Thin viscous films: I. Coating flows inside a rotating ... · • at slow rotation rates, a thin...

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Thin-film free-surface flows

Jacqueline AshmoreDAMTP, University of Cambridge, UK

APS DFD meeting, November 21st 2004

Copyright Jacqueline Ashmore, 2004

Fundamentals of coating flows:interaction of viscous stresses

& capillary stresses (due to curvature gradients)

solidsurface

low Reynolds # Newtonian coating flows characterized by capillary number:

viscosity surface tensioncharacteristic velocity

viscous stresscapillary stress

free surface

capillary pressure gradient

viscous stress

U

Copyright Jacqueline Ashmore, 2004

The Landau-Levich-Derjaguin scalingLandau & Levich (1942), Derjaguin (1943)

flat film

liquid

static meniscus: gravity balances surface tension

dynamic meniscus: viscous force balances surface tension

asymptotic matching of the surface curvature in the two regions:

ρ,η

σ

(meniscus curvature)

U

l

provided

(low capillary number limit)

Copyright Jacqueline Ashmore, 2004

Rimming flows:coating the inside of a rotating cylinder

with Anette Hosoi (MIT) & Howard A Stone (Harvard University)

Ω

R θ

free surface

cylinder

filling fraction

density

viscosity

surface tension

R

equation for is usual coating flow equation, but this problem has two unusual features:1) solutions must be periodic2) conservation of mass imposes integral BC

Copyright Jacqueline Ashmore, 2004

A rich variety of behavior …

“sharks’ teeth” with pure fluid(Thoroddsen & Mahadevan, 1997)

banding of a suspension(Tirumkudulu, Mileo & Acrivos, 2000)

Copyright Jacqueline Ashmore, 2004

Literature review(not comprehensive)

• films outside a rotating cylinder: Moffatt (1977)

• analyses in the absence of surface tension:e.g. O’Brien & Gath (1988), Johnson (1988), Wilson & Williams (1997)

• surface tension included in numerical studies:e.g. Hosoi & Mahadevan (1999), Tirumkudulu & Acrivos (2001)

• an unpublished study including analytical work:Benjamin et al. (analytical, numerical and experimental)

no previous detailed analytical study of surface tension effectsno previous detailed analytical study of surface tension effects

Copyright Jacqueline Ashmore, 2004

Focus of our study: surface tension effects• two-dimensional (axially uniform) steady states• consider significance of surface tension in “slow rotation” limit• compare theoretical predictions & numerical results

surface tension is a singular perturbationsurface tension is a singular perturbation

Ω

σAssumptions

• lubrication approximation

• negligible inertia R

filling fraction A

ρ,η

Copyright Jacqueline Ashmore, 2004

constant flux, to be determined

viscous gravitysurface tension

“higher order” gravity

nonlinear third-order differential equation

nonlinear third-order differential equation

determines film thicknessNondimensional flux equation:

boundary condition

curvature

3 nondimensional parameters when inertia is neglected:

gravitygravitysurface tensionviscous

filling fraction (note )

Copyright Jacqueline Ashmore, 2004

Dependence of solutions onin absence of higher-order gravity & surface tension no solutions for

bottom of cylinder direction of rotation

λ=12

35

1020

50

θ

h(θ)

λ

points denote value of flux from numerical simulations in low

capillary # limit; B=100, A=0.1

3 qualitatively different regimes:(“shocks”); (pool & thin film)

(uniform coating);

π 2π

Copyright Jacqueline Ashmore, 2004

approximately uniform coating

“shocks” develop

high capillary # limit: surface tension not important

(Tirumkudulu & Acrivos, 2001)

pool in bottom with thin film coating sides and toplow capillary # limit:

surface tension generates films with

LLD scaling

Overview of solutions

Copyright Jacqueline Ashmore, 2004

Film thickness when

theoretical prediction:

B=100, A=0.2

scaling of pool determined from static considerations

log

q

log λ

0.119−2(log λ)/3

2/3

log(

q λ) λ=10000, A=0.2

log B

−0.214+(log B)/6

Copyright Jacqueline Ashmore, 2004

Coating the inside of a rotating cylinder: conclusions

• inclusion of surface tension facilitates an analytical description of a steady 2-D solution at very slow rotation rates

• at slow rotation rates, a thin film is pulled out of a pool sitting at the bottom of the cylinder

• thickness of the film in low capillary # limit calculated by asymptotic matching

• dimensional film thickness:

Copyright Jacqueline Ashmore, 2004

With special thanks to …

Advisor: Howard A. Stone (Harvard)Co-advisor: Gareth H. McKinley (MIT)Eric R. Dufresne (Yale)Michael P. Brenner (Harvard)Anette (Peko) Hosoi (MIT)

Copyright Jacqueline Ashmore, 2004