Fireplaces: Good for your CO2 footprint, bad for air...

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Fireplaces: Good for your CO2 footprint, bad for air quality

Ulrich Pfeffer, Tanja Schuck, Ludger Breuer North Rhine-Westphalia State Agency for Nature, Environment and Consumer Protection

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de

23 November 2011

Air Quality in Europe: Particulate Matter

2

• EU limit values for PM10 are exceeded in many European cities

• Episodes with high PM10 levels − e. g. winter 2011 / 2012

• To reduce the PM burden we need to know the sources

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de

Background

• Combustion releases a number of substances into the air e. g. carbon monoxide, aerosol particles, hydrocarbons, PAH, …

• Each type of combustion process bears a characteristic signature

• Wood burning emissions can be identified by specific tracers such as certain – hydrocarbons – isotopic carbon “fingerprint” – a class of sugars: anhydrosugars, one of them is levoglucosan

3

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 4

Number o Stoves and Fireplaces sold in Germany

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de

Air Quality Network in NRW

5

We use Levoglucosan to get a grasp of how strongly wood burning influences local and regional air quality

North Rhine-Westphalia (NRW): − 34.000 km² − 18 million people − a dense air quality

monitoring network

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 6

PM10 Concentration in NRW

0

20

40

60

80

100

01/1

1/20

11

08/1

1/20

11

15/1

1/20

11

22/1

1/20

11

29/1

1/20

11

06/1

2/20

11

13/1

2/20

11

20/1

2/20

11

27/1

2/20

11

03/0

1/20

12

10/0

1/20

12

17/0

1/20

12

24/0

1/20

12

31/0

1/20

12

07/0

2/20

12

14/0

2/20

12

21/0

2/20

12

28/0

2/20

12

06/0

3/20

12

13/0

3/20

12

20/0

3/20

12

27/0

3/20

12

03/0

4/20

12

10/0

4/20

12

17/0

4/20

12

24/0

4/20

12

PM 10

[ µg

/m³ ]

BIEL

EIFE

DUBR

DUM2

EU daily limit value

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 7

0,0

0,5

1,0

1,5

2,0

2,5Le

vogl

ucos

an [

µg/m

³ ] BIEL

EIFEDUBRDUM2

0,0%

1,0%

2,0%

3,0%

4,0%

5,0%

1/11

8/11

15/1

1

22/1

1

29/1

1

6/12

13/1

2

20/1

2

27/1

2

3/1

10/1

17/1

24/1

31/1 7/2

14/2

21/2

28/2 6/3

13/3

20/3

27/3 3/4

10/4

17/4

24/4

Rel

ativ

e S

hare

of

Levo

gluc

osan

in P

M10

BIELEIFEDUBRDUM2

Absolute and Relative Concentrations of Levoglucosan in PM10

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 8

Project „Smoke in my Garden ...“

Source 1 Source 2

2 x LVS

In the past .....

Determination of conversion factor: PM10 = F • levoglucosan (≈ 13)

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 9

Contribution of Wood Burning to PM10

0

50

100

01/1

1/20

11

01/1

2/20

11

01/0

1/20

12

01/0

2/20

12

01/0

3/20

12

01/0

4/20

12

PM10

[ µg

/m³ ]

PM10 at Station DUM2

PM10 wood burning

PM10 other sources

EU daily limit value

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 10

PM10 Limit Value Exceedances

0

5

10

15

20

25

30

35

40

45

50

BIE

L

BO

RG

BO

TT

BU

CH

DD

CS

DM

D2

DU

BR

DU

M2

EIF

E

GE

LS

GR

GG

KR

ES

MH

HS

STY

R

VAC

W

VKT

U

VM

GR

VW

EL

WA

LS

WA

ST

# da

ys >

50

µg/m

³

Station

PM10 Exceedances caused by wood burning (Nov 2011 - April 2012)

wood burningPM10 other sources

EU limit value: 35 days per year

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 11

Sensitivity Analysis of Conversion Factor F

Percentage of days > 50 µg/m³ PM10 caused by wood burningcalculated as LG * F (with F = 6 ..... 15)

21 sites in NRW

0%

10%

20%

30%

40%

50%

60%

70%

80%

Nov 11 Dez 11 Jan 12 Feb 12 Mrz 12 Apr 12

Per

cent

age

6 8 10 11 12 13 15

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de

Some Examples across Europe

12

Maenhaut 2012:

In Flanders 10 – 15 % of winterly PM10 are from wood burning

Borrego 2010:

PM10 burden in Lisbon due to

residential wood combustion − up to 60 exceedance days total

could be avoided all over Portugal

by usage of certified appliances

Caseiro 2010:

10% of PM10 load in autumn

and winter in Vienna are related to wood smoke

Green Week, 4 -7 June 2013, Brussels ulrich.pfeffer@lanuv.nrw.de 13

Summary and Conclusions

Potential for significant reduction of exceedance days

Quality of combustion process plays a crucial role

Use stoves rather than open fire places

Replace or upgrade old installations for domestic heating

Use stoves with optimal combustion and filter techniques

Regulation of use of single stoves during episodes with high PM concentrations?

Transport of air masses plays also an important role a European Issue

Fireplaces: good for your CO2 footprint, bad for air quality

Ulrich Pfeffer, Ludger Breuer, Dieter Gladtke, Tanja Schuck North Rhine Westphalian State Agency for Nature, Environment and Consumer Protection