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A Brief Presentation:A Brief Presentation:Evaluations of CALPUFF 6.4; Experience with Modeling for 1 hour NO2 and SO2 Compliance in Baltimore; Using MM5 Data for Local Scale ModelingMM5 Data for Local Scale Modeling
For Presentation at the:h f f l d l10th Conference of Air Quality Modeling
EPA‐Research Triangle Park, NCMarch 15, 2012
M k G i A d Y ERMMark Garrison, Anand Yegnan, ERMJohn Sherwell, Maryland DNR
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Topicsp
•Evaluations of CALPUFF 6.4; •Experience with Modeling for 1 hour NO2 and SO2
Compliance in Baltimore; •Using MM5 Data for Local Scale Modeling
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Evaluations of CALPUFF 6.4
• Maryland DNR Power Plant Research Program (PPRP) has a long standing interest in the Chesapeake Bay including excess long-standing interest in the Chesapeake Bay including excess nutrient loading due to anthropogenic emissions of NOx
• CALPUFF has been used as a tool to help understand source and t t ib ti t N l di d t t source sector contributions to N loading; compare and contrast
with CMAQ• New chemistry included in v. 6.4 holds promise in terms of
improving predictions of N loading• Work-in-Progress includes evaluations of CALPUFF predictions
compared to aerosol and gas concentrations, and wet deposition, p g pmeasured at CASTNET, IMPROVE, and NADP measurement stations
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Evaluations of CALPUFF 6.4: Modeling Domain
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Evaluations of CALPUFF 6.4: Initial Observations
• Summary of NOx and SO2 Emissions (Millions of• Summary of NOx and SO2 Emissions (Millions of short tons) – NEI 2005
Pollutant Total EGU Industry Mobile Non-PointPollutant Total EGU Industry Mobile Non-PointNOx 7.09 1.85 0.39 2.69 2.14 SO2 8.81 7.27 0.61 0.06 0.87
•Preliminary Results Indicate improvements in predictions of nitric acid concentrations, particulate nitrate concentrations, and wet deposition of nitrates
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Baltimore NOx Monitors/Sources for Evaluation
T i Old T d E h •Two measurement sites – Old Town and Essex – have recorded NOx and NO2 concentrations for over 20 yearsy
•2009 actual emissions inventory prepared for AERMOD
•Focus on stationary sources (approx. 500 facilities)•Approx. 438,000 lbs/day of NOx•NOx/NO2 measurements for 2009 for comparison
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Trends in NO2/NOx Ratios
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Meteorological Data g
•Baltimore-Washington International (BWI) surface, Dulles (Sterling, VA) upper air for 2009( g, ) pp
•Utilized new AERMINUTE processing to reduce missing, calm hours
•Significant number of low (<1 m/s) winds•AERMOD in the urban mode
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Old Town: Old Town: Predicted Concentration RatiosOLMGROUP/ OLMGROUP/ 0.10 in-stack ratio
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Old Town: Old Town: Predicted Concentration RatiosPVMRM/ 0.10 PVMRM/ 0.10 in-stack ratio
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Old Town: Old Town: Measured Concentration Patterns
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Old Town: Old Town: Predicted ConcentrationsOLM/ 0.50 in-stack ratiostack ratio
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Baltimore Analysis: Observations
•OLMGROUP appears to produce better patterns of NO2/NOx ratios than PVMRM
•Evaluation suggests use of 0.1 in-stack ratio for all sources
•Problems with AERMINUTE processing; DNR currently recommending use of pre-ASOS meteorological data
•Baltimore analysis points out shortcomings of AERMOD •Baltimore analysis points out shortcomings of AERMOD application at this scale; transport times are an issue.. possible future application of CALPUFF
•Evaluating improvements in treating “urban core” plume
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Use of MM5 for Local Scale Meterology
•PPRP has used MM5 data to extract local winds for near-field analyses in a number of cases;field analyses in a number of cases;
•Evaluations of extracted winds compared to tall towers (primarily at nuclear stations) and profilers are (p y ) pencouraging;
•Initiating evaluations of beta version of MMIF•Use of MM5 (and WRF) holds promise for improving
local scale meteorology, particularly in situations where airports are somewhat remotea po ts a e so e at e ote
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