torsion angle or the nut's

    rotation angle (additionally, the nut's slippage at the

    bearing surface), the movable plate, the fixed plate, a load-cell for measuring

    the axial tension of the bolt, a fixture for fixing firmly the test bolt to a inner side of .

    A bearing plate with which the test nut keeps contact was heat-treated and its both end

    surfaces were ground.

    Quantities to be measured are the axial tension Ff, the transverse displacement of the

    movable plate x, the transverse load W, the torsion angle of the test bolt shank T, the

    rotation angle of the test nut and the slippage at the bearing surface of the test nut s. As

    shown in Figure 6(b), fixing the attachment to the test bolt shank,Tis obtained basing

    on subtraction of outputs of two gap sensors A and B, and instead fixing to the test nut,

    Pulse Board

    Strain Amp

    A/D Board

    Strain Gage

    Control Unit

    Fixed plateBolt/nut

    Servo motor

    Torsion,

    Slippage,

    Rotation

    Differential

    screw mech.

    Axial forceExt.

    force

    Displacement

    Movable plate

    Electronic

    micrometer

    Non-contact

    sensors

    Strain gages

    Strain amp.

    A/D board

    Control unit

    Pulse board

    Fig.5 Outline of the experiment apparatus

    (a) Side view of the main body

    (b) Attachment for measurement

    of torsion, etc.

    Fig.6 Detailed explanation on the

    apparatus

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    and s are obtained basing on subtraction

    and sum of outputs from A and B,

    respectively.

    Table 1 shows the summary of

    conditions for the experiments. Test thread

    sizes are M10 and M101.25, and a griplength is 28mm. An initial axial tension of

    the bolt is always set to be 10kN and

    machine oil added MoS2 powder is applied

    to the thread surfaces and the bearing

    surfaces as a lubricant.

    4. Experimental results and

    considerations

    4.1 State of progress of loosening

    Figure 7 shows changes of therotation angle of the nut under

    transversely repeated loads.

    Amplitudes of the transverse

    displacement x are 15m to 40m.

    The negative side of means the

    loosening direction. Changes of in

    these cases are small and especially

    in ~ the changes are smaller

    and can be recognized to stop on the

    way. In the cases of ~, it is

    supposed that the changes are not dueto loosening rotation, but due to

    releases of initial torsions of the bolt

    shanks and initial deflections of the

    bolt shanks which are forced to

    generate in clamping operations.

    These kinds of rotations only connect

    to initial tiny losses of Ff. On the

    other hand, in and , real

    loosening rotations probably add to

    some extent and so their values

    steadily grow greater little by little.According to Fig.7, it can be

    supposed that loosening rotation will

    go forward when the amplitude of x

    is greater than around 30m in the

    present experiments.

    4.2 Torsion of bolt shank and

    loosening rotation

    Figure 8 shows experimental

    curves of the torsion angle T and

    corresponding curves of Ffwhen the

    amplitudes of x are 15 and 60m.

    About T, the direction indicated with

    -30

    -25

    -20

    -15

    -10

    -5

    0

    0 100 200 300 400 500 600 700 800

    Numbe r of cycle n

    Rotation

    ofnut

    (

    )

    B:15m A: 15m

    A:30m B: 30mA: 35m A: 40m

    Fig.7 Progresses of the nut rotation (A: M10 hexagon nut,

    B:M101.25 hexagon nut with flange)

    0

    2

    4

    6

    8

    Tors

    ion

    T

    (

    ) 15m

    60mTcr

    2

    4

    6

    8

    10

    0 50 100 150 200 250 300Number of cycle n

    Axialtension

    F

    f

    (kN) 15m

    60m

    Fig.8 Changes of torsion angle and axial tension (M10hexagon nut)

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    the arrow mark in Fig.1 is employed

    as the positive side. It is known that

    these curves of T show a similar

    tendency to Fig.3. In the case of15m, T approaches gradually to a

    value regarded as Tcr from an initial

    value forced by the clamping

    operation and only the tiny loss ofFf

    can be recognized in the early stage

    as mentioned in 4.1. On the other

    hand, in the case of 60m, T drops

    down rapidly just after a start of the

    transverse loading and afterward

    repeats up and down in the area between zero and the value regarded as Tcr. Moreover, it

    can be seen that progress of loosening corresponds to the behavior of T. By substitutingFf=10kN, =3.03 , dp=9.03mm and Ku=1.5910

    3Nm/rad to Eq.(2), Tcr=1.5210

    3rad=5.22is found. Here, the value of Ku is from a calculation about the test bolt. This

    value agrees fairly well with the experimental value indicated in Fig.8.

    To examine in detail, a behavior of Twas detected in a process which consists of a

    stage of a manual clamping by a spanner, five cycles of loading (the amplitude of x is

    100m) and a manual loosening by the spanner. Figure 9 shows its result. In the figure, A1

    is equivalent to a point at which the fastening torque reaches a maximum, A2 a removal

    point of the fastening torque, A3a point of a maximum loosening torque and A4an ending

    point of the loosening. According to Fig.9, in the process of transverse loading except an

    initial part, T behaves up and down similarly and periodically every half cycle. Such

    feature is because the test bolt-nut is almost under the same kinetic conditions every halfcycle in whichever direction the transverse load acts. However, it is supposed that if there

    are some reasons like geometrical deviations (e.g. perpendicularity between a bolt's axis

    -10

    -5

    0

    5

    10

    15

    20

    25

    0 100 200 300 400

    T

    ors

    ion

    alang

    le

    T

    (

    )

    A1

    A2

    A3

    A4

    100m5cycles

    Time (s)

    Fig.9 Behavior of torsion angle of bolt-shank inmanual-fastening plus transverse-loading plusmanual-loosening (M10 hexagon nut)

    -0.8

    -0.4

    0

    0.4

    0.8

    Tra

    nsverseloadW

    kN

    0

    2

    4

    6

    Torsion

    T

    (

    )

    -35

    -30

    -25

    -20

    -15

    -100 -50 0 50 100

    Nutrota

    tion

    Transverse displacement x(m)

    S3

    S6

    S4

    S7

    S7S4

    S3

    S6

    S2

    S2

    S2

    S5

    S5

    S3

    S6 S7

    S5

    S4

    Fig.10 Mutually related diagrams oftransverse load, torsion angle ofbolt-shank and rotation of nut(M10 hexagon nut)

    0

    2

    4

    6

    -120 -60 0 60 120

    x (m)

    0

    2

    4

    6

    -120 -60 0 60 120

    x (m)

    T

    Fig.11 Additive diagrams of torsion angle ofbolt-shank (M10 hexagon nut)

    Table 2 Slip widths and rotation angles of nut in

    a half cycle (n=5, M10,hexagon nut)

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    and a bearing surface), relating conditions will change and consequently T will show

    some different behavior. And, during transverse loading T exhibits a bias with a positive

    value. This is considered to meet the hypothesis that an elastic torsion of a bolt shank plays

    a role to drive loosening rotation.

    Figure 10 shows diagrams of W, Tand relating to xby arranging these in parallel.

    These diagrams were obtained from a simultaneous detection in the same experiment (theamplitude of x is 100m). Since the case is supposed to correspond to the state shown by

    Fig.4(b), the symbols used there are attached at the corresponding points supposed. During

    sections of S3S4 and S6S7 in which the bolt and the nut are regarded to be unified, T

    changes just only a little, but increases during sections of S4S5and S7S2in which the mating

    threads are regarded to be forced to slip. And it is known that the nut rotates in the manner

    synchronizing with sections of S2S3and S5S6which are regarded as sections involving the

    slippage at the bearing surface. Figure 11 shows the diagrams of T versus x when the

    amplitudes ofxare 60 and 80m. Similarity is clearly recognized between the diagrams of

    Figs.10 and 11. It is considered that such behaviors and relationships show a validity of the

    theory explained in 2. It is supposed that geometrical and tribological conditions at the

    mating threads and the bearing surface are influence factors which bring fluctuations tothese relations.

    In the experiments, progresses of loosening rotation are clearly recognized when the

    amplitude ofxis greater than 60m. Table 2 shows experimental values of the width of the

    slippagesat the bearing surface and the increment of during a half cycle at the fifth cycle

    (n=5). We can confirm thatsis very small on the whole, loosening rotation occurs even in

    the case wheresis less than 10m and its value grows larger with increase of the magnitude

    of slippage.

    M10, hex. nut M101.25, hex. nut M10, hex. nut with locknut

    Fig.12 Changes of axial tension and consumed work per a cycle (amplitude ofxis 80m)

    n = 2

    n=100

    n=300

    - 0 . 8

    - 0 . 4

    0

    0. 4

    0. 8

    - 100 - 50 0 50 10 0

    x (m)

    W

    (kN

    50 100-100

    0.8

    0.4

    -0.4

    -0.8

    W

    (kN)

    0

    -0.8

    -0.4

    0

    0.4

    0.8

    -100 -50 0 50 100x (m)

    W

    (kN)

    n = 2

    100

    n = 2

    100

    300

    x (m)

    -1

    -0.6

    -0.2

    0.2

    0.6

    1

    -100 -50 0 50 100x (m)

    W

    (kN)

    n = 2

    100

    300

    M10, hex. nut M101.25, hex.nut

    M10, hex. nut with locknut

    Fig.13 Diagrams between transverse load and transverse displacement corresponding to the cases of Fig.12

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    4.3 Consumed work

    Since occurrence of loosening rotation must be closely related with the slippages at the

    mating surface on threads and the bearing surface, a work (energy) consumed by them is

    considered to involve information about loosening. For anti-loosening performances, G. H.

    Junker, et al.(19),(5)

    employed a quantity relating to the external work of vibration as an

    evaluation factor. Here, the work consumed per one loading cycle designated as Lwill beexamined. L is considered to equal an area surrounded by diagrams of W versus x like in

    Fig.4. So, measurements of L are tried every cycle through a numerical treatment with

    regard to Wandx.

    Figure 12 shows experimental examples aboutFfandLversus n. The nut samples are as

    follows, (a) a M10 hexagon nut, (b) a M101.25 hexagon nut and (c) a M10 hexagon nut

    with a locknut (so-called a "double-nut"). Figure 13 shows diagrams of W versus x

    corresponding to the cases of Fig.12. According to these figures, the following can be

    stated. In the case of (a), bothFf andLfall most rapidly. It seems to be caused by a reason

    that the slippages are easy to occur at the mating surface on threads and the bearing surface.

    In the case of (b), both of Ff andLshows a tendency of slow falling. It is supposed that the

    slippage at the mating surface on threads is hard to occur to some extent. Lastly, in the caseof (c),Ffshows no falling tendency, butLshows a quite different feature. Namely, although

    the value ofLis initially in a higher level and keep the level for a while, afterward it falls

    down steadily. It can be pointed out that the slippage is forced to occur only at the bearing

    surface, protecting strongly the slippage at the mating surface on threads by a complete

    locking by means of a locknut. In the above example, it is known that the slippage at the

    bearing surface is getting harder to occur at n=300 than at n=2 and 100. Perhaps, such a

    situation comes from tribological changing of the bearing surface.

    4.4 Tests for anti-loosening

    performance

    Anti-loosening perform-ances of several kinds of nut

    samples are compared one

    another by evaluating a loss

    rate of the axial tension .

    Table 3 presents M10 or

    M10 1.25 test samples in

    detail and the marks assigned

    for them. In the case of a M10

    hexagon nut with a locknut (a

    "double-nut"), a locking

    operation is completely doneto assure locking effect.

    Figure 14 shows the

    values of which are

    obtained from the axial

    tension losses between n=0 to

    300 under five different

    amplitudes of xup to 100m.

    Each point doted expresses

    the average of three test

    results. Speaking from the

    results shown in Table 2, theslippage at the bearing

    0

    20

    40

    60

    80

    100

    Amp. of displacement (m)

    Lossrateofaxialtension

    (%)

    15 30 60 80 100

    Fig.14 Results of anti-loosening tests

    With washer

    Coarse(1.5)

    Fine(1.25)

    Hex. Nut

    Thread

    pitch (mm)

    Without washer

    Hex. nutHex. nut

    with flange

    Hex. nut

    with locknut

    (double-

    nut)

    "Washer" means a special plain washer which was heat-treated and

    ground

    Table 3 Samples for anti-loosening tests

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    surface is estimated to be very small.

    According to Fig.14, the "hexagon nut", which is regarded as the basic sample, has the

    lowest performance. Other samples, although degrees of the effect are not alike, exhibit

    some respective effects. However, an excellent performance is only recognized in the case

    of the "hexagon nut with a locknut ("double-nut")". Other cases seem to have insufficient or

    limited effects. Progress of loosening rotation is affected by the conditions of the bearingsurface and the mating surface on threads. The performance of the "hexagon nut with a

    locknut ("double-nut")" comes from a hard obstruction against the slippage at the mating

    surface on threads. Basically, situations in which slippages may occur at both parts of the

    mating surface on threads and the bearing surface should not be permitted for preventing

    loosening rotation. Fig.14 suggests such a point well.

    5. Conclusions

    (1) With regard to the cases under repetition of small slippages at the bearing surface, a

    theoretical explanation about the mechanism for occurrence and progress of loosening

    rotation was presented. It is based on the hypothesis that the basic driving force of

    loosening rotation is the restoring force due to the elastic torsion of the bolt shank.(2) Experiments under repetition of the transverse displacement were performed about M10

    or M101.25 samples in quasi-static states. It can be said that experimental results show

    well agreements with the theory of this paper and thus the basic mechanism of loosening

    rotation can be explained well by this paper.

    (3) The consumed work in the mating surface on threads and the bearing surface was taken

    up as a factor suggesting the feature of loosening. With some examples detected in the

    experiments, relations between its value and tendency and loosening behaviors were

    explained.

    (4) Anti-loosening performances about some kinds of test samples were inspected under

    repetition of small slippages at the bearing surface. Among the present samples, only the

    case employing the "hexagon nut with a locknut", which was subjected to a stronglocking operation, showed an excellent performance. It is emphasized that when a high

    anti-loosening performance is required a firm obstruction of the slippages at the mating

    surface on threads and/or the bearing surface must be ensured.

    Acknowledgment

    The author expresses sincere thanks to Prof. Emeritus, Akira Yamamoto, Tokyo

    Institute of Technology for his guidance and suggestions over long years. The author is

    grateful to Mr. Satoshi Yoshida, Mr. Hisanori Ishibashi and Mr. Takato Komura for their

    co-operations and contributions to this study as graduate students, and also grateful to other

    students who took part in this study. Additionally, the author wishes to thank the Ministry of

    Education, Culture, Sports, Science and Technology, and Japan Society for the Promotion ofScience for their financial support (the Grant-in Aids for scientific research) to some parts

    of this study.

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